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Nanozyme catalysis in a crowded environment:The impact of diffusion and surface shielding

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Nano Research 2024年第7期17卷 5795-5800页

作者： Vasily g.Panferov Juewen liu Department of Chemistry Waterloo Institute for NanotechnologyWaterlooOntario N2L 3G1Canada

Nanozymes are widely used in various applications as nanosized catalysts for replacing *** accurate estimation of the catalytic activity of nanozymes in real conditions is *** this article,for the first time,we systematically studied the effect of macromolecular molecules co-existing in the real system on the oxidoreductase(peroxidase,oxidase,and catalase)-mimicking nanozymes made of a gold nanoparticle core and a platinum shell,Prussian Blue,Mn_(2)O_(3) and CoO *** were made with horseradish *** distinguished two main mechanisms of the negative impact of macromolecules on nanozyme catalysis—slowed diffusion and surface shielding of *** the first mechanism is typical for enzymes,the second one is specific only for *** the mechanisms is essential for developing.a.proaches to reduce the unavoidable impact of macromolecules for various analytical and biomedical applications.

关键词： molecular crowding biosensors nanoparticles

Frequency Regulation of VSC-MTDC System with Offshore Wind Farms

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Journal of Modern Power Systems and Clean Energy 2024年第1期12卷 275-286页

作者： Haoyu liu Chongru liu North China Electric Power University Beijing 102206China

Frequency regulation of voltage source converter-based multi-terminal high-voltage direct current(VSC-MTDC)system with offshore wind farms enhances the frequency stability by compensating the power for a disturbed AC ***,it is difficult to reasonably allocate frequency-regulation resources due to a lack of coordination mechanisms between wind farms and the MTDC ***,it is difficult for the frequency control of the wind farms to manage changes in wind speed;and the risk of wind-turbine stalls is ***,based on the kinetic energy of wind turbines and the power margin of the converters,the frequency-regulation capability of wind turbines is evaluated,and a dynamic frequency-support scheme considering the real-time frequency-support capability of the wind turbines and system frequency evolution is proposed to improve the frequency-support performance.A power adaptation technique at variable wind speeds is developed;the active power in the frequency-support stage and restoration stage is switched according to the wind speed.A hierarchical zoning frequency-regulation scheme is designed to use the frequency-regulation resources of different links in the MTDC system with wind *** simulation results show that the novel frequency-regulation strategy maintains frequency stability with wind-speed changes and avoids multiple frequency dips.

关键词： Wind generation voltage source converter-based multi-terminal high-voltage direct current(VSC-MTDC) frequency regulation cooperative control adaptive control variable wind speed

Artificial-intelligent-powered safety and efficiency improvement for controlling.a.d scheduling in integ.a.ed railway systems

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High-speed Railway 2024年第3期2卷 172-179页

作者： liu J. liu g. Wang Y. Zhang W. Beijing National Railway Research & Design Institute of Sig.a. & Communication group Co. Ltd Beijing 100070 China Engineering Research Center of Railway Industry of Intelligent and Autonomous Train Control Beijing 100070 China

The multi-mode integ.a.ed railway system, anchored by the high-speed railway, caters to the diverse travel requirements both within and between cities, offering safe, comfortable, punctual, and eco-friendly transportation services. With the expansion of the railway networks, enhancing the efficiency and safety of the comprehensive system has become a crucial issue in the advanced development of railway transportation. In light of the prevailing.a.plication of artificial intelligence technologies within railway systems, this study leverages large model technology characterized by robust learning capabilities, efficient associative abilities, and linkage analysis to propose an Artificial-intelligent (AI)-powered railway control and dispatching system. This system is elaborately designed with four core functions, including global optimum unattended dispatching, synergetic transportation in multiple modes, high-speed automatic control, and precise maintenance decision and execution. The deployment pathway and essential tasks of the system are further delineated, alongside the challenges and obstacles encountered. The AI-powered system promises a significant enhancement in the operational efficiency and safety of the composite railway system, ensuring.a.more effective alignment between transportation services and passenger demands. © 2024 Beijing Jiaotong University

关键词： Artificial intelligence High-speed railway Large-scale mode, system framework Multi-mode railway system Safety and efficiency improvement

A Novel Design of a Pre-separation Panel Structure to Protect Against the Impact of an Explosion in an Aircraft Plenum Chamber

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Acta Mechanica Solida Sinica 2024年第1期37卷 166-180页

作者： Zongxing liu Xiang Yang Jun liu School of Aeronautics Northwestern Polytechnical UniversityXi'an 710072China COMAC Shang.a. Aircraft Design and Research Institute Shanghai 201210China

To reduce the damage of the pressurizing panel structure of a fuselage caused by an explosion at the“least risk bomb location”in an aircraft structure,a new pre-separation panel structure was designed to resist blast ***,the dynamic strain response and morphology of impact damage of the new pre-separation panel were measured in an impact damage ***,the commercial software LS-DYNA was used to calculate the propagation of the blast shock wave,and the results were compared with empirical equations to verify the rationality of the numerical calculation ***,the fluid–structure coupling method was used to calculate the damage process of the pre-separation panel structure under the impact of an explosion wave and an impact *** calculated results were in good agreement with the test results,which showed the rationality of the calculation method and the *** residual strength of the damaged pre-separation panel was significantly higher than that of the original damaged *** results show that the new pre-separation panel structure is reasonable and has certain significance for guiding the design of plenum chambers with strong resistance to implosion for aircraft fuselages.

关键词： Pre-separation panel structure Explosive response Residual strength Aircraft plenum chamber Least risk bomb location

Effectiveness and safety of acupuncture in treatment of preg.a.cyrelated symptoms:a systematic review and Meta-analysis

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Journal of Traditional Chinese Medicine 2024年第1期44卷 16-26页

作者： liu Tingting liu Tongou liu Mingfu School of Traditional Chinese Medicine Clinical Medicine Hubei University of Traditional Chinese MedicineWuhan 430000China First Clinical College of Hubei University of Traditional Chinese Medicine Wuhan 430000China Department of Acupuncture and Tuina Affiliated Hospital of Hubei University of Traditional Chinese MedicineHubei Provincial Hospital of Traditional Chinese MedicineWuhan 430000China

OBJECTIVE:To systematically evaluate the efficacy and safety of acupuncture(AM)in the treatment of preg.a.cyrelated symptoms such as acute vomiting during ***:We comprehensively searched the available literature up to November 2021,including Pub Med,Embase,Cochrane Library,Chinese Biomedical Literature Database,and China National Knowledge Infrastructure Database,for randomized controlled trials(RCTs)on AM for the treatment of severe vomiting,insomnia,pharyng.a. and pelvic pain,mood abnormalities,and dyspepsia during ***:Sixteen RCTs with a cumulative sample size of 1178 cases were *** these,964 patients were included in the *** Meta-analysis results showed that AM was more efficient than Western medicine in treating discomfort during preg.a.cy[odds ratio(OR)=1.19,95%confidence interval(CI)(1.11,1.28),Pgroup in improving the visual analog scale scores[standard mean difference(SMD)=0.62,95%CI(0.53,0.71),Pgroup in improving Numerical Rating Scale(NRS)symptom scores[OR=7.31,95%CI(3.36,15.94),Pgnificant difference in adverse effects between the AM and sham-AM groups and the analgesic drug group[OR=0.70,95%CI(0.39,1.28),P=0.25],but the treatment and control groups had mild adverse effects with a low ***:AM is more effective than other treatments or pharmacotherapy alone in the treatment of preg.a.cy-related symptoms,and is relatively ***,the quality of the included trials was rather poor,and high-quality studies are required to confirm our findings.

关键词： acupuncture preg.a.cy nausea vomiting sleep initiation and maintenance disorders low back pain pelvic pain mood abnormalities Meta-analysis systematic review

Stochastic Unit Commitment with High-Penetration Offshore Wind Power generation in Typhoon Scenarios

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Journal of Modern Power Systems and Clean Energy 2024年第2期12卷 535-546页

作者： Yanqi liu Dundun liu Hong.a. Zhang State Key Laboratory of Internet of Things for Smart City and Department of Electrical and Computer Engineering University of MacaoMacao 999078China University of Macao Zhuhai UM Science and Technology Research Institute ZhuhaiChina

To tackle the energy crisis and climate change,wind farms are being heavily invested in across the *** China's coastal areas,there are abundant wind resources and numerous offshore wind farms are being *** secure operation of these wind farms may suffer from typhoons,and researchers have studied power system operation and resilience enhancement in typhoon ***,the intricate movement of a typhoon makes it challenging to evaluate its spatial-temporal *** published papers only consider predefined typhoon trajectories neglecting *** address this challenge,this study proposes a stochastic unit commitment model that incorporates high-penetration offshore wind power generation in typhoon *** adopts a data-driven method to describe the uncertainties of typhoon trajectories and considers the realistic anti-typhoon mode in offshore wind farms.A two-stage stochastic unit commitment model is designed to enhance power system resilience in typhoon *** formulate the model into a mixed-integer linear prog.a.ming problem and then solve it based on the computationally-efficient progressive hedging.a.gorithm(PHA).Finally,numerical experiments validate the effectiveness of the proposed method.

关键词： Unit commitment two-stage stochastic prog.a.ming offshore wind farm typhoon

Devolatilization of high viscous fluids with high g.a.ity technology

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Chinese Journal of Chemical Engineering 2024年第7期71卷 249-257页

作者： Jibing Qi Youzhi liu Yandong liu Taiyuan University Taiyuan 030032China Shanxi Province Key Laboratory of Higee-Oriented Chemical Engineering North University of ChinaTaiyuan 030051China

Volatile organic compounds(VOCs)are generally toxic and harmful substances that can cause health and environmental *** removal of VOCs from polymers has become a key *** effective devolatilization to remove VOCs from high viscous fluids such as polymer is necessary and is of great *** this study,the devolatilization effect of a rotating packed bed(RPB)was studied by using polydimethylsiloxane as the viscous fluid and acetone as the *** devolatilization rate and liquid phase volume(KLa)have been *** results indicated that the optimum conditions were the high-g.a.ity factor of 60,liquid flow rate of 10 L·h^(-1),and vacuum degree of 0.077 *** dimensionless correlation of KLa was established,and the deviations between predicted and experimental values were less than±28%.The high-g.a.ity technology will result in lower mass transfer resistance in the devolatilization process,enhance the mass transfer process of acetone,and improve the removal effect of *** work provides a promising path for the removal of volatiles from polymers in combination with high-g.a.ity *** can provide the basis for the application of RPB in viscous fluids.

关键词： High-g.a.ity technology Devolatilization rate High viscous fluid Volatile organic compounds(VOCs)

Polar solvent induced in-situ self-assembly and oxygen vacancies on Bi_(2)MoO_(6)for enhanced photocatalytic deg.a.ation of tetracycline

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Nano Research 2024年第6期17卷 4951-4960页

作者： Fang.a. liu Dongyue Su Weizhen liu Baiquan liu Chuan liu Hong Wang Mengye Wang State Key Laboratory of Optoelectronic Materials and Technologies Guangdong Province Key Laboratory of Display Material and TechnologySchool of Electronics and Information TechnologySun Yat-Sen UniversityGuangzhou 510275China School of Materials Sun Yat-Sen UniversityShenzhen 518107China School of Environment and Energy Guangdong Provincial Key Laboratory of Solid Wastes Pollution Control and RecyclingSouth China University of TechnologyGuangzhou 510006China

It has been proved to be an effective route to efficiently ameliorate photocatalytic performance of catalysts via designing three-dimensional(3D)hierarchical nanostructures and constructing oxygen vacancies(VOs).However,controlling the self-assembly of organization into 3D hierarchical nanostructures while introducing VOs in photocatalysts remains a ***,we reported an ethylene glycol(Eg)mediated approach to craft 3D hydrang.a.structure Bi_(2)MoO_(6)with VOs for efficient photocatalytic deg.a.ation of *** manipulating the Eg concentration during the fabrication process,the influence of Eg concentration on the Bi_(2)MoO_(6)structure was systematically *** could promote the self-assembly of Bi_(2)MoO_(6)nanosheets to form a 3D hierarchical *** with 2D nanoplates,3D hierarchical architecture enhanced the surface area and the amount of active sites of Bi_(2)MoO_(6).In addition,the reduction effect of Eg on metallic oxide enabled the generation of VOs in Bi_(2)MoO_(6).The VOs adjusted the electronic structure of Bi_(2)MoO_(6),which not only enhanced the light harvesting,but also facilitated the simultaneous utilization of photo-induced electrons and holes to form reactive oxygen species(·O2−and·OH)for the efficient tetracycline decomposition.3D Bi_(2)MoO_(6)hydrang.a.with VOs achieved a 79.4%removal efficiency of tetracycline after 75 *** work provides a simple yet robust Eg-mediated strategy,which not only promotes the self-assembly of nano-catalysts into 3D hierarchical architectures,but also crafts tunable VOs for highly efficient photocatalysis.

关键词： three-dimensional(3D)hierarchical nanostructures tunable oxygen vacancies ethylene glycol(Eg)-mediated strategy bismuth molybdate photocatalytic deg.a.ation tetracycline

Thermal-hydraulic performance analysis and multi-objective optimization of a microchannel with staggered semi-elliptical ribs

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Science China Technological Sciences 2024年第10期67卷 3152-3167页

作者： CUI Pan liu Wei liu ZhiChun School of Energy and Power Engineering Huazhong University of Science and Technology

To enhance the cooling capacity of traditional microchannels for high heat flux electronic devices,a microchannel design with staggered semi-elliptical ribs is proposed in this *** numerical simulations,the flow characteristics of the designed microchannel are compared with those of a smooth one,and the effects of rib width（Wr）,rib height（Hr）,and rib length（Lr）,on the thermal-hydraulic performance are investigated under laminar flow *** results show that the periodically arranged ribs induce periodic vortices within the microchannel,effectively promoting fluid mixing.a.d enhancing heat *** Hrhave similar effects on microchannel performance,with an increase in them leading to an enhanced thermal performance at the expense of deteriorated hydraulic ***,Lrhas a comparatively weaker influence,with both the heat transfer and flow resistance initially growing with increasing Lrand then *** strike a balance between the two performances,a multi-objective optimization on the three geometrical parameters is conducted at a Reynolds number（Re） *** with simulation data,artificial neural networks are trained as surrogate models,and a multi-objective genetic algorithm is employed to derive the Pareto *** the TOPSIS decision-making method,an optimal compromise solution is determined as Wr=0.2415 mm,Hr=0.0976 mm,and Lr=0.6486 *** testing on the optimized microchannel reveals that it exhibits high heat transfer,middle flow resistance,and excellent overall performance,with the performance evaluation criterion（PEC） falling between 1.572 and 1.723 within the Re range of 220–660.

关键词： heat transfer enhancement microchannel semi-elliptical rib numerical simulation multi-objective optimization

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