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Mn single-atoms decorated CNT electrodes for high-performance supercapacitors

Nano Research 2024年第5期17卷 4039-4046页

作者： Qian rong Chao Yuwen Yingkai Liu Yuanrong Liu Chunyang wang Yang wang Ding Zhang Zhen Wen Yunnan Key Laboratory of Opto-Electronic Information Technology Institute of Physics and Electronic InformationYunnan Normal UniversityKunming 650500China Faculty of Metallurgical and Energy Engineering Kunming University of Science and TechnologyKunming 650093China Department of Physics and Astronomy University of CaliforniaIrvineCA 92697USA School of Materials Science and Engineering National Institute for Advanced MaterialsSmart Sensing Interdisciplinary Science CenterNankai UniversityTianjin 300350China Jiangsu Key Laboratory for Carbon-Based Functional Materials and Devices Institute of Functional Nano and Soft Materials(FUNSOM)Soochow UniversitySuzhou 215123China

Developing highly robust and efficient electrode materials is of critical importance to promoting the energy density of current supercapacitors for ***,we report an efficient catalyst with monodispersed Mn single-atoms embedded in carbon nanotubes(Mn-CNTs)for enhancing the electrode performance of supercapacitors.A high specific capacitance(1523.6 F·g^(-1) at 1.0 A·g^(-1))can be achieved,which is about twice as high as the specific capacitance of the electrode material without the introduction of Mn ***,the asymmetric electrochemical capacitor created with Mn-CNT and activated carbon exhibits a high energy density of 180.8 Wh·kg^(-1) at a power density of 1.4 kW·kg^(-1),much higher than most reported *** study shows that the integration of Mn atoms into the CNT can enhance the charge transport capacity and the number of polar active sites of Mn-CNT and then facilitate chemical interactions between Mn-CNT and OH-.This work provides a novel strategy to enable high-energy storage in supercapacitors by introducing single-atoms into carbon nanotubes to improve electrodes’energy density and cycle life.

关键词： carbon nanotube(CNT) supercapacitor single-atoms power density energy density

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Surface water resource attenuation attribution and patterns in Hai River Basin

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Science China Earth Sciences 2024年第5期67卷 1545-1560页

作者： Qingming wang Yong ZHAO Hao wang Jiaqi ZHAI Yue ZHANG Fan HE rong LIU Mengyang MA State Key Laboratory of Simulation and Regulation of Water Cycle in River Basin China Institute of Water Resources and Hydropower Research(IWHR)Beijing 100038China Key Laboratory of Water Safety for Beijing-Tianjin-Hebei Region of Ministry of Water Resources Beijing 100038China General Institute of Water Resources and Hydropower Planning and Design Ministry of Water ResourcesBeijing 100120China

From 1956 to 2016,Hai River Basin suffered the most severe surface water resource attenuation among the 10 first-class river basins in *** on the surface water circulation process,and evolving characteristics of precipitation and underlying surface in Hai River Basin,this study attributed the causes of surface water resource attenuation to six primary impact factors,analyzed each factor's quantitative contribution,and revealed four patterns of surface water resource attenuation in Hai River *** pattern of the dominant factor:comparing the 1980–2000 period with the 1956–1979period,the variation of precipitation is the dominant factor of which contribution is 7 billion m^(3),accounting for 59%of total11.7 billion m^(3);comparing the 2001–2016 period with the 1956–1979 period,the increasing of vegetation cover in mountainous area is the dominant factor of which contribution is 2.78 billion m3,accounting for 51%of total 4.9 billion m^(3).The pattern of spatial distributions:comparing the 2001–2016 period with the 1956–1979 period,mountainous areas were more affected by increasing vegetation cover which for example contributed 42%in Luan River Basin mountainous;the plains were more impacted by farmland ridge interception which for example contributed 51%in Beisi River Basin *** pattern of attenuation trend:comparing the 2001–2016 period with the 1980–2000 period,surface water resources in mountainous areas continued to decline,owing to the increasing water consumption of large-scale vegetation restoration,while the influence of the underlying surface changes on surface water resources in plains areas tended to remain *** pattern of reversible change:among factors led to surface water resource attenuation,the human activity,including vegetation cover increase,farmland ridge interception,and urbanization expansion,contributed 36%of the attenuation,which resulted in the variation of precipitation-runoff *** study improved the traditiona

关键词： Hai River Basin Surface water resources Contribution decomposition Quantitative contribution Attenuation patterns

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WeldNet:A voxel-based deep learning network for point cloud annular weld seam detection

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Science China(Technological Sciences) 2024年第4期67卷 1215-1225页

作者： wang Hui rong YouMin XU JiaJun XIANG SongMing PENG YiFan HUANG Yu State Key Laboratory of Intelligent Manufacturing Equipment and Technology Huazhong University of Science and TechnologyWuhan 430074China School of Mechanical Science and Engineering Huazhong University of Science and TechnologyWuhan 430074China

Weld seam detection is an important part of automated *** present,few studies have been conducted on annular weld seams,and a lot of defects exist in the point cloud model of the tube sheet obtained by RGB-D cameras and photography *** at the above problems,this paper proposed an annular weld seam detection network named WeldNet where a voxel feature encoding layer was adaptively improved for annular weld seams,the sparse convolutional network and region proposal network(RPN)were used to detect annular weld seam position,and an annular weld seam detection loss function was ***,an annular weld seam dataset was established to train the *** with the random sampling consistency(RANSAC)method,WeldNet has a higher detection accuracy,as well as a higher detection success rate which has increased by 23%.Compared with U-Net,WeldNet has been proven to achieve a better detection result,and the intersection over the union of the weld seam detection is improved by 17.8%.

关键词： deep learning point cloud weld seam detection welding annular weld seam

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A new twist to the interplay between superconductivity and Kondo correlation

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Science China(Physics,Mechanics & Astronomy) 2024年第8期67卷 1-2页

作者： gui-Lu Long Department of Physics Tsinghua UniversityBeijing 100084China Beijing Academy of Quantum Information Sciences Beijing 100193China

Recently,Deng et al.[1] found a new twist to the intriguing physics resulting from the interplay between Kondo correlation and *** correlation [2,3] and superconductivity [4,5] are two fundamental phenomena in condens... 详细信息

关键词： Kondo al. twist

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Applying heteroatom co-doped carbon nanotube for manifesting high performance in the electrochemical reduction of aqueous nitrogen oxide by gold nanoparticles

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Nano Research 2024年第3期17卷 1151-1164页

作者： Jane Chung Haibo Yin rong wang Yunlong wang Junyang Zhang Yue Peng Joung Woo Han Seongyun Ryu Junhua Li State Key Joint Laboratory of Environment Simulation and Pollution Control School of EnvironmentTsinghua UniversityBeijing 100084China EHS Research Center Samsung Electronics Co.Ltd.Gyeonggi-do 18448Republic of Korea

Electrochemical NO-to-NH_(3) under ambient conditions could be a viable alternative having advantages in terms of energy consumption and exhaust gas recycling of NO,replacing a traditional ammonia synthesis method of the Haber–Bosch *** synthesizing boron(B-)and nitrogen(N-)co-doped carbon nanotube(CNT)based gold(Au)catalysts,B-dopants elevate the conductivity of carbon nanotube by sp2 hybridization on graphene and implant B–N domains within the graphene layer,and result in facilitating the embedding amount of Au accompanied by high dispersibility with low particle *** density functional theory(DFT)calculations elucidate that the electron cloud transmitted from B-dopant to the active site of Au induces the Lewis acidic site,and the O-distal pathway occurs following a spontaneous *** of the electron-deficient B-doping area accompanied by N-defects and B–O edges retains the major valence state of Au as Au^(δ+),and suppresses hydrogen evolution reaction(HER)by repulsing the hindrance of H*.This record exhibits the highest faradaic efficiency(FE)of 94.7%,and NH_(3) yield rate of 1877.4μg·h^(-1)·mg_(cat)^(-1),which is the optimal yield over energy consumption in the field of the ambient reduction of aqueous NO.

关键词： boron heteroatom nitrogen defect gold nanoparticles valence states of gold electrochemical NO-to-NH3

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Asymmetric configuration activating lattice oxygen via weakening d-p orbital hybridization for efficient C/N separation in urea overall electrolysis

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Journal of Energy Chemistry 2024年第5期92卷 233-239页

作者： Chongchong Liu Peifang wang Bin Hu Xiaoli Liu rong Huang Gang Zhou Key Laboratory of Integrated Regulation and Resource Development on Shallow Lake of Ministry of Education College of EnvironmentHohai UniversityNanjing 210098JiangsuChina

Urea oxidation reaction(UOR)is proposed as an exemplary half-reaction in renewable energy applications because of its low thermodynamical ***,challenges persist due to sluggish reaction kinetics and complex by-products *** this end,we introduce the lattice oxygen oxidation mechanism(LOM),propelling a novel UOR route using a modified CoFe layered double hydroxide(LDH)catalyst termed *** calculations and in-situ characterizations highlight the activated lattice oxygen(O_(L))within CFRO-7 as pivotal sites for UOR,optimizing the reaction pathway and accelerating the *** the urea overall electrolysis application,the LOM route only requires a low voltage of 1.54 V to offer a high current of 100 mA cm^(-2) for long-term utilization(>48 h).Importantly,the by-product NCO^(-)−is significantly suppressed,while the CO_(2)2/N_(2) separation is efficiently *** work proposed a pioneering paradigm,invoking the LOM pathway in urea electrolysis to expedite reaction dynamics and enhance product selectivity.

关键词： Lattice oxygen Urea oxidation reaction Overall electrolysis Products selectivity

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Improved error estimates for a modified exponential Euler method for the semilinear stochastic heat equation with rough initial data

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Science China Mathematics 2024年

作者： Xinping gui Buyang Li Jilu wang Beijing Computational Science Research Center Department of Applied Mathematics The Hong Kong Polytechnic University School of Science Harbin Institute of Technology

A class of stochastic Besov spaces BpL2(Ω;H~α(O)), 1≤ p ≤∞ and α ∈ [-2, 2], is introduced to characterize the regularity of the noise in the semilinear stochastic heat equation du-△udt = f(u)dt + d W(t),under the following conditions for some α ∈(0, 1]:‖(∫t)0e~(-(t-s)A)dW(S)‖_(L2(Ω;L2(O)))≤Cta/2and ‖(∫t)0e~(-(t-s)A)dW(S)‖_(B~∞L2(Ω;H~α(O)))≤C The conditions above are shown to be satisfied by both trace-class noises(with α = 1) and one-dimensional space-time white noises(with α =1/2). The latter would fail to satisfy the conditions with α =1/2 if the stochastic Besov norm ∥·∥_(B~∞L2(Ω;H~α(O)))is replaced by the classical Sobolev norm ∥·∥_(L2(Ω;H~α(O))), and this often causes reduction of the convergence order in the numerical analysis of the semilinear stochastic heat equation. In this paper, the convergence of a modified exponential Euler method, with a spectral method for spatial discretization,is proved to have order α in both the time and space for possibly nonsmooth initial data in L4(Ω;H~β(O)) withβ >-1, by utilizing the real interpolation properties of the stochastic Besov spaces and a class of locally refined stepsizes to resolve the singularity of the solution at t = 0.

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Numerical investigation and modeling of sweep effects on inlet flow field of axial compressor cascades

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Chinese Journal of Aeronautics 2024年第2期37卷 296-308页

作者： Jiancheng ZHANG Donghai JIN Xingmin gui School of Energy and Power Engineering Beihang UniversityBeijing 100191China Jiangxi Research Institue of Beihang University Nanchang 330096China

Swept blades are widely utilized in transonic compressors/fans and provide high load,high through-flow,high efficiency,and adequate stall ***,there is limited quantitative research on the mechanism of the effect of swept blades on the flow field,resulting in a lack of direct quantitative guidance for the design and analysis of swept blades in fans/*** better understand this mechanism,this study employs a reduced-dimensional force equilibrium method to analyze more than 1500 swept cascades *** verify that circumferential fluctuation terms are responsible for inducing radial migration in the inlet airflow field of the swept blade,resulting in variations in the incidence angle and consequently leading to changes in the characteristics of the swept ***,a combination of simple functions and machine learning is utilized to model the circumferential fluctuation terms and quantify the sweep *** prediction accuracy of the model is high,with coefficient of determination greater than 0.95 on the test *** the model is applied in a meridional flow analysis program,the calculation accuracy of the program for the incidence angle is improved by 0.4°and 0.6°at the design and off-design conditions respectively,compensating for the program’s original ***,the model can also provide quantitative guidance for the design of swept blades,thereby reducing the number of design iterations and improving design efficiency.

关键词： Turbomachinery Sweep aerodynamics Quasi-3D method Incidence angle Circumferential fluctuation Machine learning

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Recent advances in visible light-mediated chemical transformations of enaminones

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Chinese Chemical Letters 2024年第2期35卷 4-15页

作者： Yu Han Liyun Zhou Chengyu wang Shangti Feng rong Ma Jie-Ping Wan College of Chemistry and Chemical Engineering Jiangxi Normal UniversityNanchang 330022China School of Chemistry and Chemical Engineering Linyi UniversityLinyi 276000China Linyi Sanfeng Chemical Co. Ltd.Linyi 276000China

Enaminones,which possesses both the nucleophilic enamine as well as electrophilic enone structures,are well known versatile building blocks in organic ***,visible light-mediated reactions have emerged as useful synthetic strategy with enhanced *** the last decade,various photochemical transformations of enaminones have been developed to construct cyclic or acyclic *** this review,we describe the recent advances in visible light-mediated chemical transformations of *** discussion on the reaction mechanism of the related reactions is given to provide guide to the ***,a summary on the existing challenges and the future outlook towards the development of practical photocatalytic reactions of enaminones is also presented.

关键词： Enaminone Visible light C-H functionalization C=C bond cleavage Cyclization Multicomponent reactions

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Recent progress on electro-sorption technology for lithium recovery from aqueous sources

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Nano Research 2024年第4期17卷 2563-2573页

作者： Qichen Lu Peng Liu Tianyi Zhou Ruling Huang Kexin Zhang Lin Hu rong Liu Zhibo Ren Jinyi wang Xiaolong wang Huaneng Clean Energy Research Institute Beijing 102209China

Lithium is known as the“white petroleum”of the electrification era,and the global demand for lithium grows rapidly with the quick development of new energy *** aqueous solutions,such as salt lake brine,underground brine,and seawater,have large lithium reserves,thus this kind of lithium resource has become a research hotspot *** with other lithium extraction technologies,electro-sorption method shows good prospects for practical applications with advantages in the aspects of efficiency,recovery ratio,cost,and ***,this review covers recent progress on electro-sorption technology for lithium recovery from aqueous solutions,including the concept illustration,research progress of the applied working electrodes and counter electrodes,and the evaluation indicators of electro-sorption ***,some prospects for the development of this technology are also *** hope this review is beneficial for the construction of high-efficient electrochemical lithium recovery system to achieve an adequate lithium supply in the future.

关键词： lithium extraction electro-sorption technology lithium selective electrode counter electrode system evaluation method

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