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Frontiers in Energy 2024年第4期18卷 418-435页

作者： feng gong Yuhang JING Rui XIAO Key Laboratory of Energy Thermal Conversion and Process Measurement and Control of the Ministry of Education School of Energy and EnvironmentSoutheast UniversityNanjing 210096China

Ammonia,with its high hydrogen storage density of 17.7 wt.%(mass fraction),cleanliness,efficiency,and renewability,presents itself as a promising zero-carbon ***,the traditional Haber−Bosch(H−B)process for ammonia synthesis necessitates high temperature and pressure,resulting in over 420 million tons of carbon dioxide emissions annually,and relies on fossil fuel *** contrast,dielectric barrier discharge(DBD)plasma-assisted ammonia synthesis operates at low temperatures and atmospheric pressures,utilizing nitrogen and hydrogen radicals excited by energetic electrons,offering a potential alternative to the H−B *** method can be effectively coupled with renewable energy sources(such as solar and wind)for environmentally friendly,distributed,and efficient ammonia *** review delves into a comprehensive analysis of the low-temperature DBD plasma-assisted ammonia synthesis technology at atmospheric pressure,covering the reaction pathway,mechanism,and catalyst system involved in plasma nitrogen *** from current research,it evaluates the economic feasibility of the DBD plasmaassisted ammonia synthesis technology,analyzes existing dilemmas and challenges,and provides insights and recommendations for the future of nonthermal plasma ammonia processes.

关键词： plasma catalysis nitrogen fixation ammonia synthesis hydrogen storage catalyst carbon neutralization

Occurrence of dark septate endophytes in Phragmites australis in the Baiyang Lake and their resistance to Cd stress

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Pedosphere 2024年第2期34卷 484-496页

作者： Minghui XU Xia LI Qiannan YE feng gong Xueli HE School of Life Sciences Hebei UniversityBaoding 071002China Key Laboratory of Microbial Diversity Research and Application of Hebei Province Hebei UniversityBaoding 071002China

Heavy metal pollution poses a serious hazard to human health,and microbial remediation of heavy metals in soil has been widely studied.A group of ascomycetes classified as dark septate endophytes(DSEs)colonize plant roots and benefit host plants under abiotic stress *** this study,Phragmites australis,a common remediation plant in the Baiyang Lake in North China,was *** and roots of *** were collected in typical heavy metal-contaminated sites,and the species diversity and community structure of DSEs in *** roots were *** addition,DSE strains were isolated,cultured,and tested for their tolerance to Cd *** results showed that DSEs occurred extensively in *** roots,forming typical dark septate hyphae,with a total colonization rate of 19.7%–83.1%.Morphological and internal transcribed spacer sequencing analyses were used to identify 10 species within 9 genera of DSE *** these fungi,6 strains with considerable resistance to Cd stress were *** biomasses of Poaceascoma helicoides,Alternaria doliconidium,and Acrocalymma vagum strains increased as the Cd levels *** results can not only help to understand plant-DSE interactions in wetland environments,but also provide a theoretical basis for making full use of DSE fungi to alleviate heavy metal contamination in soil.

关键词： ascomycete colonization rate contaminated site evenness index heavy metal Shannon-Wiener index Simpson index wetland

A fibrous hydroelectric generator derived from eco-friendly sodium alginate for low-grade energy harvesting

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Frontiers in Energy 2024年第4期18卷 474-482页

作者： feng gong Jiaming SONG Haotian CHEN Hao LI Runnan HUANG Yuhang JING Peng YANG Junjie feng Rui XIAO Key Laboratory of Energy Thermal Conversion and Control of the Ministry of Education School of Energy and EnvironmentSoutheast UniversityNanjing 210096China

With the development of renewable energy technologies,the recovery and utilization of low-grade energy based on hydroelectric effect have drawn much attention owing to its environmental ***,a novel hydroelectric generator utilizing sodium alginategraphene oxide(SA-GO)fibers is proposed,which is ecofriendly and *** fibers with a length of 5 cm and a diameter of 0.15 mm can generate an open circuit voltage(Voc)of approximately 0.25 V and a short circuit current(Isc)of 4µ*** connecting SA-GO fibers in either series or parallel,this combination can power some electronic ***,these fibers enable the recovery of low-grade energy from the atmosphere or around the human *** experimental and theoretical analysis confirm that the directional flow of protons driven by water molecules is the main mechanism for power generation of SA-GO *** study not only presents a simple energy transformation method that is expected to be applied to our daily life,but also provides a novel idea for the design of humidity electricity-generation devices.

关键词： fibrous hydroelectric generator sodium alginate(SA) graphene oxide(GO) power generation

Fe-doped Co_(3)O_(4) nanowire strutted 3D pinewood-derived carbon: A highly selective electrocatalyst for ammonia production via nitrate reduction

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Nano Research 2024年第4期17卷 2276-2282页

作者： Xuwei Liu Chaozhen Liu Xun He Zhengwei Cai Kai Dong Jun Li Xiaoya Fan Ting Xie Xiya Yang Yonglan Luo Dongdong Zheng Shengjun Sun Sulaiman Alfaifi feng gong Xuping Sun Institute of Fundamental and Frontier Sciences University of Electronic Science and Technology of ChinaChengdu 610054China Key Laboratory of Energy Thermal Conversion and Control of Ministry of Education School of Energy and EnvironmentSoutheast UniversityNanjing 211189China College of Chemistry Chemical Engineering and Materials ScienceShandong Normal UniversityJinan 250014China Chemistry Department Frontier of ScienceKing Abdulaziz UniversityJeddah 21589Saudi Arabia

Nitrate(NO_(3)^(-)),a nitrogen-containing pollutant,is prevalent in aqueous solutions,contributing to a range of environmental and health-related *** electrocatalytic reduction of NO_(3)^(-)holds promise as a sustainable approach to both eliminating NO_(3)^(-)and generating valuable ammonia(NH_(3)).Nevertheless,the reduction reaction of NO_(3)^(-)(NO_(3)^(-)RR),involving 8-electron transfer process,is intricate,necessitating highly efficient electrocatalysts to facilitate the conversion of NO_(3)^(-)to NH_(3).In this study,Fe-doped Co_(3)O_(4) nanowire strutted three-dimensional(3D)pinewood-derived carbon(Fe-Co_(3)O_(4)/PC)is proposed as a high-efficiency NO_(3)^(-)RR electrocatalyst for NH_(3) *** within 0.1 M NaOH containing NO_(3)^(-),Fe-Co_(3)O_(4)/PC demonstrates exceptional performance,obtain an impressively large NH_(3) yield of 0.55 mmol·h^(-1)·cm^(-2) and an exceptionally high Faradaic efficiency of 96.5%at-0.5 V,superior to its Co_(3)O_(4)/PC counterpart(0.2 mmol·h^(-1)·cm^(-2),73.3%).Furthermore,the study delves into the reaction mechanism of Fe-Co_(3)O_(4) for NO_(3)^(-)RR through theoretical calculations.

关键词： Fe-doped Co_(3)O_(4) nanowire pinewood-derived carbon electrocatalytic NO_(3)-reduction NH_(3) synthesis density functional theory

Flotation separation of brucite and calcite in dodecylamine system enhanced by regulator potassium dihydrogen phosphate

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Transactions of Nonferrous Metals Society of China 2024年第8期34卷 2658-2670页

作者： Xiu-feng gong Jin YAO Bin YANG Wan-zhong YIN Yu-lian WANG Ya-feng FU School of Resources and Civil Engineering Northeastern UniversityShenyang 110819China School of Chemical Engineering China University of Mining and TechnologyXuzhou 221163China School of Materials Science and Engineering Shenyang Ligong UniversityShenyang 110159China Ansteel Beijing Research Institute Co. Ltd.Beijing 102200China

To achieve efficient flotation separation of brucite and calcite,flotation separation experiments were conducted on two minerals using dodecylamine(DDA)as the collector and potassium dihydrogen phosphate(PDP)as the *** action mechanism of DDA and PDP was explored through contact angle measurement,zeta potential detection,solution chemistry calculation,FTIR analysis,and XPS *** flotation results showed that when DDA dosage was 35 mg/L and PDP dosage was 40 mg/L,the maximum floating difference between brucite and calcite was 79.81%,and the selectivity separation index was *** detection analysis showed that the main dissolved component HPO_(4)^(2−)of PDP is selectively strongly adsorbed on the Ca site on the surface of calcite,promoting the adsorption of the main dissolved component RNH_(3)^(+)of DDA on calcite surface,while brucite is basically not affected by ***,PDP is an effective regulator for the reverse flotation separation of brucite and calcite in DDA system.

关键词： brucite calcite selective adsorption flotation separation

Shewanella oneidensis MR-1对地下水低渗透区中Cr(Ⅵ)和硝酸盐的协同异化还原

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中国环境科学 2024年第5期44卷 2473-2482页

作者：贡玉凤上海市环境科学研究院国家环境保护城市土壤污染控制与修复工程技术中心上海200233 同济大学环境科学与工程学院污染控制与资源化国家重点实验室上海200092

Cr(Ⅵ)和硝酸盐是地下水中常见的复合污染物,且有可能通过迁移扩散至低渗透区而导致其修复问题被忽视.利用Shewanella oneidensis MR-1作为功能微生物,分别研究了摇瓶和非均质模拟装置中两种污染物的协同异化还原过程.结果表明:摇瓶实验... 详细信息

Cr(Ⅵ)和硝酸盐是地下水中常见的复合污染物,且有可能通过迁移扩散至低渗透区而导致其修复问题被忽视.利用Shewanella oneidensis MR-1作为功能微生物,分别研究了摇瓶和非均质模拟装置中两种污染物的协同异化还原过程.结果表明:摇瓶实验中,Cr (Ⅵ)的去除主要依赖于初始菌浓度,而受硝酸盐浓度、电子供体乳酸盐浓度的影响较小.反之,硝酸盐的还原则明显受到Cr (Ⅵ)的抑制,当Cr(Ⅵ)浓度在0到0.02mmol/L时,其一级动力学还原速率从0.635h^(-1)降至0.164h^(-1).同时,乳酸盐氧化也明显受到Cr(Ⅵ)的抑制,表明Shewanella oneidensis MR-1的代谢过程可能受到了Cr(Ⅵ)的毒性干扰.在非均相装置实验中,Cr(Ⅵ)进水浓度小于等于5mg/L(约0.1mmol/L)时,15d基本可以完全去除,对应硝酸盐去除60%左右;当Cr(Ⅵ)浓度增至10mg/L (约0.2mmol/L)时,Cr(Ⅵ)和硝酸盐的去除率分别降至40%和50%左右.装置内截留的Cr(Ⅵ)还原产物以Cr(OH)_3为主,硝酸盐的还原产物以氨为主.

关键词： Shewanella oneidensis MR-1 六价铬硝酸盐

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融合机器视觉的桥梁动态称重方法

吉林大学学报（工学版） 2024年第1期54卷 188-197页

作者：龙关旭张修石辛公锋王涛杨干山东高速集团有限公司创新研究院济南250101 长安大学公路学院西安710064 山东省高速公路技术和安全评估重点实验室济南250101

为了进一步提升现有的桥梁动态称重技术,提出了一种融合机器视觉的桥梁动态称重系统。首先,利用机器视觉算法对车辆进行识别和追踪;其次,对车辆作用下的桥梁响应监测信息进行处理;然后,利用虚拟简支梁理论对轴重、轴距进行识别;最后,通... 详细信息

为了进一步提升现有的桥梁动态称重技术,提出了一种融合机器视觉的桥梁动态称重系统。首先,利用机器视觉算法对车辆进行识别和追踪;其次,对车辆作用下的桥梁响应监测信息进行处理;然后,利用虚拟简支梁理论对轴重、轴距进行识别;最后,通过模拟分析和室内试验的方式对本文方法的准确性进行检验。结果表明:本文方法在多种工况下,对车辆的轴重、轴距都具有较好的识别效果;轴重、轴距、总重识别平均相对误差分别为3.40%、4.31%和2.71%,并且具有一定的抗噪能力。

关键词：桥梁工程桥梁动态称重机器视觉虚拟简支梁

超高性能混凝土单轴拉、压循环作用下力学性能及其本构模型研究

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工程力学 2024年第4期41卷 81-93页

作者：赵继之辛公锋陶慕轩崔文涛清华大学土木工程系土木工程安全与耐久教育部重点实验室北京100084 山东高速集团有限公司创新研究院山东济南250000 山东高速基础设施建设有限公司山东济南250000

超高性能混凝土(ultra-high performance concretre,UHPC)是一种新型材料,具有抗拉、抗压强度高、开裂后应变硬化等特点,在装配式结构领域具有较为广阔的应用前景。为了明确UHPC在单轴循环荷载下的受力性能并提出适合的本构关系,通过大... 详细信息

超高性能混凝土(ultra-high performance concretre,UHPC)是一种新型材料,具有抗拉、抗压强度高、开裂后应变硬化等特点,在装配式结构领域具有较为广阔的应用前景。为了明确UHPC在单轴循环荷载下的受力性能并提出适合的本构关系,通过大量的试验建立循环荷载下UHPC的本构模型,设计具有不同钢纤维掺量的棱柱体和狗骨直拉试件,开展不同加载制度的单轴压缩试验,分析试验结果以明确钢纤维掺量、养护方式和加载制度对UHPC单轴拉压力学性能的影响情况。试验结果表明,在受压方面,钢纤维体积含量为2%的UHPC峰值压应变明显高于钢纤维体积含量为1%和3%的UHPC峰值压应变。各UHPC试件的弹性模量明显大于普通混凝土的弹性模量。在受拉方面,UHPC呈现出一定的应变硬化现象,且达到峰值后拉应力下降较为缓慢,展现出一定的受拉延性。钢纤维体积含量和蒸养处理对UHPC试件的抗拉强度有明显的提高作用。最后,在试验数据的基础上,提出了UHPC受压和受拉的骨架曲线和滞回准则,并拟合了卸载(再加载)的计算公式,可用于有限元计算中UHPC的基本本构方程。

关键词：本构模型循环荷载拉伸试验压缩试验超高性能混凝土

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金属的应变率效应及其动态本构研究进展

机械工程学报 2024年第2期60卷 81-98页

作者：徐腾邓春阳冉家琪龚峰唐恒深圳大学机电与控制工程学院深圳518060 深圳大学深圳市高性能特种制造重点实验室深圳518060

绝大多数金属均存在复杂的应变率效应,屈服强度和流变应力在不同应变速率下的值不同,不同应变速率范围内应力变化趋势也会不同,表现为应变率强化效应和应变率弱化效应。应变速率影响着金属材料的宏观力学性能以及内部微观组织结构,不同... 详细信息

绝大多数金属均存在复杂的应变率效应,屈服强度和流变应力在不同应变速率下的值不同,不同应变速率范围内应力变化趋势也会不同,表现为应变率强化效应和应变率弱化效应。应变速率影响着金属材料的宏观力学性能以及内部微观组织结构,不同变形速度下的金属材料塑性变形行为存在明显差异。在板材高速拉深等高速冷成形过程中,材料局部应变速率的提升将导致该区域内塑性变形功转化为热量造成瞬时温升,局部的高温高压使材料的拉深成形性能和表面质量受到不同程度的影响。在金属板材高速成形领域,建立考虑应变率效应以及绝热温升效应影响的动态本构模型是准确获取材料力学行为响应、实现形性一体化高精密成形的重要前提。综述金属应变率效应以及应变速率对金属塑性变形行为的影响,并对金属动态力学行为和动态本构模型研究进展进行了总结,着重对唯象本构、物理本构、人工神经网络本构这三类模型的研究工作,以及流变应力的应变率效应进行了论述和分析,最后就金属应变率效应研究和构建金属高速成形动态本构关系研究工作中的不足进行了总结讨论,为开展金属高速成形动态本构相关的研究工作给出了一定的建议和展望。

关键词：应变率效应高速成形绝热温升动态力学行为动态本构模型

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复杂环境深大基坑支护结构有限元分析

工程技术研究 2024年第10期9卷 29-31页

作者：龚峰中铁十一局集团第四工程有限公司湖北武汉430074

文章以某深基坑为研究对象,采用大型有限元软件对基坑开挖、支护方案及施工进行了较为深入的研究。研究结果表明,该基坑支护结构有效地约束了坑底隆起,基坑外侧表面土体沉降呈凹陷型分布且沉降量均在预警值以下;桩身变形呈弓形分布特征... 详细信息

文章以某深基坑为研究对象,采用大型有限元软件对基坑开挖、支护方案及施工进行了较为深入的研究。研究结果表明,该基坑支护结构有效地约束了坑底隆起,基坑外侧表面土体沉降呈凹陷型分布且沉降量均在预警值以下;桩身变形呈弓形分布特征,且随着开挖深度的增加,最大变形量不断下移。模拟结果可为同类基坑工程提供施工经验。

关键词：基坑开挖基坑支护数值模拟有限元分析