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Ag-decorated 3D flower-like Bi_(2)MoO_(6)/rGO with boosted photocatalytic performance for removal of organic pollutants

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Rare Metals 2021年第5期40卷 1086-1098页

作者： xin Liu Wei-ya huang Qin Zhou xi-Rong Chen Kai yang Dan Li Dionysios D.Dionysiou Faculty of Materials Metallurgical and ChemistryJiangxi University of Science and TechnologyGanzhou 341000China Environmental Engineering and Science Program Department of Chemical and Environmental EngineeringUniversity of CincinnatiCincinnatiOH 45221-0012USA College of Science HealthEngineering and EducationMurdoch UniversityMurdoch 6150Australia

A series of unique 3D flower-like Bi_(2)MoO_(6)(BMO)/reduced graphene oxide(rGO)heterostructured composites decorated with varying amounts of Ag nanoparticles(NPs)were *** morphological characteristics,structural features,energy band structures and photoelectrochemical properties were systematically *** the Ag/BMO/rGO ternary composites(AgBGy;y=1%,2%and 3%)demonstrated greater photocatalytic activity towards efficient removal of our selected organic models[methyl orange(MO),rhodamine B(RhB)and phenol],as compared with the BMO/rGO binary composites(BG-x;x=0.25,2,4 and 5).Particularly,AgBG-2%,which was synthesized with the addition of 2 wt% rGO and 2 wt%Ag in BMO,possessed superior photocatalytic *** fitted rate constants(k)for the photocatalytic degradation of RhB,MO and phenol using AgBG-2% were estimated to be 0.0286,0.0301 and 0.0165 min^(-1),respectively,which were over one order of magnitude greater than those obtained using pure *** factors may contribute to the observed enhancement,including greater specific surface area,enhanced light absorption,promoted spatial separation of electronhole(e^(-)-h^(+))pairs and their suppressed recombination,especially benefiting from the synergistic effects among BMO,rGO and Ag *** work suggests that the rational design of BMO/rGO/Ag ternary composite was an effective strategy to boost the photocatalytic activity of the resulting catalyst towards the highly efficient removal of organic pollutants from water.

关键词： Bi_(2)MoO_(6) Reduced graphene oxide Ag nanoparticles 3D flower-like morphology Photocatalytic degradation

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Separation of a C_(3)H_(6)/C_(2)H_(4) mixture using Pebax^(■) 2533/PEG600 blend membranes

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Chinese Journal of Chemical Engineering 2023年第2期54卷 192-198页

作者： xi Zhang xiaodong Wang Wei huang State Key Laboratory of Clean and Efficient Coal Utilization Taiyuan University of TechnologyTaiyuan 030024China Taiyuan Coal Conversion Technology Engineering Co. LtdTaiyuan 030024China

In industry, ethylene(C_(2)H_(4))/propylene(C_(3)H_(6)) separations are usually performed by a cryogenic process,which is energy intensive. Membrane separation technology is an alternative separation process that saves energy and is efficient. In this study, blend membranes were prepared by doping polyethylene glycol(PEG600) into a poly(ether-block-amide)(Pebax^(■) 2533) matrix and were used to separate the C_(2)H_(4)/C_(3)H_(6) mixture. The PEG 600 and Pebax^(■) 2533 polymers have good compatibility because they share hydrogen bonds. The addition of PEG600 is conducive to the hydrophilicity and the free volume of blend membranes, and it is also conducive to the solubility of C_(2)H_(4) and C_(3)H_(6) in the membranes, which improves the ability of the membranes to separate this gas pair. The Pebax^(■) 2533/PEG600 blend membrane with 15%(mass) PEG600 showed the highest separation performance in our investigated membranes, with a C_(3)H_(6)/C_(2)H_(4) selectivity of 8.9 and a C_(3)H_(6) permeability of 196 barrer(1 barrer = 1.33×10^(14)m^(3)(STP)·m·m^(-2)·s^(-1)·kPa^(-1)) at 238 K and 0.2 MPa, which is higher than that of the Pebax^(■) 2533/NaY-6%(mass) membrane(α_(C_(3)H_(6)/C_(2)H_(4)) =6.5, P_(C_(3)H_(6))=211 barrer) reported in our previous work. It is confirmed that incorporating PEG600 into the Pebax^(■) 2533 matrix to fabricate blend membranes is an efficient strategy for separating light olefins.

关键词： Ethylene/propylene separation Blend membranes Pebax^(■)2533 PEG600

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MODELING PHOTONIC CRYSTALS WITH COMPLEX UNIT CELLS BY DIRICHLET-TO-NEUMANN MAPS

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Journal of Computational Mathematics 2007年第3期25卷 337-349页

作者： Yuexia huang ya yan Lu Department of Mathematics City University of Hong KongKowloonHong KongChina

For a photonic crystal （PhC） of finite size, it is important to calculate its transmission and reflection spectra. For two-dimensional （2-D） PhCs composed of a square lattice of circular cylinders, the problem can be solved by an efficient method based on the Dirichlet-to-Neumann （DtN） map of the unit cell and a marching scheme using a pair of operators. In this paper, the DtN operator marching method is extended to handle 2-D PhCs with complex unit cells and arbitrary lattice structures.

关键词： Photonic crystal Periodic structure Diffractive grating Dirichlet-to-Neumannmap Operator marching.

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社区自然人群糖调节受损者5年转归及其影响因素

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中华糖尿病杂志 2010年第2期2卷 -页

作者：冯波钱巧慧李栩黄熙涯孟仲莹富明陈明慧同济大学附属东方医院内分泌科上海200120 上海市陆家嘴社区服务中心上海市潍坊社区服务中心上海市金杨社区服务中心上海市上钢社区服务中心

目的探讨糖调节受损人群发生糖尿病的危险性及其影响因素.方法 2002年6月至8月,采用抽样分层横断面现场调查方法于上海市浦东新区社区中检出192例糖调节受损者.2007年同期进行随访,观察单纯糖耐量受损、单纯空腹血糖受损、糖耐量受损... 详细信息

目的探讨糖调节受损人群发生糖尿病的危险性及其影响因素.方法 2002年6月至8月,采用抽样分层横断面现场调查方法于上海市浦东新区社区中检出192例糖调节受损者.2007年同期进行随访,观察单纯糖耐量受损、单纯空腹血糖受损、糖耐量受损合并空腹血糖受损、糖尿病人群比例,变化.使用t检验、方差分析、卡方检验进行统计学分析.结果 5年中死亡5例,存活的187例中79例发生糖尿病,糖尿病年转化率为8.4%(79/187/5年).基线单纯糖耐量受损者糖尿病年转化率为8.2%(47/114/5年),基线单纯空腹血糖受损者精尿病年转化率为6.3%(12/38/5年),基线糖耐量受损合并空腹血糖受损者糖尿病年转化率为11.4%(20/35/5年).正常糖耐量年转化率为6.3%(59/187/5年).单纯糖耐量受损者和糖耐量受损合并空腹血糖受损者发生糖尿病的风险分别是单纯空腹血糖受损者的1.4倍(95%可信区间为0.753～2.508,P=0.29)和107倍(95%可信区间为1.021～2.80,P=0.028).转化为糖尿病者较未转化为精尿病者高血压、肥胖的比例增高,基线年龄、体重指数、腰围、腰臀比和2 h血精明显升高,随访结束时体重指数和收缩压较基线时增高.结论上海市浦东新区糖耐量受损合并空腹血糖受损者糖尿病转化率最高.多种代谢异常可促进糖调节受损人群向糖球病转化.

关键词：糖调节受损糖尿病流行病学

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Role of biochar in raising blue carbon stock capacity of salt marshes

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Pedosphere 2024年第1期34卷 19-22页

作者： Yuzhou huang xi xiAO Ocean College Zhejiang UniversityZhoushan 316021China Key Laboratory of Marine Ecological Monitoring and Restoration Technologies of the Ministry of Natural Resources of China Shanghai 201306China Donghai Laboratory Zhoushan 316021China Ocean Academy Zhejiang UniversityZhoushan 316021China Key Laboratory of Watershed Non-point Source Pollution Control and Water Eco-security of Ministry of Water Resources College of Environmental and Resources SciencesZhejiang UniversityHangzhou 310058China

Salt marshes are an important blue carbon ecosystem, with surprisingly fast carbon accumulation rates that are 40 times higher than those of terrestrial forests. In recent decades, salt marshes have suffered great degradation and loss all over the world. The idea to enhance carbon stock in salt marshes(so-called blue carbon) using biochar (so-called black carbon) has recently been proposed. Although experiments and observations remain limited, significant enhancements in soil organic carbon and plant growth have been documented in most case studies. However, due to the limited number of observations and their relatively short time window ranging from months to less than one year, there still exists a knowledge gap regarding the process, mechanism, and effect of biochar in enhancing carbon stock in salt marshes. Future research is urgently needed in the following perspectives:1) exploring the relationship between carbon stock enhancement efficiency and biochar properties, 2) optimizing the physical and chemical properties of biochar to boost its efficiency, and 3)studying the in-situ responses of complex carbon pools to biochar addition, especially under tidal conditions and over a longer period of time.

关键词： soil stock char

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Theoretical and experimental study of surface texturing with laser machining

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Advances in Manufacturing 2021年第4期9卷 538-557页

作者： ya-Zhou Mao Jian-xi yang Jin-Chen Ji School of Mechatronics Engineering Henan University of Science and TechnologyLuoyang 471003HenanPeople’s Republic of China School of Mechanical and Mechatronic Engineering University of Technology SydneySydneyNSW 2007Australia

To explore the forming process and mechanism of the surface texture of laser micropits,this paper presents the thermal model of laser machining based on the Neumann boundary conditions and an investigation on the effects of various parameters on the *** surface profile and quality of the formed micropits were analyzed using NanoFocus 3D equipment through a design of experiment(DOE).The results showed that more intense melting and splashing occurred with higher power density and narrower pulse ***,the compressive stress is an important indicator of the damage effects,and the circumferential thermal stress is the primary factor influencing the diameter *** the process of laser machining,not only did oxides such as CuO and ZnO generate,the energy distribution also tended to decrease gradually from region#1 to region#3 based on an energy dispersive spectrometer(EDS)*** factors significantly affecting the surface quality of the micropit surface texture are the energy and pulse *** relationship between taper angle and energy is appropriately *** on the formation process and mechanism of the surface texture of laser micropits provides important guidance for precision machining.

关键词： Laser machining Thermal stress damage Surface texturing Design of experiment(DOE) Micropit

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Surface deflection-based reliability analysis of asphalt pavement design

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Science China(Technological Sciences) 2020年第9期63卷 1824-1836页

作者： huang Wei LIANG SiMing WEI ya Intelligent Transportation System Research Center Southeast UniversityNanjing210096China Department of Civil Engineering Tsinghua UniversityBeijing100084China

The surface deflection of asphalt pavement reflects the strength and stiffness of the entire structure, which can be used to evaluate the rutting life of asphalt pavements. However, it is influenced by various stochastic variables including traffic loads, material properties and structural thickness of each pavement course. The uncertainty of above stochastic variables is of significance for accurately predicting the rutting life of asphalt pavement. In this study, the statistical characteristics of stochastic variables of asphalt pavement were assessed based on the field data collected from asphalt pavement projects. A unique formula with a fairly good accuracy was found using multiple linear regression based on numerical simulation results to ease the calculation of pavement deflection during the reliability analysis. It is shown that the stochastic variables of asphalt pavement can be well characterized by normal distribution or logarithmic normal distribution. The regressed formula to calculate the surface deflection of pavement has a fairly good accuracy with an error of less than 6.0% compared to the numerical method. The proposed surface deflection-based reliability analysis can be used easily to evaluate the influence of input parameters on the rutting life and to guide the structure design of asphalt pavement with required reliability.

关键词： asphalt pavement surface deflection rutting life reliability regressive model to calculate pavement deflection

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Secure output synchronization of heterogeneous multi-agent systems against false data injection attacks

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Science China(Information Sciences) 2022年第6期65卷 142-154页

作者： Shicheng HUO Dalin huang ya ZHANG School of Automation Southeast University School of Cyber Science and Engineering Southeast University Key Laboratory of Measurement and Control of Complex Systems of Engineering Ministry of Education

This paper studies secure output synchronization for heterogeneous multi-agent systems against false data injection(FDI) attacks. Both the sensors and actuators of agents may be injected into FDI *** mitigate the malicious impact of these attacks on synchronization performance, a desired reference model,which is combined with an auxiliary system, is first designed for each agent to simulate its normal system dynamics. Then, based on this reference model, a state feedback cooperative controller and a static output feedback cooperative controller, which consist of adaptive compensators, are proposed, respectively. The integrated control protocols can ensure that the output synchronization error is small by adjusting some designed parameters even in the presence of FDI attacks. An illustrative example is employed to demonstrate the effectiveness of the proposed method.

关键词： output synchronization false data injection attacks adaptive compensators heterogeneous multi-agent systems secure control

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An SVM-Based Prediction Method for Solving SAT Problems

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Chinese Journal of Electronics 2019年第2期28卷 246-252页

作者： huang Shaobin LI ya LI yanmei College of Computer Science and Technology Harbin Engineering University

We show how Support vector machines(SVM) can be applied to the Satisfiability(SAT) problem and how their prediction results can be naturally applied to both incomplete and complete SAT solvers. SVM is used for the classification of the variables in the SAT problem and the classification results are the assignment of the variables. And we also present empirical results of applying SVM to instances of the SAT problem from the Center for Discrete Mathematics and Theoretical Computer Science(DIMACS) archive and compare them against the results of other incomplete and complete algorithms for the SAT problem.

关键词： Support vector machines Satisfiability Complete algorithms Incomplete algorithms

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Structure-based discovery of orally efficient inhibitors via unique interactions with H-pocket of PDE8 for the treatment of vascular dementia

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Acta Pharmaceutica Sinica B 2022年第7期12卷 3103-3112页

作者： Xu-Nian Wu Qian Zhou ya-Dan huang xi xie Zhe Li Yinuo Wu Hai-Bin Luo School of Pharmaceutical Sciences Sun Yat-sen UniversityGuangzhou510006China Key Laboratory of Tropical Biological Resources of Ministry of Education and One Health Institute School of Pharmaceutical SciencesHainan UniversityHaikou 570228China

Our previous study demonstrated that phosphodiesterase 8(PDE8)could work as a potential target for vascular dementia(Va D)using a chemical probe ***,compound 3a is a chiral compound which was obtained by chiral resolution on HPLC,restricting its usage in ***,a series of non-chiral 9-benzyl-2-chloro-adenine derivatives were discovered as novel PDE8 *** 15 exhibited potent inhibitory activity against PDE8A(IC_(50)=11 nmol/L),high selectivity over other PDEs,and remarkable drug-like properties(worthy to mention is that its bioavailability was up to 100%).Oral administration of 15 significantly improved the c AMP level of the right brain and exhibited dosedependent effects on cognitive improvement in a Va D mouse ***,the X-ray crystal structure of the PDE8A—15 complex showed that the potent affinity and high selectivity of 15 might come from the distinctive interactions with H-pocket including T-shapedπ—πinteractions with Phe785 as well as a unique H-bond network,which have never been observed in other PDE-inhibitor complex before,providing new strategies for the further rational design of novel selective inhibitors against PDE8.

关键词： Phosphodiesterase 8(PDE8) Vascular dementia Structure-based drug design MM-GB/SA Free energy prediction Structure—activity relationship Binding potencies

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