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Chemical Research in Chinese Universities 2024年第1期40卷 47-54页

作者： XIANG Shuang guo yong LIU Xiaohui WANG Yanqin Key Laboratory for Advanced Materials and Joint International Research Laboratory of Precision Chemistry and Molecular Engineering Feringa Nobel Prize Scientist Joint Research CenterResearch Institute of Industrial CatalysisSchool of Chemistry and Molecular EngineeringEast China University of Science and TechnologyShanghai 200237P.R.China

The interface between Au and support has attracted extensive interest because of its unique catalytic ability for hydrogen activation in catalytic hydrogenation/hydrogenolysis ***,we create the Au-CoO-OV interface in the 1.0%Au/Co3O4-Rod-250 catalyst,which could dissociate H2 via the heterolytic way to yield rich hydride species and achieve excellent catalytic performance in the hydrogenolysis of biomass-derived 5-hydroxymethylfurfural(HMF)to 2,5-dimethylfuran(DMF).The XRD and HRTEM analyses show that Au nanoparticles are uniformly dispersed on CoO-OV surface and in situ DRIFTS spectra show the enhancement of heterolytic dissociation of hydrogen(signals of Au-D and O-D vibration)compared with bare CoO(Co3O4-Rod-250).This work provides insights for fabricating highly active Au-support catalysts for catalytic hydrogenation/hydrogenolysis reactions.

关键词： Au-CoO-OV interface Hydride species Heterolytic dissociation 5-Hydroxymethylfurfural(HMF) 2 5-Dimethylfuran(DMF)

Air purifier or fresh air system?A comparison of energy consumption and cost in urban China residential buildings

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Science China(Technological Sciences) 2024年第9期67卷 2637-2647页

作者： guo yong SUN ZhiWei WESCHLER Louise B ZHANG YinPing Department of Building Science Tsinghua UniversityBeijing 100084China Beijing Key Laboratory of Indoor Air Quality Evaluation and Control Beijing 100084China Independent Researcher Colts Neck 07722NJUSA

Chinese urban residential buildings face serious indoor air quality *** purification systems(e.g.,air purifiers,fresh air systems)that supply fresh air or purify indoor air are widely used in residential buildings to improve indoor air *** the challenges of energy conservation and emission reduction,it is urgent to guide residents on choosing appropriate air purification *** key problem is how to identify the best air purification system with the lowest energy consumption or operating *** of air purification systems have rarely been conducted on the premise that they should deliver air such that the main indoor pollutant concentrations all meet air quality *** ignored in comparisons are the increased filtration resistance caused by dust accumulation on the filter and the cost of filter *** this study,we propose a method to compare residential air purification systems based on energy consumption and total cost,and we provide methods to select air purification systems in China's different climatic *** used a standard two-person bedroom as the example,and determined the most suitable(minimum cost or energy consumption)air purification systems for the capital cities of the provinces in Chinese mainland.

关键词： IAQ fresh air system air purifier energy consumption cost

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Mechanical Modeling and Analysis of Stability Deterioration of Production Well During Marine Hydrate Depressurization Production

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China Ocean Engineering 2024年第2期38卷 338-351页

作者： SUN Huan-zhao CHANG Yuan-jiang SUN Bao-jiang WANG Kang CHEN guo-ming LI Hao DAI yong-guo Centre for Offshore Engineering and Safety Technology China University of Petroleum(East China)Qingdao 266580China School of Petroleum Engineering China University of Petroleum(East China)Qingdao 266580China Jiangsu Shuguang Oil Tools Co. LtdTaizhou 225532China

Different from oil and gas production,hydrate reservoirs are shallow and unconsolidated,whose mechanical properties deteriorate with hydrate ***,the formations will undergo significant subsidence during depressurization,which will destroy the original force state of the production ***,existing research on the stability of oil and gas production wells assumes the formation to be stable,and lacks consideration of the force exerted on the hydrate production well by formation subsidence caused by hydrate decomposition during *** fill this gap,this paper proposes an analytical method for the dynamic evolution of the stability of hydrate production well considering the effects of hydrate *** on the mechanical model of the production well,the basis for stability analysis has been proposed.A multi-field coupling model of the force state of the production well considering the effect of hydrate decomposition and formation subsidence is established,and a solver is *** analytical approach is verified by its good agreement with the results from the numerical method.A case study found that the decomposition of hydrate will increase the pulling-down force and reduce the supporting force,which is the main reason for the stability *** higher the initial hydrate saturation,the larger the reservoir thickness,and the lower the production pressure,the worse the stability or even *** work can provide a theoretical reference for the stability maintaining of the production well.

关键词： natural gas hydrate production well depressurization production formation deformation stability deterioration

N-doping offering higher photodegradation performance of dissolved black carbon for organic pollutants: experimental and theoretical studies

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Journal of Zhejiang University-Science A(Applied Physics & Engineering) 2024年第4期25卷 340-356页

作者： yong guo Mengxia CHEN Ting CHEN Ying guo Zixuan XU guowei XU Soukthakhane SINSONESACK Keophoungeun KANMANY Key Laboratory of Integrated Regulation and Resource Development on Shallow Lakes Ministry of EducationCollege of EnvironmentHohai UniversityNanjing 210093China Key Laboratory of Environmental Engineering of Jiangsu Province Jiangsu Provincial Academy of Environmental ScienceNanjing 210036China State Key Laboratory of Pollution Control and Resource Reuse Nanjing UniversityNanjing 210023China Central Environmental Laboratory Natural Resources and Environment Research InstituteMinistry of Natural Resources and EnvironmentVientiane 999012Laos

We investigated the influence mechanism of N-doping for dissolved black carbon(DBC)photodegradation of organic *** degradation performance of N-doped dissolved black carbon(NDBC)for tetracycline(TC)(71%)is better than that for methylene blue(MB)(28%)under *** levels are both better than DBC degradation performances for TC(68%)and MB(18%)under *** species quenching experiments suggest that h and-O,are the main reactive species for NDBC photodegraded TC,while-OH and h*are the main reactive species for NDBC photodegraded MB.-OH is not observed during DBC photodegradation of *** is likely because N-doping increases valence-band(VB)energy from 1.55 eV in DBC to 2.04 eV in NDBC;the latter is strong enough to oxidize water to ***,N-doping increases the DBC band gap of 2.29 to 2.62 eV in NDBC,resulting in a higher separation efficiency of photo-generated electrons-holes in NDBC than in *** these factors give NDBC stronger photodegradation performance for TC and MB than ***-performance liquid chromatography-mass spectrometry(HPLC-MS)characterization and toxicity evaluation with the quantitative structure-activity relationship(QSAR)method suggest that TC photodegradation intermediates produced by NDBC have less aromatic structure and are less toxic than those produced by *** adopted a theoretical approach to clarify the relationship between the surface groups of NDBC and the photoactive species *** results add to the understanding of the photochemical behavior of NDBC.

关键词： Dissolved black carbon(DBC) N-doping Organic pollutants Band gap Photodegradation

Collision-avoidance strategy for a spinning electrodynamic tether system

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Astrodynamics 2024年第2期8卷 247-259页

作者： Linxiao Li Aijun Li Hongshi Lu Changqing Wang Yuriy Mikhailovich Zabolotnov yong guo School of Automation Northwestern Polytechnical UniversityXi’an 710129China Institute of IT and Cybernatics Samara National Research UniversitySamara 443086Russia

Spinning electrodynamic tether systems(SEDTs)have promising potential for the active removal of space debris,the construction of observation platforms,and the formation of artificial ***,owing to the survivability problem of long tethers,designing collision-avoidance strategies for SEDTs with space debris is an urgent *** study focuses on the design of collision-avoidance strategies for SEDTs with an electrodynamic force(Ampere force).The relative distance between the debris and the SEDT is first derived,and then two collision-avoidance strategies are proposed according to the two different *** debris collides closer to a lighter subsatellite,a stationary avoidance strategy is proposed to change the spatial position of the subsatellite by adjusting only the angular motion of the tether,which maintains the original orbit of the *** debris collides closer to a heavier main spacecraft,a comprehensive avoidance strategy is proposed to change the spatial position of the SEDT by slightly modifying the orbital height and changing the tether angular motion *** numerical results illustrate that the proposed strategies promptly avoid potential collisions of an SEDT with space debris without significant changes in the orbital parameters of the SEDT.

关键词： spinning electrodynamic tether systems(SEDTs) collision analysis collision avoidance

Upcycling of polyphenylene oxide into 2,6-dimethyl aniline via depolymerization and amination over a Pt/CeOcatalyst

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Science China Chemistry 2024年

作者： Shengchao Jia Wenke Zhao Xiaohui Liu yong guo Yanqin Wang State Key Laboratory of Green Chemical Engineering and Industrial Catalysis Research Institute of Industrial Catalysis School of Chemistry and Molecular Engineering East China University of Science and Technology Shanghai Key Laboratory of Functional Materials Chemistry School of Chemistry and Molecular Engineering East China University of Science and Technology

Upcycling of plastic waste into N-containing compound is a novel and attractive strategy for its disposal and will opens up a promising direction for the production of value-added ***,an efficient strategy for the depolymerization-amination of polyphenylene oxide （PPO） into 2,6-dimethyl aniline is developed over a simple Pt/*** C–O linkages of PPO can be selectively broken,producing 2,6-dimethyl phenol and then hydrogenated and aminated to 2,6-dimethyl cyclohexylamine over the Pt/***,2,6-dimethyl aniline was produced with high selectivity through the dehydrogenation of 2,6-dimethyl cyclohexylamine in the same *** can be used as the hydrogen-acceptor in the dehydrogenation step and enhance the selectivity of target *** N-containing compound,2,6-dimethyl aniline,is obtained and separated after HCl ***,the Pt/CeO2catalyst exhibit remarkable stability and can sustainably catalyze the synthesis of 2,6-dimethyl aniline in several cycles.

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Optimal Scheduling Strategy of Source-Load-Storage Based onWind Power Absorption Benefit

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Energy Engineering 2024年第7期121卷 1823-1846页

作者： Jie Ma Pengcheng Yue Haozheng Yu Yuqing Zhang Youwen Zhang Cuiping Li Junhui Li Wenwen Qin yong guo State Grid Henan Economic Research Institute Zhengzhou450000China Zaozhuang Power Supply Company State Grid Shandong Electric Power CompanyZaozhuang277000China Key Laboratory of Modern Power SystemSimulation and Control&Renewable Energy Technology Ministry of EducationNortheast Electric Power UniversityJilin132012China

In recent years,the proportion of installed wind power in the three north regions where wind power bases are concentrated is increasing,but the peak regulation capacity of the power grid in the three north regions of China is limited,resulting in insufficient local wind power consumption ***,this paper proposes a two-layer optimal scheduling strategy based on wind power consumption benefits to improve the power grid’s wind power consumption *** objective of the uppermodel is tominimize the peak-valley difference of the systemload,which ismainly to optimize the system load by using the demand response resources,and to reduce the peak-valley difference of the system load to improve the peak load regulation capacity of the *** lower scheduling model is aimed at maximizing the system operation benefit,and the scheduling model is selected based on the rolling *** load-side schedulingmodel needs to reallocate the absorbed wind power according to the response speed,absorption benefit,and curtailment penalty cost of the two DR dispatching ***,the measured data of a power grid are simulated by MATLAB,and the results show that:the proposed strategy can improve the power grid’s wind power consumption capacity and get a large wind power consumption benefit.

关键词： Wind power consumption two-layer optimal demand response rolling scheduling wind curtailment penalty

从同文馆到北京大学:近代中国“Peking University”概念考论

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教育学报 2024年第4期20卷 195-207页

作者：宋雪山东大学文学院济南250100

从晚清到民国,“Peking University”的指称对象先后包括京师同文馆、汇文书院、京师大学堂、私立燕京大学和国立北京大学五所驻京高等教育机构,其中既有国立最高学府,也有私立教会学校。虽然部分属于非正式名称,但仍具有广泛社会影响... 详细信息

从晚清到民国,“Peking University”的指称对象先后包括京师同文馆、汇文书院、京师大学堂、私立燕京大学和国立北京大学五所驻京高等教育机构,其中既有国立最高学府,也有私立教会学校。虽然部分属于非正式名称,但仍具有广泛社会影响。语言概念的重叠带来话语表达中的歧义,同时也投射出多元复杂的历史图景。依据档案、报刊、辞书、回忆录等材料,返回历史现场,梳理近代中国“Peking University”概念的生成和流变,从中考察新式教育的引入、中西观念的互动及文化空间的形成,有助于探求译名背后的知识建构、教育转型与社会变迁。

关键词： Peking University 同文馆京师大学堂北京大学燕京大学概念史教育转型

具有环状运动约束的悬臂输流管道的非线性振动特征

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动力学与控制学报 2024年第5期22卷 24-37页

作者：郭勇安顺学院电子与信息工程学院安顺561000

本文对具有环状运动约束的悬臂输流管道的空间弯曲振动进行研究,目的在于考察约束刚度系数、约束放置位置对管道的两类周期运动(包括平面周期运动和空间周期运动)及其稳定性的影响规律.首先,在已有文献的基础上,将运动约束对管道的作用... 详细信息

本文对具有环状运动约束的悬臂输流管道的空间弯曲振动进行研究,目的在于考察约束刚度系数、约束放置位置对管道的两类周期运动(包括平面周期运动和空间周期运动)及其稳定性的影响规律.首先,在已有文献的基础上,将运动约束对管道的作用模拟成非线性立方弹簧模,得出振动方程.其次,运用Galerkin方法将振动方程离散成常微分方程组,结合基于中心流形—范式理论的投影法与平均法,给出了决定系统定性动力学性质的相关系数(包括临界特征值随流速的变化率及非线性共振项),取模态截断数为6,在几组约束刚度值和约束位置处计算了上述系数,据此考察了运动约束对管道的周期运动的影响,总结出了如下结论:在约束位置取定时增加约束刚度,或在约束刚度取定时增大约束位置至管的固定端的距离,均会使得管道的稳定平面周期运动对应的质量比区间减小,稳定空间周期运动对应的质量比区间增大;约束位置距管的固定端越远,约束刚度的变化对管道动力学行为的影响越明显.最后,对上述通过投影法和平均法得出的结论,本文在特定的质量比处数值求解了原振动方程的6模态Galerkin离散化方程,绘制了位形图、相图和Poincaré映射图,计算了频率,从而验证了相关的分析.

关键词：输流管道平面周期运动空间周期运动约束弹簧稳定

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抗战时期大学教授的坚守与执着——《郑天挺西南联大日记》阅读札记

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教育学报 2024年第1期20卷 197-208页

作者：李玉伟北京师范大学历史学院北京100875

阅读《郑天挺西南联大日记》,能够详细了解郑天挺在西南联大时的教学、科研、人事、行政、社交等情况。从《郑天挺西南联大日记》入手,结合相关基本史料可看出,西南联大时期的郑天挺以教学为本,对学校人才培养工作贡献巨大,深受学生认... 详细信息

阅读《郑天挺西南联大日记》,能够详细了解郑天挺在西南联大时的教学、科研、人事、行政、社交等情况。从《郑天挺西南联大日记》入手,结合相关基本史料可看出,西南联大时期的郑天挺以教学为本,对学校人才培养工作贡献巨大,深受学生认可与爱戴;他潜心于读书治学,借史学以经世,所著《清史探微》一书奠定了其在史学界的地位;就任西南联大总务长一职虽非其本意,但他最终选择牺牲小我、顾全大局,任职期间任劳任怨,堪称“联大舵手”。西南联大时期郑天挺的读书治学、为人处世,反映了他潜心育人,为学校发展而克己奉公,从中亦可揭示抗战时期中国学者的不屈精神。

关键词：郑天挺西南联大《郑天挺西南联大日记》抗日战争