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Carbon nanostructures produced through ion irradiation

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Nuclear Science and Techniques 2003年第2期14卷 107-114页

作者： YU Li-Ping, WANG Zhen-Xia, ZHU Zhi-Yuan, ZhanG Hu-Yong, han jia-guang, ZhanG Wei, SUN Li-Tao,WANG Ting-Tai, MA Yu-Gang (Shanghai Institute of Nuclear Research, the Chinese Academy of Sciences, Shanghai 201800) Shanghai Institute of Nuclear Research the Chinese Academy of Sciences 上海 201800

Several nanostructures we produced by ion irradiation have been reviewed in this paper. By using ions to irradiate two ultrahigh molecular weight polyethylene targets respectively, it was found that small fullerenes C20 and C26 were grown, adding two members to the fullerene family. Meanwhile, crystalline diamonds also have been produced by Ar+ ions irradiation of graphite. In the experiment of double ions Ni+ and Ar+ irradiation, nanoscale argon bubbles formed. On the other side, when multi-wall carbon nanotubes were irradiated by C+, many MWCNTs evolved to amorphous carbon nanowires and amorphous carbon nanotubes. And there are possible welding in the crossed nanotubes.

关键词：碳纳米结构离子辐射聚乙烯

The electromagnetic Casimir effect of spherical cavity

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Nuclear Science and Techniques 2003年第2期14卷 104-106页

作者： han jia-guang, YU Li-Ping, WANG Zhen-Xia, ZHU Zhi-Yuan (Shanghai Institute of Nuclear Research, the Chinese Academy of Sciences, Shanghai 201800) Shanghai Institute of Nuclear Research the Chinese Academy of Sciences 上海 201800

The Casimir effect results from the zero-point energy of vacuum. A spherical cavity can be divided into three regions, and we make an analysis of every region and then give a formal solution of Casimir energy. The zeta-function regularization is also used to dispel the divergence of the summation. At the end, we can see the Casimir effect of a single sphere is included in our results.

关键词：球形穴电磁Casimir效应零点能 zeta函数

16.48% Efficient solution-processed CIGS solar cells with crystal growth and defects engineering enabled by Ag doping strategy

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Journal of Energy Chemistry 2025年第1期100卷 59-65页

作者： Mengyu Xu Shaocong Yan Ting Liang jia jia Shengjie Yuan Dongxing Kou Zhengji Zhou Wenhui Zhou Yafang Qi Yuena Meng Litao han Sixin Wu Key Laboratory for Special Functional Materials of MOE National & Local Joint Engineering Research Centre for High-efficiency Display and Lighting Technology School of Nanoscience and Materials Engineering Henan University

Solution-processed Cu（In,Ga）Se2（CIGS） solar cells suffer from serious carrier recombination and power conversion efficiency（PCE） loss because of the poor film properties and easy formation of ***, we propose Ag&Se co-selenization strategy to enhance the crystallization and passivate harmful defects of the CIGS films. The formation of Ag-Se phase during the selenization process enables the formation of large grains and suppresses the deep level defects. It is found that Ag doping can enlarge the depletion region width, lower the Urbach energy and prolong the carrier lifetime. As a result, a champion solution-processed CIGS solar cell presents a high efficiency of 16.48% with the highly improved opencircuit voltage（VOC） of 662 m V and fill factor（FF） of 75.8%. This work provides an efficient strategy to prepare high quality solution-processed CIGS films for high-performance CIGS solar cells.

关键词： CIGS solar cells Solution-processed method Ag doping Crystal growth Defects engineering

Anomalous quality factor evolution of induced transparency in a virtualized coupled-oscillator system

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Science China(Physics,Mechanics & Astronomy) 2025年第1期Mechanics & Astronomy) .卷 148-155页

作者： Yunhan Yang han jia Tuo Liu Yuzhen Yang Jun Yang Key Laboratory of Noise and Vibration Research Institute of Acoustics Chinese Academy of Sciences University of Chinese Academy of Sciences State Key Laboratory of Acoustics Institute of Acoustics Chinese Academy of Sciences

The phenomenon of induced transparency, characterized by a high quality(Q) factor, holds significant importance in the fields of high-precision sensing, energy storage and wave manipulation. Conventional transparency systems are often constrained by the limited experimentally accessible parameter space and the lack of independent control over intrinsic parameters, thereby hindering advanced research on high-Q effects. Here we propose a virtualized coupled-oscillator system that enables reconfigurable induced transparency in the reflection spectrum. By virtually incorporating a pair of coupled oscillators into an individual acoustic meta-atom, we achieve the manipulation of induced transparency in a decoupled, wide-ranging, and elaborate manner. Exploiting the diverse evolutions across the intrinsic parameter space, we show experimentally a counter-intuitive increase in the Q-factor of the transparency window, which is attributed to the enhanced dissipation of the bright ***, a constant group delay at the center frequency is observed accompanying this evolution. Our work demonstrates an intriguing platform as well as a novel strategy to engineer high-Q induced transparency phenomenon, and paves the way towards applications in programmable acoustic sensors, filters and slow-wave devices.

关键词： induced transparency acoustic meta-atom high quality-factor scattering programmable intrinsic parameter

Synergistic promotion strategy of “dual-site” and “dual-path” to enhance the C–C coupling between CO2 and HCHO driven by photoelectrocatalysis

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Journal of Energy Chemistry 2025年第1期100卷 39-49页

作者： Hongqiang Yang jianfeng Zheng Guoyu Wang Yifei Gao Yatao Yang jia Li Xiaojin han Yan Cui Zhanggen Huang National Key Laboratory of High Efficiency and Low Carbon Utilization of Coal Institute of Coal Chemistry Chinese Academy of Science University of Chinese Academy of Science Shenyang University of Chemical Technology

Photoelectrocatalytic coupling CO2and volatile organic compounds （VOCs） is a promising green strategy for the synergistic conversion of the two carbon-containing resources to *** catalytic efficiency is always at the mercy of chemical inertness of CO2and the competitive hydrogen evolution of ***,a modified g-C3N4/ZnAl-LDH Z-scheme heterojunction catalyst with dual reaction site was rationally designed and precisely *** Faraday efficiency of ethanol reached 68.67%with a corresponding formation rate of 227.3μmol *** revealed by in-situ characterizations and density functional theory calculations,CO2and HCHO were absorbed at Zn site and N site,***,*CO generated from CO2and HCHO was converted to*CH3O and*CHO on the dual-active-site *** detailed reaction mechanism experiments indicated that C–C coupling only occurred between*CO and*CH3O in electrocatalysis *** from the“*CO+*CH3O”path,another“*CO+*CHO”coupling path was also detected in photoelectrocatalytic *** selectivity of ethanol was significantly enhanced due to the synthesis of dual-site catalyst and the dual-path coupling path between CO2and HCHO simultaneously driven by light and electricity.

关键词： Photoelectrocatalysis Z-scheme C–C coupling Ethanol

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基于太赫兹光谱的平面应力测量方法

实验力学 2015年第1期30卷 17-22页

作者：张旭王世斌李林安王志勇韩家广天津大学机械工程学院力学系天津300072 天津大学精密仪器与光电子工程学院太赫兹研究中心天津300072

本文提出了一种基于太赫兹光谱技术的平面应力状态测量方法。该方法在传统的太赫兹时域光谱系统中引入起偏镜和检偏镜,实现了对太赫兹脉冲偏振态的调控。针对该实验系统,建立了试件所受应力与穿透试件的太赫兹波相位延迟之间的定量关系... 详细信息

本文提出了一种基于太赫兹光谱技术的平面应力状态测量方法。该方法在传统的太赫兹时域光谱系统中引入起偏镜和检偏镜,实现了对太赫兹脉冲偏振态的调控。针对该实验系统,建立了试件所受应力与穿透试件的太赫兹波相位延迟之间的定量关系,并提出了根据实验所测太赫兹波相位延迟计算平面应力状态三个应力参量的数据处理方法。将该方法得到的实验结果和应变仪测量的结果作对比,发现两种方法有很好的一致性,证明此实验方法合理可靠。

关键词：太赫兹光谱系统相位变化应力分量

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L-天冬酰胺及其一水合物的太赫兹光谱研究

物理学报 2014年第13期63卷 97-103页

作者：杨静琦李绍限赵红卫张建兵杨娜荆丹丹王晨阳韩家广天津大学太赫兹波研究中心天津大学精密仪器与光电子工程学院光电信息技术教育部重点实验室天津300072 中国科学院上海应用物理研究所上海201800

本文利用太赫兹时域光谱技术测量了室温条件下无水L-天冬酰胺与L-天冬酰胺一水合物的光谱特征,发现二者存在显著的差异,并利用太赫兹时域光谱技术实时检测L-天冬酰胺一水合物受热脱水的动态过程.结果表明太赫兹波对晶体结构变化、含结... 详细信息

本文利用太赫兹时域光谱技术测量了室温条件下无水L-天冬酰胺与L-天冬酰胺一水合物的光谱特征,发现二者存在显著的差异,并利用太赫兹时域光谱技术实时检测L-天冬酰胺一水合物受热脱水的动态过程.结果表明太赫兹波对晶体结构变化、含结晶水状况以及分子间弱相互作用敏感.结合差示扫描量热法与热重分析联用、傅里叶变换红外光谱、粉末X射线衍射等多种技术分别从热学性质、分子振动等方面进行了表征,进一步确认了太赫兹实验结果的可靠性.采用基于密度泛函理论(DFT)的第一性原理平面波赝势方法,结合广义梯度近似(GGA)下的PBE交换-关联泛函,对L-天冬酰胺一水合物进行模拟计算,对实验所得太赫兹光谱与分子结构以及相互作用间的关系进行了讨论分析.

关键词： L-天冬酰胺太赫兹时域光谱特征吸收结晶水

缩比模型的宽频时域太赫兹雷达散射截面(RCS)研究

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物理学报 2014年第21期63卷 85-94页

作者：梁达川魏明贵谷建强尹治平欧阳春梅田震何明霞韩家广张伟力天津大学太赫兹研究中心精密仪器域光电子工程学院光电信息技术教育部重点实验室天津300072 合肥工业大学光电技术研究院合肥230009

本文首次以钛宝石飞秒激光振荡级为抽运源,搭建了国内首套宽频时域太赫兹雷达(带宽0.1—1.3 THz)并进行了基于标准球的系统校正验证.利用该雷达测量了太赫兹波段三种缩比模型的散射时域信号.通过改进后的后向投影算法对模型的轮廓外形... 详细信息

本文首次以钛宝石飞秒激光振荡级为抽运源,搭建了国内首套宽频时域太赫兹雷达(带宽0.1—1.3 THz)并进行了基于标准球的系统校正验证.利用该雷达测量了太赫兹波段三种缩比模型的散射时域信号.通过改进后的后向投影算法对模型的轮廓外形进行了成像研究,验证了新型时域散射信号成像机理.太赫兹雷达更高的频率,宽谱的特征和高分辨率成像的能力有望用于隐形外形设计过程,成为新兴的太赫兹散射特征研究平台.

关键词：太赫兹雷达雷达散射截面成像

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太赫兹亚波长人工结构传感应用

物理 2013年第12期42卷 838-845页

作者：田震谷建强韩家广 J.F.O'Hara 张伟力天津大学太赫兹研究中心天津大学精密仪器与光电子工程学院天津300072 俄克拉荷马州立大学电子与计算机工程系美国俄克拉荷马州静水城74078

近年来,太赫兹科学技术在快速发展,它在毒品、爆炸物、有毒危险品等安全检查及反恐怖方面展现出独特的应用前景。常用的自由空间太赫兹时域光谱技术,尽管具有很多优越性和良好的应用前景,但影响其性能提高和进一步推广应用的一些实际问... 详细信息

近年来,太赫兹科学技术在快速发展,它在毒品、爆炸物、有毒危险品等安全检查及反恐怖方面展现出独特的应用前景。常用的自由空间太赫兹时域光谱技术,尽管具有很多优越性和良好的应用前景,但影响其性能提高和进一步推广应用的一些实际问题仍然存在,如对光斑尺寸和样品体积、质量要求等。近年来,随着亚波长人工结构(包括超材料和表面等离子激元器件)的出现,为该问题的解决提供了新的契机。文章综述了作者在太赫兹亚波长人工结构器件传感应用所开展的一系列研究工作,其中包括薄膜材料传感、不同标号汽油传感以及同位素传感等,显著地提高了被测物质的探测灵敏度,同时降低了对被测物质的体积、质量要求,实现了高灵敏、微量物质传感,为太赫兹安全检查及反恐怖应用提供了技术借鉴。此外,文章还介绍了太赫兹亚波长人工结构传感器件未来的发展前景和面临的挑战。

关键词：太赫兹亚波长人工结构传感