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Platinum quantum dots-decorated MXene-derived titanium dioxide nanowire/Ti_(3)C_(2) heterostructure for use in solar-driven gas-phase carbon dioxide reduction to yield value-added fuels

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Journal of Energy Chemistry 2023年第7期82卷 627-637,I0013页

作者： Kamakshaiah Charyulu Devarayapalli S.V.Prabhakar Vattikuti Dong Jin kim Youngsu Lim Bolam kim gyuhyeon kim Dae Sung Lee Department of Environmental Engineering Kyungpook National UniversityBuk-guDaegu 41566Republic of Korea Research Institute of Environmental Science&Technology Core Research InstituteKyungpook National UniversityBuk-guDaegu 41566Republic of Korea School of Mechanical Engineering Yeungnam UniversityGyeongsan 38541Republic of Korea School of Architecture CivilEnvironmental and Energy EngineeringKyungpook National UniversityBuk-guDaegu 41566Republic of Korea

Solar-driven photocatalytic CO_(2) reduction to produce valuable chemicals and fuels offers an attractive strategy in alleviating the energy *** quantum dots(PtQDs)with TiO_(2) nanowire(TiO_(2)NW)/Ti_(3)C_(2) MXene heterostructures(Pt-TiO_(2)NW/Ti_(3)C_(2)) with tight interfacial contacts between the various components were prepared at room temperature via oxidation *** incorporated PtQDs played crucial roles as electron conduction bridges supported by the cocatalyst effect,effectively enhancing the separation efficiencies of photoinduced electron/hole pairs and improving CO_(2) reduction under simulated solar light *** Pt-TiO_(2)NW/Ti_(3)C_(2) heterostructures exhibited remarkable carbon monoxide(CO)and methane(CH_(4)) production at respective rates of 38.14 and 36.15μmol g^(-1)after 10 h of simulated solar light irradiation,an apparent quantum yield of 1.68%,and 79.2%selectivity for *** photocatalytic activities of the Pt-TiO_(2) NW/Ti_(3)C_(2) heterostructures for CO_(2) reduction were significantly enhanced compared to those of TiO_(2)NW/Ti_(3)C_(2) and the single-component photocatalysts,and they exhibited remarkable stabilities even after five *** addition,the densities of states and electronic characteristics of Ti_(3)C_(2) MXene and Pt-TiO_(2)NW/Ti_(3)C_(2) were studied using density functional theory,and a synergistic mechanism of the improvement in CO_(2) photoreduction is proposed.

关键词： MXene CO_(2)reduction Density functional theory Quantum dot Photocatalyst

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