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Water-mediated phase-change composite electrolyte

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Green Energy & Environment 2020年第3期5卷 249-250页

作者： Mingyang Liu buxing han Beijing National Laboratory for Molecular Sciences CAS Key Laboratory of ColloidInterface and Chemical ThermodynamicsCAS Research/Education Center for Excellence in Molecular SciencesInstitute of ChemistryChinese Academy of SciencesBeijing100190China School of Chemistry and Chemical Engineering University of Chinese Academy of SciencesBeijing100049China

With the world's focus on wearable electronics, the scientific community has anticipated the plasticine-like processability of electrolytes and electrodes. A bioinspired composite of polymer and phase-changing salt with the similar bonding structure to that of natural bones is a suitable electrolyte candidate. Here, Wang et al. reported a water-mediated composite electrolyte by simple thermal mixing of crystallohydrate and polymer. The processable phase-change composites have significantly high mechanical strength and high ionic mobility.

关键词： Electrolyte Energy storage Electronic devices

Selective production of diethyl maleate from lignin

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Green Energy & Environment 2019年第4期4卷 343-344页

作者： buxing han Beijing National Laboratory for Molecular Sciences Institute of Chemistry Chinese Academy of Sciences

Lignin is an abundant and renewable carbon resource and also a by-product in the paper *** of lignin into valuable chemicals and liquid fuels has attracted extensive *** lignin depolymerization is a potentially important strategy to reduce fossil resource ***,lignin is an underutilized resource of biomass compared to either cellulose or *** has great potential for the generation of biochemicals and fuels due to its highly aromatic structure[1].However,efficient utilization of lignin requires the selective breakdown of the recalcitrant polymeric structure[1–3].Catalytic oxidation is one of the most promising routes to depolymerize lignin,which can produce value-added chemicals,such as phenols,quinines,and dicarboxylic acids[4].Nevertheless,controlling the oxidative pathways of lignin and its intermediates to get pure chemicals is a great challenge because of the complex structure of lignin.

关键词： lignin oxidative utilized

Green chemistry: a tool for the sustainable development of the chemical industry

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National Science Review 2015年第3期2卷 255-256页

作者： Jinliang Song buxing han Institute of Chemistry Chinese Academy of Sciences

Most manufactured products involve one or more chemical *** cannot imagine what our life will be like without the products produced by the chemical ***,on average,only a small proportion of the resources we take from the Earth is converted into the desired products in current chemical processes,and large amounts of wastes and hazardous materials are *** to supply humanity with enough food,

关键词： a tool for the sustainable development of the chemical industry Green chemistry

Ionic liquid-based electrolytes for CO2 electroreduction and CO2 electroorganic transformation

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National Science Review 2022年第4期9卷 168-185页

作者： Xingxing Tan Xiaofu Sun buxing han Beijing National Laboratory for Molecular Sciences CAS Key Laboratory of Colloid and Interface and ThermodynamicsCAS Research/Education Center for Excellence in Molecular SciencesInstitute of ChemistryChinese Academy of Sciences School of Chemistry and Chemical Engineering University of Chinese Academy of Sciences Shanghai Key Laboratory of Green Chemistry and Chemical Processes School of Chemistry and Molecular EngineeringEast China Normal University

CO;2;is an abundant and renewable C1 *** transformation of CO;2;can integrate CO;2;fixation with renewable electricity storage,providing an avenue to close the anthropogenic carbon *** a new type of green and chemically tailor able solvent,ionic liquids（ILs） have been proposed as highly promising alternatives for conventional electrolytes in electrochemical CO;2;*** review summarizes major advances in the electrochemical transformation of CO;2;into value-added carbonic fuels and chemicals in IL-based media in the past several *** the direct CO;2;electroreduction（CO;2;ER）and CO;2;-involved electro organic transformation（CO;2;EOT） are discussed,focusing on the effect of electrocatalysts,IL components,reactor configurations and operating conditions on catalytic activity,selectivity and *** reasons for the enhanced CO;2;conversion performance by ILs are also discusse d,providing guidance for the rational design of novel IL-based electro chemical processes for CO;2;***,the critical challenges remaining in this research area and promising directions for future research are proposed.

关键词： ionic liquid carbon dioxide electrocatalysis green synthesis value-added fuels and chemicals

Transformation of CO2 and H2 to C2+ chemicals and fuels

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National Science Review 2023年第9期10卷 17-19页

作者： Qingli Qian buxing han Beijing National Laboratory for Molecular Sciences CAS Key Laboratory of Colloid Interface and Chemical Thermodynamics CAS Research/Education Center for Excellence in Molecular Sciences Center for Carbon Neutral Chemistry Institute of ChemistryChinese Academy of Sciences 2. Physical Science Laboratory Huairou National Comprehensive Science Center School of Chemistry and Chemical Engineering University of Chinese Academy of Sciences Shanghai Key Laboratory of Green Chemistry and Chemical Processes School of Chemistry and Molecular Engineering East China Normal University

CO2is a greenhouse gas,and is also a cheap,easily available and renewable carbon *** of CO2into chemicals has been extensively investigated in the forms of thermo catalysis,electrocatalysis and photo ***2is the highes...

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Large Scale Synthesis of Transition Metal Single Atom Catalysts by a Universal Ligand Mediated Method

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Chemical Research in Chinese Universities 2019年第6期35卷 951-952页

作者： han buxing Institute of Chemistry Chinese Academy of SciencesBeijing 100190P.R.China

Series of transition metal single atom catalysts containing Cr,Mn,Fe,Co,Ni,Cu,Zn,Ru,Pt or combinations thereof were synthesized in a large scale by a universal ligand mediated *** as-synthesized single atom catalysts ... 详细信息

关键词： method. Transition catalysts

Basic ionic liquids promoted chemical transformation of CO_2 to organic carbonates

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Science China Chemistry 2018年第12期61卷 1486-1493页

作者： Jiayin Hu Huizhen Liu buxing han Tianjin Key Laboratory of Marine Resources and Chemistry College of Chemical Engineering and Materials ScienceTianjin University of Science and Technology Beijing National Laboratory for Molecular Sciences CAS Key Laboratory of Colloid Interface and Chemical ThermodynamicsInstitute of Chemistry Chinese Academy of Sciences

Ionic liquids(ILs), especially basic ILs with unique physicochemical properties, have wide application in catalysis. Using basic ILs as catalysts for the conversion of cheap, abundant, nontoxic, and renewable CO_2 into value-added organic carbonates is highly significant in view of environmental and economic issues. This review aims at giving a detailed overview on the recent advances on basic ILs promoted chemical transformation of CO_2 to cyclic and linear carbonates. The structures of various basic ILs, as well as the basic ILs promoted reactions for the transformation of CO_2 to organic carbonates are discussed in detail,including the reaction conditions, the yields of target products, the catalytic activities of basic ILs and the reaction mechanism.

关键词： basic ionic liquid CO_2 chemical transformation organic carbonates

Preface:special issue on green chemistry

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Science China Chemistry 2017年第7期60卷 837-838页

作者： Mingyuan He buxing han Research Institute of Petrochem Processing SINOPECBeijing 100083China Shanghai Key Laboratory of Green Chemistry&Chemical Processes Department of ChemistryEast China Normal UniversityShanghai 200062China Beijing National Laboratory for Molecular Sciences CAS Key Laboratory of Colloid and Interface and ThermodynamicsInstitute of ChemistryChinese Academy of SciencesBeijing 100190China University of Chinese Academy of Sciences Beijing 100049China

The growing up of green chemistry has now a history of more than twenty years,with a blooming development demonstrated by its great contribution to sustainable development and economical benefit to our *** is well acc... 详细信息

关键词： sustainable economical morethan manufacture hazardous creativity technological reflecting imagination biomass

Special Topic on Ionic Liquids： Energy, Materials ＆ Environment

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Science China Chemistry 2016年第5期59卷 505-506页

作者： Suojiang Zhang buxing han Jianji Wang Beijing Key Laboratory of Ionic Liquids Clean Chemical Process Institute of Process and EngineeringChinese Academy of SciencesBeijing 100190China Beijing National Laboratory for Molecular Sciences CAS Key Laboratory of ColloidInterface and Chemical ThermodynamicsInstitute of ChemistryChinese Academy of SciencesBeijing 100190China Collaborative Innovation Center of Henan Province for Green Manufacturing of Fine Chemicals Key Laboratory of Green Chemical Media and ReactionsMinistry of EducationSchool of Chemistry and Chemical EngineeringHenan Normal UniversityXinxiang 453007China

Ionic liquids （ILs） are organic salts with low melting points, which have many unusual properties like negligible vapor pressure, good thermal stability, non-flammability, wide liquid range and electrochemical window, and excellent solvation power for both organic and inorganic substances. The unique characteristics of ILs endow them with great potential for applications in different fields including chem- ical reactions, extraction and separation, material science, renewable energy, environment, and photoelectric trans- formations. Their properties can be tuned to suit various applications by changing the structures of the cations and/or anions.

关键词： Chemistry Synthesis (chemical)