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Horticultural Plant Journal 2024年第4期10卷 1035-1048页

作者： hao Hu Fengqun Yu Agriculture and Agri-Food Canada Saskatoon Research and Development Centre107 Science PlaceSaskatoonSKS7N OX2Canada

Clubroot disease is a severe threat to Brassica crops globally,particularly in western *** resistance,achieved through pyramiding clubroot resistance(CR)genes with different modes of action,is the most important strategy for managing the ***,studies on the CR gene functions are quite *** this study,we have conducted investigations into the temporal,structural,and interacting features of a newly cloned CR gene,Rcr1,using CRISPR/Cas9 *** temporal functionality,we developed a novel CRISPR/Cas9-based binary vector,pHHIGR-Hsp18.2,to deliver Rcr1 into a susceptible canola line(DH12075)and observed that early expression of Rcr1 is critical for conferring *** structural functionality,several independent mutations in specific domains of Rcr1 resulted in loss-offunction,highlighting their importance for CR *** the study of the interacting features of Rcr1,a cysteine protease gene and its homologous allele in canola were successfully disrupted via CRISPR/Cas9 as an interacting component with Rcr1 protein,resulting in the conversion from clubroot resistant to susceptible in plants carrying intact *** results indicated an indispensable role of these two cysteine proteases in Rcr1-mediated resistance *** study,the first of its kind,provides valuable insights into the functionality of ***,the new vector p HHIGR-Hsp18.2 demonstrated an inducible feature on the removal of add-on traits,which should be useful for functional genomics and other similar research in brassica crops.

关键词： Clubroot resistance Brassica crops Canola Rcr1 CRISPR/Cas9 system Gene knock-out Timing control Non-synonymous mutation Protein-protein interaction

Constraint on the focal mechanism of the 2011 Tohoku earthquake from the radial modes

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Geodesy and Geodynamics 2024年第1期15卷 27-32页

作者： Weikun Chen hao Ding School of Geodesy and Geomatics Hubei LuoJia LaboratoryWuhan UniversityWuhan 430079China

Different from other normal modes of the Earth’s free oscillation that depend on all the six components(M_(rr),M_(tt),M_(pp),M_(rt),M_(rp),and M_(tp))of the centroid moment tensor,the amplitudes of the radial modes depend on the M_(rr)component(e.g.,scalar moment(M_(0)),dip(δ),and slip(λ))and hypocenter depth of the focal mechanism,and hence can be easily used to constrain these parameters of the focal *** this study,we use the superconducting gravimeter(SG)records after the 2011 Tohoku earthquake to analyze the radial modes_(0)S_(0)and_(1)S_(0).Based on the solutions of the focal mechanism provided by the GCMT and USGS,we can obtain the theoretical amplitudes of these two radial *** the theoretical amplitudes with the observation amplitudes,it is found that there are obvious differences between the former and the latter,which means that the GCMT and USGS focal mechanisms cannot well represent the real focal mechanism of the 2011 *** the GCMT solution as a reference and changing the depth and the three parameters of the M_(rr)moment,the scalar moment(M_(0))and the dip(δ)have significant influences,but the effects of the slip(λ)and the depth are *** comparisons,we provide a new constraint(M_(0)=5.8±0.09×10^(22)N·m,δ=10.1±0.08°,λ=88°,and depth=20 km)for the focal mechanism of the 2011 *** addition,we further determine the center frequency(1.631567±2.6e^(-6)mHz)and quality factor(2046.4±50.1)of the_(1)S_(0)mode.

关键词： Focal mechanism Radial modes Gravity observation

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特殊拓扑结构聚硅氧烷的研究进展

中国材料进展 2018年第3期37卷 161-167页

作者：李泽汪旭红郝超伟杨雄发来国桥杭州师范大学有机硅化学及材料技术教育部重点实验室浙江杭州311121

聚硅氧烷是一类以重复的Si-O键为主链的聚合物。Si-O键较长,具有部分双键特性和较强的离子性,裂解能较高,Si-O-Si键角较大。Si-O键所具有的特性使得聚硅氧烷具有耐高低温、耐辐射、耐气候老化、耐臭氧、电气绝缘、憎水、难燃、无毒、无... 详细信息

聚硅氧烷是一类以重复的Si-O键为主链的聚合物。Si-O键较长,具有部分双键特性和较强的离子性,裂解能较高,Si-O-Si键角较大。Si-O键所具有的特性使得聚硅氧烷具有耐高低温、耐辐射、耐气候老化、耐臭氧、电气绝缘、憎水、难燃、无毒、无腐蚀和生理惰性等优异的性能。聚硅氧烷在航空航天、建筑、电子电器、日用化学品和医药等领域具有重要用途。由于制备聚硅氧烷的原料丰富,所以聚硅氧烷的普及应用有助于减少人类对不可再生资源的依赖。提高聚硅氧烷的性能可以进一步拓展其应用范围,而高分子材料的性能主要取决于其主链结构。因此,制备具有特殊拓扑结构的聚硅氧烷至关重要。主要介绍了大环、密闭多环、高度支化、笼型、半笼型、双甲板型和梯型等几种具有特殊拓扑结构聚硅氧烷的合成、性能与应用方面的研究进展。

关键词：特殊拓扑结构聚硅氧烷合成性能应用

Effect of Fe Addition on Dehydrogenation Performance of Methylcyclohexance over Pt/Al_(2)O_(3)

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China Petroleum Processing & Petrochemical Technology 2024年第1期26卷 12-18页

作者： Tong Fengya Tian hao Wang hao Miao Changxi Song Lei Shanghai Research Institute of Petrochemical Technology SINOPEC Shanghai201208

Catalysts with varying Fe contents were prepared using a sequential impregnation method to investigate the effects of Fe addition on the physicochemical properties of Pt/Al_(2)O_(3) and their performance in methylcyclohexane(MCH)*** results demonstrated that the addition of Fe to Pt/Al_(2)O_(3) enhanced the electron density of Pt and improved catalytic activity,while exhibiting negligible influence on the catalytic selectivity for *** the Fe content was 0.057%,the catalyst exhibited the highest MCH consumption rate,which was approximately two times higher than that of the catalyst without ***,the incorporation of Fe inhibited the formation of coke and reduced the quantity of coke deposits on the catalyst,thereby improving its catalytic ***,Fe shows promise as a prospective secondary element for Pt/Al_(2)O_(3) to enhance the MCH dehydrogenation performance.

关键词： methylcyclohexane dehydrogenation hydrogen storage deactivation Fe addition

Very long wave infrared quantum dot photodetector up to 18μm

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Light(Science & Applications) 2024年第4期13卷 772-782页

作者： Xiaomeng Xue Qun hao Menglu Chen School of Optics and Photonics Beijing Institute of TechnologyBeijing 100081China. Westlake Institute for Optoelectronics FuyangHangzhou 311421China. Physics Department Changchun University of Science and TechnologyChangchun 130022China

Colloidal quantum dots(CQDs)are of interest for optoelectronic devices because of the possibility of high-throughput solution processing and the wide energy gap tunability from ultraviolet to infrared *** may question about the upper limit on the CQD wavelength *** date,although the CQD absorption already reaches terahertz,the practical photodetection wavelength is limited within mid-wave *** figure out challenges on CQD photoresponse in longer wavelength,would reveal the ultimate property on these ***’s more,it motivates interest in bottom-up infrared photodetection with less than 10%cost compared with epitaxial growth semiconductor *** this work,developing a re-growth method and ionic doping modification,we demonstrate photodetection up to 18μm wavelength on HgTe *** liquid nitrogen temperature,the responsivity reaches 0.3 A/W and 0.13 A/W,with specific detectivity 6.6×108 Jones and 2.3×109 Jones for 18μm and 10μm CQD photoconductors,*** work is a step toward answering the general question on the CQD photodetection wavelength limitation.

关键词： quantum wave ultraviolet

CFD-DEM study of impacts of the porous distributor medium on fluidization characteristics of a 2D-fluidized bed

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Particuology 2024年第4期87卷 54-73页

作者： Fei Wang Yishan Zeng hao Yan School of Mechanical Engineering Hefei University of TechnologyHefei230009China

Gas-solid bubbling fluidized beds are widely used in chemical,energy,construction,and other industrial fields due to their excellent fluidization performance.2D-fluidized beds with planar rectangular columns of finite thickness are widely used in fluidized bed studies,and it is essential for understanding the hydrodynamics of gas-particle ***,the distributor(porous medium)at the bottom of the bed has a crucial influence on the fluidization performance of the 2D-fluidized *** this work,the fluidization mechanism and gas-solid dynamic characteristics of the fluidized bed under three porous media are studied by CFD-DEM coupled with the porous medium model,and the accuracy of numerical simulation is verified by a high-speed photography *** show that with the increase in the flow resistance of the porous medium,the average and standard deviation of the bubble diameter decrease,and the time and position of particles in the dead zone to participate in the core-annular flow *** a low fluidization velocity,the dead zone in the bed can be considerably reduced by increasing the flow resistance.

关键词： Fluidized bed CFD-DEM Porous medium Bubble dynamics Solid mixing

Challenges and perspectives of air pollution control in China

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Frontiers of Environmental Science & Engineering 2024年第6期18卷 9-16页

作者： Bin Zhao Shuxiao Wang Jiming hao State Key Joint Laboratory of Environmental Simulation and Pollution Control School of EnvironmentTsinghua UniversityBeijing 100084China State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex Beijing 100084China

Air pollution is one of the most challenging environmental issues in the *** has achieved remarkable success in improving air quality in last decade as a result of aggressive air pollution control ***,the average fine particulate matter(PM2.5)concentration in China is still about six times of the World Health Organization(WHO)Global Air Quality Guidelines(AQG)and causing significant human health *** emission reductions of multiple air pollutants are required for China to achieve the *** we identify the major challenges in future air quality improvement and propose corresponding control *** main challenges include the persistently high health risk attributed to PM2.5 pollution,the excessively loose air quality standards,and coordinated control of air pollution,greenhouse gases(GHGs)emissions and emerging *** further improve air quality and protect human health,a health-oriented air pollution control strategy shall be implemented by tightening the air quality standards as well as optimizing emission reduction pathways based on the health risks of various *** the meantime,an“oneatmosphere”concept shall be adopted to strengthen the synergistic control of air pollutants and GHGs and the control of non-combustion sources and emerging pollutants shall be enhanced.

关键词： Air pollution China Health impact Air quality standards GHGs Emerging pollutants

Discovery of Partial Differential Equations from Highly Noisy and Sparse Data with Physics-Informed Information Criterion

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Research 2024年第1期2023卷 247-259页

作者： hao Xu Junsheng Zeng Dongxiao Zhang BIC-ESAT EREand SKLTCSCollege of EngineeringPeking UniversityBeijing 100871P.R.China Institute of Applied Physics and Computational Mathematics Beijing 100088P.R.China Eastern Institute for Advanced Study Eastern Institute of TechnologyNingbo 315200ZhejiangP.R.China National Center for Applied Mathematics Shenzhen(NCAMS) Southern University of Science and TechnologyShenzhen 518055GuangdongP.R.China Department of Mathematics and Theories Peng Cheng LaboratoryShenzhen 518000GuangdongP.R.China

Data-driven discovery of partial differential equations(PDEs)has recently made tremendous progress,and many canonical PDEs have been discovered successfully for proof of ***,determining the most proper PDE without prior references remains challenging in terms of practical *** this work,a physics-informed information criterion(PIC)is proposed to measure the parsimony and precision of the discovered PDE *** proposed PIC achieves satisfactory robustness to highly noisy and sparse data on 7 canonical PDEs from different physical scenes,which confirms its ability to handle difficult *** PIC is also employed to discover unrevealed macroscale governing equations from microscopic simulation data in an actual physical *** results show that the discovered macroscale PDE is precise and parsimonious and satisfies underlying symmetries,which facilitates understanding and simulation of the physical *** proposition of the PIC enables practical applications of PDE discovery in discovering unrevealed governing equations in broader physical scenes.

关键词： process canonical proof

Numerical study on local failures of reinforced concrete slabs against underwater close-in explosions

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Journal of Zhejiang University-Science A(Applied Physics & Engineering) 2024年第8期25卷 650-669页

作者： Fei ZHOU Hedong LI hao WU College of Civil Engineering Tongji UniversityShanghai 200092China School of Civil Engineering and Architecture Zhejiang Sci-Tech UniversityHangzhou 310018China

Reinforced concrete(RC)slabs are the primary load-carrying member of underwater *** can suffer severe local failures such as cratering,spalling,or breaching as a result of underwater close-in(UWCI)*** this study,we established a fully validated high-fidelity finite element analysis approach to precisely reproduce the local failures of RC slabs after a UWCI explosion.A recently proposed dynamic constitutive model is used to describe wet *** effects of free water content on the material properties,including the tensile/compressive strength,elastic modulus,strain rate effect,failure strength surface,and equation of state,are comprehensively calibrated based on existing test *** calibrated material parameters are then verified by a single-element test.A high-fidelity finite element analysis(FEA)approach of an RC slab subjected to a UWCI explosion is established using an arbitrary Lagrangian-Eulerian(ALE)*** previous UWCI explosion tests on RC orifice targets and underwater contact explosion tests on saturated concrete slabs showed that the established FEA approach could accurately reproduce the pressure-time history in water and damage patterns,including the cracking,cratering,and spalling,of the RC orifice target and saturated concrete ***,parametric studies conducted by simulating an RC slab subjected to a UWCI explosion showed that:(i)the local failure of an RC slab enlarges with increased charge weight,reduced standoff distance,and reduced structural thickness;(ii)compared to a water-backed RC slab,an air-backed RC slab exhibits much more obvious local and structural ***,to aid the anti-explosion design of relevant underwater facilities,based on over 90 simulation cases empirical formulae are summarized to predict local failure modes,i.e.,no spall,spall,and breach,of water-and air-backed RC slabs subjected to a UWCI explosion.

关键词： Reinforced concrete slab(RC) Underwater close-in(UWCI)explosion Saturated concrete Failure modes Numerical simulation

Polyelectrolyte Complexes and Coacervates Formed by De novo-Designed Peptides and Oligonucleotide

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Chinese Journal of Polymer Science 2024年第9期42卷 1333-1340,I0007页

作者： Tian-hao Ren De-Hai Liang Beijing National Laboratory for Molecular Sciences Department of Polymer Science and Engineering and the Key Laboratory of Polymer Chemistry and Physics of the Ministry of EducationCollege of Chemistry and Molecular EngineeringPeking UniversityBeijing100871China

The liquid-liquid phase separation of biopolymers in living cells contains multiple interactions and occurs in a dynamic *** the regulation mechanism is still a *** this work,we designed a series of peptides(XXLY)_(6)SSSGSS and studied their complexation and coacervation behavior with single-stranded ***“X”and“Y”are varied to combine known amounts of charged and non-charged amino acids,together with the introduction of secondary structures and pH *** show that the electrostatic interaction,which is described as charge density,controls both the strength of complexation and the degree of chain relaxation,and thus determines the growth and size of the *** hydrophobic interaction is prominent when the charges are ***,the secondary structures of peptides exhibit profound effect on the morphology of the phases,such as solid phase to liquid phase *** study gains insight into the phase separation under physiological *** is also helpful to create coacervates with desirable structures and functions.

关键词： Polyelectrolyte complex Coacervate Peptides Secondary structure Electrostatic interaction