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Precise construction of RuPt dual single-atomic sites to optimize oxygen electrocatalytic behaviors for high-performance Zn-air batteries

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Journal of Energy Chemistry 2024年第10期97卷 520-528,I0011页

作者： xiaolin hu Zhenkun Wu Chaohe Xu School of Science Chongqing Key Laboratory of New Energy Storage Materials and DevicesChongqing University of TechnologyChongqing 400054China School of Chemistry and Engineering Chongqing UniversityChongqing 400044China College of Materials Science and Engineering Chongqing UniversityChongqing 400044China

The development of redox bifunctional electrocatalysts with high performance,low cost,and long lifetimes is essential for achieving clean energy *** study proposed an atom capture strategy for anchoring dual single atoms(DSAs)in a zinc-zeolitic imidazolate framework(Zn-ZIF),followed by calcination under an N_(2) atmosphere to synthesize ruthenium-platinum DSAs supported on a nitrogendoped carbon substrate(RuPt DSAs-NC).Theoretical calculations showed that the degree of Ru 5dxz-~*O 2p_x orbital hybridization was high when^(*)O was adsorbed at the Ru site,indicating enhanced covalent hybridization of metal sites and oxygen ligands,which benefited the adsorption of intermediate *** presence of the RuPtN_6 active center optimized the absorption-desorption behavior of intermediates,improving the electrocatalytic performance of the oxygen reduction reaction(ORR)and the oxygen evolution reaction(DER),RuPt DSAs-NC exhibited a 0.87 V high half-wave potential and a 268 mV low overpotential at 10 mA cm^(-2)in an alkaline ***,rechargeable zinc-air batteries(ZABs)achieved a peak power density of 171 MW cm^(-2).The RuPt DSAs-NC demonstrated long-term cycling for up to 500 h with superior round-trip *** study provided an effective structural design strategy to construct DSAs active sites for enhanced electrocata lytic performance.

关键词： Dual single atoms catalysts Atom capture Oxygen reduction reaction Oxygen evolution reaction Rechargeable Zn-air batteries

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Ultrafast laser-chemical modification hybrid fabrication of hydrostatic bearings with a superhydrophobicity solid-liquid interface

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Science China(Technological Sciences) 2024年第3期67卷 696-708页

作者： GUO Minghui RONG YouMin huANG Yu FENG xiaolin hu HaiDong WU CongYi ZHANG GuoJun State Key Laboratory of Intelligent Manufacturing Equipment and Technology Huazhong University of Science and Technology Wuhan 430074China School of Mechanical Science and Engineering Huazhong University of Science and TechnologyWuhan 430074China Faculty of Engineering and Life Sciences Universiti Selangor Bestari JayaSelangor 45600Malaysia

Oil film vortex severely reduces the stability of hydrostatic bearings. A solid-liquid interface with drag and slip properties can weaken the oil film vortex of the bearing. Here, a combined picosecond laser ablation and chemical modification method is proposed to prepare surfaces with microbulge array structure on 6061 aluminum alloy substrates. Because of the low surface energy of the perfluorododecyltriethoxysilane modification and the bulge geometry of the microbulge array structure, the surface shows excellent superhydrophobicity. The optimum contact angle in air for water is 164°, and that for oil is 139°. Two surfaces with “lotus-leaf effect” and “rose-petal effect” were obtained by controlling the processing parameters. The drag reduction properties of superhydrophobic surfaces were systematically investigated with slip lengths of 22.26 and 36.25 μm for deionized water and VG5 lubricant, respectively. In addition, the superhydrophobic surface exhibits excellent mechanical durability and thermal stability. The proposed method provides a new idea for vortex suppression in hydrostatic bearings and improves the stability of bearings in high-speed operation.

关键词： superhydrophobicity surface ultrafast laser drag reduction solid-liquid interface microbulge array structure

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Waldenström macroglobulinemia:a challenging case treated with anti-CD19 CAR-T cell therapy

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Journal of Zhejiang University-Science B(Biomedicine & Biotechnology) 2024年第8期25卷 719-722页

作者： Yang YANG xiaolin GU Jingsong HE Yongxian hu Zhen CAI Bone Marrow Transplantation Center Department of Hematologythe First Affiliated HospitalSchool of MedicineZhejiang UniversityHangzhou 310006China Department of Hematology Putuo People’s HospitalZhoushan 316100China

Waldenström macroglobulinemia(WM)is characterized by lymphoplasmacytic lymphoma associated with large amounts of monoclonal immunoglobulin M(IgM)protein(Owen et al.,2003).Common signs and symptoms include fatigue due to anemia,lymph node enlargement,hepatosplenomegaly,thrombocytopenia,symptoms related to high viscosity,and peripheral neuropathy,among *** significant advances in WM treatment,this type of indolent lymphoma remains incurable,with a wide array of patient outcomes(Ruan et al.,2020).In recent years,chimeric antigen receptor T(CAR-T)cell therapy targeting cluster of differentiation 19(CD19)has shown unprecedented response rates and durability in the treatment of B-cell *** this report,we describe a challenging case of WM that involved multiple extramedullary sites,relapsed,and was refractory to chemotherapy,immunotherapy,and targeted *** anti-CD19 CAR-T cell therapy,the tumor burden significantly decreased and the patient’s condition remained stable at the writing of this report.

关键词： CD19 globulin durability

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How variable progenitor clones construct a largely invariant neocortex

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National Science Review 2024年第1期11卷 129-144页

作者： Zhongfu Shen Jiajun Yang Qiangqiang Zhang Kuiyu Wang Xiaohui Lv xiaolin hu Jian Ma Song-Hai Shi New Cornerstone Science Laboratory IDG/McG overn Institute for Brain Research Tsinghua-Peking Center for Life Sciences Beijing Frontier Research Center for Biological Structure School of Life Sciences Tsinghua University Department of Computer Sciences Tsinghua University College of Life Sciences Nankai University Chinese Institute for Brain Research

The neocortex contains a vast collection of diverse neurons organized into distinct layers. While nearly all neocortical neurons are generated by radial glial progenitors(RGPs), it remains largely unclear how a complex yet organized neocortex is constructed reliably and robustly. Here, we show that the division behavior and neuronal output of RGPs are highly constrained with patterned variabilities to support the reliable and robust construction of the mouse neocortex. The neurogenic process of RGPs can be well-approximated by a consistent Poisson-like process unfolding over time, producing deep to superficial layer neurons progressively. The exact neuronal outputs regarding layer occupation are variable; yet, this variability is constrained systematically to support all layer formation, largely reflecting the variable intermediate progenitor generation and RGP neurogenic entry and exit timing differences. Together, these results define the fundamental features of neocortical neurogenesis with a balanced reliability and variability for the construction of the complex neocortex.

关键词： neocortex radial glial progenitor intermediate progenitor neurogenesis clonal variability layer formation

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A New Method for Solving the Continuous Multi-Object Optimization Problems

A New Method for Solving the Continuous Multi-Object Optimiz...

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智能计算及其应用国际会议

作者： hu Yefa1 CHENG Hao1 hu xiaolin2 huANG Zhangcan3 (1. School of Mechanical and Electrical Engineering Wuhan University of Technology Wuhan 430070 China) (2. Department of Automation & Computer-Aided Engineering The Chinese University of Hong Kong Hong Kong SAR China) (3. State Key Laboratory of Software Engineering Wuhan University Wuhan 430072 China)

In this paper, we proposed a new multi-object evolutionary algorithm (MOEA), neighborhood exploring evolutionary strategy (NEES), which focused on search operators to generate new individuals in MOEA.

关键词： Neighborhood exploring evolution strategy multi-objective optimization evolutionary algorithm evolution strategy

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非牛顿流固耦合问题的半隐式分区ALE有限元-间断有限元耦合算法研究

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浙江大学学报（理学版） 2024年第4期51卷 450-458页

作者：高普阳胡小林长安大学理学院陕西西安710064

针对非牛顿流固耦合问题,提出了任意拉格朗日-欧拉(arbitrary Lagrangian-Eulerian,ALE)框架下的半隐式分区有限元-间断有限元耦合算法。其数学模型主要包括非牛顿流体和固体结构的控制方程,以及流体-固体交界面上的边界条件。固体结构... 详细信息

针对非牛顿流固耦合问题,提出了任意拉格朗日-欧拉(arbitrary Lagrangian-Eulerian,ALE)框架下的半隐式分区有限元-间断有限元耦合算法。其数学模型主要包括非牛顿流体和固体结构的控制方程,以及流体-固体交界面上的边界条件。固体结构由弹性材料组成,非牛顿流体由幂律型本构模型描述。用分裂格式对非牛顿流体控制方程进行解耦,得到若干子方程;通过有限元、间断有限元方法求解对应恰当类型的子方程。用中心差分及标准有限元方法分别对固体结构弹性动力学方程进行时间和空间离散;用修正的Laplace移动网格方法处理固体结构的形变及流体区域网格的变化过程。最后用数值算法研究了带有圆弧顶端梯形结构体的非牛顿流固耦合问题,并详细分析了结构体高度、入口速度及流体特性等因素对流固耦合问题的影响及机理。

关键词：流固耦合非牛顿流体幂律模型半隐式有限元

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LncRNA CCRR maintains Ca^(2+)homeostasis against myocardial infarction through the FTO-SERCA2a pathway

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Science China(Life Sciences) 2024年第8期67卷 1601-1619页

作者： hua Yang Lina Xuan Shengjie Wang huishan Luo Xiaomeng Duan Jianjun Guo Shijia Cui Jieru Xin Junwei Hao Xiufang Li Jun Chen Feihan Sun xiaolin hu Siyun Li Ying Zhang Lei Jiao Baofeng Yang Lihua Sun Department of Pharmacology Harbin Medical University(State Key Laboratory of Frigid Zone Cardiovascular Diseasethe State-Province Key Laboratories of Biomedicine-Pharmaceutics of ChinaKey Laboratory of Cardiovascular ResearchMinistry of EducationJoint International Research Laboratory of Cardiovascular Medicine ResearchMinistry of EducationChina)College of PharmacyHarbin Medical UniversityHarbin 150081China

Cardiac conduction regulatory RNA(CCRR)has been documented as an antiarrhythmic lncRNA in our earlier *** study aimed to evaluate the effects of CCRR on SERCA2a and the associated Ca^(2+)homeostasis in myocardial infarction(MI).Overexpression of CCRR via AAV9-mediated delivery not only partially reversed ischemia-induced contractile dysfunction but also alleviated abnormal Ca^(2+)homeostasis and reduced the heightened methylation level of SERCA2a following *** effects were also observed in CCRR overexpressing transgenic mice.A conserved sequence domain of CCRR mimicked the protective function observed with the full ***,silencing CCRR in healthy mice led to intracellular Ca^(2+)overloading of *** increased SERCA2a protein stability by upregulating FTO *** direct interaction between CCRR and FTO protein was characterized by RNA-binding protein immunoprecipitation(RIP)analysis and RNA pulldown *** of NFATc3 was identified as an upstream mechanism responsible for CCRR downregulation in *** study demonstrates that CCRR is a protective lncRNA that acts by maintaining the function of FTO,thereby reducing the m^(6)A RNA methylation level of SERCA2a,ultimately preserving calcium homeostasis for myocardial contractile function in ***,CCRR may be considered a promising therapeutic strategy with a beneficial role in cardiac pathology.

关键词： CCRR calcium homeostasis FTO myocardial infarction SERCA2a

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基于改进YOLO v5的复杂环境下花椒簇识别与定位方法

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农业机械学报 2024年第3期55卷 243-251页

作者：黄华张昊胡晓林聂兴毅兰州理工大学机电工程学院兰州730050

花椒树产果量大,枝干纵横交错,树叶茂密,给花椒的自动化采摘带来了困难。因此,本文设计一种基于改进YOLO v5的复杂环境下花椒簇的快速识别与定位方法。通过在主干提取网络CSPDarknet的CSPLayer层和Neck的上采样之后增加高效通道注意力EC... 详细信息

花椒树产果量大,枝干纵横交错,树叶茂密,给花椒的自动化采摘带来了困难。因此,本文设计一种基于改进YOLO v5的复杂环境下花椒簇的快速识别与定位方法。通过在主干提取网络CSPDarknet的CSPLayer层和Neck的上采样之后增加高效通道注意力ECA(Efficient channel attention)来简化CSPLayer层的计算量,提升了特征提取能力。同时在下采样层增加协同注意力机制CA(Coordinate attention),减少下采样过程中信息的损失,强化特征空间信息,配合热力图(Grad-CAM)和点云深度图,来完成花椒簇的空间定位。测试结果表明,与原YOLO v5相比较,改进的网络将残差计算减少至1次,保证了模型轻量化,提升了效率。同帧数区间下,改进后的网络精度为96.27%,对比3个同类特征提取网络YOLO v5、YOLO v5-tiny、Faster R-CNN,改进后网络精确度P分别提升5.37、3.35、15.37个百分点,连株花椒簇的分离识别能力也有较大提升。实验结果表明,自然环境下系统平均识别率为81.60%、漏检率为18.39%,能够满足花椒簇识别要求,为移动端部署创造了条件。

关键词：花椒簇识别农业机器人深度学习目标检测 YOLO v5

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改进YOLOv5s的桥梁表观病害检测方法

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重庆大学学报 2024年第9期47卷 91-100页

作者：董绍江谭浩刘超胡小林重庆交通大学机电与车辆工程学院重庆400074 重庆工业大数据创新中心有限公司重庆404100

针对已有目标检测方法在混凝土桥梁表观病害检测的应用中识别精度低且伴随较多误检和漏检的问题,提出了一种改进的YOLOv5s桥梁表观病害检测方法。针对目前桥梁表观病害特征成分较复杂的问题,为了更有效地利用不同尺度的缺陷特征,在主干... 详细信息

针对已有目标检测方法在混凝土桥梁表观病害检测的应用中识别精度低且伴随较多误检和漏检的问题,提出了一种改进的YOLOv5s桥梁表观病害检测方法。针对目前桥梁表观病害特征成分较复杂的问题,为了更有效地利用不同尺度的缺陷特征,在主干网中添加修改后的空间金字塔池化模块,提高了整体网络对缺陷特征信息的获取能力,同时减少了运算工作量;针对由病害图像中不同缺陷特征交叉分布导致的误检率、漏检率高的问题,在YOLOv5s网络中加入轻量化注意力模块;针对桥梁缺陷尺寸差异大、分类困难和数据集小而导致的边界回归不匹配的问题,采用考虑了向量角度的损失函数。实验证明,改进后的YOLOv5s检测器在桥梁表观病害目标检测识别任务中能够有效提高精度、降低误检率和漏检率。

关键词：病害检测 YOLOv5s 特征融合平均精度

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变曲率立面自适应爬壁机器人结构的设计与分析

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机器人 2024年第5期46卷 576-590页

作者：胡晓林郭润兰黄华张存东兰州理工大学机电工程学院甘肃兰州730000

针对爬壁机器人在变曲率壁面作业时稳定性差和自适应能力不足等问题,设计了一种自适应模块与机身相对独立的分离式结构爬壁机器人,并研究它在壁面上的移动性能。首先根据机器人的壁面运动原理建立力学模型,计算无滑移和无倾覆时纵/横移... 详细信息

针对爬壁机器人在变曲率壁面作业时稳定性差和自适应能力不足等问题,设计了一种自适应模块与机身相对独立的分离式结构爬壁机器人,并研究它在壁面上的移动性能。首先根据机器人的壁面运动原理建立力学模型,计算无滑移和无倾覆时纵/横移动方向切换、沿壁面移动和越障所需的吸附力,并分析在周向曲面和径向曲面上纵向移动和横向移动时机身姿态的变化情况。然后通过永磁体装置的磁路设计和参数化仿真,分析气隙间距和壁面厚度对吸附力的影响,对机器人在不同曲面和不同运动模式下的吸附力进行仿真,优化永磁体的设计。最后通过实验验证了爬壁机器人在不同变曲率壁面上的移动性能和自适应性能。结果表明,所设计的爬壁机器人具有纵/横切换移动灵活、吸附稳定、变曲率壁面自适应能力强的特点,最小可适应曲率为0.46 m的壁面,且在90°壁面可承载7.2 kg的设备。

关键词：爬壁机器人永磁吸附变曲率立面运动分析

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