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Revolutionizing plasmonic platform via magnetic field-assisted confined ultrafast laser deposition of high-density,uniform,and ultrafine nanoparticle arrays

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International journal of Extreme Manufacturing 2024年第3期6卷 428-438页

作者： jin Xu Lingfeng Wang Peilin Yang Haoqing jiang Huai Zheng Licong An Xingtao Liu gary j cheng School of Industrial Engineering Purdue UniversityWest LafayetteIN 47906United States of America Institute of Technological Sciences Wuhan UniversityWuhanHubei 430072People’s Republic of China

The remarkable capabilities of 2D plasmonic surfaces in controlling optical waves havegarnered significant ***,the challenge of large-scale manufacturing of uniform,well-aligned,and tunable plasmonic surfaces has hindered their *** address this,we present a groundbreaking tunable plasmonic platform design achieved throughmagnetic field(MF)assisted ultrafast laser direct deposition in *** precise control of metal nanoparticles(NPs),with cobalt(Co)serving as the model material,employing an MF,and fine-tuning ultrafast laser parameters,we have effectively converted coarse and non-uniform NPs into densely packed,uniform,and ultrafine NPs(~3 nm).This revolutionary advancement results in the creation of customizable plasmonic‘hot spots,’which play a pivotal role insurface-enhanced Raman spectroscopy(SERS)*** profound impact of this designable plasmonic platform lies in its close association with plasmonic resonance and *** the plasmonic nanostructures resonate with incident light,they generate intense local electromagnetic fields,thus vastly increasing the Raman scattering *** enhancement leads to an outstanding 2–18 fold boost in SERS performance and unparalleled sensing sensitivity down to 10^(-10)***,the plasmonic platform also demonstratesrobustness,retaining its sensing capability even after undergoing 50 cycles of rinsing andre-loading of ***,this work adheres to green manufacturing standards,making it an efficient and environmentally friendly method for customizing plasmonic‘hot spots’inSERS *** study not only achieves the formation of high-density,uniform,and ultrafine NP arrays on a tunable plasmonic platform but also showcases the profound relation betweenplasmonic resonance and energy *** outstanding results observed in SERS sensors further emphasize the immense potential of this technology for energy-relatedapplications,including photocatalysis,ph

关键词： magnetic field manipulation laser deposition metasurface SERS

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Leflunomide: A versatile additive for defect reduction, enhanced optoelectronic properties and environmental stability of perovskite films

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Nano Research 2024年第4期17卷 2628-2637页

作者： Dingyue Sun Ming Peng Taijin Wang Longju Yi Shizuo Zhang Feng Liu gary j.cheng The Institute of Technological Sciences Wuhan UniversityWuhan 430072China School of Power and Mechanical Engineering Wuhan UniversityWuhan 430072China School of Industrial Engineering Purdue UniversityWest LafayetteIN 47906USA

The development of perovskite photoelectric devices with excellent performance is largely dependent on the defects in the perovskite *** address this issue,a specific drug,leflunomide(LF,C_(12)H_(9)F_(3)N_(2)O_(2)),was incorporated into the perovskite to reduce defects and improve its photoelectric *** is believed that the C=O bond on LF molecule can interact with the uncoordinated Pb2+of the perovskite,thereby reducing non-radiative *** novel approach of incorporating LF into perovskite films has the potential to revolutionize the development of high-performance perovskite photoelectric *** trifluoromethyl functional(–CF_(3))group on LF can form a protective layer on the surface of the perovskite film,shielding it from water ***,LF can be utilized to alter the nucleation position of perovskite,thus minimizing the number of defects and optimizing the film ***,the LF-doped perovskite film displays low trap density and high photoelectric *** LF-doped perovskite film showed a trap density of 8.28×10^(11),which is notably lower than the 2.04×10^(12) of the perovskite film without *** responsivity and detectivity of the LF-doped perovskite photodetector were 0.771 A/W and 2.81×10^(11) jones,respectively,which are much higher than the 0.23 A/W and 1.06×10^(10) jones of the LF-undoped perovskite ***,the LF-doped photodetector maintained an initial photocurrent of 86%after 30 days of storage in air,indicating drastically increased environmental *** strongly suggests that LF is an effective additive for perovskites utilized in optoelectronic devices with high performance.

关键词： leflunomide additive engineering defect passivation perovskite

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Electronic properties of 2D materials and their junctions

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Nano Materials Science 2024年第1期6卷 1-23页

作者： Taposhree Dutta Neha Yadav Yongling Wu gary j.cheng Xiu Liang Seeram Ramakrishna Aoussaj Sbai Rajeev Gupta Aniruddha Mondal Zheng Hongyu Ashish Yadav Department of Chemistry Indian Institute of Engineering Science and TechnologyShibpurWest Bengal711103India Center for Advanced Laser Manufacturing(CALM) Shandong University of TechnologyZibo255000PR China School of Industrial Engineering Purdue University315 N.Grant St.West LafayetteIN47907United States Birck Nanotechnology Center Purdue University1205 W State St.West LafayetteIN47907United States Advanced Materials Institute Qilu University of TechnologyShandong Academy of SciencesJinan250014PR China Nanoscience and Nanotechnology Initiative National University of Singapore10 Kent Ridge Crescent119260Singapore Faculty of Applied Phsyics and Mathematics Gdansk University of Technology Narutowicza 11/1280233GdanskPoland Department of Physics School of EngineeringUniversity of Petroleum&Energy StudiesDehradun248007UttarakhandIndia Department of Physics National Institute of Technology DurgapurDurgapur713209West BengalIndia

With an extensive range of distinctive features at nano meter-scale thicknesses,two-dimensional(2D)materials drawn the attention of the scientific *** tremendous advancements in exploratory research on 2D materials,knowledge of 2D electrical transport and carrier dynamics still in its ***,here we highlighted the electrical characteristics of 2D materials with electronic band structure,electronic transport,dielectric constant,carriers *** atomic thinness of 2D materials makes substantially scaled field-effect transistors(FETs)with reduced short-channel effects conceivable,even though strong carrier mobility required for high performance,low-voltage device *** also discussed here about factors affecting 2D materials which easily enhanced the activity of those materials for various ***,Those 2D materials used in state-of-the-art electrical and optoelectronic devices because of the extensive nature of their electronic band structure.2D materials offer unprecedented freedom for the design of novel p-n junction device topologies in contrast to conventional bulk *** also,describe the numerous 2D p-n junctions,such as homo junction and hetero junction including mixed dimensional ***,we talked about the problems and potential for the future.

关键词： 2D materials Electrical properties p-n junctions Mixed hereto junctions Homo junctions Electrical transport

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Origins of Ultrafast Pulse Laser-Induced Nano Straight Lines with Potential Applications in Detecting Subsurface Defects in Silicon Carbide Wafers

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Nanomanufacturing and Metrology 2022年第2期5卷 167-178页

作者： Tan Shu Feng Liu Shuai Chen Xingtao Liu Chen Zhang gary j.cheng The Institute of Technological Sciences Wuhan UniversityWuhan430072People’s Republic of China School of Power and Mechanical Engineering Wuhan UniversityWuhan430072People’s Republic of China School of Industrial Engineering Purdue UniversityWest LafayetteIN47906USA

The inspection of silicon carbide(SiC)wafer quality has attracted considerable attention because internal microstructure defects are challenging to detect in production *** and destructive methods are usually employed to detect dislocations and stacking faults inside SiC *** optical methods to monitor internal defects are in *** this work,an ultrafast pulse laser was used to address this *** formation of surface nanostructures under the ultrafast laser processing of SiC wafers was explored *** study discovered the origins of a typical surface nanostructure to the subsurface dislocation structure,called low-energy laser-induced nano straight lines(LLINSs),which forms under low-energy ultrafast pulse laser irradiation on a SiC *** specific laser fluence ranges to form grooves,laser-induced periodic surface structures,LLINSs,and their hybrids were *** formation of LLINSs required an ultrafast laser(pulse width 280 fs)energy density less than 0.224 j/mm2,whereas that of pure LLINSs required a small range of 0.1–0.08 j/mm2 for *** and their surrounding microstructures were observed using scanning transmission electron microscopy to identify their origin,which is related to the subsurface dislocation *** dynamics analysis revealed that the subsurface defect area has a high energy level,which can facilitate amorphous transformation under the irradiation of an ultrafast laser,and the amorphous area had a tendency to evolve into ***,subsurface lattice defects can be detected *** work opens new ways to detect the subsurface quality of semiconductor wafers in a green and sustainable manner.

关键词： Ultrafast laser processing Surface nanostructure SiC wafer Dislocation Molecular dynamics

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MOF-Like 3D Graphene-Based Catalytic Membrane Fabricated by One-Step Laser Scribing for Robust Water Purification and Green Energy Production

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Nano-Micro Letters 2022年第11期14卷 48-61页

作者： Xinyu Huang Liheng Li Shuaifei Zhao Lei Tong Zheng Li Zhuiri Peng Runfeng Lin Li Zhou Chang Peng Kan-Hao Xue Lijuan Chen gary j.cheng Zhu Xiong Lei Ye School of Optical and Electronic Information and Wuhan National Laboratory for Optoelectronics Huazhong University of Science and TechnologyWuhan 430074People’s Republic of China Hubei Yangtze Memory Laboratories Wuhan 430205People’s Republic of China Institute for Frontier Materials Deakin UniversityGeelongVIC 3216Australia Key Laboratory of New Processing Technology for Nonferrous Metal and Materials(Ministry of Education) Guangxi Key Laboratory of Optical and Electronic Materials and DevicesCollege of Materials Science and EngineeringGuilin University of TechnologyGuilin 541004People’s Republic of China College of Chemistry and Materials Science Hunan Agricultural UniversityHunan 410128People’s Republic of China School of Material Science and Engineering Hunan University of Science and TechnologyXiangtanHunan ProvincePeople’s Republic of China School of Industrial Engineering and Birck Nanotechnology Centre Purdue UniversityWest LafayetteIN 47907USA Institute of Environmental Research at Greater Bay Key Laboratory for Water Quality and Conservation of the Pearl River DeltaMinistry of EducationGuangzhou UniversityGuangzhou 510006GuangdongPeople’s Republic of China

Increasing both clean water and green energy demands for survival and development are the grand challenges of our ***,we successfully fabricate a novel multifunctional 3D graphene-based catalytic membrane(3D-GCM)with active metal nanoparticles(AMNs)loading for simultaneously obtaining the water purification and clean energy generation,via a“green”one-step laser scribing *** as-prepared 3D-GCM shows high porosity and uniform distribution with AMNs,which exhibits high permeated fluxes(over 100 L m^(−2) h^(−1))and versatile super-adsorption capacities for the removal of tricky organic pollutants from wastewater under ultra-low pressure-driving(0.1 bar).After adsorption saturating,the AMNs in 3D-GCM actuates the advanced oxidization process to self-clean the fouled membrane via the catalysis,and restores the adsorption capacity well for the next time membrane *** importantly,the 3D-GCM with the welding of laser scribing overcomes the lateral shear force damaging during the long-term ***,the 3D-GCM could emit plentiful of hot electrons from AMNs under light irradiation,realizing the membrane catalytic hydrolysis reactions for hydrogen energy ***“green”precision manufacturing with laser scribing technology provides a feasible technology to fabricate high-efficient and robust 3D-GCM microreactor in the tricky wastewater purification and sustainable clean energy production as well.

关键词： 3D graphene Laser scribing Catalytic membrane Water purification Hydrogen production

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Laser-induced microjet-assisted ablation for high-quality microfabrication

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International journal of Extreme Manufacturing 2022年第3期4卷 122-130页

作者： Yang Guo Pei Qiu Shaolin Xu gary j cheng School of Mechatronics Engineering Harbin Institute of TechnologyHarbin 150001People’s Republic of China Department of Mechanical and Energy Engineering Southern University of Science and TechnologyShenzhen 518055People’s Republic of China School of Industrial Engineering Purdue UniversityWest LafayetteIN 47906United States of America

Liquid-assisted laser ablation has the advantage of relieving thermal effects of common laser ablation processes, whereas the light scattering and shielding effects by laser-induced cavitation bubbles, suspended debris, and turbulent liquid flow generally deteriorate laser beam transmission stability, leading to low energy efficiency and poor surface quality. Here, we report that a continuous and directional high-speed microjet will form in the laser ablation zone if laser-induced primary cavitation bubbles asymmetrically collapse sequentially near the air-liquid interface under a critical thin liquid layer. The laser-induced microjet can instantaneously and directionally remove secondary bubbles and ablation debris around the laser ablation region, and thus a very stable material removal process can be obtained. The shadowgraphs of high-speed camera reveal that the average speed of laser-induced continuous microjet can be as high as 1.1 m sin its initial 500 μm displacement. The coupling effect of laser ablation, mechanical impact along with the collapse of cavitation bubbles and flushing of high-speed microjet helps achieve a high material removal rate and significantly improved surface quality. We name this uncovered liquid-assisted laser ablation process as laser-induced microjet-assisted ablation(LIMjAA) based on its unique characteristics. High-quality microgrooves with a large depth-to-width ratio of 5.2 are obtained by LIMjAA with a single-pass laser scanning process in our experiments. LIMjAA is capable of machining various types of difficult-to-process materials with high-quality arrays of micro-channels, square and circle microscale through-holes. The results and disclosed mechanisms in our work provide a deep understanding of the role of laser-induced microjet in improving the processing quality of liquid-assisted laser micromachining.

关键词： liquid-assisted laser ablation laser-induced microjet cavitation bubbles laser microfabrication

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A review on microstructures and properties of high entropy alloys manufactured by selective laser melting

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International journal of Extreme Manufacturing 2020年第3期2卷 64-84页

作者： Chen Zhang junkai Zhu Huai Zheng Hui Li Sheng Liu gary j cheng The Institute of Technological Sciences Wuhan UniversityWuhan 430072People's Republic of China School of Power and Mechanical Engineering Wuhan UniversityWuhan 430072People's Republic of China School of Industrial Engineering Purdue UniversityWest LafayetteIN 47906United States of America

High entropy alloys(HEAs)with multi-component solid solution microstructures have the potential for large-scale industrial applications due to their excellent mechanical and functional ***,the mechanical properties of HEAs limit the selection of processing *** manufacturing technology possesses strong processing adaptability,making itthe best candidate method to overcome this *** comprehensive review examines the current state of selective laser melting(SLM)of *** SLM to HEAs processing is motivated by its high quality for dimensional accuracy,geometric complexity,surface roughness,and *** review focuses on analyzing the current developments and challenges in SLM of HEAs,including defects,microstructures,and properties,as well as strengthing prediction models of fabricated *** review also offers directions for future studies to address existing challenges and promote technological advancement.

关键词： high entropy alloys selective laser melting microstructure property strengthening model

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Isolated atomic catalysts encapsulated in MOF for ultrafast water pollutant treatment

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Nano Research 2021年第7期14卷 1287-1293页

作者： Shuailong Guo Hao Yuan Wei Luo Xiaoqing Liu Xiantao Zhang Haoqing jiang Feng Liu gary j.cheng The Institute of Technological Sciences Wuhan UniversityWuhan430072China Birck Nanotechnology Centre School of Industrial EngineeringPurdue UniversityWest LafayetteIN47906USA School of Power and Mechanical Engineering Wuhan UniversityWuhan430072China Center for materials research and analysis Wuhan University of TechnologyWuhan430072China

Atomic noble metals stand as one of the most advanced catalysts because of their unique properties and interaction with the ***,due to their high activity,noble atomic catalysts tend to aggregate and deactivate in practical ***,supports aimed to disperse these atomic catalysts often suffer from weak confinement and poor porosity,thus limited the catalytic efficiency of noble ***,we report the facile encapsulation of atomic noble catalyst in cheap cerous metal-organic framework(Ce-MOF)crystals to create a robust catalyst that could deliver high catalytic performance for the reduction of 4-nitrophenol without decay in long-term cycling ***,Au atoms encapsulated in Ce-MOF exhibited ultrahigh turnover frequency(TOF)of 131 min−1 for the reduction of 4-nitrophenol in minutes,consuming only 10%precious metals compared with state-of-the-art catalysts operated under same condition.

关键词： atomic catalysts metal-organic framework reduction of 4-nitrophenol porous

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New insights into nitric oxide biosynthesis underpin lateral root development

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Molecular Plant 2024年第5期17卷 691-693页

作者： Kapuganti jagadis Gupta Nidhi Yadav Aprajita Kumari gary j.Loake National Institute for Plant Genome Research Aruna Asaf Ali MargNew Delhi 110070India Institute of Molecular Plant Sciences School of Biological SciencesUniversity of EdinburghEH93BF EdinburghUK Centre for Engineering Biology School of Biological SciencesUniversity of EdinburghEH93BF EdinburghUK

In recent years,nitric oxide(NO)has emerged as a key redox signaling molecule in plants functioning in the regulation of key developmental programs and the orchestration of responses to a plethora of environmental cues(Kolbert et al.,2019).The predominant route for the transfer of NO bioactivity is through S-nitrosylation,the addition of an NO moiety to a protein cysteine thiol to form an S-nitrosothiol(Yun et al.,2011).Specificity for this process is established by the structural constraints imposed by tertiary protein structure in gating access to given cysteine redox switches and associated proteins that can either facilitate the addition or removal of the NO moiety at these residues(Umbreen et al.,2018).

关键词： moiety addition redox

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Parallel Nanoimprint Forming of One-Dimensional Chiral Semiconductor for Strain-Engineered Optical Properties

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Nano-Micro Letters 2020年第11期12卷 242-254页

作者： Yixiu Wang Shengyu jin Qingxiao Wang Min Wu Shukai Yao Peilin Liao Moon jKim gary jcheng Wenzhuo Wu School of Industrial Engineering Purdue UniversityWest LafayetteIN 47907USA Flex Laboratory Purdue UniversityWest LafayetteIN 47907USA Department of Materials Science and Engineering University of Texas at DallasRichardsonTX 75080USA School of Materials Engineering Purdue UniversityWest LafayetteIN 47907USA Birck Nanotechnology Center Purdue UniversityWest LafayetteIN 47907USA Regenstrief Center for Healthcare Engineering Purdue UniversityWest LafayetteIN 47907USA

The low-dimensional,highly anisotropic geometries,and superior mechanical properties of one-dimensional(1D) nanomaterials allow the exquisite strain engineering with a broad tunability inaccessible to bulk or thin-film *** capability enables unprecedented possibilities for probing intriguing physics and materials science in the 1-D *** the techniques for introducing controlled strains in 1D materials,nanoimprinting with embossed substrates attracts increased attention due to its capability to parallelly form nanomaterials into wrinkled structures with controlled periodicities,amplitudes,orientations at large scale with nanoscale ***,we systematically investigated the strain-engineered anisotropic optical properties in Te nanowires through introducing a controlled strain field using a resist-free thermally assisted nanoimprinting *** magnitude of induced strains can be tuned by adjusting the imprinting pressure,the nanowire diameter,and the patterns on the *** observed Raman spectra from the chiral-chain lattice of 1D Te reveal the strong lattice vibration response under the *** results suggest the potential of 1D Te as a promising candidate for flexible electronics,deformable optoelectronics,and wearable *** experimental platform can also enable the exquisite mechanical control in other nanomaterials using substrate-induced,on-demand,and controlled strains.

关键词： Chiral semiconductor Nanowires Nanoimprinting Strain engineering Optical property

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