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Construction of 3D porous Cu_(1.81)S/nitrogen-doped carbon frameworks for ultrafast and long-cycle life sodium-ion storage

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International Journal of Minerals,Metallurgy and Materials 2025年第1期32卷 191-200页

作者： chen chen Hongyu Xue Qilin Hu Mengfan Wang Pan Shang Ziyan Liu Tao Peng Deyang Zhang Yongsong Luo Key Laboratory of Microelectronics and Energy of Henan Province Henan Joint International Research Laboratory of New Energy Storage TechnologyCollege of Physics and Electronic EngineeringXinyang Normal UniversityXinyang 464000China School of Physics and Electronic Engineering Nanyang Normal UniversityNanyang 473061China

Transition metal sulfides have great potential as anode mterials for sodium-ion batteries(SIBs)due to their high theoretical specific ***,the inferior intrinsic conductivity and large volume variation during sodiation-desodiation processes seriously affect its high-rate and long-cyde performance,unbeneficial for the application as fast-charging and long-cycling SIBs ***,the three-dimensional porous Cu_(1.81)S/nitrogen-doped carbon frameworks(Cu_(1.81)S/NC)are synthesized by the simple and facile sol-gel and annealing processes,which can accommodate the volumetric expansion of Cu_(1.81)S nanoparticles and accelerate the transmission of ions and electrons during Na^(+)insertion/extraction processes,exhibiting the excellent rate capability(250.6 mA·g^(-1)at 20.0 A·g^(-1))and outstanding cycling stability(70% capacity retention for 6000 cycles at 10.0 A·g^(-1))for ***,the Na-ion full cells coupled with Na_(3)V_(2)(PO_(4))_(3)/C cathode also demonstrate the satisfactory reversible specific capacity of 330.5 mAh·g^(-1)at 5.0 A·g^(-1)and long-cycle performance with the 86.9% capacity retention at 2.0 A·g^(-1)after 750 *** work proposes a promising way for the conversionbased metal sulfides for the applications as fast-charging sodium-ion battery anode.

关键词： copper sulfide nanoparticles porous carbon framework fast charging long-cycle performance sodium-ion full batteries

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ru doping triggering reconstruction of cobalt phosphide for coupling glycerol electrooxidation with seawater electrolysis

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Journal of Energy Chemistry 2025年第1期100卷 317-326页

作者： Binglu Deng Jie Shen Jinxing Lu Chuqiang Huang Zhuoyuan chen Feng Peng Yunpeng Liu School of Materials Science and Hydrogen Energy Foshan University School of Chemistry and Chemical Engineering Guangzhou University Guangdong Key Laboratory for Hydrogen Energy Technologies

Seawater electrolysis is a promising approach for sustainable energy without relying on precious ***,the large-scale seawater electrolysis is hindered by low catalytic efficiency and severe anode corrosion caused by the harmful *** contrast to the oxygen evolution reaction （OER）and chlorin ion oxidation reaction （ClOR）,glycerol oxidation reaction （GOR） is more thermodynamically and kinetically favorable ***,a ru doping cobalt phosphide （ru-CoP2） is proposed as a robust bifunctional electrocatalyst for seawater electrolysis and GOR,for the concurrent productions of hydrogen and value-added *** in situ and ex situ characterization analyses demonstrated that ru doping featured in the dynamic reconstruction process from ru-CoP2to ru-CoOOH,accounting for the superior GOR *** coupling GOR with hydrogen evolution was realized by employing ru-CoP2as both anode and cathode,requiring only a low voltage of 1.43 V at 100 mA cm-2,which was 250 m V lower than that in alkaline *** work guides the design of bifunctional electrocatalysts for energy-efficient seawater electrolysis coupled with biomass resource upcycling.

关键词： Glycerol electrooxidation Hydrogen evolution ru doping Cobalt phosphide Bifunctional electrocatalysts

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Metabolic reprogramming: a new option for the treatment of spinal cord injury

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Neural Regeneration Research 2025年第4期20卷 1042-1057页

作者： Jiangjie chen Jinyang chen Chao Yu Kaishun Xia Biao Yang Ronghao Wang Yi Li Kesi Shi Yuang Zhang Haibin Xu Xuesong Zhang Jingkai Wang Qixin chen chengzhen Liang Department of Orthopedics The Second Affiliated Hospital of Zhejiang University School of MedicineHangzhouZhejiang ProvinceChina Orthopedics Research Institute of Zhejiang University Zhejiang UniversityHangzhouZhejiang ProvinceChina Key Laboratory of Motor System Disease Research and Precision Therapy of Zhejiang Province HangzhouZhejiang ProvinceChina Clinical Research Center of Motor System Disease of Zhejiang Province HangzhouZhejiang ProvinceChina Qiandongnan Prefecture People’s Hospital KailiGuizhou ProvinceChina Department of Orthopedics Fourth Medical CenterChinese PLA General HospitalBeijingChina

Spinal cord injuries impose a notably economic burden on society,mainly because of the severe after-effects they *** the ongoing development of various therapies for spinal cord injuries,their effectiveness remains ***,a deeper understanding of metabolism has opened up a new therapeutic opportunity in the form of metabolic *** this review,we explore the metabolic changes that occur during spinal cord injuries,their consequences,and the therapeutic tools available for metabolic *** spinal cord metabolism is characterized by independent cellular metabolism and intercellular metabolic ***,spinal cord injury results in metabolic disorders that include disturbances in glucose metabolism,lipid metabolism,and mitochondrial *** metabolic disturbances lead to corresponding pathological changes,including the failure of axonal regeneration,the accumulation of scarring,and the activation of *** rescue spinal cord injury at the metabolic level,potential metabolic reprogramming approaches have emerged,including replenishing metabolic substrates,reconstituting metabolic couplings,and targeting mitochondrial therapies to alter cell *** available evidence suggests that metabolic reprogramming holds great promise as a next-generation approach for the treatment of spinal cord *** further advance the metabolic treatment of the spinal cord injury,future efforts should focus on a deeper understanding of neurometabolism,the development of more advanced metabolomics technologies,and the design of highly effective metabolic interventions.

关键词： axons glycolysis metabolic reprogramming metabolism mitochondria neural regeneration neuroprotection oxidative phosphorylation spinal cord injury therapy

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身体活动与执行功能领域研究主题的动态演化

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中国组织工程研究 2025年第14期29卷 3043-3050页

作者：邓青邱晨王庆军黄贵张业廷南京师范大学体育科学学院江苏省南京市210012 南京晓庄学院体育学院江苏省南京市211171 南京师范大学新闻与传播学院江苏省南京市210012 中国民用航空飞行学院航空安全保卫学院四川省广汉市618307

背景:身体活动与执行功能领域的相关研究不断涌现,目前尚未有学者使用可视化工具探讨这一领域研究主题的动态演化路径。目的:通过文献计量学方法,探究身体活动与执行功能领域研究主题的动态演化过程,从而理清其发展状态及知识结构的变... 详细信息

背景:身体活动与执行功能领域的相关研究不断涌现,目前尚未有学者使用可视化工具探讨这一领域研究主题的动态演化路径。目的:通过文献计量学方法,探究身体活动与执行功能领域研究主题的动态演化过程,从而理清其发展状态及知识结构的变化。方法:通过检索式:TS=(“Physical activity”AND“Executive function*”)OR TS=(Exercise AND“Executive function*”)检索Web of Science数据库,依照纳入排除标准选取4386篇相关文献为研究内容,利用SciMAT软件进行可视化分析。结果与结论:身体活动与执行功能领域的研究呈现蓬勃发展态势,相关研究日趋深入,未来发展空间较大;该领域可分为执行功能、儿童、老年人和干预措施4个方向,并形成了11条主要演化路径;“运动技能”“生活方式”“有氧运动”和“干预措施”等主题可能是未来的研究重点,“青少年”和“老年人”群体是该领域研究的重点关注人群。

关键词：身体活动执行功能认知 SciMAT 可视化分析动态演化

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Co-production of hydrogen, oxygen, and electricity via an integrated solar-driven system with decoupled water electrolyzer and Na-Zn ion battery

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Journal of Energy Chemistry 2025年第1期100卷 621-627页

作者： Fei Lv Longjie Liu Jiazhe Wu Pengfei Wang Lixia Pan Dengwei Jing Yubin chen International Research Center for Renewable Energy State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University

Combining water electrolysis and rechargeable battery technologies into a single system holds great promise for the co-production of hydrogen （H2） and ***,the design and development of such systems is still in its ***,an integrated hydrogen-oxygen （O2）-electricity co-production system featuring a bipolar membrane-assisted decoupled electrolyzer and a Na-Zn ion battery was established with sodium nickelhexacyanoferrate （NaNiHCF） and Zn2+/Zn as dual redox *** decoupled electrolyzer enables to produce H2and O2in different time and space with almost 100%Faradaic efficiency at 100 mA ***,the charged NaNiHCF and Zn electrodes after the electrolysis processes formed a Na-Zn ion battery,which can generate electricity with an average cell voltage of 1.75 V at 10 m A *** connecting Si photovoltaics with the modular electrochemical device,a well-matched solar driven system was built to convert the intermittent solar energy into hydrogen and electric energy with a solar to hydrogen-electricity efficiency of 16.7%,demonstrating the flexible storage and conversion of renewables.

关键词： Hydrogen Electricity Decoupled water electrolyzer Na-Zn ion battery Solar energy

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Flexible organic-inorganic hybrid photodetectors with n-type phenyl-C61-butyric acid methyl ester （PCBM） and p-type pearl-like GaP nanowires

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Nano Research 2014年第12期7卷 1777-1787页

作者： gui chen Xuming Xie Guozhen Shen State Key Laboratory for Superlattices and Microstructures Institute of Semiconductors Chinese Academy of Sciences Beijing100083 China

Flexible photodetectors have become a focus of current researches because they may offer some unique applications in various new areas that require flexible, lightweight, and mechanical shock-resistive sensing elements. In this work, we designed flexible organic-inorganic hybrid photodetectors on various flexible substrates, including polyethylene terephthalate （PET）, common Sellotape and polydimethylsiloxane （PDMS）, with n-type phenyl-C61-butyric acid methyl ester （PCBM） and p-type pearl-like GaP nanowires （NWs） as the active materials. The as-fabricated hybrid devices exhibited an optimized performance superior to the device made of pristine GaP NWs, with a fast response time （43 ms） and high on/off ratio （-170）. Under different bending conditions, the flexible hybrid photodetectors demonstrated excellent flexibility and electrical stability, which make them very promising for further large-scale, high sensitivity and high speed photodetector applications.

关键词： nanowires flexible photodetectors hybrid

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Advancing intestinal organoid technology to decipher nano-intestine interactions and treat intestinal disease

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Nano Research 2023年第3期16卷 3976-3990页

作者： Lin Bao Xuejing Cui ru Bai Chunying chen CAS Key Laboratory for Biomedical Effects of Nanomaterials and Nanosafety&CAS Center for Excellence in Nanoscience National Center for Nanoscience and Technology of ChinaChinese Academy of SciencesBeijing 100190China The GBA National Institute for Nanotechnology Innovation Guangzhou 510700China University of Chinese Academy of Sciences Beijing 100049China

With research burgeoning in nanoscience and nanotechnology,there is an urgent need to develop new biological models that can simulate native structure,function,and genetic properties of tissues to evaluate the adverse or beneficial effects of nanomaterials on a *** the current biological models,three-dimensional(3D)organoids have developed as powerful tools in the study of nanomaterial-biology(nano-bio)interactions,since these models can overcome many of the limitations of cell and animal models.A deep understanding of organoid techniques will facilitate the development of more efficient nanomedicines and further the fields of tissue engineering and personalized ***,we summarize the recent progress in intestinal organoids culture systems with a focus on our understanding of the nature and influencing factors of intestinal organoid *** also discuss biomimetic extracellular matrices(ECMs)coupled with *** particular,we analyze the application prospects for intestinal organoids in investigating nano-intestine *** integrating nanotechnology and organoid technology,this recently developed model will fill the gaps left due to the deficiencies of traditional cell and animal models,thus accelerating both our understanding of intestine-related nanotoxicity and the development of nanomedicines.

关键词： intestinal organoid biomimetic extracellular matrices(ECMs) intestinal tissue engineering nano-intestine interaction

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A novel negative quantum capacitance field-effect transistor with molybdenum disulfide integrated gate stack and steep subthreshold swing for ultra-low power applications

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Science China(Information Sciences) 2023年第6期66卷 71-77页

作者： Liang chen Huimin WANG Qianqian HUANG ru HUANG School of Integrated Circuits Peking University Beijing Advanced Innovation Center for Integrated Circuits

Various steep-slope devices based on novel structures and mechanisms garnered considerable attention for their potential in ultra-low power logic applications. In this work, a novel steep-slope negative quantum capacitance field-effect transistor(NQCFET)with molybdenum disulfide(MoS2)-integrated gate stack was realized by theoretical analysis and experimental evaluation. By combining the MoS+2 equivalent capacitance model calibrated with experimental results, the NQCFET device model is further *** results demonstrated that the optimized MoS2-integrated NQCFET can achieve a subthreshold swing(SS)of sub-60 mV/dec over a current range of 5 decades, with the minimum SS reaching 29 mV/dec,indicating the remarkable potential of MoS2-integrated NQCFETs for ultra-low power applications.

关键词： negative quantum capacitance molybdenum disulfide field-effect transistor subthreshold swing ultra-low power device

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One-pot synthesis of Fe/Cu-SSZ-13 catalyst and its highly efficient performance for the selective catalytic reduction of nitrogen oxide with ammonia

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Journal of Environmental Sciences 2021年第2期33卷 306-316页

作者： Jie Wan Jiawei chen ru Zhao Renxian Zhou Energy Research Institute Nanjing Institute of TechnologyNanjing 211167China Institute of Catalysis Zhejiang UniversityHangzhou 310028China

Series of Fe/Cu-SSZ-13 catalysts with different Fe loading content were synthesized by simple one-pot *** obtained catalysts were subjected to selective catalytic reduction(SCR)of NO x with NH 3 and were characterized by various *** results show that Fe 0.63/Cu 1.50-SSZ-13 catalyst with proper Fe content exhibits excellent catalytic activity with widest operation temperature window from 160 to 580℃,excellent hydrothermal stability as well as good resistance to sulfur poisoning when compared with Cu-SSZ-13,signifying its great potential for practical *** characterizations reveal that the synthesized Fe/Cu-SSZ-13 catalysts present typical chabazite(CHA)structure with good crystallinity,while isolated Cu^2+and monomeric Fe 3+are revealed as the predominant copper and iron *** low temperatures,isolated Cu^2+species act as primary active sites for SCR reaction,while monomeric Fe^3+species provide sufficient active sites for sustain the SCR activity at high ***,Fe over doping would lead to the damage of zeolite structure,destruction of isolated Cu^2+site,as well as the formation of highly oxidizing Fe2O3,thus causing deterioration of catalytic performances.

关键词： NH3-SCR Fe/Cu-SSZ-13 One-pot synthesis Active species

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Multifunctional Nacre-Like Nanocomposite Papers for Electromagnetic Interference Shielding via Heterocyclic Aramid/MXene Template-Assisted In-Situ Polypyrrole Assembly

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NANO-MICRO LETTERS 2025年第1期17卷 1-18页

作者： Xiong, Jinhua Zhao, Xu Liu, Zonglin chen, He Yan, Qian Lian, Huanxin chen, Yunxiang Peng, Qingyu He, Xiaodong Harbin Inst Technol Ctr Composite Mat & Struct Natl Key Lab Sci & Technol Adv Composites Special Harbin 150080 Peoples R China

The large-scale, high-strength, super-tough, and multifunctional nacre-like heterocyclic aramid (HA)/MXene@polypyrrole (PPy) (HMP) nanocomposite papers were fabricated using the in-situ assembly of PPy onto the HA/MXene hydrogel *** "brick-and-mortar" layered structure and abundant hydrogen-bonding interactions among MXene, PPy, and HA respond cooperatively to external stress and effectively increase the mechanical properties of HMP nanocomposite *** templating effect from HA/MXene was utilized to guide the assembly of conducting polymers, leading to high electrical conductivity and outstanding electromagnetic interference shielding performance. Robust, ultra-flexible, and multifunctional MXene-based electromagnetic interference (EMI) shielding nanocomposite films exhibit enormous potential for applications in artificial intelligence, wireless telecommunication, and portable/wearable electronic equipment. In this work, a nacre-inspired multifunctional heterocyclic aramid (HA)/MXene@polypyrrole (PPy) (HMP) nanocomposite paper with large-scale, high strength, super toughness, and excellent tolerance to complex conditions is fabricated through the strategy of HA/MXene hydrogel template-assisted in-situ assembly of PPy. Benefiting from the "brick-and-mortar" layered structure and the strong hydrogen-bonding interactions among MXene, HA, and PPy, the paper exhibits remarkable mechanical performances, including high tensile strength (309.7 MPa), outstanding toughness (57.6 MJ m-3), exceptional foldability, and structural stability against ultrasonication. By using the template effect of HA/MXene to guide the assembly of conductive polymers, the synthesized paper obtains excellent electronic conductivity. More importantly, the highly continuous conductive path enables the nanocomposite paper to achieve a splendid EMI shielding effectiveness (EMI SE) of 54.1 dB at an ultra-thin thickness (25.4 mu m) and a high specific EMI SE of 17,204.7 dB cm2 g-1. In addit

关键词： MXene Remarkable mechanical properties Heterocyclic aramid Electromagnetic interference shielding Polypyrrole Multifunctionality

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