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Nano Research 2024年第6期17卷 4943-4950页

作者： rui Li Xiayan Yan Meng Liu Qingkai Zhao Jie Du Xinxin Tan Jingwen ba.Rongguang Zeng Wenhua Luo Jingsong Xu Institute of Materials China Academy of Engineering PhysicsJiangyou 621907China Science and Technology on Surface Physics and Chemistry Laboratory Jiangyou 621908China

Top-down strategy has been widely applied for synthesis of metal single atom catalysts(SACs)via converting metal nanoparticles or bulk metals into atomically dispersed ***,we report a simple electrochemical atomic migration strategy for top-down synthesis of SACs via a facile cathodic corrosion process without involving high temperature or harsh *** of metal nanoparticles on cathode are firstly disba.ded under high negative voltage,and emitted into the electrolyte in the form of atomic metal anions in Zintl *** escaped atomically dispersed metal species are then oxidized by water molecules and captured by the defects on the pre-added nitrogen doped carbon carriers in the *** cathodic corrosion strategy is confirmed to be suitable for scalable synthesis of kinds of metal SACs(e.g.,Pt,Pd,and Ir)on doped carbon ***,the as-prepared nitrogen doped carbon powder supported Pt SACs exhibit superior catalytic activity toward hydrogen evolution reaction(HER)with a low overpotential of 0.024 V at 10 mA·cm^(−2)and a low Tafel slope of 29.7 mV·dec^(−1)as well as a long-term durability.

关键词： cathodic corrosion top-down strategy powdery single atom catalysts hydrogen evolution reaction scalable synthesis

Products of Commutator Ideals of Some Lie-admissible Algebras

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Acta Mathematica Sinica,English Series 2024年第8期40卷 1875-1892页

作者： Ivan KAYGORODOV Farukh MASHUROV Tran Giang NAM Ze rui ZhaNG CMA-UBI Universidade da Beira InteriorCovilhaPortugal Shenzhen International Center for Mathematics(SICM) Southern University of Science and TechnologyShenzhen 518055P.R.China Institute of Mathematics VAST18 Hoang Quoc VietCau GiayHanoiVietnam School of Mathematical Sciences South China Normal UniversityGuangzhou 510631P.R.China

In this article,we mainly study the products of commutator ideals of Lie-admissible algebras such as Novikov algebras,bicommutative algebras,and assosymmetric *** precisely,we first study the properties of the lower central chains for Novikov algebras and bicommutative *** we show that for every Lie nilpotent Novikov algebra or Lie nilpotent bicommutative algebra A,the ideal of A generated by the set{ab−ba.a,b∈A}is ***,we study properties of the lower central chains for assosymmetric algebras,study the products of commutator ideals of assosymmetric algebras and show that the products of commutator ideals have a similar property as that for associative algebras.

关键词： Novikov algebra bicommutative algebra assosymmetric algebra Lie nilpotent algebra

Is convenience really king? Comparative evaluation of catastrophic costs due to tuberculosis in the public and private healthcare sectors of Viet Nam: a longitudinal patient cost study

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贫困所致传染病(英文) 2024年第2期13卷 17-28页

作者： Nguyen Hoa Binh Quang Vo Luan Nguyen Forse Rachel Jeanette Wiemers Anja Maria Christine Huynh Huy ba.Dong Thuy Thi Thu Phan Yen Thi Hoang Creswell Jacob Dang Thi Minh ha Nguyen Lan Huu Shedrawy Jad L?nnroth Knut Nguyen Tuan Dinh Van Dinh Luong Annerstedt Kristi Sidney Codlin Andrew James National Lung Hospital Ha Noi Viet Nam Friends for International TB Relief Ha Noi Viet Nam Department of Globa. Public Health WHO Collaboration Centre On Tuberculosis and Social Medicine Karolinska Institute Stockholm Sweden Stop TB Partnership Geneva Switzerland Pham Ngoc Thach Hospital Ho Chi Minh City Viet Nam

ba.kground In Viet Nam, tuberculosis (TB) represents a devastating life-event with an exorbitant price tag, partly due to lost income from daily directly observed therapy in public sector care. Thus, persons with TB may seek care in the private sector for its flexibility, convenience, and privacy. Our study aimed to measure income changes, costs and catastrophic cost incurrence among TB-affected households in the public and private *** Between October 2020 and March 2022, we conducted 110 longitudinal patient cost interviews, among 50 patients privately treated for TB and 60 TB patients treated by the National TB Program (NTP) in ha Noi, hai Phong and Ho Chi Minh City, Viet Nam. Using a local adaptation of the WHO TB patient cost survey tool, participants were interviewed during the intensive phase, continuation phase and post-treatment. We compared income levels, direct and indirect treatment costs, catastrophic costs using Wilcoxon rank-sum and chi-squared tests and associated risk factors between the two cohorts using multivariate *** The pre-treatment median monthly household income was significantly higher in the private sector versus NTP cohort (USD 868 vs USD 578;P=0.010). However, private sector treatment was also significantly costlier (USD 2075 vs USD 1313;P=0.005), driven by direct medical costs which were 4.6 times higher than costs reported by NTP participants (USD 754 vs USD 164;P<0.001). This resulted in no significant difference in catastrophic costs between the two cohorts (Private: 55% vs NTP: 52%;P=0.675). Factors associated with catastrophic cost included being a single-person household [adjusted odds ratio [(aOR=13.71; 95% confidence interval (CI): 1.36–138.14;P=0.026], unemployment during treatment (aOR=10.86; 95%CI: 2.64–44.60;P<0.001) and experiencing TB-related stigma (aOR=37.90; 95%CI: 1.72–831.73;P=0.021).Conclusions Persons with TB in Viet Nam face similarly high risk of catastrophic costs whether treated in the

关键词： Tuberculosis Patient cost Catastrophic cost Private sector Comparative analysis Viet Nam

靶向泛素特异性蛋白酶1小分子抑制剂的研究进展

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药学学报 2024年第4期59卷 866-885页

作者：徐嘉浩李宏瑞把睿先刘同超熊兵江西中医药大学药学院江西南昌330004 沈阳药科大学辽宁沈阳110016 中国科学院上海药物研究所上海201203 长三角药物高等研究院江苏南通226133

泛素特异性蛋白酶1(ubiquitin-specific protease 1,USP1)是在癌症研究中越发受关注的去泛素化酶之一。USP1在许多肿瘤中过度表达,现已发现USP1能通过调控与肿瘤相关的多种蛋白质的表达来控制肿瘤的发生和进展,如SIK2、GSK-3β和Bcl-2... 详细信息

泛素特异性蛋白酶1(ubiquitin-specific protease 1,USP1)是在癌症研究中越发受关注的去泛素化酶之一。USP1在许多肿瘤中过度表达,现已发现USP1能通过调控与肿瘤相关的多种蛋白质的表达来控制肿瘤的发生和进展,如SIK2、GSK-3β和Bcl-2等。基因敲除或药物抑制USP1能有效抑制肿瘤,同时还有望解决顺铂以及聚腺苷二磷酸核糖聚合酶(poly ADP-ribose polymerase,PARP)抑制剂耐药性问题。本综述介绍了USP1的结构、功能以及USP1靶点与肿瘤的关系,并系统地总结2013年至2023年公开的USP1小分子抑制剂的结构、活性以及构效关系。最后,本综述讨论了开发USP1小分子抑制剂的挑战和机遇。

关键词：泛素特异性蛋白酶1 小分子抑制剂合成致死耐药性构效关系

Clinical efficacy of endovascular revascularization combined with vacuum-assisted closure for the treatment of diabetic foot

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World Journal of Diabetes 2024年第7期15卷 1499-1508页

作者： Feng-rui Lei Xiao-Fei Shen Chuang Zhang Xin-Qing Li hao Zhuang Hong-Fei Sang Department of Vascular Surgery The Second Affiliated Hospital of Soochow UniversitySuzhou 215004Jiangsu ProvinceChina

ba.KGROUND The diabetic foot is a common cause of disability and death,and comorbid foot infections usually lead to prolonged hospitalization,high healthcare costs,and a significant increase in amputation *** most diabetic foot trauma is complicated by lower extremity arteriopathy,which becomes an independent risk factor for major amputation in diabetic foot *** To establish the efficacy and safety of endovascular revascularization(ER)combined with vacuum-assisted closure(VAC)for the treatment of diabetic *** Clinical data were collected from 40 patients with diabetic foot admitted to the Second Affiliated Hospital of Soochow University from April 2018 to April *** foot lesions were graded according to Wagner’s classification,and blood flow to the lower extremity was evaluated using the ankle-brachial index test and computerized tomography angiography of the lower extremity *** subcutaneous insulin infusion pumps were used to achieve glycemic *** limb revascularization was facilitated by percutaneous transluminal ba.loon angioplasty(ba.or *** were cleaned by nibbling *** granulation tissue growth was induced by VAC,and wound repair was performed by skin grafting or skin flap *** Of the 35 cases treated with lower limb revascularization,34 were successful with a revascularization success rate of 97%.Of these,6 cases underwent stenting after ba.of the superficial femoral artery,and 1 received popliteal artery stent *** the 25 cases treated with infrapopliteal artery revascularization,39 arteries were reconstructed,7 of which were treated by drug-coated ba.and the remaining 32 with plain old *** was performed in 32 ***-four cases of skin grafting and 2 cases of skin flap transplantation were *** patients underwent major amputations,whereas 17 had minor amputations,accounting for a success limb salvage rate of 95%.CONCLUSION ER in

关键词： Diabetic foot Revascularization Vacuum-assisted closure ba.loon angioplasty Wound repair

Woody plant taxonomic,functional,and phylogenetic diversity decrease along elevational gradients in Andean tropical montane forests:Environmental filtering and arrival of temperate taxa

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Plant Diversity 2024年第4期46卷 491-501页

作者： Guillermo ba.ares-de-Dios Manuel J.Macía Gabriel Arellano Íñigo Granzow-de la Cerda Julia Vega-álvarez Itziar Arnelas Carlos I.Espinosa Norma Salinas Luis Cayuela Departamento de Biología y Geología Física y Química InorgánicaUniversidad Rey Juan CarlosCalle Tulipán s/nMóstolesMadridES-28933Spain Departamento de Biología Área de BotánicaUniversidad Autónoma de MadridCalle Darwin 2MadridES-28049Spain Centro de Investigación en Biodiversidad y Cambio Globa.(CIBC-UAM) Universidad Autónoma de MadridCalle Darwin 2MadridES-28049Spain Ecology and Evolutionary Biology University of MichiganAnn ArborMI 48109USA Oikobit LLC ***AlbuquerqueNM87120USA Real Jardín Botánico–CSIC Plaza Murillo 2MadridES-28014Spain Departamento de Biología Animal EcologíaParasitologíaEdafología y Química AgrícolaUniversidad de SalamancaCalle Donantes de Sangre s/nSalamancaES-37007Spain Departamento de Biodiversidad Ecología y EvoluciónUniversidad Complutense de MadridCalle JoséAntonio Nováis 12Ciudad UniversitariaES-28040Spain Departamento de Ciencias Biológicas y Agropecuarias Universidad Técnica Particular de LojaA.P.11-01-608 LojaEcuador Sección Química Pontificia Universidad Católica del PerúA.P.Lima 32LimaPeru ECI School of Geography and EnvironmentUniversity of OxfordOX13QYOxfordshireUnited Kingdom Instituto de Investigación en Cambio Globa.(IICG-URJC) Universidad Rey Juan CarlosCalle Tulipán s/nMóstolesMadridES-28933Spain

Mountains are paramount for exploring biodiversity patterns due to the mosaic of topographies and climates encompassed over short *** research has traditionally focused on taxonomic diversity when investigating changes along elevational gradients,but other facets should be *** first time,we simultaneously assessed elevational trends in taxonomic,functional,and phylogenetic diversity of woody plants in Andean tropical montane forests and explored their underlying ecological and evolutionary *** investigation covered four transects(traversing ca.2200 m a.s.l.) encompassing 114 plots of 0.1 ha across a broad latitudinal range(ca.10°).Using Hill numbers to quantify abundance-ba.ed diversity among 37,869 individuals we observed a consistent decrease in taxonomic,functional,and phylogenetic diversity as elevation increased,although the decrease was less pronounced for higher Hill *** exception was a slight increase in phylogenetic diversity when dominant species were *** decrease in taxonomic and functional diversity might be attributed to an environmental filtering process towards highlands,where the increasingly harsher conditions exclude species and functional ***,the differences in steepness decrease between Hill orders suggest that rare species disproportionately contribute to functional *** phylogenetic diversity the shifting elevational trend between Hill orders indicates a greater than previously considered influence in central Andean highlands of tropical lowlands originated species with strong niche conservatism relative to distantly related temperate *** could be explained by a decreasing presence and abundance of temperate,extratropical taxa towards the central Andes relative to northern or southern Andes,where they are more prevalent.

关键词： Altitudinal gradients Andes Environmentalﬁltering Out of the Tropical Lowlands Functional rarity Tropical Niche Conservatism

Pushing the high-k scalability limit with a superparaelectric gate layer

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Journal of Advanced Ceramics 2024年第4期13卷 539-547页

作者： Kun Wang Chao Liu Yuan Zhang Fuyu Lv Jun Ouyang Houbing Huang rui-Long Yang Yu-Yao Zhao Hongbo Cheng hanfei Zhu Xiaoming Shi Yun Tian Institute of Advanced Energy Materials and Chemistry Jinan Engineering Laboratory for Multi-scale Functional MaterialsSchool of Chemistry and Chemical EngineeringQilu University of Technology(Shandong Academy of Sciences)Jinan 250353China Key Laboratory for Liquid-Solid Structure Evolution and Processing of Materials(Ministry of Education) School of Materials Science and EngineeringShandong UniversityJinan 250061China China Toba.co Shandong Industrial Co. Ltd.Jinan 250104China Department of Materials Science and Engineering Southern University of Science and TechnologyShenzhen 518055China Key Laboratory of Key Film Materials&Application for Equipments(Hunan Province) School of Material Sciences and EngineeringXiangtan UniversityXiangtan 411105China Advanced Research Institute of Multidisciplinary Science and School of Materials Science and EngineeringBeijing Institute of TechnologyBeijing 100081China Key Laboratory of Magnetic Molecules and Magnetic Information Materials of Ministry of Education School of Chemistry and Materials ScienceShanxi Normal UniversityTaiyuan 030032China

To meet the expectation set by Moore’s law on transistors,the search for thickness-scalable high dielectric constant(k)gate layers has become an emergent research *** investigations have failed to solve the“polarizability–scalability–insulation robustness”*** this work,we show that this trilemma can be solved by using a gate layer of a high k ferroelectric oxide in its superparaelectric(SPE)*** the SPE,its polar order becomes local and is dispersed in an amorphous matrix with a crystalline size down to a few nanometers,leading to an excellent dimensional scalability and a good field-stability of the k *** an example,a stable high k value(37±3)is shown in ultrathin SPE films of(ba.(0.95),Sr_(0.05))(Zr_(0.2),Ti_(0.8))O_(3)deposited on LaNiO_(3)-buffered Pt/Ti/SiO_(2)/(100)Si down to a 4 nm thickness,leading to a small equivalent oxide thickness of~0.46 *** aforementioned characteristic microstructure endows the SPE film a high breakdown strength(~10.5 MV·cm^(−1)for the 4 nm film),and hence ensures a low leakage current for the operation of the complementary metal oxide semiconductor(CMOS)***,a high electrical fatigue resistance is displayed by the SPE *** results reveal a great potential of superparaelectric materials as gate dielectrics in the next-generation microelectronics.

关键词： high-k transistors Moore's law superparaelectric insulation robustness

西藏巴松错夏季浮游植物优势种生态位及其种间联结性

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水生态学杂志 2024年第2期45卷 111-120页

作者：刘洋安瑞志王陈潘成梅巴桑西藏大学地球第三极碳中和研究中心西藏拉萨850000 西藏大学生态环境学院青藏高原湿地与流域生态实验室西藏拉萨850000

为了解青藏高原高寒湖泊不同空间维度浮游植物群落优势种的生态位及种间联结性,选取青藏高原东南部最大的高寒冰山堰塞湖之一的巴松错为研究地点,2020年7月进行了浮游植物定性和定量采集,共采集水平和垂直维度浮游植物水样275个,结合生... 详细信息

为了解青藏高原高寒湖泊不同空间维度浮游植物群落优势种的生态位及种间联结性,选取青藏高原东南部最大的高寒冰山堰塞湖之一的巴松错为研究地点,2020年7月进行了浮游植物定性和定量采集,共采集水平和垂直维度浮游植物水样275个,结合生态位宽度、生态位重叠值、生态响应速率、总体联结性、χ^(2)检验、联结系数(AC)、共同出现百分比(PC)以及点相关系数(φ)等方法,分析优势种的生态位及种间联结性。结果显示:(1)共鉴定出浮游植物优势种5属8种,均属于硅藻门;(2)生态位宽度值差异较大,可分为3大生态位类群,水平维度对二维生态位宽度影响较明显;(3)在水平维度上,生态位重叠度达到有意义的种对比例较高,具有明显的同质性;在垂直和水平-垂直维度上,生态位重叠度达到有意义的种对比例较低,具有明显的异质性;(4)夏季浮游植物群落优势种生态响应速率在水平维度上形成正反馈,在垂直和水平-垂直维度上形成负反馈,表明巴松错夏季浮游植物群落存在多稳态,垂直和水平-垂直维度群落较水平维度更稳定;(5)夏季浮游植物群落总体处于演替初期,有正向演替趋势,物种间联结性不强,种间关系较为松散。研究结果为进一步研究高寒湖泊优势种生态位和群落多稳态提供了基础资料。

关键词：浮游植物优势种生态位种间联结巴松错

贵州紫皮百香果果腐病病原菌的鉴定及其与各发育阶段真菌微生物群落的关系

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湖南农业大学学报（自然科学版） 2024年第2期50卷 57-64页

作者：雷霁卿石银娜巴良杰吉宁王瑞贵阳学院食品科学与工程学院贵州贵阳550005

对分离自贵州紫皮百香果果腐病病原菌进行形态学及分子鉴定,确定致病菌15株,分属可可毛色二孢菌(Lasiodiplodia brasiliensis),层出镰孢菌(Fusarium proliferatum),间作壳菌(Diaporthe tectonendophytica、***、***、***);致病性观察显示,15株致病菌中包括弱致病力菌株1株、中致病力菌株4株、较强致病力菌株4株、强致病力菌株6株,***菌株BXG-Z-1及***菌株均为强致病力菌株。分析百香果不同发育阶段真菌微生物多样性,结果表明,百香果花、百香果幼果、百香果成熟果实真菌OTU数量分别为26、23、20,Simpson指数为0.095~0.113,真菌群落多样化程度低;Shannon指数均低于0.5,真菌微生物类群落分布均匀程度低,与之相对应的,Microdium spp.相对丰度在百香果不同发育阶段均超过90%;百香果花中Cladosporium spp.、ruinenia spp.相对丰度最高,幼果时降至最低,至成熟果实期又再次上升;百香果花中Trichoderma spp.、Bipolaris spp.、Amanita spp.、Monilinia spp.、Cercospora spp.相对丰度显著高于百香果幼果的,并随着果实发育成熟降至最低。

关键词：紫皮百香果病原菌微生物多样性贵州

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Brachiopods from the Silurian “Lower Red Beds” of Wuhan（E. Hubei， South China）: paleoecological and paleogeographical implications

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Journal of Earth Science 2024年

作者： Jia-Yi Yin Yi-Long Liu Lie-Bin Huang Yi-Ming Gong rui-Wen Zong School of Earth Sciences， China University of Geosciences Faculty of Land and Resources Engineering， Kunming University of Science and Technology State Key Laboratory of Biogeology and Environmental Geology， China University of Geosciences

The age and sedimentary environment of the Silurian “Lower Red Beds” (LRBs)， which occur widely in South China， have long been controversial because of the scarcity of index fossils. Recently， these beds have been dated by trilobites as middle-late Aeronian to early Telychian in age. Here， we report abundant brachiopods from the LRBs in Wuhan， Middle Yangtze Region， including atrypides (Meifodia hunanensis， Zygospiraella sp. 1， Zygospiraella sp. 2 and Nalivkinia? sp.)， spiriferides (Striispirifer acuminiplicatus， Striispirifer? sp.)， strophomenides (Eostropheodonta? sp. and Katastrophomena modesta)， and linguliformeans (Anomaloglossa? sp. and Orbiculoidea? sp.). Most of these are common in the Leijiatun， Xiangshuyuan， Shihniulan， Niuchang， Lojoping， and Shamao formations in the Upper Yangtze Region. The discovery of brachiopods from the LRBs in Wuhan not only enrich the biodiversity of the LRBs in the Yangtze Region， where Meifodia， Zygospiraella， Katastrophomena and Eostropheodonta are first found in the LRBs， but also expand the paleogeographical distribution of brachiopods to Middle-Lower Yangtze Region that first radiated after the end-Ordovician extinction. In addition， this brachiopod fauna also provides important implications for the sedimentary environment of LRBs during the Llandovery， which is usually developed in the nearshore shallow-water (ba.-2)， althought this paper extends to the deeper parts of the shallow-marine (ba.-4).

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