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Rational modulation of fluorophosphate cathode by anionic groups to reduce the polarization behavior for fast-charging sodium-ion batteries

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Journal of Energy Chemistry 2025年第1期100卷 509-521页

作者： Xinyuan Wang Fan Zhang Xingyu Zhou Qian Wang Changyu liu Yangyang liu hui Wang Xiaojie liu Key Laboratory of Synthetic and Natural functional Molecule of the Ministry of Education College of Chemistry & Materials Science Northwest University

Na3V2（PO4）2O2F （VP） is recognized as a promising cathode material for sodium-ion batteries due to its stable structural framework and high specific *** functional theory （DFT） and finite element simulations show that incorporating SO42-into VP decreases its band gap,lowers the migration energy barrier,and ensures a uniform Na+concentration gradient and stress distribution during charge and discharge ***,the average Na+diffusion coefficient of Na3V2（PO4）1.95（SO4）0.05O2F（VPS-1） is roughly double that of VP,leading to enhanced rate capability (80 C,75.5 mAh g-1) and cycling stability (111.0 mAh g-1capacity after 1000 cycles at 10 C current density) for ***-1 exhibits outstanding fast-charging capabilities,achieving an 80%state of charge in just 8.1 *** assembled VPS-1//SbSn/NPC full cell demonstrated stable cycling over 200 cycles at a high 5 C current,maintaining an average coulombic efficiency of 95.35%.

关键词： Anionic group modulation Polarization behavior Fast-charging Sodium-ion battery Fluorophosphate Cathode

Pancreatic stent improves the success rate of needle-knife papillotomy in patients with difficult biliary cannulation

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World Journal of Gastroenterology 2025年第1期31卷 58-67页

作者： Mu-Hsien Lee Cheng-hui Lin Chi-Huan Wu Yung-Kuan Tsou Kai-Feng Sung Sheng-fu Wang Nai-Jen liu Department of Gastroenterology and Hepatology Chang Gung Memorial Hospital and Chang Gung University College of MedicineTaoyuan 33305Taiwan School of Medicine Chang Gung UniversityTaoyuan 33305Taiwan

BACKGROUND Needle-knife precut papillotomy(NKP)is typically performed ***,it remains unclear whether pancreatic stent(PS)placement can improve the outcomes of *** To explore whether PS placement improves the success rate of NKP in patients with difficult biliary *** This single-center retrospective study included 190 patients who underwent NKP between January 2017 and December 2021 after failed conventional biliary *** cases with incidental pancreatic duct cannulation during conventional biliary cannulation,the decision for pre-NKP PS placement was made at the endoscopist's *** primary outcome was the difference in the NKP success rate between patients with and without PS placement;the secondary outcome was the adverse event *** Among the 190 participants,82 received pre-NKP PS(PS-NKP group)whereas 108 did not[freehand or freehand NKP(FH-NKP)group].Post-NKP selective biliary cannulation was successful in 167(87.9%)patients,and the PS-NKP had a significantly higher success rate than the FH-NKP group(93.9%vs 83.3%,P=0.027).The overall adverse event rates were 7.3%and 11.1%in the PS-NKP and FH-NKP groups,respectively(P=0.493).A periampullary diverticulum(PAD)and significant intraoperative bleeding during NKP were independently associated with NKP failure;however,a pre-NKP PS was the only predictor of NKP *** the 44 participants with PADs,the PS-NKP group had a non-significantly higher NKP success rate than the FH-NKP group(87.5%and 65%,respectively;P=0.076).CONCLUSION PS significantly improved the success rate of NKP in patients with difficult biliary cannulation.

关键词： Difficult biliary cannulation Endoscopic retrograde cholangiopancreatography Needle-knife papillotomy Pancreatic stent Selective biliary cannulation

我国按疾病诊断相关分组预付费改革进展及建议

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中国卫生政策研究 2017年第9期10卷 32-38页

作者：胡广宇刘婕付婷辉刘远立北京协和医学院公共卫生学院北京100730 中国中医科学院西苑医院北京100091 首都医科大学附属北京妇产医院北京100020

按疾病诊断相关分组预付费是国际上应用较成熟的一种住院患者医保费用支付方式,2017年我国将选择部分地区开展按疾病诊断相关分组预付费试点。本文从省、市、县层面,对国内按疾病诊断相关分组预付费改革典型地区进行个案分析,总结改革... 详细信息

按疾病诊断相关分组预付费是国际上应用较成熟的一种住院患者医保费用支付方式,2017年我国将选择部分地区开展按疾病诊断相关分组预付费试点。本文从省、市、县层面,对国内按疾病诊断相关分组预付费改革典型地区进行个案分析,总结改革方案设计的特点,比较政策实施的差异,讨论改革的经验和启示。在分析当前改革进展和问题的基础上,提出推进我国按疾病诊断相关分组预付费改革的相关建议。

关键词：医疗改革疾病诊断相关分组预付费制度试点项目

Unraveling brain aging through the lens of oral microbiota

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Neural Regeneration Research 2025年第7期20卷 1930-1943页

作者： Qinchao Hu Si Wang Weiqi Zhang Jing Qu Guang-hui liu State Key Laboratory of Membrane Biology Institute of ZoologyChinese Academy of SciencesBeijingChina Hospital of Stomatology Guanghua School of StomatologyGuangdong Provincial Key Laboratory of StomatologySun Yat-sen UniversityGuangzhouGuangdong ProvinceChina Advanced Innovation Center for Human Brain Protection and National Clinical Research Center for Geriatric Disorders Xuanwu HospitalCapital Medical UniversityBeijingChina Aging Translational Medicine Center International Center for Aging and CancerBeijing Municipal Geriatric Medical Research CenterXuanwu HospitalCapital Medical UniversityBeijingChina CAS Key Laboratory of Genomic and Precision Medicine Beijing Institute of GenomicsChinese Academy of Sciences and China National Center for BioinformationBeijingChina University of Chinese Academy of Sciences BeijingChina Institute for Stem Cell and Regeneration Chinese Academy of SciencesBeijingChina Aging Biomarker Consortium BeijingChina State Key Laboratory of Stem Cell and Reproductive Biology Institute of ZoologyChinese Academy of SciencesBeijingChina Beijing Institute for Stem Cell and Regenerative Medicine BeijingChina

The oral cavity is a complex physiological community encompassing a wide range of *** of oral microbiota can lead to various oral infectious diseases,such as periodontitis and tooth decay,and even affect systemic health,including brain aging and neurodegenerative *** studies have highlighted how oral microbes might be involved in brain aging and neurodegeneration,indicating potential avenues for intervention *** this review,we summarize clinical evidence demonstrating a link between oral microbes/oral infectious diseases and brain aging/neurodegenerative diseases,and dissect potential mechanisms by which oral microbes contribute to brain aging and *** also highlight advances in therapeutic development grounded in the realm of oral microbes,with the goal of advancing brain health and promoting healthy aging.

关键词： Alzheimer's disease brain aging multiple sclerosis neurodegeneration neurodegenerative diseases oral microbiota Parkinson's disease periodontitis bacteria Porphyromonas gingivalis

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基于全相位谱分析的剪切光束成像目标重构

物理学报 2017年第2期66卷 141-146页

作者：陈明徕罗秀娟张羽兰富洋刘辉曹蓓夏爱利中国科学院西安光学精密机械研究所西安710119

剪切光束成像技术是一种非传统散斑成像技术,能透过扰动介质对远距离目标进行高分辨率成像.本文提出了一种基于全相位谱分析的图像重构算法,利用全相位谱分析对回波信号数据进行预处理,可有效抑制频谱泄露,校正散斑频谱,消除多种因素引... 详细信息

剪切光束成像技术是一种非传统散斑成像技术,能透过扰动介质对远距离目标进行高分辨率成像.本文提出了一种基于全相位谱分析的图像重构算法,利用全相位谱分析对回波信号数据进行预处理,可有效抑制频谱泄露,校正散斑频谱,消除多种因素引起的频率漂移误差,得到准确的散斑强度和相位差,提高实际成像环境的系统成像能力.仿真结果表明:该图像重构算法有效抑制了频率漂移对成像质量的影响,当信号存在频率误差时,其成像效果大大优于基于传统傅里叶变换谱分析的重构算法.

关键词：剪切光束成像散斑全相位谱分析目标重构

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我国行政审判中调解制度的改革与完善

现代法学 2002年第5期24卷 34-37页

作者：朱福惠刘伟光厦门大学福建厦门361005

我国行政审判中的调解制度不仅在立法上存在矛盾 ,而且在法律适用上也有冲突。因此 ,本文从调解适用范围、适用原则以及调解模式等四个方面出发 ,提出了改革和完善我国行政审判中的调解制度之设想。

关键词：中国行政审判调整制度行政赔偿诉讼案件国家赔偿法

Real-world evidence on the efficacy and safety of vonoprazanamoxicillin dual therapy for Helicobacter pylori treatment in elderly patients

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World Journal of Gastroenterology 2025年第1期31卷 68-78页

作者： Wen Gao Jing-Wen Li hui Ye Xue-Zhi Zhang Jian-Xiang liu Hong Cheng Department of Gastroenterology Peking University First HospitalBeijing 100034China School of Medicine Tsinghua MedicineTsinghua UniversityBeijing 100034China Department of Traditional Chinese Medicine and Integrative Medicine Peking University First HospitalBeijing 100034China

BACKGROUND A dual therapy regimen containing amoxicillin is a common treatment option for the eradication of Helicobacter pylori(***).While substantial research supports the efficacy and safety of vonoprazan and amoxicillin(VA)dual therapy in the general population,there is still a lack of studies specifically focusing on its safety in elderly *** To evaluate efficacy and safety of VA dual therapy as first-line or rescue treatment for *** in elderly *** As a real-world retrospective study,data were collected from elderly patients aged 60 years and above who accepted VA dual therapy(vonoprazan 20 mg twice daily+amoxicillin 1000 mg thrice daily for 14 days)for *** eradication in the Department of Gastroenterology at Peking University First Hospital between June 2020 and January *** status was evaluated by^(13)C-urease breath test 6 weeks after *** adverse events(AEs)during treatment were *** In total,401 cases were ***-one cases were excluded due to loss to follow-up,lack of re-examination,or unwillingness to take *** total of 380 included cases comprised 250 who received VA dual therapy as first-line treatment and 130 who received VA dual therapy as rescue *** was successfully eradicated in 239 cases(95.6%)in the first-line treatment group and 116 cases(89.2%)in the rescue treatment *** overall incidence of AEs was 9.5%for both ***,9.2%of patients experienced an AE in the first-line treatment group and 10.0%in the rescue treatment *** patients discontinued treatment due to AE,with a discontinuation rate of 1.3%.No serious AE *** The VA dual therapy regimen as a first-line treatment and a rescue therapy was effective and safe for elderly patients aged 60 and older.

关键词： Helicobacter pylori Vonoprazan Amoxicillin Dual therapy Elderly

Synthesis and glycosidase inhibitory activity ofandrographolide cyclophosphate detrivatives

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Synthesis and glycosidase inhibitory activity ofandrographol...

Continuous high-temperature rapid nanomanufacturing of electrocatalysts

第七届全国磷化学化工暨第四届海峡化学生物学、生物技术与医药发展讨论会

作者： XU Hai-Wei, liu Gai-Zhi, DAI Gui-fu, Li hui-Na, liu Hong-Min (New Drug Research & Development Center Zhengzhou University Zhengzhou 450052) (Department of Chemistry Zhengzhou University Zhengzhou 450052)

Andrographolide (1) is one of the major labdane diterpenoidal constituents of Andrographis paniculate (Burm) Nees, which is widely used in Traditional Chinese and Indian Medicine. It has been reported to exhibit a wide spectrum of biological activities The results reported here were that a series of cyclophosphate andrographolide derivatives were synthesised from andrographolide. The activity results showed that compounds 2,5,6 were selective inhibitors of α-

关键词： Synthesis and glycosidase inhibitory activity ofandrographolide cyclophosphate detrivatives

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Nano Research 2025年第1期18卷 225-235页

作者： Xiaoyang Wang Ziyi Luo Baihua Cui Ziqi fu Yanchang liu Weidi liu Jia Ding Jianrong Zeng Yanan ChenWenbin Hu School of Materials Science and Engineering Tianjin UniversityTianjin 300350China Australian Institute for Bioengineering and Nanotechnology The University of QueenslandSt.LuciaBrisbane 4072Australia Shanghai Synchrotron Radiation Facility Shanghai Advanced Research InstituteChinese Academy of SciencesShanghai 201204China Shanghai Institute of Applied Physics Chinese Academy of SciencesShanghai 201800China

Encapsulating metal nanoparticles in carbon shells(Metal@C)to enhance catalytic activity and stability has been certified ***,most existing methods for preparing Metal@C are complex,time-consuming,and lack of *** this study,a novel method that couples the high-temperature shock(HTS)with ultrasonic spray pyrolysis is reported,which can realize facile and scalable production of various Metal@C through the pyrolysis of glucose and metal chloride *** proposed HTS ultrasonic spray pyrolysis offers several advantages,including compact size,short reaction time(~120 ms),and uniform *** the Ni@C-40 nanocomposite as an example,the ultrasmall Ni nanoparticles(~10 nm)with thin carbon protective shells(~2 nm)are uniformly dispersed in the carbon matrix and applied for oxygen evolution reaction(OER)in alkaline *** Ni@C-40 optimized by tuning the thickness of carbon shell exhibits significantly enhanced OER activity with low overpotential of 242 mV at 10 mA·cm^(-2) and stability,which is attributed to the optimized interactions between Ni nanoparticles and carbon *** method also shows promise for continuous pyrolysis synthesis of various extreme materials at ultra-high temperatures using alternative electric heating materials.

关键词： ultrasonic spray pyrolysis high-temperature shock carbon shell oxygen evolution reaction Metal@C nanocomposite