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Modulated noble metal/2D MOF heterostructures for improved hydrogen storage of MgH_(2)

Rare Metals 2024年第4期43卷 1672-1685页

作者： Zeng-Yi Li Li-xian Sun Fen Xu Yu-Mei Luo Yong-Peng xia Sheng Wei Chen-Chen Zhang Ri-guang Cheng Chao-Feng Ye Meng-Yuan Liu Ju-Lan Zeng Zhong Cao Hong-Ge Pan School of Material Science and Engineering Guilin University of Electronic TechnologyGuilin541004China School of Chemistry and Chemical Engineering Changsha University of Science and TechnologyChangsha410114China Institute of Science and Technology for New Energy Xi’an Technological UniversityXi’an710021China

The conjugation of external species with twodimensional(2D)materials has broad application *** this study,we have explored the potential of noble metal/2D MOF heterostructures in hydrogen ***,the MgH_(2)-Ni-MOF@Pd system has shown remarkable hydrogen desorption/sorption performances,starting to liberate hydrogen at 1810C,which is 2300C lower than that of pristine *** the catalytic effect of Ni-MOF@Pd,the dehydrogenation apparent activation energy of MgH2 is noticeably decreased from(133.5±17.5)to(34.58±1.87)kJ·moL^(-1),and the hydrogenation apparent activation energy is reduced from(70.41±7.43)to(25.78±4.64)kJ·moL^(-1),which is lowered by 63.4%.The fully-dehydrogenated MgH2-NiMOF@Pd composite rapidly uptakes hydrogen,with 2.62wt%at 100℃and 6.06 wt%at 150℃within 300 s,*** mechanism analysis of MgH2 catalyzed by Ni-MOF@Pd has revealed that the transformation of Mg_2Ni and Mg_2NiH_4 could act as a"hydrogen pump",providing numerous channels for fast diffusion and transport of hydrogen ***,in the dehydrogenation process,the element Pd reacts with MgH_(2)to form the MgPd alloy phase,which makes MgH_(2)take precedence to decompose through the Mg-Pd alloy rather than self-decomposition,further reducing thermal stability and improving de/hydrogenation *** synergistic effect of Mg-Pd,Mg_2Ni,and the special ultra-thin 2D sheet structure of the additive is the main reason for the good hydrogen storage property of MgH_(2)-Ni-MOF@*** findings provide inspiration for designing efficient multifunctional additives with unique morphologies to optimize the hydrogen desorption/sorption behaviors of hydrogen storage materials.

关键词： Hydrogen storage Magnesium hydride 2D metal-organic framework nanosheets Ni/Pd Synergistic catalysis

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A Deep-Learning and Transfer-Learning Hybrid Aerosol Retrieval Algorithm for FY4-AGRI:Development and Verification over Asia

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Engineering 2024年第7期38卷 164-174页

作者： Disong Fu Hongrong Shi Christian AGueymard Dazhi Yang Yu Zheng Huizheng Che Xuehua Fan Xinlei Han lin Gao Jianchun Bian Minzheng Duan xiangao xia Key Laboratory of Middle Atmosphere and Global Environment Observation Institute of Atmospheric PhysicsChinese Academy of SciencesBeijing 10029China Key Laboratory of Cloud-Precipitation Physics and Severe Storms Institute of Atmospheric PhysicsChinese Academy of SciencesBeijing 100029China Solar Consulting Services ColebrookNH 03576USA School of Electrical Engineering and Automation Harbin Institute of TechnologyHarbin 150006China State Key Laboratory of Severe Weather&Key Laboratory of Atmospheric Chemistry Institute of Atmospheric Composition and Environmental MeteorologyChinese Academy of Meteorological SciencesChina Meteorological AdministrationBeijing 100081China National Institute of Natural Hazards Ministry of Emergency Management of ChinaBeijing100085China Key Laboratory of Compound and Chained Natural Hazards Dynamics Ministry of Emergency Management of ChinaBeijing 100085China h National Satellite Meteorological Center China Meteorological AdministrationBeijing 100081China University of Chinese Academy of Sciences Beijing 100049China

The Advanced Geosynchronous Radiation Imager(AGRI)is a mission-critical instrument for the Fengyun series of *** acquires full-disk images every 15 min and views East Asia every 5 min through 14 spectral bands,enabling the detection of highly variable aerosol optical depth(AOD).Quantitative retrieval of AOD has hitherto been challenging,especially over *** this study,an AOD retrieval algorithm is proposed that combines deep learning and transfer *** algorithm uses core concepts from both the Dark Target(DT)and Deep Blue(DB)algorithms to select features for the machinelearning(ML)algorithm,allowing for AOD retrieval at 550 nm over both dark and bright *** algorithm consists of two steps:①A baseline deep neural network(DNN)with skip connections is developed using 10 min Advanced Himawari Imager(AHI)AODs as the target variable,and②sunphotometer AODs from 89 ground-based stations are used to fine-tune the DNN ***-of-station validation shows that the retrieved AOD attains high accuracy,characterized by a coefficient of determination(R2)of 0.70,a mean bias error(MBE)of 0.03,and a percentage of data within the expected error(EE)of 70.7%.A sensitivity study reveals that the top-of-atmosphere reflectance at 650 and 470 nm,as well as the surface reflectance at 650 nm,are the two largest sources of uncertainty impacting the *** a case study of monitoring an extreme aerosol event,the AGRI AOD is found to be able to capture the detailed temporal evolution of the *** work demonstrates the superiority of the transfer-learning technique in satellite AOD retrievals and the applicability of the retrieved AGRI AOD in monitoring extreme pollution events.

关键词： Aerosol optical depth Retrieval algorithm Deep learning Transfer learning Advanced Geosynchronous Radiation Imager

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A Nonparametric Model Checking Test for Functional linear Composite Quantile Regression Models

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Journal of Systems Science & Complexity 2024年第4期37卷 1714-1737页

作者： xia Lili DU Jiang ZHANG Zhongzhan Faculty of Science Beijing University of TechnologyBeijing 100124China

This paper is focused on the goodness-of-fit test of the functional linear composite quantile regression model.A nonparametric test is proposed by using the orthogonality of the residual and its conditional expectation under the null *** proposed test statistic has an asymptotic standard normal distribution under the null hypothesis,and tends to infinity in probability under the alternative hypothesis,which implies the consistency of the ***,it is proved that the test statistic converges to a normal distribution with nonzero mean under a local alternative *** simulations are reported,and the results show that the proposed test has proper sizes and is sensitive to the considered model *** proposed methods are also applied to two real datasets.

关键词： Composite quantile regression consistent test functional data nonparametric test quadratic form

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Effects of intensive psychological intervention on treatment compliance,psychological status,and quality of life of patients with epilepsy

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World Journal of Psychiatry 2024年第5期14卷 670-677页

作者： Su-Hua Zhang Jie-Hua Wang Hong-Yu Liu Yue-xia Zhang Ya-ling lin Bi-Yu Wu Department of Neurology Quanzhou First HospitalQuanzhou 362000Fujian ProvinceChina Department of Nursing Quanzhou First HospitalQuanzhou 362000Fujian ProvinceChina

BACKGROUND Epilepsy is a nervous system disease characterized by recurrent attacks,a long disease course,and an unfavorable *** is associated with an enduring therapeutic process,and finding a cure has been *** with epilepsy are predisposed to adverse moods,such as resistance,anxiety,nervousness,and anxiety,which compromise treatment compliance and overall *** To explored the influence of intensive psychological intervention on treatment compliance,psychological status,and quality of life(QOL)of patients with *** The clinical data of 105 patients with epilepsy admitted between December 2019 and July 2023 were retrospectively analyzed,including those of 50 patients who underwent routine intervention(control group)and 55 who underwent intensive psychological intervention(research group).Treatment compliance,psychological status based on the Self-Rating Anxiety Scale(SAS)and Depression Scale Self-Rating Depression Scale(SDS)scores,hope level assessed using the Herth Hope Scale(HHS),psychological resilience evaluated using the Psychological Resilience Scale,and QOL determined using the QOL in Epilepsy-31 Inventory(QOLIE-31)were comparatively *** Treatment compliance in the research group was 85.5%,which is significantly better than the 68.0%of the control *** notable intergroup differences in preinterventional SAS and SDS scores were identified(P>0.05);however,after the intervention,the SAS and SDS scores decreased significantly in the two groups,especially in the research group(P0.05).After 6 months of intervention,the research group showed evidently higher HHS,CD-RISC,tenacity,optimism,strength,and QOLIE-31 scores(P<0.05).CONCLUSION Intensive psychological intervention enhances treatment compliance,psychological status,and QOL of patients with epilepsy.

关键词： Intensive psychological intervention Epilepsy Treatment compliance Psychological status Quality of life

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Robust optimal dispatch strategy of integrated energy system considering CHP-P2G-CCS

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Global Energy Interconnection 2024年第1期7卷 14-24页

作者： Bin Zhang Yihui xia xiaotao Peng School of Electrical Engineering Naval University of EngineeringWuhan 430000P.R.China School of Electrical Engineering Wuhan UniversityWuhan 430072P.R.China

Integrated energy systems(IESs)can improve energy efficiency and reduce carbon emissions,essential for achieving peak carbon emissions and carbon *** study investigated the characteristics of the CHP model considering P2G and carbon capture systems,and a two-stage robust optimization model of the electricity-heat-gascold integrated energy system was ***,a CHP model considering the P2G and carbon capture system was established,and the electric-thermal coupling characteristics and P2G capacity constraints of the model were derived,which proved that the model could weaken the electric-thermal coupling characteristics,increase the electric power regulation range,and reduce carbon ***,a two-stage robust optimal scheduling model of an IES was constructed,in which the objective function in the day-ahead scheduling stage was to minimize the start-up and shutdown *** objective function in the real-time scheduling stage was to minimize the equipment operating costs,carbon emission costs,wind curtailment,and solar curtailment costs,considering multiple ***,after the objective function is linearized with a ψ-piecewise method,the model is solved based on the C&CG *** results show that the proposed model can effectively absorb renewable energy and reduce the total cost of the system.

关键词： Combined heat and power Power-to-gas Carbon capture system Integrated energy system Robust optimization

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Nuclei-rich galvanizing strategy for suppressing zinc dendrite growth

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Rare Metals 2024年第8期43卷 4016-4018页

作者： Hai-xia Wu Kai-Lu Guo College of Chemistry and Chemical Engineering Henan Key Laboratory of Function-Oriented Porous MaterialsLuoyang Normal UniversityLuoyang 471934China

The uncontrolled growth of zinc dendrites on zinc anode hinders the application of zinc ion *** solve this problem,Lu's group proposed a nuclei-rich galvanizing strategy for suppressing the zinc dendrite *** allows the nuclei-rich zinc electrode to cycle steadily for1200 h and have a high Coulombic efficiency of 99.7%at15 mA·cm^(-2)with a deposited amount of 10 mAh·cm^(-2).Moreover,the Zn-MnO_(2) battery with a low N/P ratio of 1.9exhibited sustained cycling life.

关键词： cycling sustained battery

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A modified smoothed particle hydrodynamics method considering residual stress for simulating failure and its application in layered rock mass

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Journal of Mountain Science 2024年第6期21卷 2091-2112页

作者： xia Chengzhi SHI Zhenming KOU Huanjia Department of Geotechnical Engineering College of Civil EngineeringTongji UniversityShanghai 200092China Key Laboratory of Geotechnical and Underground Engineering of Ministry of Education Tongji UniversityShanghai 200092China

Residual strength is an indispensable factor in evaluating rock fracture,yet the current Smoothed Particle Hydrodynamics(SPH)framework rarely considers its influence when simulating *** improved cracking strategy considering residual stress in the base bond SPH method was proposed to simulate failures in layered rocks and slopes and verified by experimental results and other simulation methods(i.e.,the discrete element method).Modified Mohr–Coulomb failure criterion was applied to distinguish the mixed failure of tensile and *** fracture markψwas introduced to improve the kernel function after tensile damage,and the calculation of residual stress after the damage was derived after shear *** simulations were carried out to evaluate its performance under different stress and scale conditions and to verify its effectiveness in realistically reproducing crack initiation and propagation and coalescence,even fracture and *** results indicate that the improved cracking strategy precisely captures the fracture and failure pattern in layered rocks and rock *** residual stress of brittle tock is correctly captured by the improved SPH *** improved SPH method that considers residual strength shows an approximately 13%improvement in accuracy for the safety factor of anti-dip layered slopes compared to the method that does not consider residual strength,as validated against analytical *** infer that the improved SPH method is effective and shows promise for applications to continuous and discontinuous rock masses.

关键词： Smoothed particle hydrodynamics Cracking strategy Residual stress Layered rock Crack propagation

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A Probing Model of Secret Key Generation Based on Channel Autocorrelation Function

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China Communications 2024年第6期21卷 163-175页

作者： xia Enjun Hu Binjie Shen Qiaoqiao School of Electronic and Information Engineering South China University of TechnologyGuangzhou 510641China

Secret key generation(SKG)is a promising solution to the problem of wireless communications *** the first step of SKG,channel probing affects it *** there have been some probing schemes,there is a lack of research on the optimization of the probing *** study investigates how to optimize correlated parameters to maximize the SKG rate(SKGR)in the time-division duplex(TDD)***,we build a probing model which includes the effects of transmitting power,the probing period,and the dimension of sample *** on the model,the analytical expression of the SKGR is ***,we formulate an optimization problem for maximizing the SKGR and give an algorithm to solve *** conclude the SKGR monotonically increases as the transmitting power *** mathematical proofs are given in this *** the simulation results,increasing appropriately the probing period and the dimension of the sample vector could increase the SKGR dramatically compared to a yardstick,which indicates the importance of optimizing the parameters related to the channel probing phase.

关键词： channel autocorrelation function channel probing optimization problem physical layer security secret key generation

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Recent advances in transition-metal catalyzed nitrene transfer reactions with carbamates

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Chinese Chemical Letters 2024年第3期35卷 76-86页

作者： Yanshu Luo Xinyu Zhang Yuanzhi xia College of Chemistry and Materials Engineering Wenzhou UniversityWenzhou 325035China

Nitrene transfer reactions are powerful tools in synthetic organic *** recent years,transitionmetal catalyzed nitrene transfer reactions with carbamates as the nitrene precursors have been widely *** species undergoes facile C-H amination,aziridination,and bifunctionalization of alkenes under the catalysis of different transition metals including Rh,Fe,Ru and others,enabling the efficient construction of various nitrogen-containing *** this review,the recent developments in nitrene transfer reactions with carbamates via N-O bond cleavage were introduced based on different types of reaction,and the key mechanistic information and synthetic applications of the methodologies were discussed.

关键词： Transition-metal catalysis Nitrene transfer Carbamate C—H amination Aziridination Bifunctionalization

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Prediction and scheduling of multi-energy microgrid based on BiGRU self-attention mechanism and LQPSO

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Global Energy Interconnection 2024年第3期7卷 347-361页

作者： Yuchen Duan Peng Li Jing xia School of Automation and Intelligence Beijing Jiaotong UniversityBeijing 100044P.R.China Goldwind Science&Technology Co.Ltd. Beijing 100176P.R.China

To predict renewable energy sources such as solar power in microgrids more accurately,a hybrid power prediction method is presented in this ***,the self-attention mechanism is introduced based on a bidirectional gated recurrent neural network(BiGRU)to explore the time-series characteristics of solar power output and consider the influence of different time nodes on the prediction ***,an improved quantum particle swarm optimization(QPSO)algorithm is proposed to optimize the hyperparameters of the combined prediction *** final proposed LQPSO-BiGRU-self-attention hybrid model can predict solar power more *** addition,considering the coordinated utilization of various energy sources such as electricity,hydrogen,and renewable energy,a multi-objective optimization model that considers both economic and environmental costs was constructed.A two-stage adaptive multi-objective quantum particle swarm optimization algorithm aided by a Lévy flight,named MO-LQPSO,was proposed for the comprehensive optimal scheduling of a multi-energy microgrid *** algorithm effectively balances the global and local search capabilities and enhances the solution of complex nonlinear *** effectiveness and superiority of the proposed scheme are verified through comparative simulations.

关键词： Microgrid Bidirectional gated recurrent unit Self-attention Lévy-quantum particle swarm optimization Multi-objective optimization

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