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Na_(3)P interphase reduces Na nucleation energy enabling stable anode-less sodium metal batteries

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Journal of energy chemistry 2024年第9期96卷 448-455页

作者： Haizhao Yang Haifeng Lv en Zhou Xiaohao Ji chunnian c.en Haolei Yu Zhaowei Sun Dawei Zhang Hongchang Jin Xianghua Kong Hengxing Ji Department of chemistry and chemical engineering Hefei University of TechnologyHefei 230009AnhuiChina Hefei National Research center for Physical Sc.ences at the Microscale School of Chemistry and Materials ScienceUniversity of Science and Technology of ChinaHefei 230026AnhuiChina

Sodium metal batteries(SMBs)are rising as viable alternatives to lithium-ion systems due to their superior energy density and sodium's relative ***,SMBs face significant impediments,particularly the exceedingly high negative-to-positive capacity ratios(N/P ratios)which severely encumber energy density and hinder their practical ***,a novel nucleophilic Na_(3)P interphase on aluminum foil has been designed to significantly lower the nucleation energy barrier for sodium atom deposition,resulting in a remarkable reduction of nucleation overpotential and effic.ent mitigation of dendritic growth at high sodium deposition of 5 mA h cm^(−2).The interphase promotes stable cycling in anode-less SMB configurations with a low N/P ratio of 1.4 and high cathode mass loading of 11.5 mg cm^(−2),and demonstrates a substantial increase in high capacity retention of 92.4%after 500 cycles even under 1 c rate *** innovation signifies a promising leap forward in the development of high-energy-density,anode-less SMBs,offering a potential solution to the longstanding issues of cycle stability and energy effic.ency.

关键词： Anode-less Phosphorus anode Nucleation buffer layer Sodium metal Dendrite-free

磁序与拓扑的耦合:从基础物理到拓扑磁电子学

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物理学报 2024年第1期73卷 24-30页

作者：刘恩克中国科学院物理研究所磁学国家重点实验室北京100190

磁学与拓扑物理是两大较为成熟的学科,二者的结合是新一代磁电子学的需求和基础.磁性拓扑材料是磁序与拓扑物理耦合的重要产物,为新兴的拓扑物理提供了材料载体和调控自由度.磁性外尔半金属实现了时间反演对称破缺下的外尔费米子拓扑物... 详细信息

磁学与拓扑物理是两大较为成熟的学科,二者的结合是新一代磁电子学的需求和基础.磁性拓扑材料是磁序与拓扑物理耦合的重要产物,为新兴的拓扑物理提供了材料载体和调控自由度.磁性外尔半金属实现了时间反演对称破缺下的外尔费米子拓扑物态,通过拓扑增强的贝利曲率产生了一系列新奇的磁/电/热/光效应;而外尔电子与磁序的相互作用也使得拓扑电子物理有望成为磁电子学应用的新原理和驱动力.当前,新物态与新效应的发现是磁性拓扑材料第一阶段的主要任务和特征,而动量空间拓扑电子与实空间磁序的相互作用已经开始进入人们的视野.这两个阶段的深入发展,将为拓扑磁电子学积累必要的物理基础和应用尝试.本文着眼于磁性拓扑材料发展的两个阶段,讲述磁性拓扑材料的提出和实现、均一磁序下的拓扑电子态及新奇物性、局域磁态与拓扑电子的相互作用3个方面,阐述当前领域内的热点内容和发展趋势,并对拓扑磁电子学的未来发展进行了思考和展望,以助力未来拓扑自旋量子器件的快速发展.

关键词：拓扑物理磁性外尔半金属拓扑磁电子学

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Mixing states and secondary formation processes of organic nitrogen-containing single particles in Guangzhou,china

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Journal of environmental Sc.ences 2024年第4期138卷 62-73页

作者： Lijun Yun chunlei c.eng Suxia Yang Zaihua Wang Mei Li Qi en Zhong LiyuanMao Sulin Liu Xiaoya c.eng Duanying c.en Fan Yang Zhen Zhou Institute of Mass Spectrometry and Atmospheric.environment Guangdong Provincial Engineering Research Center for on-line source apportionment system of air pollutionJinan UniversityGuangzhou 510632China Guangdong-Hongkong-Macao Joint Laboratory of collaborative Innovation for environmental Quality Guangzhou 510632China State Key Laboratory of Loess and Quaternary Geology Institute of Earth EnvironmentChinese Academy ScienceXi’an 710061China Institute for environment and climate Research Jinan UniversityGuangzhou 510632China Guangdong Academy of Sc.ences Institute of Resources Utilization and Rare Earth DevelopmentGuangzhou 510650China environmental Monitoring Station of Pudong New District Shanghai 201200China

Organic nitrogen(ON)compounds play a significant role in the light absorption of brown carbon and the formation of organic aerosols,however,the mixing state,secondary formation processes,and influencing factors of ON compounds are still *** paper reports on the mixing state of ON-containing particles based on measurements obtained using a highperformance single particle aerosol mass spectrometer in January 2020 in *** ON-containing particles accounted for 21% of the total detected single particles,and the particle count and number fraction of the ON-containing particles were two times higher at night than during the *** prominent increase in the content of ON-containing particles with the enhancement of NO_xmainly occurred at night,and accompanied by high relative humidity and nitrate,which were associated with heterogeneous reactions between organics and gaseous NO_(x)and/or NO_(3)*** synchronous decreases in ON-containing particles and the mass absorption coeffic.ent of water-soluble extracts at 365 nm in the afternoon may be associated with photo-bleaching of the ON species in the *** addition,the positive matrix factorization analysis found five factors dominated the formation processes of ON particles,and the nitrate factor(33%)mainly contributed to the production of ON particles at *** results of this study provide unique insights into the mixing states and secondary formation processes of the ON-containing particles.

关键词： Organic nitrogen compounds Single particles Mixing state Secondary formation Nighttime chemistry

Mechanical Behavior and Failure Mechanism of an As-Extruded Mg-11wt%Y Alloy at Elevated Temperature

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Acta Metallurgica Sinica(english Letters) 2024年第6期37卷 969-981页

作者： Lan Zhang Dao-Kui Xu Bao-Jie Wang cui-Lan Lu Shuo Wang Xiang-Bo Xu Dong-Liang Wang Xin Lv en-Hou Han School of Materials Sc.ence and engineering University of Science and Technology of ChinaShenyang110016China Key Laboratory of Nuclear Materials and Safety Assessment Institute of Metal ResearchChinese Academy of SciencesShenyang110016China School of environmental and chemical engineering Shenyang Ligong UniversityShenyang110159China Key Lab of Electromagnetic Processing of Materials Ministry of EducationNortheastern UniversityShenyang110819China Institute of corrosion Sc.ence and Technology Guangdong510070China

Through carrying out the high-temperature tensile experiments on an as-extruded Mg-11wt%Y alloy at 350℃,400℃,450℃,500℃and 550℃,the mechanical behavior and fracture mechanisms at elevated temperatures are investigated and *** results show that with the increase of temperature,the yield strength and ultimate tensile strength of the alloy increase at first and then decrease,while that the elongation ratio decreases firstly and then *** the sample being tested at 350℃,the values of yield strength,ultimate tensile strength and the elongation ratio are 188 MPa,266 MPa and 11%,*** 400℃,the yield strength and ultimate tensile strength reach the maximum values of,respectively,198 MPa and 277 MPa,but the elongation ratio is the lowest and its value is only 8%.When the applied temperature is increased to 550℃,the values of yield strength and ultimate tensile strength,respectively,decrease to 140 MPa and 192 MPa and the elongation ratio increases to 38%.Failure analysis demonstrates that the fracture surfaces of different samples are mainly composed of plastic dimples and exhibit the typical characteristic of ductile *** observation to the fracture side surfaces indicates that at the temperatures of 350℃and 400℃,microcracks mainly initiate in the interior of Mg_(24)Y_(5)*** the temperatures are 450℃,500℃and 550℃,the cracks preferentially initiate at the Mg_(24)Y_(5)/α-Mg interfaces.

关键词： Mg-Y alloy High-temperature tensile properties Fracture mechanism Failure analysis

A novel clinical data management platform for acute pancreatitis

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Journal of Zhejiang University-Sc.ence B(Biomedicine & Biotechnology) 2024年第8期25卷 711-718页

作者： Shiyin c.en c.eng ZHANG Zhi’en WANG Jian ZHANG Wenqiao YU Yanshuai WANG Weiwei SI Tingbo LIANG Yun ZHANG Department of Hepatobiliary and Pancreatic Surgery Zhejiang Provincial Key Laboratory of Pancreatic Diseasethe First Affiliated HospitalZhejiang University School of MedicineHangzhou 310003China Department of Rehabilitation Medicine the First Affiliated HospitalZhejiang University School of MedicineHangzhou 310003China Department of comprehensive Intensive care Unit the First Affiliated HospitalZhejiang University School of MedicineHangzhou 310003China

This study presents a multi-center clinical data management platform that facilitates unified and structured management of real-world data and serves as an ideal tool to enhance the quality and progress of clinical research related to severe acute pancreatitis(SAP).The use of the platform enables clinical teams to obtain safe,accurate,structurally unified,traceable,sceneclear,and fully functional real-world medical data in the diagnosis,treatment,and research of acute pancreatitis(AP).

关键词： clinical pancreatitis acute

Microstructure and texture evolution of cu-cr-co-Ti alloys during the two-stage cryorolling

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Rare Metals 2024年第9期43卷 4535-4547页

作者： Jia-Jun Zhang Long-Jian Li Zhi-Feng Liu Zong-Ning c.en en-Yu Guo Hui-Jun Kang Ren-Geng Li Tong-Min Wang Key Laboratory of Solidification control and Digital Preparation Technology(Liaoning Province) School of Materials Science and EngineeringDalian University of TechnologyDalian 116024China center of Hyper-Gravity Experimental and Interdisciplinary Research Zhejiang UniversityHangzhou 310058China Ningbo Institute of Dalian University of Technology Ningbo 315000China Key Laboratory for Light-Weight Materials Nanjing Tech UniversityNanjing 210009China

This study entailed an investigation of the mechanical properties,microstructural and texture orientation evolutions of cu-cr-co-Ti alloys prepared via twostage cryorolling and intermediate aging *** this end,X-ray diffraction and electron backscatter diffraction were *** results indicate that the two-stage cryorolling and intermediate aging treatments led to the development of profuse twin bundles and significantly enhanced the mechanical *** initial cryorolling led to coplanar slip and developed a strong Y({111})orientation,accelerating the formation of Goss({011})orientation and a Brass-type *** intermediate aging treatment relieved the restriction on dislocation slip and reoriented the grains toward the copper({112})and Z({111})*** Z orientation,with a relatively high volume fraction,dominated the *** cryorolling intensified twinning and shear banding,transforming the copper-type shear bands into Brass-type shear bands with rhomboidal prism *** areas inside the Brasstype shear bands exhibited a Y orientation,and the areas outside the shear bands exhibited a stable Brass-type *** evident decrease in the weighted Schmid factors demonstrated that the two-stage cryorolling and intermediate aging treatment can modify the texture evolution and aid the design of high-performance cu alloys.

关键词： copper alloys Two-stage cryorolling Macrotexture evolution Electron backscatter diffraction Schmid factor

Transcriptome analysis suggests broad jejunal alterations in Linghu’s obesity-diarrhea syndrome:A pilot study

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World Journal of Gastroenterology 2024年第21期30卷 2777-2792页

作者： Xiao-Tong Niu Xiang-Yao Wang Yan Wang Ke Han Nan Ru Jing-Yuan Xiang en-Qiang Linghu Medical School of chinese PLA Chinese PLA General HospitalBeijing 100853China Department of Gastroenterology The First Medical Center of Chinese PLA General HospitalBeijing 100853China School of Medicine Nankai UniversityTianjin 300071China

BAcKGROUND Obesity is associated with a significantly increased risk for chronic diarrhea,which has been proposed as Linghu’s obesity-diarrhea syndrome(ODS);however,its molecular mechanisms are largely *** To reveal the transcriptomic changes in the jejunum involved in *** In a cohort of 6 ODS patients(JOD group),6 obese people without diarrhea(JO group),and 6 healthy controls(Jc group),high-throughput sequencing and bioinformatics analyses were performed to identify jejunal mucosal mRNA expression alterations and dysfunctional biological *** another cohort of 16 ODS patients(SOD group),16 obese people without diarrhea(SO group),and 16 healthy controls(Sc group),serum diamine oxidase(DAO)and D-lactate(DLA)concentrations were detected to assess changes in intestinal barrier *** The gene expression profiles of jejunal mucosa in the JO and Jc groups were similar,with only 1 differentially expressed gene(DEG).The gene expression profile of the JOD group was significantly changed,with 411 DEGs compared with the JO group and 211 DEGs compared with the Jc group,129 of which *** enrichment analysis of these DEGs showed that the biological processes such as digestion,absorption,and transport of nutrients(especially lipids)tended to be up-regulated in the JOD group,while the biological processes such as rRNA processing,mitochondrial translation,antimicrobial humoral response,DNA replication,and DNA repair tended to be down-regulated in the JOD *** DEGs(cDT1,NHP2,EXOSc5,EPN3,NME1,REG3A,PLA2G2A,and PRSS2)may play a key regulatory role in the pathological process of ODS,and their expression levels were significantly decreased in ODS patients(Pcond cohort,compared with healthy controls,the levels of serum intestinal barrier function markers(DAO and D-LA)were significantly increased in all obese individuals(PcONcLUSION compared with health

关键词： Obesity chronic diarrhea Jejunum Transcriptome Intestinal barrier

Interconnections between diabetic corneal neuropathy and diabetic retinopathy:diagnostic and therapeutic implications

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Neural Regeneration Research 2025年第8期20卷 2169-2180页

作者： Mingyi Yu Faith Teo en Ning chang Liu Yu-chi Liu Tissue engineering and Stem cell Group Singapore Eye Research InstituteSingapore Yong Loo Lin School of Medicine National University of SingaporeSingapore Department of cornea and External Eye Disease Singapore National Eye CenterSingapore Ophthalmology and Visual Sc.ences Academic clinical Program Duke-NUS Medical SchoolSingapore

Diabetic corneal neuropathy and diabetic retinopathy are ocular complications occurring in the context of diabetes *** corneal neuropathy refers to the progressive damage of corneal *** retinopathy has traditionally been considered as damage to the retinal ***,growing evidence suggests that diabetic retinopathy is a complex neurovascular disorder resulting from dysfunction of the neurovascular unit,which includes both the retinal vascular structures and neural *** retinopathy is one of the leading causes of blindness and is frequently screened for as part of diabetic ocular ***,diabetic corneal neuropathy is commonly overlooked and underdiagnosed,leading to severe ocular surface *** studies have found that these two conditions tend to occur together,and they share similarities in their pathogenesis pathways,being triggered by a status of chronic *** review aims to discuss the interconnection between diabetic corneal neuropathy and diabetic retinopathy,whether diabetic corneal neuropathy precedes diabetic retinopathy,as well as the relation between the stage of diabetic retinopathy and the severity of corneal *** also endeavor to explore the relevance of a corneal screening in diabetic eyes and the possibility of using corneal nerve measurements to monitor the progression of diabetic retinopathy.

关键词： cornea corneal nerves diabetes diabetic corneal neuropathy diabetic retinopathy retina

Research on the High-Quality Development of Agricultural Supply chain Financial Ecosystem Empowered by Sc.ence and Technology

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Proceedings of Business and Economic Studies 2024年第5期7卷 98-105页

作者： chunhui Wang Qi’en Zhang School of Finance Jilin Business and Technology CollegeChangchun 130507China

A systematic perspective on agricultural supply chain finance can offer fresh insights into its *** high-quality development of the agricultural supply chain finance ecosystem is crucial for the comprehensive revitalization of rural areas and the realization of agricultural *** on the current state of development of this ecosystem,this paper identifies several bottlenecks,such as insuffic.ent policy and technical support in the macro-environment system,weak incentives for independent circulation within the industrial environment system,and inadequate motivation for stakeholders to participate in the micro-environment *** address these issues,this paper proposes that the visualization,digitalization,and authenticity characteristics of the“blockchain+Internet of Things”technology architecture can effectively resolve these ***,targeted strategies are suggested to promote the high-quality development of the agricultural supply chain finance ecosystem.

关键词： Agricultural supply chain finance ecosystem High-quality development Blockchain+Internet of Things