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Mechanism investigation of A-site doping on modulating electronic band structure and photocatalytic performance towards CO_(2) reduction of LaFeO_(3) perovskite

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Nano Research 2024年第5期17卷 3733-3744页

作者： Chi cao Jinshuo Li yang Hu Lin Zhang Wensheng yang State Key Laboratory of Inorganic Synthesis and Preparative Chemistry College of ChemistryJilin UniversityChangchun 130012China Engineering Research Center for Nanomaterials Henan UniversityKaifeng 475004China

Three kinds of metal atoms with different valence electronic configurations,Bi(6s^(2)6p^(3)),Y(4d^(1)5s^(2)),and Ce(4f^(1)5d^(1)6s^(2)),were selected to investigate the effect of A-site(La^(3+))doping on electronic band structure,photoelectric properties,and photocatalytic performance of LaFeO_(3) *** was identified that the Bi doped LaFeO_(3) presented significantly improved photocatalytic activity towards the reduction of CO_(2),while the Y or Ce doped LaFeO_(3) displayed decreased photocatalytic activity compared to the pristine LaFeO_(3).It was revealed that doping of all the three metal atoms resulted in narrowed band gap and thus extended light absorption of LaFeO_(3) by lowering its conduction band minimum(CBM).The recombination rate and mobility of the charge carriers were represented by the relative effective mass(D)between holes and electrons for pristine and A-site doped LaFeO_(3).The doping of Bi resulted in increased D value,attributed to the Bi 6s electron states at the valence band maximum(VBM),and thus promoted separation and transfer of the charge carriers and improved photocatalytic activity of LaFeO_(3).In contrast,the doping of Ce resulted in significantly decreased D value,induced by the highly localized Ce 4f hole states at the CBM,and thus higher recombination rate of the charge carriers and decreased photocatalytic activity of LaFeO_(3).furthermore,the Y doped LaFeO_(3) with a slightly decreased D value presented slightly increased recombination rate of the charge carriers and thus decreased photocatalytic *** a work provides new insights into the A-site doping in LaFeO_(3) perovskite,which should be helpful for optimizing the electronic band structure and activity of perovskite-type photocatalysts at atomic level.

关键词： A-site doping electronic band structure charge carrier behavior photocatalytic CO_(2)reduction perovskite-type photocatalytsts

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Estimation of Hammerstein nonlinear systems with noises using filtering and recursive approaches for industrial control

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Frontiers of Information Technology & Electronic Engineering 2024年第2期25卷 260-271页

作者： Mingguang ZHANG Feng LI yang YU Qingfeng cao School of Electrical&Information Engineering Jiangsu University of TechnologyChangzhou213001China College of Electrical Energy and Power EngineeringYangzhou UniversityYangzhou225127China

This paper discusses a strategy for estimating Hammerstein nonlinear systems in the presence of measurement noises for industrial control by applying filtering and recursive *** proposed Hammerstein nonlinear systems are made up of a neural fuzzy network(NFN)and a linear state`-space *** estimation of parameters for Hammerstein systems can be achieved by employing hybrid signals,which consist of step signals and random ***,based on the characteristic that step signals do not excite static nonlinear systems,that is,the intermediate variable of the Hammerstein system is a step signal with different amplitudes from the input,the unknown intermediate variables can be replaced by inputs,solving the problem of unmeasurable intermediate variable *** the presence of step signals,the parameters of the state-space model are estimated using the recursive extended least squares(RELS)***,to effectively deal with the interference of measurement noises,a data filtering technique is introduced,and the filtering-based RELS is formulated for estimating the NFN by employing random ***,according to the structure of the Hammerstein system,the control system is designed by eliminating the nonlinear block so that the generated system is approximately equivalent to a linear system,and it can then be easily controlled by applying a linear *** effectiveness and feasibility of the developed identification and control strategy are demonstrated using two industrial simulation cases.

关键词： Hammerstein nonlinear systems Neural fuzzy network Data filtering Hybrid signals Industrial control

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Distributed generalized Nash equilibrium seeking:event-triggered coding-decoding-based secure communication

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Science China(Information Sciences) 2024年第7期67卷 271-284页

作者： Shaofu yang Wenying XU Wangli HE Jinde cao School of Computer Science and Engineering Southeast University School of Mathematics Southeast University Key Laboratory of Advanced Control and Optimization for Chemical Processes East China University of Science and Technology

In this paper, we consider the distributed generalized Nash equilibrium(GNE) seeking problem in strongly monotone games. The transmission among players is implemented through a digital communication network with limited bandwidth. For improving communication efficiency or/and security, an event-triggered coding-decoding-based communication is first proposed, where the data(decision variable) are first mapped to a series of finite-level codewords and, only when an event condition is satisfied, then sent to the neighboring agents. Moreover, a distributed communication-efficient GNE seeking algorithm is constructed accordingly,and the overrelaxation scheme is further taken into consideration. Through primal-dual analysis, the proposed algorithm is proven to converge to a variational GNE with fixed step-sizes by recasting it as an inexact forward-backward iteration. Finally, numerical simulations illustrate the benefit of the proposed algorithms in terms of saving communication resources.

关键词： noncooperative games event-triggered communication coding-decoding quantization

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Effect of Active–Passive Deformation on the Thrust by the Pectoral Fins of Bionic Manta Robot

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Journal of Bionic Engineering 2024年第2期21卷 718-728页

作者： yang Lu Shaomin Meng Cheng Xing Yiwei Hao Yonghui cao Guang Pan Yong cao School of Marine Science and Technology Northwestern Polytechnical UniversityXi’an710072China Unmanned Vehicle Innovation Center Ningbo Institute of NPUNingbo315103China State Key Lab of Fluid Power and Mechatronic Systems School of Mechanical EngineeringZhejiang UniversityHangzhou310027China Zhejiang Key Laboratory of Advanced Manufacturing Technology School of Mechanical EngineeringZhejiang UniversityHangzhou310027China

Bionic manta underwater vehicles will play an essential role in future oceans and can perform tasks,such as long-duration reconnaissance and exploration,due to their efficient *** manta wings’deformation is evident during the swimming *** improve the propulsion performance of the unmanned submersible,the study of the deformation into the bionic pectoral fin is *** this research,we designed and fabricated a flexible bionic pectoral fin,which is based on the Fin Ray®effect with active and passive deformation(APD)*** APD fin was actively controlled by two servo motors and could be passively deformed to variable *** APD fin was moved at 0.5 Hz beat frequency,and the propulsive performance was experimentally verified of the bionic pectoral fins equipped with different extents of *** results showed that the pectoral fin with active–passive deformed capabilities could achieve similar natural biological deformation in the wingspan *** average thrust(T)under the optimal wingspan deformation is 61.5%higher than the traditional passive deformed pectoral *** obtained results shed light on the design and optimization of the bionic pectoral fins to improve the propulsive performance of unmanned underwater vehicles(UUV).

关键词： Manta ray Bionic pectoral fin Fin Ray®effect Active-passive deformation(APD)

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Adsorption limitation investigation on olefins for Cu–BTC

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Friction 2024年第4期12卷 606-617页

作者： Xiao yang Yunbo WANG Weihua cao Ruizheng JIANG Guoxin XIE Yuying cao Xiaowen QI School of Mechanical Engineering Yanshan UniversityQinhuangdao 066004China Key Laboratory of Self-Lubricating Spherical Plain Bearing Technology of Hebei Province Yanshan UniversityQinhuangdao 066004China State Key Laboratory of Tribology in Advanced Equipment Department of Mechanical EngineeringTsinghua UniversityBeijing 100084China Aviation Key Laboratory of Science and Technology on Generic Technology of Self-Lubricating Spherical Plain Bearing Yanshan UniversityQinhuangdao 066004China

To utilize Cu-benzene-1,3,5-tricarboxylate(Cu-BTC)adsorbed lubricant oils in the self-lubricating field,the adsorption properties of Cu-BTC on different 1-olefins must be *** this work,1-hexene,1-octene,1-nonene,1-decene,1-undecene,and 1-dodecene were studied by the Monte Carlo method and *** adsorption limit of Cu-BTC for n-olefins was determined as 1-undecene by the adsorption *** suggested a limit for even straight-chain molecules to the adsorption of *** maximum ratio of the olefin length of the largest pore diameter(L/D)of Cu-BTC was approximately ***,theoretical calculations(radial distribution function(RDF))and experiments(infrared(IR)spectra)confirmed the interaction of n-olefin adsorbates and the Cu-BTC framework occurred between the-CH=of olefins and the Cu and O atoms of the Cu-BTC *** work adds to the understanding and investigation of the adsorption of liquid lubricants using Cu-BTC as a metal-organic framework(MOF).

关键词： metal-organic framework(MOF) Cu-benzene-1,3,5-tricarboxylate(Cu-BTC) Monte Carlo method adsorption properties 1-olefins

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Structural optimization design of semi-rigid base asphalt pavement using modulus matching criterion and multi-indicator range analysis

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Journal of Traffic and Transportation Engineering(English Edition) 2024年第1期11卷 131-159页

作者： Zhihao yang Linbing Wang Dongwei cao Yinghao Miao Hailu yang China Airport Planning&Design Institute Co. Ltd.Beijing 101312China Department of Road and Urban Railway Engineering Beijing University of TechnologyBeijing 100124China National Center for Materials Service Safety University of Science and Technology BeijingBeijing 100083China School of Environmental CivilAgricultural and Mechanical EngineeringUniversity of GeorgiaAthensGA 30602USA China-Road Transportation Verification&Inspection Hi-Tech Co. Ltd.Beijing 100088China

Damage to semi-rigid base asphalt pavement is related to improper matching of the pavement structure *** study mainly focused on the modulus matching of structural layers and the development of a pavement structure optimization ***,the modulus loss of existing pavement structures was analysed,and a three-dimensional finite element model was established based on the existing ***,the influence of the modulus of each structural layer on the mechanical response indicators and fatigue life was *** on the results,a pavement structure design method using the smoothness of the stress-strain curve as the modulus matching criterion of the structural layers was *** it was found that a strain convex point was present and that the stress mutation between the structural layers was significant when the modulus matching of the pavement structure was ***,the evaluation indicators were divided into two groups,namely,mechanical indicators and fatigue life *** it was proposed an optimized pavement structure design method based on modulus matching and multi-indicator range ***,the optimal modulus combination of pavement structure was determined by this *** research systematically studied the influence of the modulus of each structural layer on the mechanical response and fatigue life of the pavement,and proposed the concept and specific executive criteria of modulus matching for the first ***,it also provided an effective optimization method for pavement structure design.

关键词： Stress-strain curve Modulus matching Structural optimization design Multi-indicator range analysis Fatigue life

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A comprehensive review on microchannel heat sinks for electronics cooling

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International Journal of Extreme Manufacturing 2024年第2期6卷 133-162页

作者： Zhi-Qiang Yu Mo-Tong Li Bing-yang cao Key Laboratory for Thermal Science and Power Engineering of Ministry of Education Department of Engineering MechanicsTsinghua UniversityBeijing 100084People’s Republic of China

The heat generation of electronic devices is increasing dramatically,which causes a serious bottleneck in the thermal management of electronics,and overheating will result in performance deterioration and even device *** the development of micro-machining technologies,the microchannel heat sink(MCHS)has become one of the best ways to remove the considerable amount of heat generated by high-power *** has the advantages of large specific surface area,small size,coolant saving and high heat transfer *** paper comprehensively takes an overview of the research progress in MCHSs and generalizes the hotspots and bottlenecks of this *** heat transfer mechanisms and performances of different channel structures,coolants,channel materials and some other influencing factors are ***,this paper classifies the heat transfer enhancement technology and reviews the related studies on both the single-phase and phase-change flow and heat *** comprehensive review is expected to provide a theoretical reference and technical guidance for further research and application of MCHSs in the future.

关键词： microchannel heat sink thermal management of electronics microscale heat transfer heat transfer enhancement

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Controlling of coordination state of Ru_(x)N_(y) clusters for efficient oxygen reduction electrocatalysis

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Nano Research 2024年第3期17卷 1035-1041页

作者： Weiyang fu Yihuan Yu Tongtong Liu Yinliang cao Zhengping Zhang Feng Wang State Key Laboratory of Chemical Resource Engineering Beijing Key Laboratory of Electrochemical Process and Technology for MaterialsBeijing University of Chemical TechnologyBeijing 100029China Beijing Advanced Innovation Center for Soft Matter Science and Engineering Beijing University of Chemical TechnologyBeijing 100029China Zhejiang Tianneng Hydrogen Energy Technology Co. Ltd.Huzhou 313100China

Ruthenium(Ru)is an attractive potential alternative to platinum as an electrocatalyst for the oxygen reduction reaction(ORR),in virtue of its high catalytic selectivity and relatively low *** this work,a series of well-dispersed nitrogen-coordinated Ru-clusters on carbon black(Ru_(x)N_(y)/C)were prepared by pyrolyzing different Ru-containing sandwich compounds as the Ru *** higher thermal stability of these complexed sandwich precursors(bis(1,2,3,4,5-pentamethylcyclopentadienyl)Ru(II)monomer,dichloro(p-cymene)Ru(II)dimer,and chloro(1,2,3,4,5-pentamethylcyclopentadienyl)Ru(II)tetramer)affords the control of coordinated state for the resulting Ru-clusters,in comparison of that derived from ruthenium *** the pyrolysis treatment,the Ru coordinated state in Ru_(x)N_(y)/C,with the Ru–N and Ru–Ru bonds,still showed the structural inheritance from the Ru(II)monomer,dimer,and tetramer,but using ruthenium chlorides as the Ru source resulted in the nanoscale Ru *** ORR testing exhibited that the Ru_(x)N_(y)/C sample derived from the Ru(II)tetramer(Ru_(x)N_(y)/C-T)presents the higher catalytic activity than the other obtained samples in either alkaline or acidic *** in the acidic electrolyte,Ru_(x)N_(y)/C-T shows the comparable ORR activity to that of Pt/C catalysts,and it shows the superior tolerance against methanol and *** X-ray absorption spectroscopy and density functional theory calculations demonstrate that these tetra-nuclear Ru-clusters could be the most active site due to their broadened d-orbital bands and lower energy d-band center than those of other subnano species and nanocrystals,and their favorable Yeager-type adsorption of O_(2)-molecules is also contributed to promoting O–O bond cleavage and accelerating the ORR process.

关键词： ruthenium clusters coordination environment sandwich compounds electrocatalysis oxygen reduction reaction

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Spontaneous anchoring Cl intoα-Co(OH)_(2) as efficient and stable oxygen reduction electrocatalysts for seawater battery

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Rare Metals 2024年第7期43卷 3074-3083页

作者： Wang Zheng Xue-Rong Zheng Qi Lu Yan-Hui cao yang Wang Hai-Peng fu Jin-Feng Zhang Yi-Da Deng Wen-Bin Hu School of Materials Science and Engineering Key Laboratory of Advanced Ceramics and Machining Technology of Ministry of EducationTianjin UniversityTianjin 300072China State Key Laboratory of Marine Resource Utilization in South China Sea School of Materials Science and EngineeringHainan UniversityHaikou 570228China Key Laboratory of Electromagnetic Processing of Materials Ministry of EducationNortheastern UniversityShenyang 110819China

Seawater battery is an advanced energy storage system that enables conversion of chemical energy to electricity by consuming metals,dissolved oxygen and seawater in anode,cathode and electrolyte,***,the oxygen reduction reaction(ORR)activity and stability of electrocatalysts can be easily deactivated due to the severe Cl~-permeation and corrosion in seawater ***,we developed a structural buffer engineering strategy by spontaneously anchoring Cl~-intoα-Co(OH)_(2) as efficient and stable ORR electrocatalysts,in which the ultrathinα-Co(OH)_(2) nanosheets were synthesized using an ultrafast solution high-temperature shock(SHTS)*** large lattice space(~0.8 nm)of layeredα-Co(OH)_(2) ensured the spontaneously penetration of Cl~-into the lattice structure and replaced part of OH~-to formα-Co(OH)_(2-x)Cl_*** continuous leaching and compensating of saturated Cl inα-Co(OH)_(2-x)Cl_x could enhance the Cl~-corrosion resistance and modulate electronic structure of Co metallic sites,thus improving the ORR electrocatalytic activity and stability in seawater ***α-Co(OH)_(2-x)Cl_x seawater batteries display superior onset and half-wave potentials of 0.71 and 0.66 V,respectively,which are much better than the counterparts ofα-Co(OH)_(2) and ofβ-Co(OH)_(2) with no Cl~-penetrating and no buffer ***α-Co(OH)_(2-x)Cl_x-based seawater batteries display stable open-circuit potential of 1.69 V and outstanding specific capacity of 1345 mAh·g^(-1).

关键词： Seawater battery Oxygen reduction electrocatalyst Solution high-temperature shock Structural buffer engineering

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A novel method for vibration signal transmission and attenuation analysis in complex planetary gearboxes

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Science China(Technological Sciences) 2024年第9期67卷 2939-2953页

作者： WEI ChaoHu cao HongRui SHI JiangHai yang yang DU MingGang National and Local Joint Engineering Research Center of Equipment Operation Safety and Intelligent Monitoring Xi’an Jiaotong UniversityXi’an 710049China School of Mechanical Engineering Xi’an Jiaotong UniversityXi’an 710049China China North Vehicle Research Institute Beijing 100072China

Planetary gearboxes play a crucial role in altering rotary speed and transmitting power in large machines like wind turbines and sophisticated vehicles. There are many nonlinear interfaces, such as splines, bearings, and gear pairs, in planetary gearboxes, and the resulting vibration signal transmission and attenuation mechanisms are still unknown. In this study, a novel method for quantitatively analyzing the transmission and attenuation of vibration signals is proposed. A multibody dynamic model of the planetary gearbox considering nonlinear gear meshing is presented and experimentally validated. To avoid the interference of foundation vibration on the transmission of the fault signal, the fault impact factor(FIF) is used to describe the intensity of the failure, which aligns well with the experimental signals. Based on the FIF, the vibration signal attenuation of nonlinear interfaces such as splines, bearings, and gear meshing interfaces is quantitatively evaluated. To clarify the transfer paths of fault vibration signals inside the gearbox, the transfer path area method(TPAM) based on FIF is proposed. According to the simulated results,the primary transfer paths of fault vibration signals within the gearbox have been identified, which is of great help in understanding the transmission and attenuation of vibration signals in planetary gearboxes.

关键词： planetary gearbox nonlinear interface fault mechanism vibration transmission vibration attenuation

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