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Change trend of natural gas hydrates in permafrost on the Qinghai-Tibet Plateau(1960-2050)under the background of global warming and their impacts on carbon emissions

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China Geology 2022年第3期5卷 475-509页

作者： Zhen-quan lu Chu-guo Wu Neng-you Wu hai-long lu Ting Wang Rui Xiao Hui Liu Xin-he Wu Oil and Gas Survey China Geological SurveyMinistry of Natural ResourcesBeijing 100083China Information Center Ministry of Natural ResourcesBeijing 100036China Qingdao Institute of Marine Geology China Geological SurveyQingdao 266237China School of Earth and Space Sciences Peking UniversityBeijing 100871China

Global warming and the response to it have become a topic of concern in today’s society and are also a research focus in the global scientific community.As the world’s third pole,the global warming amplifier,and the starting region of China’s climate change,the Qinghai-Tibet Plateau is extremely sensitive to climate change.The permafrost on the Qinghai-Tibet Plateau is rich in natural gas hydrates(NGHs)resources.Under the background of global warming,whether the NGHs will be disassociated and enter the atmosphere as the air temperature rises has become a major concern of both the public and the scientific community.Given this,this study reviewed the trend of global warming and accordingly summarized the characteristics of the temperature increase in the Qinghai-Tibet Plateau.Based on this as well as the distribution characteristics of the NGHs in the permafrost on the Qinghai-Tibet Plateau,this study investigated the changes in the response of the NGHs to global warming,aiming to clarify the impacts of global warming on the NGHs in the permafrost of the plateau.A noticeable response to global warming has been observed in the Qinghai-Tibet Plateau.Over the past decades,the increase in the mean annual air temperature of the plateau was increasingly high and more recently.Specifically,the mean annual air temperature of the plateau changed at a rate of approximately 0.308-0.420℃/10a and increased by approximately 1.54-2.10℃in the past decades.Moreover,the annual mean ground temperature of the shallow permafrost on the plateau increased by approximately 1.155-1.575℃and the permafrost area decreased by approximately 0.34×10^(6)km^(2) from about 1.4×10^(6)km^(2) to 1.06×10^(6)km^(2) in the past decades.As indicated by simulated calculation results,the thickness of the NGH-bearing permafrost on the Qinghai-Tibet Plateau has decreased by 29-39 m in the past 50 years,with the equivalent of(1.69-2.27)×10^(10)-(1.12-1.51)×10^(12)m^(3) of methane(CH_(4))being released due to NGHs dissociation.It is predicted that the thicknes

关键词： Climate change Global warming Permafrost Gas hydrate Greenhouse effect Carbon emission Peak carbon dioxide emissions Carbon neutrality Qinghai-Tibet Plateau Environment geological survey engineering China

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Distributed optical fiber acoustic sensor for in situ monitoring of marine natural gas hydrates production for the first time in the Shenhu Area,China

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China Geology 2022年第2期5卷 322-329页

作者： Xiang-ge He Xue-min Wu Lei Wang Qian-yong Liang Li-juan Gu Fei Liu hai-long lu Yi Zhang Min Zhang Beijing International Center for Gas Hydrate Peking UniversityBeijing 100871China Guangzhou Marine Geological Survey China Geological SurveyMinistry of Natural ResourcesGuangzhou 510075China School of Earth and Space Sciences Peking UniversityBeijing 100871China Dongguan Institute of Optics and Electronics Peking UniversityDongguan 523000China Southern Marine Science and Engineering Guangdong Laboratory(Guangzhou) Guangzhou 511458China School of Computer and Communication Engineering University of Science and Technology BeijingBeijing 100083China SinoProbe Center Chinese Academy of Geological Sciences and China Geological SurveyMinistry of Natural ResourcesBeijing 100037China

The distributed acoustic sensor(DAS)uses a single optical cable as the sensing unit,which can capture the acoustic and vibration signals along the optical cable in real-time.So it is suitable for monitoring downhole production activities in the process of oil and gas development.The authors applied the DAS system in a gas production well in the South China Sea for in situ monitoring of the whole wellbore for the first time and obtained the distributed acoustic signals along the whole wellbore.These signals can clearly distinguish the vertical section,curve section,and horizontal production section.The collected acoustic signal with the frequency of approximately 50 Hz caused by the electric submersible pump exhibit a signal-to-noise ratio higher than 27 dB.By analyzing the acoustic signals in the production section,it can be located the layers with high gas production rates.Once an accurate physical model is built in the future,the gas production profile will be obtained.In addition,the DAS system can track the trajectory of downhole tools in the wellbore to guide the operation.Through the velocity analysis of the typical signals,the type of fluids in the wellbore can be distinguished.The successful application of the system provides a promising whole wellbore acoustic monitoring tool for the production of marine gas hydrate,with a good application prospect.

关键词： Gas hydrate production monitoring Optical fiber sensor Distributed acoustic sensor In situ monitoring Fluid type NGHs exploration trial engineering Oil and gas exploration engineering Shenhu Area South China Sea

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Sediment permeability change on natural gas hydrate dissociation induced by depressurization

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China Geology 2020年第2期3卷 221-229页

作者： Lei Wang Li-juan Gu hai-long lu Beijing International Center for Gas Hydrate Peking UniversityBeijing 100871China Department of Energy and Resources Engineering College of EngineeringPeking UniversityBeijing 100871China

The permeability of a natural gas hydrate reservoir is a critical parameter associated with gas hydrate production.Upon producing gas from a hydrate reservoir via depressurization,the permeability of sediments changes in two ways with hydrate dissociation,increasing with more pore space released from hydrate and decreasing due to pore compression by stronger effective stress related to depressurization.In order to study the evolution of sediment permeability during the production process with the depressurization method,an improved pore network model(PNM)method is developed to establish the permeability change model.In this model,permeability change induced by hydrate dissociation is investigated under hydrate occurrence morphology of pore filling and grain coating.The results obtained show that hydrate occurrence in sediment pore is with significant influence on permeability change.Within a reasonable degree of pore compression in field trial,the effect of pore space release on the reservoir permeability is greater than that of pore compression.The permeability of hydrate containing sediments keeps increasing in the course of gas production,no matter with what hydrate occurrence in sediment pore.

关键词： Natural gas hydrate Reservoir sediment Permeability Pore network model Depressurization Oil gas exploration engineering South China Sea China

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Coexistence of natural gas hydrate,free gas and water in the gas hydrate system in the Shenhu Area,South China Sea

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China Geology 2020年第2期3卷 210-220页

作者： Xu-wen Qin Jing-an lu hai-long lu hai-jun Qiu Jin-qiang Liang Dong-ju Kang Lin-sen Zhan Hong-feng lu Zeng-gui Kuang China Geological Survey Ministry of Natural ResourcesBeijing 100037China Guangzhou Marine Geological Survey China Geological SurveyMinistry of Natural ResourcesGuangzhou 510075China Beijing International Center for Gas Hydrate Peking UniversityBeijing 100871China Southern Marine Science and Engineering Guangdong Laboratory(Guangzhou) Guangzhou 510000China

Shenhu Area is located in the Baiyun Sag of Pearl River Mouth Basin,which is on the northern continental slope of the South China Sea.Gas hydrates in this area have been intensively investigated,achieving a wide coverage of the three-dimensional seismic survey,a large number of boreholes,and detailed data of the seismic survey,logging,and core analysis.In the beginning of 2020,China has successfully conducted the second offshore production test of gas hydrates in this area.In this paper,studies were made on the structure of the hydrate system for the production test,based on detailed logging data and core analysis of this area.As to the results of nuclear magnetic resonance(NMR)logging and sonic logging of Well GMGS6-SH02 drilled during the GMGS6 Expedition,the hydrate system on which the production well located can be divided into three layers:(1)207.8–253.4 mbsf,45.6 m thick,gas hydrate layer,with gas hydrate saturation of 0–54.5%(31%av.);(2)253.4–278 mbsf,24.6 m thick,mixing layer consisting of gas hydrates,free gas,and water,with gas hydrate saturation of 0–22%(10%av.)and free gas saturation of 0–32%(13%av.);(3)278–297 mbsf,19 m thick,with free gas saturation of less than 7%.Moreover,the pore water freshening identified in the sediment cores,taken from the depth below the theoretically calculated base of methane hydrate stability zone,indicates the occurrence of gas hydrate.All these data reveal that gas hydrates,free gas,and water coexist in the mixing layer from different aspects.

关键词： Mixing layer Gas hydrate NMR logging Sonic logging Core analysis Oil gas exploration engineering Shenhu Area South China Sea China

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Preliminary results of environmental monitoring of the natural gas hydrate production test in the South China Sea

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China Geology 2018年第2期1卷 202-209页

作者： Jian-liang Ye Xu-wen Qin hai-jun Qiu Qian-yong Liang Yi-fei Dong Jian-gong Wei hai-long lu Jing-an lu Yao-hong Shi Chao Zhong Zhen Xia Guangzhou Marine Geological Survey China Geological SurveyGuangzhou 510075China Gas Hydrate Engineering Technology Center China Geologtcal SurveyGuangzhou 510075China College of Engineering Peking UniversityBeijing 100871China

Natural gas hydrate (NGH)is considered as one of the new clean energy sources of the 21st century with the highest potential.The environmental issues of NGH production have attracted the close attention of scientists in various countries.From May 10 to July 9,2017,the first offshore NGH production test in the South China Sea (SCS)was conducted by the China Geological Survey.In addition,environmental security has also been effectively guaranteed via a comprehensive environmental monitoring system built during the NGH production test.The monitoring system considered sea-surface atmosphere methane and carbon dioxide concentrations,dissolved methane in the sea water column,and the seafloor physical oceanography and marine chemistry environment.The whole process was monitored via multiple means, in multiple layers,in all domains,and in real time.After the production test,an environmental investigation was promptly conducted to evaluate the environmental impact of the NGH production test. The monitoring results showed that the dissolved methane concentration in seawater and the near-seabed environment characteristics after the test were consistent with the background values,indicating that the NGH production test did not cause environmental problems such as methane leakage.

关键词： South China Sea Natural gas hydrate Production test Methane leakage Environmental momtoring

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The first offshore natural gas hydrate production test in South China Sea

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China Geology 2018年第1期1卷 5-16页

作者： Jin-fa Li Jian-liang Ye Xu-wen Qin hai-jun Qiu Neng-you Wu hai-long lu Wen-wei Xie Jing-an lu Fei Peng Zhen-qiang Xu Cheng lu Zeng-gui Kuang Jian-gong Wei Qian-yong Liang Hong-feng lu Bei-bei Kou China Geological Survey Beijing 100037China Guangzhou Marine Geologtcal Survey China Geologtcal SurveyGuangzhou 510075China Qingdao Institute of Marine Geology China Geological SurveyQingdao 266071China Peking University Beijing 100871China Institute of Exploration Techmques China Academy of Geological SciencesLangfang 065000China CNPC Offshore Engineering Company Ltd Beijing 100102China Center of Oil & Natural Gas Resource Exploration China Geological SurveyBeijing 100083China

Natural gas hydrates (NGH)is one of key future clean energy resources.Its industrialized development will help remit the huge demand of global natural gas,relieve the increasing pressure of the environment, and play a vital role in the green sustainable growth of human societies.Based on nearly two decades' studying on the reservoir characteristics in the South China Sea (SCS)and the knowledge of reservoir system,the China Geological Survey (CGS)conducted the first production test on an optimal target selected in Shenhu area SCS in 2017.Guided by the "three-phase control"exploitation theory which focused on formation stabilization,technologies such as formation fluid extraction,well drilling and completing, reservoir stimulating,sand controlling,environmental monitoring,monitoring and preventing of secondary formation of hydrates were applied.The test lasted for 60 days from May 10^th when starting to pump, drop pressure and ignite to well killing on July 9^th,with gas production of 3.09×10^5 m^3 in total,which is a world record with the longest continuous duration of gas production and maximal gas yield.This successful test brings a significant breakthrough on safety control of NGH production.

关键词： Natural gas hydrate (NGH) Production test Shenhu area South Chma Sea (SCS)

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The second natural gas hydrate production test in the South China Sea

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China Geology 2020年第2期3卷 197-209页

作者： Jian-liang Ye Xu-wen Qin Wen-wei Xie hai-long lu Bao-jin Ma hai-jun Qiu Jin-qiang Liang Jing-an lu Zeng-gui Kuang Cheng lu Qian-yong Liang Shi-peng Wei Yan-jiang Yu Chunsheng Liu Bin Li Kai-xiang Shen Hao-xian Shi Qiu-ping lu Jing Li Bei-bei Kou Gang Song Bo Li He-en Zhang Hong-feng lu Chao Ma Yi-fei Dong Hang Bian China Geological Survey Ministry of Natural ResourcesBeijing 100037China Guangzhou Marine Geological Survey China Geological SurveyMinistry of Natural ResourcesGuangzhou 510075China Institute of Exploration Techniques China Geological SurveyMinistry of Natural ResourcesLangfang 065000China Peking University Beijing 100871China CNPC Offshore Engineering Company Limited Beijing 100102China Oil and Gas Resources Survey China Geological SurveyMinistry of Natural ResourcesBeijing 100083China Southern Marine Science and Engineering Guangdong Laboratory(Guangzhou) Guangzhou 510000China

Clayey silt reservoirs bearing natural gas hydrates(NGH)are considered to be the hydrate-bearing reservoirs that boast the highest reserves but tend to be the most difficult to exploit.They are proved to be exploitable by the first NGH production test conducted in the South China Sea in 2017.Based on the understanding of the first production test,the China Geological Survey determined the optimal target NGH reservoirs for production test and conducted a detailed assessment,numerical and experimental simulation,and onshore testing of the reservoirs.After that,it conducted the second offshore NGH production test in 1225 m deep Shenhu Area,South China Sea(also referred to as the second production test)from October 2019 to April 2020.During the second production test,a series of technical challenges of drilling horizontal wells in shallow soft strata in deep sea were met,including wellhead stability,directional drilling of a horizontal well,reservoir stimulation and sand control,and accurate depressurization.As a result,30 days of continuous gas production was achieved,with a cumulative gas production of 86.14×104 m3.Thus,the average daily gas production is 2.87×10^4 m^3,which is 5.57 times as much as that obtained in the first production test.Therefore,both the cumulative gas production and the daily gas production were highly improved compared to the first production test.As indicated by the monitoring results of the second production test,there was no anomaly in methane content in the seafloor,seawater,and atmosphere throughout the whole production test.This successful production test further indicates that safe and effective NGH exploitation is feasible in clayey silt NGH reservoirs.The industrialization of hydrates consists of five stages in general,namely theoretical research and simulation experiments,exploratory production test,experimental production test,productive production test,and commercial production.The second production test serves as an important step from the exploratory production test to experim

关键词： Natural gas hydrates Second production test Horizontal well Reservoir stimulation Environmental impact NGH exploration trial engineering South China Sea

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Comprehensive study on the spatial distribution of heavy metals and their environmental risks in high-sulfur coal gangue dumps in China

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Journal of Environmental Sciences 2024年第2期136卷 486-497页

作者： Yingbo Dong Huan lu hai Lin School of Energy and Environmental Engineering University of Science and Technology BeijingBeijing 100083China Beijing Key Laboratory on Resource-oriented Treatment of Industrial Pollutants Beijing 100083China

The accumulation of coal gangue(CG)from coal mining is an important source of heavy metals(HMs)in soil.Its spatial distribution and environment risk assessment are extremely important for the management and remediation of HMs.Eighty soil samples were collected from the high-sulfur CG site in northern China and analyzed for six HMs.The results showed that the soil was heavily contaminated by Mn,Cr and Ni based on the Nemerow index,and posed seriously ecological risk depended on the geo-accumulation index,potential ecological risk index and risk assessment code.The semi-variogram model and ordinary kriging interpolation accurately portrayed the spatial distribution of HMs.Fe,Mn,and Cr were distributed by band diffusion,Ni was distributed by core,the distribution of Cu had obvious patchiness and Zn was more uniform.The spatial autocorrelation indicated that all HMs had strong spatial heterogeneity.The BCR sequential extraction was employed to qualify the geochemical fractions of HMs.The data indicated that Fe and Cr were dominated by residual fraction;Cu,Ni and Zn were dominated by reducible and oxidizable fractions;Mn was dominated by reducible and acid-extractable(25.38%-44.67%)fractions.Pearson correlation analysis showed that pH was the main control factor affecting the non-residue fractions of HMs.Therefore,acid production from high sulfur CG reduced soil pH by 2-3,which indirectly promoted the activity of HMs.Finally,the conceptual model of HMs contamination at the CG site was proposed,which can be useful for the development of ecological remediation strategies.

关键词： High-sulfur coal gangue Soil contamination Heavy metals Spatial distribution Geochemical fractions Risk assessment

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Constructing S-scheme charge separation in cobalt phthalocyanine/oxygen-doped g-C_(3)N_(4) heterojunction with enhanced photothermal-assisted photocatalytic H_(2) evolution

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Rare Metals 2024年第1期43卷 198-211页

作者： Wei-long Shi Zheng Xu Yu-Xing Shi Ling-Ling Li Jia-Lin lu Xin-hai Sun Xin Du Feng Guo Chang-Yu lu School of Material Science and Engineering Jiangsu University of Science and TechnologyZhenjiang 212003China School of Energy and Power Jiangsu University of Science and TechnologyZhenjiang 212003JiangsuChina College of Chemistry Zhengzhou UniversityZhengzhou 450001China School of Water Resource and Environment Hebei Province Key Laboratory of Sustained Utilization and Development of Water RecourseHebei Center for Ecological and Environmental Geology ResearchHebei Geo UniversityShijiazhuang 050031China

Hydrogen acquisition from solar energy is an effective way to address energy crisis,which makes the development of efficient photocatalysts become the main direction of scientific research.Herein,cobalt phthalocyanine/oxygen-doped g-C_(3)N_(4)(CoPc/OCN) S-scheme heterojunction photocatalyst was designed by coupling multi-step calcination with solvothermal method for enhanced photothermal-assisted photocatalytic H_(2) evolution.The multistep calcined g-C_(3)N_(4) is easier for O-doping formation,and the ethanol solvothermal strategy is utilized to enhance the dispersion of CoPc on OCN nano sheet surface and forms sufficient S-scheme heterojunction through H-bonds.In addition,the active sites and excellent photothermal properties of CoPc itself further improve the integrated photocatalytic activity of CoPc/OCN S-scheme heterojunction.The optimal photocatalytic hydrogen evolution rate of CoPc/OCN S-scheme heterojunction photocatalyst reached 9.56 mmol·g^(-1)·h^(-1),which is 2.69 and 1.23 times higher than that of CN and OCN,respectively.This work provides a valuable design idea and scheme for enhancing the multi-factor co-assisted photocatalytic H_(2) evolution performance.

关键词： Photothermal Photocatalytic H_(2)evolution Cobalt phthalocyanine Oxygen-doped g-C_(3)N_(4) Sscheme heterojunction

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Layer Hall effect induced by hidden Berry curvature in antiferromagnetic insulators

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National Science Review 2024年第2期11卷 15-23页

作者： Rui Chen hai-Peng Sun Mingqiang Gu Chun-Bo Hua Qihang Liu hai-Zhou lu X.C.Xie Shenzhen Institute for Quantum Science and Engineering and Department of Physics Southern University of Science and Technology(SUSTech) International Quantum Academy Institute for Theoretical Physics and Astrophysics University of Würzburg School of Electronic and Information Engineering Hubei University of Science and Technology Guangdong Provincial Key Laboratory of Computational Science and Material Design Southern University of Science and Technology Shenzhen Key Laboratory of Quantum Science and Engineering International Center for Quantum Materials School of PhysicsPeking University Collaborative Innovation Center of Quantum Matter CAS Center for Excellence in Topological Quantum Computation University of Chinese Academy of Sciences

The layer Hall effect describes electrons spontaneously deflected to opposite sides at different layers, which has been experimentally reported in the MnBi2Te4thin films under perpendicular electric fields. Here, we reveal a universal origin of the layer Hall effect in terms of the so-called hidden Berry curvature, as well as material design principles. Hence, it gives rise to zero Berry curvature in momentum space but non-zero layer-locked hidden Berry curvature in real space. We show that, compared to that of a trivial insulator, the layer Hall effect is significantly enhanced in antiferromagnetic topological insulators. Our universal picture provides a paradigm for revealing the hidden physics as a result of the interplay between the global and local symmetries, and can be generalized in various scenarios.

关键词： layerHall effect hidden Berry curvature antiferromagnetic insulator axion insulator, quantum transport

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