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Buried interface bridging for inverted cesium-formamidinium triiodide perovskite solar cells with long operational stability

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Science China Chemistry 2025年第1期68卷 163-173页

作者： Chenhui Zhang Chunjun Liang Fulin Sun Ting zhu Xinghai Huang Yuzhu guo Xinyu guo Kunyang Ge Dan Li Fangtian You Zhiqun he Key Laboratory of Luminescence and Optical Information Ministry of Education Institute of Optoelectronic TechnologyBeijing Jiaotong University Department of Physics School of Physical Science and Engineering Beijing Jiaotong University

In the field of perovskite solar cells(PSCs), the research on defects in the buried interface has been relatively limited due to its non-exposure; however, this interface significantly impacts the performance enhancement of inverted PSCs. This study employs phenylethylammonium chloride(PEACl) molecules as a buffer layer to modify the buried interface of p-i-n structured PSCs,aiming to enhance the uniformity of self-assembled monolayers(SAMs) and facilitate the uniform nucleation and growth of perovskite films on the substrate. Furthermore, the introduction of the PEACl buffer layer effectively passivates defects at the bottom of the perovskite layer and notably enhances the crystal quality of the perovskite film by mitigating residual stress,thereby reducing nonradiative recombination loss. Following these optimizations, the MA-free PSCs treated with PEACl achieve a power conversion efficiency(PCE) of 24.11%, with significant improvements in storage, thermal stability, and operational stability. Particularly noteworthy is the device's performance in an unencapsulated state, whereas after 1,500 hours of continuous light operation stability testing, it retains 97% of its original efficiency. This study not only enriches the systematic understanding of the characteristics of the buried interface in PSCs but also contributes significantly to advancing the commercial production of perovskite photovoltaic technology.

关键词： defect-induced recombination buried interfaces inverted perovskite solar cells crystallization lattice mismatch

Sequence-activated chemiluminescence probes: programmable illumination for high-contrast in vivo sensing and imaging

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Science China Chemistry 2025年第1期68卷 26-34页

作者： Yutao Zhang Juan Li Wei-Hong zhu Zhiqian guo Shanghai Key Laboratory of Functional Materials Chemistry Joint International Research Laboratory of Precision Chemistry and Molecular Engineering Institute of Fine Chemicals School of Chemistry and Molecular Engineering East China University of Science and Technology State Key Laboratory of Bioreactor Engineering Shanghai Frontier Science Research Base of Optogenetic Techniques for Cell MetabolismEast China University of Science & Technology

Sequence-activated chemiluminescence(CL) technique offers a unique approach to detecting specific biomolecules or cellular events with high sensitivity and spatial resolution. The fundamental principle behind sequence-activated CL probes involves tailoring highly-controllable CL signals in response to specific sequences or events of interest, thus enabling high-contrast signals under complex physiological conditions. This sequential activation could be triggered by enzymes, reactive oxygen species(ROS), biothiols or changes in the microenvironment. These unique sequence-activated CL probes bestow several advantages, including minimal background, deep-tissue penetration, and the ability of non-invasive or minimally invasive detection. The sequence-activated CL techniques represent a significant advancement in molecular imaging and diagnostics. In this mini-review, we focus on the latest developments in sequential CL probes, addressing the technical challenges and discussing the future trajectory by harnessing CL signaling and molecular recognition.

关键词： chemiluminescnece sequence-activation in-vivo bioimaging cyclic peroxide

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大口径新型顶管力学行为现场试验研究

岩土工程学报 2017年第10期39卷 1842-1850页

作者：张耀闫治国朱合华同济大学土木工程防灾国家重点实验室上海200092 同济大学土木工程学院地下建筑与工程系上海200092

通过对新型预应力钢筒混凝土顶管(JPCCP)开展现场试验,得到了在施工荷载、水土压力等三维荷载作用下顶管各部位的应变时程响应;同时也获得了顶进过程中管–土接触应力时程变化。根据对数据的分析,得出预应力钢筒混凝土顶管具有较大的纵... 详细信息

通过对新型预应力钢筒混凝土顶管(JPCCP)开展现场试验,得到了在施工荷载、水土压力等三维荷载作用下顶管各部位的应变时程响应;同时也获得了顶进过程中管–土接触应力时程变化。根据对数据的分析,得出预应力钢筒混凝土顶管具有较大的纵向抗压刚度,而纵向抗拉刚度不足。由于预应力的效应,内层混凝土与中间层混凝土能够承受较大的环向拉应力。通过对管节的纵向受力分析,计算出管–土平均摩阻力随顶进距离的变化规律,结合施工记录得出平均摩阻力随顶进距离先增大后减小,最小值为1.27 k Pa;同时,施工顶进间隔越短,平均摩阻力越小。此外,实测结果表明,管–土接触应力对管节运动较为敏感,最大瞬时值可达500 k Pa;施工结束后,接触应力沿管周分布并不对称或均匀,但与实测管节环向应变分布对应。

关键词：预应力钢筒混凝土顶管管–土接触应力管–土平均摩阻力应变时程响应

OPTIMIZATION OF OLEO-PNEUMATIC SHOCK ABSORBER OF AIRCRAFT

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Chinese Journal of Aeronautics 1993年第2期 101-107页

作者： Liu Li (Beijing Institute of Technology,Beijing,China,100081) Yang guo-zhu,he Qing-zhi (Beijing University of Aeronautics and Astronautics,Beijing,China,100083)

The influence of the oleo-pneumatic shock absorber on aircraft response during bothtaxiing and landing impact is considered. For improving the dynamic response characteristicsof the aircraft during taxiing, the model and method for optimization of shock absorberparameters are proposed, in which the mean square value of the heave accelerationof the aircraft during taxiing is taken as the objective function and the landing impact energyto be absorbed as the constraint conditions. As an example, the optimization of themain landing gear system is studied based on the model and method proposed above. Becausethe PSD method is used in the analyses, the optimization procedure is easy and simple.

关键词： ab OPTIMIZATION OF OLEO-PNEUMATIC SHOCK ABSORBER OF AIRCRAFT

Cross-section measurement for the ^(93)Nb(n,2n)^(92g)Nb reaction at the neutron energy of 14.6 MeV by the AMS method

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Chinese Physics C 2018年第7期42卷 37-40页

作者： guo-zhu he Bin Shi Ming he Zhen-Yu Li Shi-Long Liu Xiong-Jun Chen Xi-Chao Ruan Qi-Wei Zhang Qi-Wen Fan heng Li Shao-Yong Wu Shan Jiang Zu-Ying Zhou Key Laboratory of Nuclear Data China Institute of Atomic Energy Beijing 102413 China Department of Nuclear Physics China Institute of Atomic Energy Beijing 102413 China College of Physics Science and Technology Guizhou Normal University Guiyang 530004 China Institute of High Energy Physics Chinese Academy of Science Beijing 100049 China

The cross-section for the 93Nb（n, 2n）92gNb reaction has been measured at the neutron energy of 14.6 MeV using neutron activation and accelerator mass spectrometry （AMS） determination of the long-lived product nuclide 92gNb. The neutron energy was generated from the D＋T neutron source at the China Institute of Atomic Energy （CIAE）. The neutron flux was monitored by measuring the activity of 92mNb produced in the competing reaction channel of 93Nb（n, 2n）92mNb. At the neutron energy of 14.6 MeV, the 93Nb（n, 2n）92gNb reaction cross-section of （736±220） mb was obtained for the first time.

关键词： 93Nb(n,2n)92gNb reaction cross-section D+T neutron source accelerator mass spectrometry

Influence of hot deformation quantity on impact fatigue resistance of low alloy wear resistant cast iron

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材料科学与工程（中英文版） 2009年第8期3卷 60-64页

作者： LIU Jian-hua MENG De-liang guo Yu-xing zhu guo-he ZHANG Rui-jun State Key Laboratory of Metastable Materials Science and Technology Yanshan University Qinhuangdao 066004 China School of Civil Engineering and Mechanics Yanshan University Qinhuangdao 066004 China Thin Strip Co. Ltd. of Baosteel Shanghai 200431 China

Defect Engineering with Rational Dopants Modulation for High‑Temperature Energy Harvesting in Lead‑Free Piezoceramics

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Nano-Micro Letters 2025年第3期17卷 87-101页

作者： Kaibiao Xi Jianzhe guo Mupeng Zheng Mankang zhu Yudong Hou Key Laboratory of Advanced Functional Materials Ministry of EducationCollege of Materials Science and EngineeringBeijing University of TechnologyBeijing 100124People’s Republic of China

High temperature piezoelectric energy harvester(HTPEH)is an important solution to replace chemical battery to achieve independent power supply of HT wireless ***,simultaneously excellent performances,including high figure of merit(FOM),insulation resistivity(ρ)and depolarization temperature(Td)are indispensable but hard to achieve in lead-free piezoceramics,especially operating at 250°C has not been reported ***,well-balanced performances are achieved in BiFeO3–BaTiO3 ceramics via innovative defect engineering with respect to delicate manganese *** to the synergistic effect of enhancing electrostrictive coefficient by polarization configuration optimization,regulating iron ion oxidation state by high valence manganese ion and stabilizing domain orientation by defect dipole,comprehensive excellent electrical performances(Td=340°C,ρ250°C>10^(7)Ωcm and FOM_(250°C)=4905×10^(–15)m^(2)N^(−1))are realized at the solid solubility limit of manganese *** HT-PEHs assembled using the rationally designed piezoceramic can allow for fast charging of commercial electrolytic capacitor at 250°C with high energy conversion efficiency(η=11.43%).These characteristics demonstrate that defect engineering tailored BF-BT can satisfy high-end HT-PEHs requirements,paving a new way in developing selfpowered wireless sensors working in HT environments.

关键词： Lead-free piezoceramic Defect engineering Dopants modulation High-temperature Piezoelectric energy harvester

Dip2a regulates stress susceptibility in the basolateral amygdala

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Neural Regeneration Research 2025年第6期20卷 1735-1748页

作者： Jing Li Zixuan he Weitai Chai Meng Tian Huali Yu Xiaoxiao he Xiaojuan zhu Key Laboratory of Molecular Epigenetics Ministry of Education Institute of Genetics and CytologyNortheast Normal UniversityChangchunJilin ProvinceChina

Dysregulation of neurotransmitter metabolism in the central nervous system contributes to mood disorders such as depression, anxiety, and post–traumatic stress disorder. Monoamines and amino acids are important types of neurotransmitters. Our previous results have shown that disco-interacting protein 2 homolog A(Dip2a) knockout mice exhibit brain development disorders and abnormal amino acid metabolism in serum. This suggests that DIP2A is involved in the metabolism of amino acid–associated neurotransmitters. Therefore, we performed targeted neurotransmitter metabolomics analysis and found that Dip2a deficiency caused abnormal metabolism of tryptophan and thyroxine in the basolateral amygdala and medial prefrontal cortex. In addition, acute restraint stress induced a decrease in 5-hydroxytryptamine in the basolateral amygdala. Additionally, Dip2a was abundantly expressed in excitatory neurons of the basolateral amygdala, and deletion of Dip2a in these neurons resulted in hopelessness-like behavior in the tail suspension test. Altogether, these findings demonstrate that DIP2A in the basolateral amygdala may be involved in the regulation of stress susceptibility. This provides critical evidence implicating a role of DIP2A in affective disorders.

关键词： 5-hydroxytryptamine acute restraint stress basolateral amygdala CaMKII neurons DIP2A metabolomics neurotransmitters principal component analysis stress susceptibility tryptophan

Structural and microwave absorption properties of CoFe_(2)O_(4)/residual carbon composites

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International Journal of Minerals,Metallurgy and Materials 2025年第1期32卷 221-232页

作者： Yuanchun Zhang Shengtao Gao Xingzhao Zhang Dacheng Ma Chuanlei zhu Jun he Joint National-Local Engineering Research Centre for Safe and Precise Coal Mining Anhui University of Science and TechnologyHuainan 232001China School of Chemical and Blasting Engineering Anhui University of Science and TechnologyHuainan 232001China

Electromagnetic interference,which necessitates the rapid advancement of substances with exceptional capabilities for bsorbing electromagnetic waves,is of urgent concern in contemporary *** this work,CoFe_(2)O_(4)/residual carbon from coal gasification fine slag(CFO/RC)composites were created using a novel hydrothermal *** mechanisms for microwave absorption,including conductive loss,natural resonance,interfacial dipole polarization,and magnetic flux loss,are involved in these ***,compared with pure residual carbon materials,this composite offers superior capabilities in microwave *** 7.76GHz,the CFO/RC-2 composite achieves an impressive minimum reflection loss(RL_(min))of-43.99 dB with a thickness of 2.44 ***,CFO/RC-3 demonstrates an effective absorption bandwidth(EAB)of up to 4.16 GHz,accompanied by a thickness of *** study revealed the remarkable capability of the composite to diminish electromagnetic waves,providing a new generation method for microwave absorbing materials of superior quality.

关键词： coal gasification slag residual carbon hydrothermal method microwave absorption CoFe_(2)O_(4)