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Ultra-homogeneous dense Ag nano layer enables long lifespan solid-state lithium metal batteries

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Journal of Energy Chemistry 2024年第9期96卷 110-119页

作者： Yaning Liu Tianqi Yang Ruyi Fang Chengwei Lu Ruojian Ma Ke Yue Zhen Xiao Xiaozheng Zhou Wenkui zhang Xinping He Yongping Gan jun zhang Xinhui Xia hui huang Xinyong tao Yang Xia College of Materials Science and Engineering Zhejiang University of TechnologyHangzhou 310014ZhejiangChina Key Laboratory of Rare Earth Optoelectronic Materials and Devices of Zhejiang Province Institute of Optoelectronic Materials and DevicesChina Jiliang UniversityHangzhou 310018ZhejiangChina

The unstable electrolyte/lithium(Li)anode interface has been one of the key challenges in realizing high energy density solid-state lithium metal batteries(LMBs)***,a dense and uniform silver(Ag)nano interlayer with a thickness of∼35 nm is designed accurately by magnetron sputtering technology to optimize the electrolyte/Li anode *** Ag nano layer reacts with Li metal anode to in-situ form Li-Ag alloy,thus enhancing the physical interfacial contact,and further improving the interfacial wettability and *** particular,the Li-Ag alloy is inclined to form AgLi phase proved by cryo-TEM and DFT,effectively preventing SN from continuously“attacking”the Li metal anode due to the lower adsorption of succinonitrile(SN)molecules on AgLi than that of pure Li metal,thereby significantly reinforcing the interfacial ***,the enhanced physical and chemical stability of electrolyte/Li anode interface promotes the homogeneous deposition of Li^(+)and inhibits the dendrite *** Li-symmetric cell maintains stable operation for up to 1700 h and the cycling stability of LiFePO_(4)|SPE|Li full cell is remarkably improved at room temperature(capacity retention rate of 91.9%for 200 cycles).This work opens an effective way for accurate and controllable interface design of long lifespan solid-state LMBs.

关键词： Silvernano layer Poly(ethylene oxide) Solid polymer electrolyte Succinonitrile Lithium metal battery

Shifts in reproductive strategies in the evolutionary trajectory of plant lineages

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Science China(Life Sciences) 2024年第11期67卷 2499-2510页

作者： Xin-Jian zhang Xian-Han huang Jacob BLandis Quan-sheng Fu jun-Tong Chen Peng-Rui Luo Li-Juan Li Heng-Yi Lu Hang Sun tao Deng State Key Laboratory of Plant Diversity and Specialty Crops Kunming Institute of BotanyChinese Academy of SciencesKunming 650201China Yunnan International Joint Laboratory for Biodiversity of Central Asia Kunming Institute of BotanyChinese Academy of SciencesKunming 650201China University of Chinese Academy of Sciences Beijing 100049China School of Integrative Plant Science Section of Plant Biology and the L.H.Bailey HortoriumCornell UniversityNew York 14850USA BTI Computational Biology Center Boyce Thompson InstituteNew York 14853USA CAS Key Laboratory of Plant Germplasm Enhancement and Specialty Agriculture Wuhan Botanical GardenChinese Academy of SciencesWuhan 430074China

Understanding the maintenance and shift in reproductive strategies is a fundamental question in evolutionary *** many efforts have been made to compare different reproductive strategies,the association between reproductive strategies and lineage divergence is largely *** explore the impact of different reproductive strategies on lineage divergence,we investigated the evolution of clonality in Saxifraga ***+*** integrating several lines of evidence,we found that the loss of clonality in Irregulares+Heterisia was associated with a progressive increase in diversification rate and intraspecific morphological diversity but with a reduction in species distribution *** findings provide insights into the ecological and evolutionary effects of different reproductive strategies,suggesting the necessity of integrating clonality into ecological and evolutional research.

关键词： Saxifragaceae diversification reproduction clonality phenotype niche

A reinvestigation of low molecular weight components in SOA produced by cyclohexene ozonolysis

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Nuclear Science and Techniques 2018年第11期29卷 238-246页

作者： jun Chen Zhao-hui Li Ye-Peng Yu Xuan Lin Hang zhang Yan-Bo Li Huan-Huan Wang Rui-Rui Sun Qing-hui Meng Chao-Qun huang Xiao-Bin Shan Fu-Yi Liu Chang-Jin Hu Wei-jun zhang Liu-Si sheng National Synchrotron Radiation Laboratory School of Nuclear Science and TechnologyUniversity of Science and Technology of China Laboratory Medical Optical and Mass Spectrometry Center of Medical Physics and TechnologyHefei Institutes of Physical ScienceChinese Academy of Sciences Laboratory of Atmospheric Physico-Chemistry Anhui Institute of Optics and Fine MechanicsChinese Academy of Sciences School of Environmental Science and Optoelectronic Technology University of Science and Technology of China

The ozonolysis of cyclohexene is an important model system for understanding the more complex reaction of O_3 with monoterpenes; however, many previous studies have come to qualitatively different conclusions about the composition of the secondary organic aerosol(SOA)formed in this system. In the present study, the composition of the SOA produced by cyclohexene ozonolysis in the absence of seed aerosols has been investigated online and off-line using synchrotron-based thermal desorption/tunable vacuum ultraviolet photoionization time-of-flight aerosol mass spectrometry(TD-VUV-TOF-PIAMS) in conjunction with a custom-built smog chamber. On the basis of the molecular ions observed by mass spectrometry at 11.5 e V, it was found that dicarboxylic acids, dialdehydes, and cyclic anhydrides are the predominant low molecular weight components in the particle phase. The results also indicated that TD-VUV-TOF-PIAMS coupled with filter sampling is a potentially useful tool for the investigation of SOA composition both in the field and in the laboratory.

关键词： Cyclohexene Ozonolysis SOA Smog chamber Aerosol mass spectrometry

Effects of fluid balance on prognosis of acute respiratory distress syndrome patients secondary to sepsis

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World Journal of Emergency Medicine 2020年第4期11卷 216-222页

作者： Yu-ming Wang Yan-jun Zheng Ying Chen Yun-chuan huang Wei-wei Chen Ran Ji Li-li Xu Zhi-tao Yang hui-qiu sheng Hong-ping Qu En-qiang Mao Er-zhen Chen Department of Emergency Ruijin Hospital Affi liated to Shanghai Jiao Tong University School of MedicineShanghaiChina Department of Critical Care Medicine Ruijin Hospital Affi liated to Shanghai Jiao Tong University School of MedicineShanghaiChina

BACKGROUND:Fluid management is crucial to acute respiratory distress syndrome(ARDS)secondary to ***,choices of fluid resuscitation strategies and fluid input volumes remain a thorny *** study aimed to elucidate the relationship between fluid balance and prognosis of ARDS patients secondary to ***:Our study included 322 sepsis patients from Ruijin Hospital between 2014 and 2018,and 84 patients were diagnosed as ARDS within 72 hours after onset of sepsis according to Berlin ARDS Defi ***:Among the 322 sepsis patients,84(26.1%)were complicated with ARDS within 72 *** patients had a lower oxygenation index(PaO2/FiO2166.4±71.0 vs.255.0±91.2,P<0.05),longer duration of mechanical ventilation(11[6-24]days vs.0[0-0]days,P<0.05)than those without *** patients with ARDS showed daily positive net fl uid balance during seven days compared with those without ARDS who showed daily negative net fluid balance since the second day with signifi cant statistical *** the 84 sepsis patients with ARDS,58(69.0%)*** daily fl uid input volumes were much lower in survivors than in non-survivors(43.2±16.7 mL/kg vs.51.0±25.2 mL/kg,P<0.05)while output volumes were much higher in survivors(45.2±19.8 mL/kg vs.40.2±22.7 mL/kg,P<0.05).Using binary logistic regression analysis,we found that the mean daily fl uid balance was independently associated with mortality of sepsis patients complicating with ARDS(P<0.05).CONCLUSIONS:Early negative fluid balance is independently associated with a better prognosis of sepsis patients complicated with ARDS.

关键词： Sepsis Acute respiratory distress syndrome Fluid balance Prognosis

NAD^(+) exhaustion by CD38 upregulation contributes to blood pressuree elevation and vascular damage in hypertension

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Signal Transduction and Targeted Therapy 2023年第10期8卷 4964-4977页

作者： Yumin Qiu Shiyue Xu Xi Chen Xing Wu Zhe Zhou Jianning zhang Qiang Tu Bing Dong Zhefu Liu Jiang He Xiaoyu zhang Shuangshuang Liu Chen Su hui huang Wenhao Xia jun tao Department of Hypertension and Vascular Disease The First Affiliated Hospital of Sun Yat-sen University510080 GuangzhouChina National-Guangdong Joint Engineering Laboratory for Diagnosis and Treatment of Vascular Diseases 510080 GuangzhouChina Key Laboratory on Assisted Circulation Ministry of Health510080 GuangzhouChina Department of Cardiology The Eighth Affiliated Hospital of Sun Yat-sen University518033 ShenzhenChina Guangxi Hospital Division of The First Affiliated Hospital Sun Yat-sen University530022 NanningChina

Hypertension is characterized by endothelial dysfunction and arterial stiffness,which contribute to the pathogenesis of atherosclerotic cardiovascular *** adenine dinucleotide(NAD^(+))is an indispensable cofactor in all living cells that is involved in fundamental biological ***,in hypertensive patients,alterations in NAD^(+)levels and their relation with blood pressure(BP)elevation and vascular damage have not yet been studied.

关键词： damage arterial hypertension

Effect of Crossbreed on the Muscle Quality(Chemical Composition) in Yun-Ling Black Goats

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Agricultural Sciences in China 2009年第1期8卷 108-114页

作者： JIA jun-jing TIAN Yun-bo zhang Xi huang Qi-chao WEN sheng-ping GU Feng-ying GE Chang-rong CAO Zhen-hui CHENG Zhi-bin M. Jois Yunnan Provincial Key Laboratory of Animal Nutrition and Feed Science Yunnan Agricultural University Kunming 650201 P.R.China College of Zhongkai Agricultural Technology and Science Guangzhou 510225 P.R. China College of Food Science and Technology Yunnan Agricultural University Kunming 650201 P.R.China Department of Agriculture School of Life Sciences La Trobe University Bundoora 3086 Victoria Australia

Twenty castrated male goats, each of Yun-Ling Black goats （YLB goat）, N × YLB hybrid goats （Nubian ♂ ×Yun-Ling Black goats 9） and B × YLB hybrid goats （Boer ♂× Yun-Ling Black goats ♀）, were used to evaluate the effect of crossbreeding on the meat chemical composition in the YLB goats of China. After weaning of 90 days, all the experimental goats were reared on natural pasture when they were slaughtered at an age of 730 days. The longissimus dorsi （LD） and biceps femoris （BF） muscles were sampled from each carcass to determine chemical compositions. Both hybrid goats had higher protein content （P 〈 0.01） and lower fat content （P 〈 0.05） than the YLB goats in the two types of muscle. The inosinic acid contents of LD muscle for the YLB goats and the B × YLB hybrid goats were significantly higher （P 〈 0.05） than that for the N × YLB hybrid goats. The LD muscle from the YLB goats contained higher essential amino acid （P 〈 0.01）, total amino acid （P 〈 0.01）, and some individual amino acid （P 〈 0.05） than those from the hybrid goats. The concentration of unsaturated fatty acid （USFA） of LD muscle from the N × YLB hybrid goats was significantly higher than the other two goat breeds （P〈0.05） but did not differ between the other two goat breeds （P〉0.05）. The YLB goats had significantly higher （P〈0.05） concentrations of oleic acid （C18：1） and linolenic acid （C18：3） of LD muscle than the hybrid goats, had significantly higher （P 〈 0.05） proportion of mono-unsaturated （Sum for C 16：1 and C 18：1） than the B ×YLB hybrid goats, and tended to be higher than the N × YLB hybrid goats （P 〉 0.05）. In contrast, the proportion of poly-unsaturated in the YLB goats was significantly lower （P 〈 0.05） than that in the hybrid goats.

关键词： Yun-Ling Black goat crossbreed muscle amino acids muscle fatty acids

Activin A receptor type 1C single nucleotide polymorphisms associated with esophageal squamous cell carcinoma risk in Chinese population

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World Journal of Gastrointestinal Oncology 2025年第1期17卷 39-51页

作者： Si-Yun Lin Hou huang Jin-Jie Yu Feng Su Tian Jiang Shao-Yuan zhang Lu Lv tao Long hui-Wen Pan jun-Qing Qi Qiang Zhou Wei-Feng Tang Guo-Wen Ding Li-Ming Wang Li-Jie Tan jun Yin Department of Thoracic Surgery Zhongshan Hospital Affiliated to Fudan UniversityShanghai 200032China Shanghai Key Laboratory of Clinical Geriatric Medicine Huadong Hospital Affiliated to Fudan UniversityShanghai 200040China Department of Cardiothoracic Surgery The Affiliated People's Hospital of Jiangsu UniversityZhenjiang 212002Jiangsu ProvinceChina Department of Thoracic Surgery Sichuan Cancer Hospital&InstituteChengdu 610042Sichuan ProvinceChina Department of Cardiothoracic Surgery Nanjing Drum Tower HospitalThe Affiliated Hospital of Nanjing University Medical SchoolNanjing 210000Jiangsu ProvinceChina Department of Respiratory and Critical Care Medicine Shanghai Xuhui Central HospitalShanghai 200032China

BACKGROUND Transforming growth factor-β(TGF-β)superfamily plays an important role in tumor progression and *** A receptor type 1C(ACVR1C)is a TGF-βtype I receptor that is involved in tumorigenesis through binding to dif-ferent *** To evaluate the correlation between single nucleotide polymorphisms(SNPs)of ACVR1C and susceptibility to esophageal squamous cell carcinoma(ESCC)in Chinese Han *** In this hospital-based cohort study,1043 ESCC patients and 1143 healthy controls were *** SNPs(rs4664229,rs4556933,rs77886248,rs77263459,rs6734630)of ACVR1C were assessed by the ligation detection reaction ***-Weinberg equilibrium test,genetic model analysis,stratified analysis,linkage disequi-librium test,and haplotype analysis were *** Participants carrying ACVR1C rs4556933 GA mutant had significantly decreased risk of ESCC,and those with rs77886248 TA mutant were related with higher risk,especially in older male *** the haplotype analysis,ACVR1C Trs4664229Ars4556933Trs77886248Crs77263459Ars6734630 increased risk of ESCC,while Trs4664229Grs4556933Trs77886248Crs77263459Ars6734630 was associated with lower susceptibility to *** ACVR1C rs4556933 and rs77886248 SNPs were associated with the susceptibility to ESCC,which could provide a potential target for early diagnosis and treatment of ESCC in Chinese Han population.

关键词： Activin A receptor type 1C Single nucleotide polymorphisms Esophageal squamous cell carcinoma Genetic susceptibility Hospital-based cohort study

Expert consensus of Chinese Association for the Study of Pain on the radiofrequency therapy technology in the Department of Pain

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World Journal of Clinical Cases 2021年第9期9卷 2123-2135页

作者： Jin-Feng Liu Wen Shen Dong huang tao Song Wei tao Qing Liu You-Qing huang Xiao-Mei zhang Ling-Jie Xia Da-sheng Wu hui Liu Fu-Yong Chen Tang-Hua Liu Bao-Gan Peng Yan-Qing Liu Department of Algology The Second Affiliated Hospital of Harbin Medical UniversityHarbin 150086Heilongjiang ProvinceChina Department of Algology Affiliated Hospital of Xuzhou Medical UniversityXuzhou 221000Jiangsu ProvinceChina Department of Algology The Third Xiangya Hospital of Central South UniversityChangsha 410000Hunan ProvinceChina Department of Algology The First Affiliated Hospital of China Medical UniversityShenyang 110000Liaoning ProvinceChina Department of Neurosurgery Shenzhen University General HospitalShenzhen 518000Guangdong ProvinceChina Department of Algology The Affiliated T.C.M Hospital of Southwest Medical UniversityLuzhou 646000Sichuan ProvinceChina Department of Algology The Second Affiliated Hospital of Kunming Medical UniversityKunming 650000Yunnan ProvinceChina Department of Algology The First Affiliated Hospital of Kunming Medical UniversityKunming 650000Yunnan ProvinceChina Department of Algology Henan Provincial HospitalZhengzhou 450000Henan ProvinceChina Department of Algology Jilin Province People's HospitalChangchun 130000Jilin ProvinceChina Department of Algology West China Hospital of Sichuan UniversityChengdu 610000Sichuan ProvinceChina Department of Algology The Third People's Hospital of YibinYibin 644000Sichuan ProvinceChina Department of Orthopedics The Third Medical CenterGeneral Hospital of the Chinese People’s Liberation ArmyBeijing 100039China Department of Algology Beijing Tiantan HospitalCapital Medical UniversityBeijing 100070China

On the basis of continuous improvement in recent years,radiofrequency therapy technology has been widely developed,and has become an effective method for the treatment of various intractable *** therapy is a technique that uses special equipment and puncture needles to output ultra-high frequency radio waves and accurately act on local *** order to standardize the application of radiofrequency technology in the treatment of painful diseases,Chinese Association for the Study of Pain(CASP)has developed a consensus proposed by many domestic experts and scholars.

关键词： Radiofrequency therapy Standard radiofrequency therapy Pulsed radiofrequency Bipolar radiofrequency therapy Expert consensus Pain

Magnetic-biased chiral molecules enabling highly oriented photovoltaic perovskites

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National Science Review 2024年第2期11卷 221-230页

作者： Jing Chen Caner Deger Zhen-huang Su Kai-Li Wang Guang-Peng Zhu jun-Jie Wu Bing-Chen He Chun-Hao Chen tao Wang Xing-Yu Gao Ilhan Yavuz Yan-hui Lou Zhao-Kui Wang Liang-sheng Liao Institute of Functional Nano&Soft Materials(FUNSOM) Laboratory of Advanced Negative Carbon TechnologiesSoochow University Department of Physics Marmara University Shanghai Synchrotron Radiation Facility(SSRF) Shanghai Advanced Research InstituteChinese Academy of Sciences College of Energy Soochow Institute for Energy and Materials Innovations Soochow University Macao Institute of Materials Science and Engineering Macau University of Science and Technology

The interaction between sites A, B and X with passivation molecules is restricted when the conventional passivation strategy is applied in perovskite（ABX3） photovoltaics. Fortunately, the revolving A-site presents an opportunity to strengthen this interaction by utilizing an external field. Herein, we propose a novel approach to achieving an ordered magnetic dipole moment, which is regulated by a magnetic field via the coupling effect between the chiral passivation molecule and the A-site（formamidine ion） in *** strategy can increase the molecular interaction energy by approximately four times and ensure a well-ordered molecular arrangement. The quality of the deposited perovskite film is significantly optimized with inhibited nonradiative recombination. It manages to reduce the open-circuit voltage loss of photovoltaic devices to 360 mV and increase the power conversion efficiency to 25.22%. This finding provides a new insight into the exploration of A-sites in perovskites and offers a novel route to improving the device performance of perovskite photovoltaics.

关键词： perovskite photovoltaics magnetic moment A-site regulation chiral molecules