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Pressure drop analysis on the positive half-cell of a cerium redox flow battery using computational fluid dynamics: mathematical and modelling aspects of porous media

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Frontiers of Chemical Science and Engineering 2021年第2期15卷 399-409,F0004页

作者： Fernando F.Rivera Berenice Miranda-Alcantara german orozco Carlos Ponce de Leon Luis F.Arenas National Council of Science and Technology(CONACYT) Mexico City 03940Mexico Center of Research and Technological Development in Electrochemistry(CIDETEQ) Queretaro 76703Mexico Electrochemical Engineering Laboratory Energy Technology Research GroupFaculty of Engineering and Physical SciencesUniversity of SouthamptonSouthampton SO171BJUK

Description of electrolyte fluid dynamics in the electrode compartments by mathematical models can be a powerful tool in the development of redox flow batteries(RFBs)and other electrochemical *** order to determine their predictive capability,turbulent Reynolds-averaged Navier-Stokes(RANS)and free flow plus porous media(Brinkman)models were applied to compute local fluid velocities taking place in a rectangular channel electrochemical flow cell used as the positive half-cell of a cerium-based RFB for laboratory *** different platinized titanium electrodes were considered,a plate plus a turbulence promoter and an expanded metal *** pressure drop was validated against experimental data obtained with typical cerium *** was found that the pressure drop values were better described by the RANS approach,whereas the validity of Brinkman equations was strongly dependent on porosity and permeability values of the porous media.

关键词： CFD simulation porous media porous electrode pressure drop redox flow battery

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Comparison of Nine Membrane Pairs for Electrodialytic Removal of Nitrate Ions

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Journal of Water Resource and Protection 2011年第6期3卷 387-397页

作者： Lopez-Garcia Ulises Antano-Lopez Rene orozco german Torres-Gonzalez Julieta Castaneda Federico Centro de Investigacion y Desarrollo Tecnologico en electroquimica(CIDETEQ) Parque Tecnologico Queretaro-SanfandilaPedro EscobedoMexico

Electrodialysis (ED) of NaNO3 solutions was performed to stress the role of the membrane pair as a unit i.e. the behavior as a whole of Anion Exchange Membrane (AEM) and Cation Exchange Membrane (CEM), in the process at room temperature. The membrane pair was also tested in the reclamation of nitric acid and sodium hydroxide. It was found that the membrane pair ranking in Limiting Current Density does not agree with that of ions leakage and both rankings are not the same as for Current Efficiency or Specific Power Consumption, each parameter for a specific membrane pair depends on the associated membrane and at a lesser degree on the flow rate. Results show that one cannot select a membrane or a membrane pair only by its limiting current density i.e. it is necessary to evaluate several parameters of the process by characterizing the whole membrane pair and to decide the parameter of interest, i.e. denitrification speed, ions leakage, proton back migration, current efficiency or specific power consumption.

关键词： Electrodialysis Ion Exchange Membranes Nitrate Removal Nitric Acid Sodium Hy-droxide

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Comparison of Nine Membrane Pairs for Electrodialytic Removal of Nitrate Ions

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Journal of Water Resource and Protection（水资源与保护） 2011年第6期 387-397页

作者： López-García Ulises Anta？o-López René orozco german Torres-González Julieta Casta？eda Federico

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