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Nano Research 2024年第5期17卷 4307-4313页

作者： Zhiquan Lang guang-ling song Xingpeng Liao Wenzhong Huang Yixing Zhu Haipeng Wang Dajiang Zheng Center for Marine Materials Corrosion and Protection College of MaterialsXiamen UniversityXiamen 361005China Department of Ocean Science and Engineering Southern University of Science and TechnologyShenzhen 518055China State Key Laboratory of Physical Chemistry of Solid Surfaces Xiamen UniversityXiamen 361005China The University of Queensland St.LuciaOLD 4072Australia State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan 430070China Department of Mechanical Engineering Tsinghua UniversityBeijing 100084China

Controllable and scalable preparation of electrocatalyst materials holds significant importance for their practical application.Magnetron sputtering is a highly effective synthesis method,known for its producing uniform films and allowing easy control of component compositions.In this paper,we propose an in-situ synthesis method for layered double hydroxide(LDH)electrocatalysts through sacrificing magnetron sputtered films.The resulting FeCo-LDH catalyst demonstrated a low overpotential of only 300 mV at 10 mA·cm^(-2).Furthermore,we conducted spectroscopic analysis to investigate the surface changes of the catalysts during the oxygen evolution reaction(OER)process.Our findings indicated that the formation of Co oxyhydroxides plays a beneficial role in enhancing the catalytical performance of the FeCo-LDH for OER reaction.This restructuring strategy of converting a magnetron-sputtered sacrificial film into a catalytical LDH introduces a new avenue to the synthesis of transition metal-based electrocatalysts.

关键词： magnetron co-sputtering surface reconstruction electrocatalyst oxygen evolution reaction

Recently deepened insights regarding Mg corrosion and advanced engineering applications of Mg alloys

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Journal of Magnesium and Alloys 2023年第11期11卷 3948-3991页

作者： guang-ling song Andrej Atrens Department of Ocean Science and Engineering Southern University of Science and Technology1088 Xueyuan BoulevardShenzhen 518055China The University of Queensland School of Mechanical and Mining EngineeringCentre for Advanced Materials Processing and Manufacturing(AMPAM)St LuciaQld 4072 Australia State Key Laboratory of Physical Chemistry of Solid Surfaces Xiamen University422 S.Siming RdXiamen 361005China

This review summarizes recent insights into the Mg corrosion mechanism, clarifies many critical controversial points regarding the Mg corrosion behaviour, and updates some efforts made to extend the industrial application of Mg alloys. Based on the new understandings gained so far, future research directions are also suggested in the review. This review has the following logic. The first section "1. Scope"is a consolidation of the new understandings or developments regarding the Mg corrosion mechanism and the new applications for Mg alloys. It also highlights some key points for the review. The second section "2. Widely accepted knowledge" briefly summarizes the general understanding of Mg corrosion gained so far, which acts as the foundation for the following sections. The third section "3. Recently deepened insights" mainly briefs on some new insights into Mg corrosion phenomena based on recent findings. Different interpretations on the corrosion behaviours are comprehensively discussed in the fourth section "4. Controversial points" and the conclusions are drawn in the subsection"4.5 Clarified points". Apart from the fundamental understandings, various efforts in the application of Mg alloys are presented in the fifth section "5. New applications". Following the research tendency as indicated in the review, prioritized research areas are suggested in "6.Future directions". The review is concluded with "7. Concluding remarks" at last.

关键词： Mg Corrosion Hydrogen Anode Intelligentization

A corrosion-reconstructed and stabilized economical Fe-based catalyst for oxygen evolution

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Nano Research 2023年第2期16卷 2224-2229页

作者： Zhiquan Lang guang-ling song Pengpeng Wu Dajiang Zheng Center for Marine Materials Corrosion and Protection Xiamen UniversityXiamen 361005China Department of Ocean Science and Engineering Southern University of Science and TechnologyShenzhen 518055China State Key Laboratory of Physical Chemistry of Solid Surfaces Xiamen UniversityXiamen 361005China The University of Queensland St.LuciaQLD 4072Australia

The anode activity can to a great degree limit the cathodic hydrogen evolution efficiency in an electrolyte cell.Thus,cost-efficient electrocatalysts with good water oxidation performance and stability are highly desired in widespread implementation of the hydrogen production from water splitting.This paper proposes a facile corrosion-reconstruction strategy to transform Fe surface into a Fe-Co hydroxide layer to improve the oxygen evolution activity.The as-prepared catalyst was measured to have an over-potentential as low as 320 mV at 100 mA·cm^(−2),and its stability even exceeded 600 h.Surface and Raman spectroscopy analyses indicated that the catalyst experienced chemical changes from hydroxides to oxyhydroxides and Co^(2+)to Co^(3+)during oxygen evolution reaction(OER).The corrosion-reconstruction is not only an economical method to synthesize a highly efficient,stable and durable Fe-based catalysts,it also converses the detrimental corrosion into a beneficial catalyst fabrication process.

关键词： oxygen evolution reaction electrocatalyst corrosion stability

Self-repairing functionality and corrosion resistance of in-situ Mg-Al LDH film on Al-alloyed AZ31 surface

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Journal of Magnesium and Alloys 2023年第5期11卷 1567-1579页

作者： Yi-Xing Zhu guang-ling song Peng-Peng Wu Center for Marine Materials Corrosion and Protection College of MaterialsXiamen University422 S.Siming RdXiamenFujian 361005China State Key Laboratory of Physical Chemistry of Solid Surfaces Xiamen University422 S.Siming RdXiamenFujian 361005China School of Mechanical and Mining Engineering The University of QueenslandBrisbaneQueensland 4072Australia

A novel Mg-Al LDH film was in-situ prepared hydrothermally in an alkaline aqueous solution on an Al-alloyed AZ31 substrate.The structural,chemical and functional characteristics of the film were explored by means of scanning electron microscope(SEM),X-ray diffraction(XRD),energy dispersive spectrometer(EDS),polarization curve,AC impedance and salt immersion tests,respectively.The anti-corrosion results indicated that the Mg-Al LDH film on the Al-alloyed AZ31 surface could effectively protect the AZ31 from corrosion attack even after 90 days of immersion in 3.5 wt.%NaCl solution.The protection performance is surprisingly better than most of the reported coatings on Mg alloys.More interestingly,when the Mg-Al LDH film was scratched,the exposed Al-alloyed surface might gradually release metal ions and re-generate dense LDH nano-sheets in the corrosive environment to inhibit the further corrosion there,exhibiting a self-repairing behavior.The combination of the benign long-term protection and desirable self-repairing performance in this new process of surface-alloying and LDH-formation may significantly extend the practical application of magnesium alloys.

关键词： LDH film Surface alloying Corrosion resistance Self-repairing

Bio-inhibitive effect of an algal symbiotic bacterium on corrosion of magnesium in marine environment

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Journal of Magnesium and Alloys 2023年第12期11卷 4603-4618页

作者： Yuqiao Dong guang-ling song Yuqing Xu Dajiang Zheng College of Materials Xiamen UniversityXiamen 361005China Department of Ocean Science and Engineering Southern University of Science and TechnologyShenzhenChina State Key Laboratory of Physical Chemistry of Solid Surfaces Xiamen University422 S.Siming RdXiamen361005China The University of Queensland School of Mechanical and Mining EngineeringDivision of Materials EngineeringSt LuciaQld 4072 Australia Institute of Corrosion Science and Technology Guangzhou510530GuangdongChina

It is a longstanding and challenging task to develop sustainable environment-friendly and cost-effective corrosion-protection technologies for Mg alloys, especially under marine conditions in which corrosion can normally be significantly accelerated by bacterial activity. However,this paper reports on the corrosion of highly active Mg interestingly inhibited by an algal-symbiotic bacterium Bacillus altitudinis. The corrosion of Mg in the presence of the bacterium drastically reduced by one order of magnitude after 14 days of immersion. This means that the algal-symbiotic bacterium widely available in natural ocean environments may be employed as a green and sustainable inhibitor in the marine industry. Based on electrochemical measurements, surface analyses and microbe experiments, a combined inhibition mechanism is proposed in the paper to interpret the interesting corrosion behavior of Mg.

关键词： Magnesium Corrosion inhibition Marine environment Biofilm Bacterium

Cross-species transmission and host range genes in poxviruses

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Virologica Sinica 2024年第2期39卷 177-193页

作者： Chen-Hui Yang A-ling song Ye Qiu Xing-Yi Ge College of Biology Hunan Provincial Key Laboratory of Medical VirologyHunan UniversityChangsha410012China

The persistent epidemic of human mpox, caused by mpox virus (MPXV), raises concerns about the future spread ofMPXV and other poxviruses. MPXV is a typical zoonotic virus which can infect human and cause smallpox-likesymptoms. MPXV belongs to the Poxviridae family, which has a relatively broad host range from arthropods tovertebrates. Cross-species transmission of poxviruses among different hosts has been frequently reported andresulted in numerous epidemics. Poxviruses have a complex linear double-strand DNA genome that encodeshundreds of proteins. Genes related to the host range of poxvirus are called host range genes (HRGs). This reviewbriefly introduces the taxonomy, phylogeny and hosts of poxviruses, and then comprehensively summarizes thecurrent knowledge about the cross-species transmission of poxviruses. In particular, the HRGs of poxvirus aredescribed and their impacts on viral host range are discussed in depth. We hope that this review will provide acomprehensive perspective about the current progress of researches on cross-species transmission and HRGvariation of poxviruses, serving as a valuable reference for academic studies and disease control in the future.

关键词： Poxvirus Host range gene(HRG) Host spectrum Cross-species transmission

The anodically polarized Mg surface products and accelerated hydrogen evolution

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Journal of Magnesium and Alloys 2023年第1期11卷 230-248页

作者： Jufeng Huang guang-ling song Yixing Zhu Dajiang Zheng Ziming Wang Center for Marine Materials Corrosion and Protection College of MaterialsXiamen UniversityPeople’s Republic of China State Key Laboratory of Physical Chemistry of Solid Surfaces Xiamen UniversityXiamen 361005People’s Republic of China School of Engineering The University of QueenslandSt.LuciaQld 4072Australia

To clarify the anodic dissolution mechanism of Mg,the hydrogen evolution from pure Mg in acidic solutions under galvanostatic conditions were systematically measured.With increasing anodic current density,the cathodic hydrogen evolution rate decreased,and the anodic hydrogen evolution became faster while some surface area on the Mg was becoming dark under anodic polarization.Based on the surface analysis results and the generally accepted basic electrochemical equations,the evolution kinetics of hydrogen from Mg was deduced,and the most possible surface intermediate active species that could facilitate the anodic Mg dissolution and anodic hydrogen evolution were proposed.This paper further develops the model of incomplete film Mg^(+) dissolution,explains many reported experimental phenomena,and clarifies misunderstandings of current mechanism.

关键词： Magnesium Corrosion Hydrogen evolution Negative difference effect

Mathematical Model,Numerical Simulation and Convergence Analysis of a Semiconductor Device Problem with Heat and Magnetic Influences

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Acta Mathematicae Applicatae Sinica 2024年第2期40卷 302-319页

作者： Chang-feng LI Yi-rang YUAN Huai-ling song School of Economics Shandong UniversityJinan 250100China Institute of Mathematics Shandong UniversityJinan 250100China College of Mathematics and Econometrics Hunan UniversityChangsha 410082China

In this paper,the authors discuss a three-dimensional problem of the semiconductor device type involved its mathematical description,numerical simulation and theoretical analysis.Two important factors,heat and magnetic influences are involved.The mathematical model is formulated by four nonlinear partial differential equations(PDEs),determining four major physical variables.The influences of magnetic fields are supposed to be weak,and the strength is parallel to the z-axis.The elliptic equation is treated by a block-centered method,and the law of conservation is preserved.The computational accuracy is improved one order.Other equations are convection-dominated,thus are approximated by upwind block-centered differences.Upwind difference can eliminate numerical dispersion and nonphysical oscillation.The diffusion is approximated by the block-centered difference,while the convection term is treated by upwind approximation.Furthermore,the unknowns and adjoint functions are computed at the same time.These characters play important roles in numerical computations of conductor device problems.Using the theories of priori analysis such as energy estimates,the principle of duality and mathematical inductions,an optimal estimates result is obtained.Then a composite numerical method is shown for solving this problem.

关键词： three-dimensional conductor device problem with heat and magnetic influences upwind blockcentered differences elemental conservation of mass numerical analysis

Mesenchymal stem cell-derived extracellular vesicles in skin wound healing:roles,opportunities and challenges

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Military Medical Research 2024年第3期11卷 400-429页

作者： Jia-Yi Ding Min-Jiang Chen ling-Feng Wu Gao-Feng Shu Shi-Ji Fang Zhao-Yu Li Xu-Ran Chu Xiao-Kun Li Zhou-guang Wang Jian-song Ji Key Laboratory of Imaging Diagnosis and Minimally Invasive Intervention Research Institute of Imaging Diagnosis and Minimally Invasive Intervention Researchthe Fifth Affiliated Hospital of Wenzhou Medical UniversityZhejiangLishui 323000China Oujiang Laboratory(Zhejiang Lab for Regenerative Medicine Vision and Brain Health)School of Pharmaceutical ScienceWenzhou Medical UniversityWenzhou 325035ZhejiangChina Clinical College of the Affiliated Central Hospital School of MedicineLishui UniversityLishui 323000ZhejiangChina Department of Overseas Education College Jimei UniversityXiamen 361021FujianChina Department of Medicine II Internal MedicineCardio-Pulmonary Institute(CPI)Universities of Giessen and Marburg Lung Center(UGMLC)Member of the German Center for Lung Research(DZL)Justus-Liebig University Giessen35392 GiessenGermany Pulmonary and Critical Care Department of Medicine VInternal MedicineInfectious Diseases and Infection ControlUniversities of Giessen and Marburg Lung Center(UGMLC)Member of the German Center for Lung Research(DZL)Justus-Liebig University Giessen35392 GiessenGermany

Skin wounds are characterized by injury to the skin due to trauma,tearing,cuts,or contusions.As such injuries are common to all human groups,they may at times represent a serious socioeconomic burden.Currently,increasing numbers of studies have focused on the role of mesenchymal stem cell(MSC)-derived extracellular vesicles(EVs)in skin wound repair.As a cell-free therapy,MSC-derived EVs have shown significant application potential in the field of wound repair as a more stable and safer option than conventional cell therapy.Treatment based on MSC-derived EVs can significantly promote the repair of damaged substructures,including the regeneration of vessels,nerves,and hair follicles.In addition,MSC-derived EVs can inhibit scar formation by affecting angiogenesis-related and antifibrotic pathways in promoting macrophage polarization,wound angiogenesis,cell proliferation,and cell migration,and by inhibiting excessive extracellular matrix production.Additionally,these structures can serve as a scaffold for components used in wound repair,and they can be developed into bioengineered EVs to support trauma repair.Through the formulation of standardized culture,isolation,purification,and drug delivery strategies,exploration of the detailed mechanism of EVs will allow them to be used as clinical treatments for wound repair.In conclusion,MSCderived EV-based therapies have important application prospects in wound repair.Here we provide a comprehensive overview of their current status,application potential,and associated drawbacks.

关键词： Mesenchymal stem cell(MSC) Extracellular vesicles(EVs) Wound repair Engineered nanoparticles

Biocorrosion induced by red-tide alga-bacterium symbiosis and the biofouling induced by dissolved iron for carbon steel in marine environment

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Journal of Materials Science & Technology 2022年第33期128卷 107-117页

作者： Yuqiao Dong guang-ling song Jiawei Zhang Yahui Gao Zi Ming Wang Dajiang Zheng Center for Marine Materials Corrosion and Protection College of MaterialsXiamen UniversityXiamen 361005China School of Life Sciences and Key Laboratory of Ministry of Education for Coastal and Wetland Ecosystems Xiamen UniversityXiamen 361102China Department of Ocean Science and Engineering Southern University of Science and TechnologyShenzhen 518055China The University of Queensland School of Mechanical and Mining EngineeringDivision of Materials EngineeringSt LuciaQld 4072Australia

The assemblages of unicellular microalgae and bacteria in phytoplankton communities can generally result in biodeterioration of metals in marine environment.In this study,the self-promoted biofouling mechanism underneath red-tide alga Phaeodactylum tricornutum and its symbiotic bacterium Bacillus altitudinis was systematically revealed.The mutualistic interaction of the bacteria and algae quadrupled the corrosion rate in comparison to the individual effect of the bacterium or algal strain alone.Reversely,the corroded metal appeared to be an accelerator that can stimulate the activity of the P.tricornutum and aggravate the biological pollution based on the result of 62.3%up-regulation of the key photosynthesis genes.The corrosion-biofouling-accelerated corrosion-deteriorated biofouling formed a vicious cycle.

关键词： Algal-bacterial symbiosis Marine biofouling Carbon steel Corrosion products