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Synthesis,Structure and Chemical Bonding of Polyantimony Clusters Containing Coinage Metals[M_(2)Sb_(14)]^(4-)(M=Cu,Ag)

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Chinese Journal of Chemistry 2024年第6期42卷 617-622页

作者： Wei-xing Chen Yu-He Xu Cui-Cui Wang Lei Qiao Zi-Yan guo Wen-Juan Tian Zhong-Ming Sun State Key Laboratory of Element-Organic Chemistry Tianjin Key Lab for Rare Earth Materials and ApplicationsSchool of Materials Science and EngineeringNankai UniversityTianjin300350 China Institute of Molecular Science Shanxi UniversityTaiyuanShanxi030006 China

Binary polyantimony clusters,namely[Cu_(2)Sb_(14)]^(4–) and [Ag_(2)Sb_(14)]^(4–),containing coinage metals,were successfully synthesized and characterized,in which two homoatomic Sb73–subunits are bridged by two coinage metals in η^(4):η^(1) and η^(1):η^(1) coordination modes,***[M_(2)Sb_(14)]^(4-),two bridging Cu ions and two Sb atoms form a planar rhombic unit,which was revealed to have antiaromatic properties by theoretical *** electron structure and bonding analysis confirmed the presence of delocalized bonds in the rhombic unit and the metallophilic interaction between two formal M^(+) ions.

关键词： Polyantimony cluster Copper Silver Antiaromaticity Metallophilic interaction Quantum chemical calculations

Is there a place for endoscopic management in postcholecystectomy iatrogenic bile duct injuries?

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World Journal of Gastrointestinal Surgery 2024年第5期16卷 1218-1222页

作者： Hong-Qiao Cai guo-qiang Pan Shou-Jing Luan Jing Wang Yan Jiao Department of Hepatobiliary and Pancreatic Surgery General Surgery CenterThe First Hospital of Jilin UniversityChangchun 130021Jilin ProvinceChina Department of General Surgery Qilu HospitalShandong UniversityJinan 250000Shandong ProvinceChina Department of Endocrinology and Metabolism Weifang People’s HospitalWeifang 261041Shandong ProvinceChina Shandong Medical College Jinan 250000Shandong ProvinceChina

In this editorial we comment on the article by Emara et al published in the recent issue of the World Journal of Gastrointestinal ***,surgery was the primary treatment for bile duct injuries(BDI).The treatment of BDI has advanced due to technological breakthroughs and minimally invasive *** and percutaneous treatments have largely supplanted surgery as the primary treatment for most instances in recent *** management,including the specific technique,is typically impacted by local knowledge and the kind and severity of the *** therapy is a highly successful treatment for postoperative benign bile duct stenosis and offers superior long-term outcomes compared to surgical *** on the damage features of BDI,therapeutic options include endoscopic duodenal papillary sphincterotomy,endoscopic nasobiliary drainage,and endoscopic biliary stent implantation.

关键词： Post-cholecystectomy Iatrogenic Bile duct injuries Endoscopic management Benign bile duct stenosis

Enhancing growth, liver health, and bile acid metabolism of tilapia(Oreochromis niloticus) through combined cholesterol and bile acid supplementation in plant-based diets

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Animal Nutrition 2024年第2期17卷 335-346页

作者： Jiayuan Jiang xing Lu Lixue Dong Juan Tian Jianmin Zhang Zhongbao guo Yongju Luo Zongbin Cui Hua Wen Ming Jiang College of Fisheries and Life Science Shanghai Ocean University Yangtze River Fisheries Research Institute Chinese Academy of Fishery Sciences Guangdong Provincial Key Laboratory of Microbial Culture Collection and Application State Key Laboratory of Applied Microbiology Southern ChinaInstitute of MicrobiologyGuangdong Academy of Sciences Guangxi Institute of Fisheries

The present study aimed to compare the nutritional effects of cholesterol, bile acids, and combination of cholesterol with bile acids in plant-based diets on juvenile genetically improved farmed tilapia(GIFT;Oreochromis niloticus). The isonitrogenous(321 g/kg crude protein) and isolipidic(76 g/kg crude fat) diets(Con diet) were based on plant protein sources, which included corn gluten meal, soybean meal, cottonseed meal and rapeseed meal. The Con diet was supplemented with 12 g/kg cholesterol(CHO diet), 0.2 g/kg bile acids(BAs diet), a combination of 12 g/kg cholesterol and 0.2 g/kg bile acids(CHO-BAs diet),respectively. Each diet was fed to three tanks in an indoor recirculating aquaculture system for 9 *** showed that compared to the Con group, fish had a higher weight gain rate, hepatosomatic index,and a lower feed conversion ratio in the CHO-BAs group. The highest levels of whole-fish fat and ash were found in the Con group. Serum parameters, including activities of alanine aminotransferase(ALT) and aspartate transaminase(AST), along with levels of glucose(GLU) and triglyceride(TG) except for total cholesterol(TCHO), were lower in the CHO, BAs, and CHO-BAs groups than those in the Con group(P <0.001). Histological examination revealed that fish in the Con group exhibited severe hepatocyte vacuolization and diminished hepatocyte proliferation. Gene expression analysis indicated that the transcriptional levels of bile acid metabolism-related genes(including fxr, fgf19, bsep) were up-regulated in the CHO-BAs group(P < 0.05), whereas cholesterol metabolism-related genes(acly and hmgcr) were downregulated in both CHO and CHO-BAs groups(P < 0.001). Moreover, UPLC-MS/MS analysis revealed that the higher taurine-conjugated bile acids(T-BAs), followed by free bile acids(Free-BAs) and glycine(G-BAs)were determined in tilapia bile. Among these, taurochenodeoxycholic bile acid was the predominant bile acid. Dietary bile acids supplementation also increased the pr

关键词： Bile acid metabolism Tilapia Plant-based feed Cholesterol Liver health

Sustainability-oriented prioritization of nuclear fuel cycle transitions in China:a holistic MCDM framework under uncertainties

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Nuclear Science and Techniques 2024年第9期35卷 196-212页

作者： Lei Wang Ru-xing Gao Hyo On Nam Hong Jang Won Il Ko Chun-Dong Zhang guo-An Ye Wen-Heng Jing State Key Laboratory of Materials-Oriented Chemical Engineering College of Chemical EngineeringNanjing Tech UniversityNanjing 211816China School of Energy Science and Engineering Nanjing Tech UniversityNanjing 211816China Korea Atomic Energy Research Institute 989-111 Daedeok-daeroYuseong-GuDaejeon 34057Republic of Korea China Institute of Atomic Energy P.O.Box 275-1Beijing 102413China

A sustainability-oriented assessment of the nuclear energy system can provide informative and convincing decision-making support for nuclear development strategies in *** our previous study,four authentic nuclear fuel cycle(NFC)transi-tion scenarios were proposed,featuring different development stages and exhibiting distinct environmental,economic,and technical ***,because of the multiple and often conflicting criteria embedded therein,determining the top-priority NFC alternative for a sustainability orientation remains *** address this issue,this study proposed a novel hybrid multi-criteria decision-making framework comprising fuzzy AHP,PROMETHEE GAIA,and ***,an improved fuzzy AHP weighting model was developed to determine criteria weights under uncertainty and investigate the influence of various weight aggregation and defuzzification ***,PROMETHEE GAIA was used to address conflicts among the criteria and prioritize alternatives on a visualized k-dimensional GAIA *** a result,the alternative for direct recycling PWR spent fuel in fast reactors is considered the most ***,a sensitivity analysis was conducted to examine the influence of criteria weight variation and validate the screening ***,using MOORA,some significant optimization ideas and valuable insights were provided to support decision-makers in shaping nuclear development strategies.

关键词： Nuclear energy systems Nuclear fuel cycle Fuzzy AHP PROMETHEE GAIA

Functional nanoemulsions: Controllable low-energy nanoemulsification and advanced biomedical application

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Chinese Chemical Letters 2024年第2期35卷 57-69页

作者： Maojie Zhang qiang Cao Yuming Yuan Xiaohan guo Dawei Pan Rui Xie Xiaojie Ju Zhuang Liu Wei Wang Liangyin Chu College of Engineering Sichuan Normal UniversityChengdu 610101China School of Chemical Engineering Sichuan UniversityChengdu 610065China State Key Laboratory of Polymer Materials Engineering Sichuan UniversityChengdu 610065China

Nanoemulsions are widely used as advanced pharmaceutical delivery systems in biomedical field, due to their high encapsulation efficiency and good therapy *** techniques that produce nanoemulsions with controllable sizes and compositions are promising for creating advanced nanoemulsion systems for pharmaceutical *** review summarizes recent advances on low-energy emulsification techniques for producing nanoemulsions, and the use of these nanoemulsions as advanced pharmaceutical delivery systems and as templates to create drug-loaded functional particles for biomedical ***, nanoemulsification techniques that utilize elaborate interfacial physics/chemistry and micro-/nano-fluidics, featured with relatively-low energy input, to produce nanoemulsions with controllable sizes and compositions, are *** of these nanoemulsions to create nanoemulsionincorporated milli-particles, drug-loaded nanoparticles and nanoparticle-incorporated microparticles with sizes ranging from several millimeters to sub-10 nm are *** and efficient use of the nanoemulsions, functional nanoparticles and milli-/micro-particles integrated with nanoemulsions or nanoparticles for advanced pharmaceutical delivery in biomedical field are highlighted, with focus on how the interplay between their sizes and compositions achieve desired pharmaceutical-delivery ***, perspectives on further advances on the controllable production of nanoemulsions are provided.

关键词： Nanoemulsions Interfaces Drug delivery Template synthesis Nanoparticles

Characteristics and drivers of the soil multifunctionality under different land use and land cover types in the drylands of China

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Regional Sustainability 2024年第3期5卷 99-110页

作者： SONG Boyi ZHANG Shihang LU Yongxing guo Hao guo xing WANG Mingming ZHANG Yuanming ZHOU Xiaobing ZHUANG Weiwei College of Life Sciences Xinjiang Normal UniversityUrumqi830054China State Key Laboratory of Desert and Oasis Ecology Key Laboratory of Ecological Safety and Sustainable Development in Arid LandsXinjiang Institute of Ecology and GeographyChinese Academy of SciencesUrumqi830011China Xinjiang Key Laboratory of Biodiversity Conservation and Application in Arid Lands Xinjiang Institute of Ecology and GeographyChinese Academy of SciencesUrumqi830011China Xinjiang Field Scientific Observation Research Station of Tianshan Wild Fruit Forest Ecosystem Ili Botanical GardenXinjiang Institute of Ecology and GeographyChinese Academy of SciencesIli844900China University of Chinese Academy of Sciences Beijing100049China

The drylands of China cover approximately 6.6×106 km2 and are home to approximately 5.8×10^(8)people,providing important ecosystem services for human survival and ***,dryland ecosystems are extremely fragile and sensitive to external environmental *** use and land cover(LULC)changes significantly impact soil structure and function,thus affecting the soil multifunctionality(SMF).However,the effect of LULC changes on the SMF in the drylands of China has rarely been *** this study,we investigated the characteristics of the SMF changes based on soil data in the 1980s from the National Tibetan Plateau Data *** explored the drivers of the SMF changes under different LULC types(including forest,grassland,shrubland,and desert)and used structural equation modeling to explore the main driver of the SMF *** results showed that the SMF under the four LULC types decreased in the following descending order:forest,grassland,shrubland,and *** main driver of the SMF changes under different LULC types was mean annual temperature(MAT).In addition to MAT,pH in forest,soil moisture(SM)and soil biodiversity index in grassland,SM in shrubland,and aridity index in desert are crucial factors for the SMF ***,the SMF in the drylands of China is regulated mainly by MAT and pH,and comprehensive assessments of the SMF in drylands need to be performed regarding LULC *** results are beneficial for evaluating the SMF among different LULC types and predicting the SMF under global climate change.

关键词： Soil multifunctionality(SMF) Land use and land cover(LULC)changes Structural equation modeling(SEM) Climate change Dryland ecosystems

In-situ SEM characterization of fracture mechanism of TiB/Ti-2Al-6Sn titanium matrix composites after electroshocking treatment

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Rare Metals 2024年第6期43卷 2805-2818页

作者： Ya-Ya Wu Jian Zhou guo-Lei Han Yan Wen Zhou Wang Li-qiang Wang Wei-Jie Lv Le-Chun Xie Lin Hua Hubei Key Laboratory of Advanced Technology for Automotive Components Wuhan University of TechnologyWuhan 430070China Hubei Collaborative Innovation Center for Automotive Components Technology Wuhan 430070China Faculty of Materials and Manufacturing Beijing University of TechnologyBeijing 100124China State Key Laboratory of Metal Matrix Composites School of Materials Science and EngineeringShanghai Jiao Tong UniversityShanghai 200240China

In this article,in-situ scanning electron microscope characterization of the tensile properties of TiB/Ti-2Al-6Sn titanium matrix composite(TMC)was conducted before and after electroshocking treatment(EST).After EST,the tensile strength increased by 113.2 *** effect of EST on the tensile strength and fracture behavior of TiB was investigated using in-situ characterization of the fracture morphology and crack propagation path of the matrix and *** EST,TiB fracture introduced cracks that extended into the matrix,resulting in material *** EST,the refined TiB improved the bearing capacity of the matrix,thereby improving TMC ***,after EST,the cracks were introduced into the matrix,and resulting the fracture of matrix *** an increase in the external load,cracks in the matrix were observed to propagate to TiB,and the refined TiB was fractured,detached,and pulled out,resulting in the formation of *** the propagation path of the main crack after EST showed that the deflection angle of the main crack *** micro structure of the fracture surface indicated that the fracture of the matrix was plastic,whereas that of TiB was *** EST,the size and area of the dimples increased,confirming the increase in *** results revealed that the comprehensive mechanical properties of TiB/Ti-2Al-6Sn improved after ***,EST is an efficient method for tailoring the micro structures and mechanical properties of TMCs.

关键词： TiB/Ti-2Al-6Sn In-situ microstructure characterization Tensile properties Reinforcement Electroshocking treatment(EST)

Lithium-induced graphene layer containing Li_(3)P alloy phase to achieve ultra-stable electrode interface for lithium metal anode

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Rare Metals 2024年第2期43卷 562-574页

作者： Jia-Xin Chen guo-qiang Zhang Xian-Ying Qin Kui Lin Zi-Jin Yang Ge-Meng Liang Yue Xia guo-Bin Zhang Hai-Kun Wu Qiu-Chan Cai Hai Lin Bao-Hua Li Shenzhen Key Laboratory on Power Battery Safety Research and Shenzhen Geim Graphene Center Tsinghua Shenzhen International Graduate SchoolShenzhen518055China Shenzhen Graphene Innovation Center Co. Ltd.Shenzhen518107China School of Chemical Engineering and Advanced Materials The University of AdelaideAdelaideSA5005Australia Department of Chemistry City University of Hong KongHong Kong990077China

Uncontrolled growth of lithium dendrite will lead to low Coulombic efficiency and poor cycle stability,which hinders the commercialization of lithium metal ***,a novel modified lithium anode with reduced graphene oxide conductive network containing trace lithiophilic phosphorus(P-rGO/Cu)is prepared by electrospraying technique combined with heat treatment *** rGO layer has a concave and undulating conductive structure,which can significantly improve the effective electrical contact between lithium metal and the current collector,speed up the kinetics of interfacial electron transport and reaction,and improve the resistance of the negative electrode to the internal stress caused by volume change of the lithium,which is advantageous for the stability of the SEI *** extremely small and uniformly distributed red phosphorus element avoids the volume change caused by lithiation to the maximum *** two-phase compound Li_(3)P obtained by alloying P with Li can directionally induce the homogeneous nucleation and dense deposition of lithium metal,address the issue of lithium dendrites and extend the cycle life of the *** obtained P-rGO/Cu exhibits excellent electrochemical performance with an average Coulombic efficiency(CE)of 98%at a current density of 1 mA·cm^(−2) for 400 cycles,and the capacity retention rate of the full cell matched with lithium iron phosphate(LFP)is 83%after 400 cycles at 1C.

关键词： Lithium anode Dendrite-free Lithiophilicity Induced nucleation deposition

XOR spin logic operated by unipolar current based on field-free spin-orbit torque switching induced by a lateral interface

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Rare Metals 2024年第8期43卷 3868-3875页

作者： Yan-Ru Li Mei-Yin Yang guo-qiang Yu Bao-Shan Cui Jin-Biao Liu Yong-Liang Li Qi-Ming Shao Jun Luo Key Laboratory of Microelectronic Devices and Integrated Technology Institute of MicroelectronicsChinese Academy of Sciences(IMECAS)Beijing 100029China University of Chinese Academy of Sciences(UCAS) Beijing 100049China Songshan Lake Materials Laboratory Dongguan 523808China Institute of Physics Chinese Academy of SciencesBeijing 100190China Key Laboratory for Magnetism and Magnetic Materials of Ministry of Education Lanzhou UniversityLanzhou 730000China Department of Electronic and Computer Engineering The Hong Kong University of Science and TechnologyHong Kong 999077China

Spin logics have emerged as a promising avenue for the development of logic-in-memory *** particular,the realization of XOR spin logic gates using a single spin-orbit torque device shows great potential for low-power stateful logic circuits in the next *** this study,we successfully obtained the XOR logic gate by utilizing a spin-orbit torque device with a lateral interface,which was created by local ion implantation in the Ta/Pt/Co/Ta Hall device exhibiting perpendicular magnetic *** angle of the lateral interface is set at 45°relative to the current direction,leading to the competition between symmetry breaking and current-driven Néel-type domain wall ***,the field-free magnetic switching reversed is realized by the same sign of current amplitude at this *** on this field-free magnetic switching behavior,we successfully proposed an XOR logic gate that could be implemented using only a single spin-orbit torque Hall *** study provides a potentially viable approach toward efficient spin logics and in-memory computing architectures.

关键词： Filed-free magnetic switching Spin-orbit torque XOR logic gate Lateral interface