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A surface engineering strategy for the stabilization of zinc metal anodes with montmorillonite layers toward long-life rechargeable aqueous zinc ion batteries

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Journal of Energy Chemistry 2025年第1期100卷 94-105页

作者： Wenbo Wang Ruifeng Xu Xu Zhang Peiyu Wang Bao Yang Bingjun Yang Juan Yang Kailimai su Pengjun Ma Yanan Deng Xianfeng Fan Wanjun Chen Key Laboratory for Electronic Materials College of Electrical Engineering Northwest Minzu University Resource Chemistry and Energy Materials Research Center State Key Laboratory of Solid Lubrication Lanzhou Institute of Chemical Physics Chinese Academy of Sciences University of Chinese Academy of Sciences Institute for Materials and Processes School of Engineering University of Edinburgh

Rechargeable aqueous zinc-ion batteries （AZIBs） exhibit appreciable potential in the domain of electrochemical energy ***,there are serious challenges for AZIBs,for instance zinc dendrite growth,hydrogen evolution reaction （HER）,and corrosion side ***,we propose a surface engineering modification strategy for coating the montmorillonite （MMT） layer onto the surface of the Zn anode to tackle these issues,thereby achieving high cycling stability for rechargeable *** results reveal that the MMT layer on the surface of the Zn anode is able to provide ordered zincophilic channels for zinc ions migration,facilitating the reaction kinetics of zinc *** functional theory（DFT） calculations and water contact angle （CA） tests prove that MMT@Zn anode exhibits superior adsorption capacity for Zn2+and better hydrophobicity than the bare Zn anode,thereby achieving excellent cycling ***,the MMT@Zn||MMT@Zn symmetric cell holds the stable cycling over 5600 h at 0.5 mA cm-2and 0.125 m A h cm-2,even exceeding 1800 h long cycling under harsh conditions of 5 m A cm-2and 1.25 m A h *** MMT@Zn||V2O5full cell reaches over 3000 cycles at 2 A g-1with excellent rate ***,this surface engineering modification strategy for enhancing the electrochemical performance of AZIBs represents a promising application.

关键词： Hydrogen evolution reaction

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Holographic Dark Energy Model is Consistent with Pantheon SN Ia Data

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Communications in Theoretical Physics 2019年第4期71卷 421-426页

作者： Xin Li su-Ping Zhao Li Tang hai-Nan lin Department of Physics Chongqing University

We constrain three cosmological models,i.e.,ACDM model, holographic dark energy(HDE) model and R_h = ct model by using the recent Pantheon compilation of type la supernovae(SN la), the direction measurements of Hubble parameter H(z), and the baryon acoustic oscillations(BAO). The spatial curvature is considered in the ACDM model and the HDE model. We show that the HDE model in a spatially flat and HDE dominate universe has the same behavior as Rh = ct model if the characteristic parameter of the HDE model C_0 approaches to infinity. Numerical results show that the ACDM model is the best favoured one among the three models. The HDE model is consistent with observational data, the best fitting value of C_0 is around 0.8, which implies that the Rh = ct model should be modified to be compatible with the present cosmological observational data. Combing all the datasets, we give strict constraint on the Hubble constant,where h_0=0.694 ± 0.020 for the ACDM model and h_0= 0.689 ±0.019 for the HDE *** results imply that the tension of Hubble constant between Planck collaborations and Riess et al. has been partially relaxed. The constraint on the spatial curvature is also given,where Ω_(k0) =-0.066 ± 0.165 for the ACDM model andΩ_(k0)=0.029 ± 0.067 for the HDE model.

关键词： holographic dark energy cosmological observations supernova general

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Quantum Fidelity and Thermal Phase Transitions in a Two-Dimensional Spin System

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Chinese Physics Letters 2012年第12期29卷 9-12页

作者： WANG Bo HUANG hai-lin suN Zhao-Yu KOU su-Peng Department of Physics Beijing Normal UniversityBeijing 100875 School of Electrical and Electronic Engineering Wuhan Polytechnic UniversityWuhan 430000

We investigate the ability of quantum fidelity in detecting the classical phase transitions(CPTs)in a two-dimensional Heisenberg-Ising mixed spin model,which has a very rich phase diagram and is exactly *** a two-site subsystem of the model,the reduced fidelity(including the operator fidelity and the fidelity susceptibility)at finite temperatures is calculated,and it is found that an extreme value presents at the critical temperature,thus shows a signal for the *** some parameter region,the signal becomes *** propose to use the"normalized fidelity susceptibility"to solve this problem.

关键词： susceptibility Transition extreme

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Probing the universality of acceleration scale in modified Newtonian dynamics with SPARC galaxies

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Chinese Physics C 2021年第2期45卷 598-605页

作者： Xin Li su-Ping Zhao hai-Nan lin Yong Zhou Department of Physics Chongqing UniversityChongqing 401331China CAS Key Laboratory of Theoretical Physics Institute of Theoretical PhysicsChinese Academy of SciencesBeijing 100190China

We probe the universality of acceleration scale a_(0) in Milgrom's modified Newtonian dynamics(MOND)using the recently released rotation curve data from SPARC *** divide the SPARC data into different subsamples according to the morphological types of galaxies,and fit the rotation curve data of each subsample with the theoretical prediction of *** involves an arbitrary interpolation function which connects the Newtonian region and the MOND *** we consider five different interpolation functions that are widely discussed in the *** is shown that the best-fitting a_(0) significantly depends on the interpolation *** a specific interpolation function, a_(0) also depends on the morphological types of galaxies,implying that a_(0) may be not a universal *** a dipole correction to a_(0) can significantly improve the *** dipole directions for four of the five interpolation functions point towards an approximately consistent direction,but a_(0) still varies for different interpolation functions.

关键词： kinematics and dynamics dark matter modified Newtonian dynamics

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PRECISE SYNTHESIS OF OLEFIN BLOCK COPOLYMERS USING A SYNDIOSPECIFIC LIVING POLYMERIZATION SYSTEM

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Chinese Journal of Polymer Science 2013年第4期31卷 541-549页

作者：蔡正国 hai-hui su Takeshi Shiono State Key Lab for Modification of Chemical Fibers and Polymer Materials College of Material Science and EngineeringDonghua University Graduate School of Engineering Hiroshima University

This feature article summarizes the synthesis of novel olefin block copolymers using fast syndiospecific living homo- and copolymerization of propylene, higher 1-alkene, and norbornene with ansa-fluorenylamidodimethyltitanium- based catalyst according to the authors＇ recent results. The catalytic synthesis of monodisperse polyolefin and olefin block copolymer was also described using this living system.

关键词： Single-site catalyst Propylene Norbomene Living polymerization Block copolymer.

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Sniffing with mass spectrometry

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Science Bulletin 2018年第20期63卷 1351-1357页

作者： Miao-Miao Chen hai-Feng su Ying Xie Li-Fang He Shui-Chao lin Mei-lin Zhang Cheng Wang su-Yuan Xie Rong-Bin Huang Lan-sun Zheng State Key Laboratory for Physical Chemistry of Solid surfaces Collaborative Innovation Center of Chemistry for Energy Materials Department of Chemistry College of Chemistry and Chemical Engineering Xiamen University School of Information Science and Engineering Xiamen University

Gaseous compounds are usually on-line detectable on sensors. The limitations of conventional sensors are suffering from incapability for exactly identifying multiple components as well as incompatibility to possible toxicants in every odor sample. Herein, we discuss an inlet modification to the laboratory standard mass spectrometer, inspired by the sensitive olfactory systems of animals, for direct sniffing,established by connecting a mini pump to the nebulizer gas tubing. The modified mass spectrometry method—sniffing-mass spectrometry(sniffing-MS)—can acquire detailed fingerprint spectra of mixed odors and shows high tolerance to toxicants. Furthermore, the method has a low limit of detection in the order of parts per trillion and is a ‘sampling-free' technique for analyzing various gaseous compounds simultaneously, thus offering versatility for smelling daily commodities, tracking diffusion, and locating position of odors. Sniffing-MS can mimic or even surpass the olfaction of animals and is applicable for analyzing gaseous/volatile compounds, especially those polar compounds, in a simple manner depending on the intrinsic molecular mass-to-charge ratio.

关键词： Ambient mass spectrometry Volatile compounds Gas source locating On-line monitoring Olfaction

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The Singularly Perturbed Problem of Vector Integro-differential Equations

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Acta Mathematicae Applicatae Sinica 2010年第2期26卷 267-276页

作者： su-rong lin Department of Computer Fujian Broadcasting TV University Fuzhou 350003 China

The singularly perturbed boundary value problem of scalar integro-differential equations has been studied extensively by the differential inequality method . However, it does not seem possible to carry this method over to a corresponding nonlinear vector integro-differential equation. Therefore , for n-dimensional vector integro-differential equations the problem has not been solved fully. Here, we study this nonlinear vector problem and obtain some results. The approach in this paper is to transform the appropriate integro-differential equations into a canonical or diagonalized system of two first-order equations.

关键词： Integro-differential equation singular perturbation boundary value problem diagonalization method

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πN Elastic Scattering and Resonances in Quark Potential Model

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Communications in Theoretical Physics 2008年第4期49卷 987-992页

作者： WANG hai-Jun su Jun-Chen Center for Theoretical Physics Jilin University Changchun 130023 China

The quark potential model is used to investigate the low-energy elastic scattering of πN system. The model potential consists of the t-channel and s-channel one-gluon exchange potentials and the harmonic oscillator confining potential. By means of the resonating group method, a nonlocal effective potential for the πN system is derived from the interquark potentials and used to calculate the πN elastic scattering phase shifts. By considering the effect of QCD renormalization, the suppression of the spin-orbital coupling and the contribution of the color octet of the clusters （qq） and （qqq）, the numerical results are in fairly good agreement with the experimental data. The same model and method are employed to investigate the possible πN resonances. For this purpose, the resonating group equation is transformed into a standard Schrodinger equation in which the nonlocal effective πN interaction potential is included. Solving the Schrodinger equation by the variational method, we are able to reproduce the masses of some currently concerned πN resonances.

关键词： quark potential model pion-baryon interactions pion elastic scattering

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RNA-based nanomedicines and their clinical applications

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Nano Research 2023年第12期16卷 13182-13204页

作者： lin-Jia su Zi-Han Ji Mo-Xi Xu Jia-Qing Zhu Yi-hai Chen Jun-Fei Qiao Yi Wang Yao-Xin lin CAS Key Laboratory for Biomedical Effects of Nanomaterials and Nanosafety National Center for Nanoscience and Technology(NCNST)Beijing 100190China University of Chinese Academy of Sciences(UCAS) Beijing 100149China Department of Breast surgery Harbin Medical University Cancer HospitalHarbin 150081China School of Chemical and Environmental Engineering Wuhan Polytechnic UniversityWuhan 430023China Institute of Bioengineering and Institute of Materials Science&Engineering École Polytechnique Fédérale de Lausanne(EPFL)Lausanne1015Switzerland

RNA-based nanomedicines encompass a range of therapeutic approaches that utilize RNA molecules or molecules that target RNAs for the treatment or prevention of *** include antisense oligonucleotides(ASOs),small interfering RNAs(siRNAs),endogenous microRNAs(miRNAs),messenger RNAs(mRNAs),clustered regularly interspersed short palindromic repeats-associated protein 9(CRISPR/Cas9),single guide RNAs(sgRNAs),as well as RNA *** therapeutic agents exert their effects through various mechanisms such as gene inhibition,addition,replacement,and *** advancement of RNA biology and the field of RNA therapy has paved the way for the development and utilization of RNA-based nanomedicine in human *** remarkable example of RNA-based nanomedicine is the mRNA-based vaccines including mRNA-1273(Moderna)and BNT162b2(Pfizer/BioNTech)that have been successfully employed in response to the coronavirus disease 2019(COVID-19)*** review aims to highlight the advantages of RNA-based nanomedicines,provides an overview of significant developments in delivery systems,elucidates the molecular mechanisms of action underlying RNA-based nanomedicines,and discusses their clinical ***,the review will address the existing challenges and innovations in delivery platforms while exploring the future possibilities for these promising RNA-based nanomedicines.

关键词： RNA-based nanomedicine conjugate-based delivery system nanoparticle-based delivery system clinical trial

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Refractory lipoatrophy treated with autologous whole blood injection:A case report

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World Journal of Clinical Cases 2025年第2期13卷 33-38页

作者： Wonnam Kim Jun su Park En Hyung Kim Department of Pharmacology School of Korean MedicinePusan National UniversityYangsan 50612GyeongnamSouth Korea Department of Dermatology College of MedicineChungbuk National UniversityCheongju 28644ChungbukSouth Korea Department of Dermatology Chungbuk National University HospitalCheongju 28644ChungbukSouth Korea

BACKGROUND Intramuscular corticosteroid injection may cause adverse effects such as dermal and/or subcutaneous atrophy,alopecia,hypopigmentation,and *** cutaneous atrophy can spontaneously resolve,several treatment options have been suggested for this *** suMMARY In this paper,we report a case of corticosteroid injection induced lipoatrophy treated with autologous whole blood(AWB)injection,as the condition had been unresponsive to fractional laser therapy.A 29-year-old female patient visited the dermatology clinic complaining of skin depression on her right buttock area,which had appeared six months *** had been only subtle improvement at the margins after fractional CO_(2) laser treatment;therefore,after obtaining informed consent from the patient,AWB treatment was *** month after the first AWB injection,the size and depth of the lesion had noticeably improved,and a slight improvement was also observed in *** Close observation is the initial treatment of choice for steroid induced skin atrophy;however,for patients in need of immediate cosmetic improvement,AWB injection may be a safe and cost-effective alternative.

关键词： Atrophy Corticosteroid subcutaneous fat Autologous whole blood injection Laser therapy Case report

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