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Chinese Chemical Letters 2024年第8期35卷 545-548页

作者： Junhua Wang Xin Lian Xichuan Cao Qiao Zhao Baiyan Li Xian-He bu School of Materials Science and Physics China University of Mining and TechnologyXuzhou 221116China School of Chemical Engineering and Technology China University of Mining and TechnologyXuzhou 221116China School of Materials Science and Engineering National Institute for Advanced MaterialsTKL of Metal and Molecule-Based Material ChemistryNankai UniversityTianjin 300350China

The purification of low-grade coal-bed methane is extremely important,but challenging,due to the very similar physical properties of CH_(4)and ***,we proposed a dual polarization strategy by employing triazine and polyfluoride sites to construct polar pores in COF materials,achieving the efficient separa-tion of CH_(4)from *** expected,the dual polarized F-CTF-1 and F-CTF-2 exhibit higher CH_(4)adsorption capacity and CH_(4)/n_(2)selectivity than CTF-1 and CTF-2,***,the CH4 uptake capacity and CH_(4)/n_(2)selectivity of F-CTF-2 is 1.76 and 1.42 times than that of *** work not only developed promising COF materials for CH4/n_(2)separation,but also provided important guidance for the separation of other adsorbates with similar properties.

关键词： Dual polarization strategy Covalent organic frameworks(COFs) Coal-bed methane purification Chemical/thermal stability Cycling stability

Combination of nitrogen-Rich Skeleton and Coordination Group:Synthesis of a High-Energy Primary Explosive Based on 1H-Tetrazole-5-Carbohydrazide

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Defence Technology（防务技术） 2024年第1期31卷 271-277页

作者： Tingwei Wang Zujia Lu Shu bu Baolong Kuang Lu Zhang Zhenxin Yi Kun Wang Shunguan Zhu Jianguo Zhang State Key Laboratory of Explosion Science and Technology Beijing Institute of TechnologyBeijing 100081China School of Chemical Engineering Nanjing University of Science and Technology200 Xiaolingwei StreetXuanwuNanjing 210094China Department of Chemistry Laboratory of Structure and Functional Regulation of Hybrid MaterialsAnhui UniversityMinistry of EducationHefei 230601China

The high energy coordination compounds Cu(TZCA)_(2)(ClO_(4))_(2)(ECCs-1) was prepared by 1H-tetrazole-5-carbohydrazide(TZCA) with a high energy skeleton and a strong coordination ability *** the same time,the reaction activity of the ligand was explored,and the single crystal structure of it and intermediate were *** structures of all substances were characterized by IR and *** the structure and composition of ECCs-1 are confirmed by ESP,AC,SEM and *** and chemical properties tests show that ECCs-1 has an acceptable thermal stability(T_(d)=177℃) and extremely sensitive mechanical stimulation(IS=1 J,FS=5 n).The comprehensive performance test results show that ECCs-1 has excellent initiation *** addition,the decomposition mechanism of ECCs-1 is explored from two aspects of experiment and theoretical calculation.

关键词： 1H-tetrazole-5-carbohydrazide Primary explosive Decomposition mechanism Coordination polymers Laser

Effect of red clover isoflavones on hormone, immune, inflammatory, and plasma biochemistry in lactating dairy cows

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Animal nutrition 2024年第1期16卷 306-312页

作者： Shiqi Zhang Xiaoyin Zhang Zhanbo Xiong Kexin Li Yuan Gao Ying bu nan Zheng Shengguo Zhao Jiaqi Wang State Key Laboratory of Animal nutrition Institute of Animal Sciences Chinese Academy of Agricultural Sciences Beijing 100193 China

This study was to conducted to investigate the effect of red clover isoflavones on the health indicated by immune status and blood biochemistry in dairy cows. Sixty-eight healthy Holstein lactating cows were randomly divided into four treatments (n= 17 per treatment) from 5 blocks according to milk yield using a randomized complete block design. no initial differences in parity (2.13 ± 1.21), days in milk (165 ± 21 d), and milk yield (33.93 ± 3.81 kg/d) between groups. Cows were fed the basal diet supplemented with 0, 2, 4, or 8 g/kg red clover extract (RCE) in diet (dry matter based). Feeding, refusal feed weights, and milk yield were recorded three consecutive days in weeks 0, 4, 8, and 12. Blood was collected from the tail vein of the cows on the last day of weeks 4, 8 and 12, 1 h after the morning feeding, and analyzed for hormones, immunoglobulins, inflammatory markers, and markers of liver and kidney activities. The dry matter intake was significantly decreased by 3.7% in the 8 g/kg group (Pnificantly higher in both of the 2 and 4 g/kg groups (Pnd prolactin showed a quadratic effect with increasing RCE levels, with the highest in the 4 g/kg group (Pnecrosis factor (TnF)-α, interleukin (IL)-6, and IL-1β levels decreased linearly with increasing dietary RCE levels. Plasma IL-18 levels showed a quadratic effect with increasing dietary RCE levels, with significantly lower levels in both of the 2 and 4 g/kg groups (Pnoglobulin A and D-lactic acid levels showed a quadratic effect with increasing dietary RCE levels, with significantly higher level in the 4 g/kg group (Pnction and kidney activity makers were similar (P> 0.05). These results recommend the supplementation of RCE at a level from 2 to 4 g/kg DM.

关键词： Dairy cow Red clover isoflavone Immunity Anti-inflammatory

Efficacy comparison of multipoint and single point scanning panretinal laser photocoagulation in non-proliferative diabetic retinopathy treatment

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World Journal of Diabetes 2024年第8期15卷 1734-1741页

作者： Yang-Zhou Zhang Hua Gong Juan Yang Ji-Pu bu Hui-Ling Yang Institute of Molecular Precision Medicine and Hunan Key Laboratory of Molecular Precision Medicine Xiangya HospitalCentral South UniversityChangsha 410008Hunan ProvinceChina Department of Ophthalmology Xingsheng HospitalYiyang 413200Hunan ProvinceChina Department of Ophthalmology Boshi Eye HospitalLiuyang 410300Hunan ProvinceChina Department of Ophthalmology Hunan Children‘s HospitalChangsha 410007Hunan ProvinceChina

BACKGROUnD non-proliferative diabetic retinopathy(nPDR)poses a significant challenge in diabetes management due to its microvascular changes in the *** photocoagulation,a conventional therapy,aims to mitigate the risk of progressing to proliferative diabetic retinopathy(PDR).AIM To compare the efficacy and safety of multi-spot vs single-spot scanning panretinal laser photocoagulation in nPDR *** Forty-nine nPDR patients(86 eyes)treated between September 2020 and July 2022 were *** were randomly allocated into single-spot(n=23,40 eyes)and multi-spot(n=26,46 eyes)*** outcomes,including bestcorrected visual acuity(BCVA),central macular thickness(CMT),and mean threshold sensitivity,were assessed at predetermined intervals over 12 *** reactions were also *** Energy levels did not significantly differ between groups(P>0.05),but the multi-spot group exhibited lower energy density(Pnd CMT improvements were noted in the multi-spot group at one-month posttreatment(Pn incidence was similar between groups(P>0.05).COnCLUSIOn While energy intensity and safety were comparable between modalities,multi-spot scanning demonstrated lower energy density and showed superior short-term improvements in BCVA and CMT for nPDR patients,with reduced laser-induced damage.

关键词： Panretinal laser photocoagulation non-proliferative diabetic retinopathy Efficacy comparison Multipoint Single point Treatment assessment

IMpower210:A phase Ⅲ study of second-line atezolizumab vs. docetaxel in East Asian patients with non-small cell lung cancer

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Chinese Journal of Cancer Research 2024年第2期36卷 103-113页

作者： Yi-Long Wu Shun Lu Gongyan Chen Jianxing He Jifeng Feng Yiping Zhang Liyan Jiang Hongming Pan Jianhua Chang Jian Fang Amy Cai Lilian bu Jane Shi Jinjing Xia Guangdong Lung Cancer Institute Guangdong Provincial Key Laboratory of Translational Medicine in Lung CancerGuangdong Provincial People's Hospital&Guangdong Academy of Medical SciencesSouthern Medical UniversityGuangzhou 510080China Shanghai Lung Cancer Center Shanghai Chest HospitalSchool of MedicineShanghai Jiao Tong UniversityShanghai 200025China Department of Respiration Harbin Cancer HospitalHarbin Medical UniversityHarbin 150081China Department of Thoracic Oncology and Surgery the First Affliated Hospital of Guangzhou Medical UniversityGuangzhou 510120China Department of Medical Oncology Jiangsu Cancer HospitalNanjing 210009China Department of Medical Oncology Zhejiang Cancer HospitalHangzhou 330022China Department of Pulmonary Medicine Shanghai Chest HospitalShanghai Jiao Tong UniversityShanghai 200030China Department of Medical Oncology Sir Run Run Shaw HospitalZhejiang University School of MedicineHangzhou 310016China Department of Medical Oncology Shenzhen HospitalCancer Hospital of Chinese Academy of Medical SciencesShenzhen 518116China Department of Thoracic Oncology Beijing Cancer HospitalBeijing 100142China Product Development Shanghai Roche Pharmaceutical LtdShanghai 201203China

Objective: IMpower210(nCT02813785) explored the efficacy and safety of single-agent atezolizumab *** as second-line treatment for advanced non-small cell lung cancer(nSCLC) in East Asian ***: Key eligibility criteria for this phase Ⅲ, open-label, randomized study included age ≥18 years;histologically documented advanced nSCLC per the Union for International Cancer Control/American Joint Committee on Cancer staging system(7th edition);Eastern Cooperative Oncology Group performance status of 0 or 1;and disease progression following platinum-based chemotherapy for advanced or metastatic nSCLC. Patients were randomized 2:1 to receive either atezolizumab(1,200 mg) or docetaxel(75 mg/m^(2)). The primary study endpoint was overall survival(OS) in the intention-to-treat(ITT) population with wild-type epidermal growth factor receptor expression(ITT EGFR-WT) and in the overall ITT ***: Median OS in the ITT EGFR-WT population(n=467) was 12.3 [95% confidence interval(95% CI),10.3-13.8] months in the atezolizumab arm(n=312) and 9.9(95% CI, 7.8-13.9) months in the docetaxel arm[n=155;stratified hazard ratio(HR), 0.82;95% CI, 0.66-1.03]. Median OS in the overall ITT population was 12.5(95% CI, 10.8-13.8) months with atezolizumab treatment and 11.1(95% CI, 8.4-14.2) months(n=377) with docetaxel treatment(n=188;stratified HR, 0.87;95% CI, 0.71-1.08). Grade 3/4 treatment-related adverse events(TRAEs) occurred in 18.4% of patients in the atezolizumab arm and 50.0% of patients in the docetaxel ***: IMpower210 did not meet its primary efficacy endpoint of OS in the ITT EGFR-WT or overall ITT populations. Atezolizumab was comparatively more tolerable than docetaxel, with a lower incidence of grade3/4 TRAEs.

关键词： Atezolizumab East Asia non-small cell lung cancer programmed death-ligand 1 inhibitors monoclonal antibody

Unveiling a novel metal-to-metal transition in LuH_(2):Critically challenging superconductivity claims in lutetium hydrides

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Matter and Radiation at Extremes 2024年第3期9卷 65-73页

作者： Dong Wang ningning Wang Caoshun Zhang Chunsheng Xia Weicheng Guo Xia Yin Kejun bu Takeshi nakagawa Jianbo Zhang Federico Gorelli Philip Dalladay-Simpson Thomas Meier Xujie Lü Liling Sun Jinguang Cheng Qiaoshi Zeng Yang Ding Ho-kwang Mao Center for High-Pressure Science and Technology Advanced Research Beijing 100094China Beijing national Laboratory for Condensed Matter Physics and Institute of Physics Chinese Academy of SciencesBeijing 100190China Shanghai Key Laboratory of Material Frontiers Research in Extreme Environments(MFree) Shanghai Advanced Research in Physical Sciences(SHARPS)Shanghai 201203China

Following the recent report by Dasenbrock-Gammon et al.[nature 615,244–250(2023)]of near-ambient superconductivity in nitrogendoped lutetium trihydride(LuH_(3-δ)n_(ε)),significant debate has emerged surrounding the composition and interpretation of the observed sharp resistance ***,we meticulously revisit these claims through comprehensive characterization and *** definitively identify the reported material as lutetium dihydride(LuH_(2)),resolving the ambiguity surrounding its *** similar conditions(270–295 K and 1–2 GPa),we replicate the reported sharp decrease in electrical resistance with a 30%success rate,aligning with the observations by Dasenbrock-Gammon et ***,our extensive investigations reveal this phenomenon to be a novel pressure-induced metal-to-metal transition intrinsic to LuH_(2),distinct from ***,nitrogen doping exerts minimal impact on this *** work not only elucidates the fundamental properties of LuH_(2)andLuH_(3),but also critically challenges the notion of superconductivity in these lutetium hydride *** findings pave the way for future research on lutetium hydride systems,while emphasizing the crucial importance of rigorous verification in claims of ambient-temperature superconductivity.

关键词： resistance hydride superconductivity

基于AR-ECM平均差异模型的串联电池组SOC、容量多尺度联合估计方法

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中国电机工程学报 2024年第10期44卷 3937-3948,I0016页

作者：刘芳余丹苏卫星卜凡涛天津市自主智能技术与系统重点实验室(天津工业大学) 天津市西青区300387 东软睿驰汽车技术(沈阳)有限公司辽宁省沈阳市110000

考虑电池单体老化差异所致的电池组不一致性,针对串联电池组荷电状态(state of charge,SOC)、容量估计问题,提出一种基于自回归等效电路模型(autoregression equivalent circuit model,AR-ECM)的平均差异模型(mean-difference model,MDM)。基于此模型,提出串联电池组SOC、容量多尺度联合估计算法。该算法由2个部分组成,一是基于AR-ECM的MDM及差异化模型参数辨识策略:条件辨识策略和定频分组辨识策略;二是基于多时间尺度H无穷滤波(multi-timescale H infinity filter,Mts-HIF)的电池组SOC、容量联合估计算法。通过将所提出MDM中的自回归平均模型(autoregression mean model,AR-MM)与传统MDM中的n阶RC平均模型(nRC mean model,nRC-MM)比较,结果表明所提出的AR-MM在复杂运行工况下具有更优的动态跟随性能。依据最小化信息量准则(akaike information criterion,AIC),AR-MM具有更优的复杂度与精度的权衡。通过与基于多时间尺度扩展卡尔曼滤波(multi-timescale extended Kalman filter,Mts-EKF)联合状态估计算法比较,结果表明所提出的Mts-HIF状态估计算法具有更优的鲁棒性、精度和收敛速度。

关键词：串联电池组自回归等效电路模型平均差异模型容量荷电状态 H无穷滤波

UASB-MSBR-混凝处理高浓度屠宰废水的研究与工业应用

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应用化工 2024年第4期53卷 982-985页

作者：陈步青湖南师范大学人事处湖南长沙410081

采用UASB-MSBR-混凝工艺处理某生猪屠宰场废水,总处理规模70 m^(3)/d,其工艺稳定运行7 d后,对COD、SS、nH_(3)-n、TP和动植物油的去除率分别达到97%,98%,94%,96%和97%,经处理后的出水达到国家《污水综合排放标准》(GB 8978—1996)一级... 详细信息

采用UASB-MSBR-混凝工艺处理某生猪屠宰场废水,总处理规模70 m^(3)/d,其工艺稳定运行7 d后,对COD、SS、nH_(3)-n、TP和动植物油的去除率分别达到97%,98%,94%,96%和97%,经处理后的出水达到国家《污水综合排放标准》(GB 8978—1996)一级排放标准。

关键词：高浓度屠宰废水 UASB MSBR 混凝

ERROR ESTIMATES FOR THE TIME DISCRETIZATIOn FOR nOnLInEAR MAXWELL'S EQUATIOnS

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Journal of Computational Mathematics 2008年第5期26卷 677-688页

作者： Mavián Slodika Ján bua Jr. Department of Mathematical Analysis Ghent University

This paper is devoted to the study of a nonlinear evolution eddy current model of the type δtB（H）＋ △↓× （ △↓ × H） =0 subject to homogeneous Dirichlet boundary conditions H × v = 0 and a given initial datum. Here, the magnetic properties of a soft ferromagnet are linked by a nonlinear material law described by B（H）. We apply the backward Euler method for the time discretization and we derive the error estimates in suitable function spaces. The results depend on the nonlinearity of B（H）.

关键词： Electromagnetic field nonlinear eddy current problem Time discretization,Error estimate.

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高速地铁隧道洞口及风井对压力波的影响研究

铁道工程学报 2024年第4期41卷 90-95,101页

作者：那艳玲牟野叶天震卜永和江崇旭中国铁路设计集团有限公司天津300308 天津大学天津300350

研究目的:地铁车辆由明线高速驶入隧道洞口和经过中间风井时,由于断面突变引起车厢内部压力剧烈波动,导致乘客不舒适,为解决该问题,本文使用三维可压缩黏性流体n-S方程和RnG k-ε两方程模型,研究不同中间风井位置和采取不同形式洞口缓... 详细信息

研究目的:地铁车辆由明线高速驶入隧道洞口和经过中间风井时,由于断面突变引起车厢内部压力剧烈波动,导致乘客不舒适,为解决该问题,本文使用三维可压缩黏性流体n-S方程和RnG k-ε两方程模型,研究不同中间风井位置和采取不同形式洞口缓冲结构工况对地铁隧道的空气动力学效应的影响。研究结论:(1)中间风井位置的不合理设置会导致膨胀波叠加使车厢内压力梯度不满足要求,可根据列车长度、列车运行速度等因素计算出中间风井的合理位置;(2)隧道洞口采取断面扩大型和喇叭型缓冲结构分别能使车厢表面压力梯度最大值下降29.3%和38.2%;(3)按照现行标准中人体舒适性的考核指标进行评价,140 km/h高速磁浮列车系统隧道口缓冲结构缓压段的长度设置为2倍的隧道断面水力直径更合理;(4)本文研究可以为优化高速地铁列车驶入隧道洞口时的气动效应问题提供参考。

关键词：高速地铁列车空气动力学压力波风井位置缓冲结构