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Electronic structure and mechanical properties of layered compound YB_2C_2:A promising precursor for making two dimensional(2D) B_2C_2 nets

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Journal of Materials Science & Technology 2017年第9期33卷 1044-1054页

作者： Yanchun zhou Huimin xiang Xiaohui Wang Wei Sun fu-Zhi Dai Zhihai Feng Science and Technology of Advanced functional Composite Laboratory Aerospace Research Institute of Materials & Processing Technology Shenyang National Laboratory for Materials Science Institute of Metal ResearchChinese Academy of Sciences

Layered compounds play pivotal roles as precursors for producing 2D materials through mechanical exfoliation(micro-mechanical cleavage) or chemical approaches. Therefore, searching for layered compounds with sharp anisotropic chemical bonding and properties becomes emergent. In this work, the stability, electronic structure, elastic properties, and lattice dynamics of YBCwere investigated. Strong anisotropy in elastic properties is revealed, i.e., high Young’s modulus in a-b plane but low Young’s modulus in c direction. The maximum to minimum Young’s modulus ratio is 2.41 and 2.45 for YBCwith P42/mmc and P4/mbm symmetry, respectively. The most likely systems for shear sliding or microdelaminating are(001)[100] and(001)[010]. The anisotropic elastic properties are underpinned by the anisotropic chemical bonding, i.e., strong bonding within the BCnets and weak bonding between Y atom layers and BCnets. YBCis electrically conductive and the contributions to the electrical conductivity are from delocalized Y 4deas well as Bpandpzelectrons. The layered crystal structure, sharp anisotropic mechanical properties, and metallic conductivity endorse YBCpromising as a precursor for new 2D BCnets.

关键词： YB2C2 Layered compounds Electronic structure Mechanical properties 2D graphite like materials

Phase pure and well crystalline Cr2AlB2:A key precursor for two-dimensional CrB

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Journal of Materials Science & Technology 2019年第8期35卷 1593-1600页

作者： Haiming Zhang fu-Zhi Dai Huimin xiang Xiaohui Wang Zhili Zhang Yanchun zhou School of Mechanical Electronic and Control EngineeringBeijing Jiaotong UniversityBeijing 100044 China Science and Technology on Advanced functional Composite Laboratory Aerospace Research Institute of Materials & Processing TechnologyNo. 1 South Dahongmen Road Beijing 100076 China Shenyang National Laboratory for Materials Sciences Institute of Metal ResearchChinese Academy of Sciences72 Wenhua Road Shenyang 110016 China

Phase pure and well crystalline Cr2AlB2 powders are synthesized by heating the mixtures of CrB and Al powders at 900~℃.Cr2AlB2 exhibits nanolaminated morphology which transforms from flake-like crystallite to needle-like grain with the increase of holding *** morphology-structure relationships of Cr2AlB2 are delicately ***,as the precursor for fabrication of Cr2AlB2,high purity CrB powders are also prepared by high-temperature reaction of B and Cr elemental powders at 1800℃.CrB grains grow into regular plate-like *** Rietveld structure refinement,new sets of diffraction data are presented for both CrB and Cr2AlB2 and overlapped peak positions and intensities are revealed which make up for the deficiency of the existing data in ICDD PDF#32-0277(CrB)and ICDD PDF#72-1847(Cr2AlB2).Moreover,since MAB phases are precursors for preparing MBenes,2D-CrBnanosheets are successfully prepared by completely etching out Al atomic layers from Cr2AlB2.2D-CrB crystalizes in CrB structure with two-dimensional lamellar *** the formation mechanism of 2D-CrB is vividly depicted.A system of materials preparation from CrB to Cr2AlB2 and then to 2D-CrB is well established.

关键词： Cr2AlB2 CrB MAB phases 2D-CrB Ultrahigh temperature ceramics

Photothermal Nano-Vaccine Promoting Antigen Presentation and Dendritic Cells Infiltration for Enhanced Immunotherapy of Melanoma via Transdermal Microneedles Delivery

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Research 2023年第2期2022卷 139-157页

作者： Jiaojiao Zhu Ruimin Chang Benliang Wei Yao fu xiang Chen Hong Liu Wenhu zhou xiangya School of Pharmaceutical Sciences Central South UniversityChangshaHunan 410013China Department of Dermatology Hunan Engineering Research Center of Skin Health and DiseaseHunan Key Laboratory of Skin Cancer and PsoriasisXiangya HospitalCentral South UniversityChangsha410008 HunanChina National Engineering Research Center of Personalized Diagnostic and Therapeutic Technology Xiangya Hospital.Central South UniversityChangsha410008 HunanChina Department of Thoracic Surgery Xiangya HospitalCentral South UniversityChangshaHunan 410008China

Immunotherapy has demonstrated the potential to cure melanoma,while the current response rate is still unsatisfactory in *** evidence indicates the correlation between the eficacy and pre-existing T-cell in tumors,whe... 详细信息

关键词： melanoma Antigen Vaccine

Digital twin-driven green material optimal selection and evolution in product iterative design

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Advances in Manufacturing 2023年第4期11卷 647-662页

作者： Feng xiang Ya-Dong zhou Zhi Zhang Xiao-fu Zou Fei Tao Ying Zuo Key Laboratory of Metallurgical Equipment and Control Technology Ministry of EducationWuhan University of Science and TechnologyWuhan430081People’s Republic of China Hubei Key Laboratory of Mechanical Transmission and Manufacturing Engineering Wuhan University of Science and TechnologyWuhan430081People’s Republic of China Institute of Artificial Intelligence Beihang UniversityBeijing100191People’s Republic of China School of Automation Science and Electrical Engineering Beihang UniversityBeijing100191People’s Republic of China Research Institute for Frontier Science Beihang UniversityBeijing100191People’s Republic of China

In recent years,green concepts have been integrated into the product iterative design in the manufacturing field to address global competition and sustainability ***,previous efforts for green material optimal selection disregarded the interaction and fusion among physical entities,virtual models,and users,resulting in distortions and inaccuracies among user,physical entity,and virtual model such as inconsistency among the expected value,predicted simulation value,and actual performance value of evaluation ***,this study proposes a digital twin-driven green material optimal selection and evolution method for product iterative ***,a novel framework is ***,an analysis is carried out from six perspectives:the digital twin model construction for green material optimal selection,evolution mechanism of the digital twin model,multi-objective prediction and optimization,algorithm design,decision-making,and product function ***,taking the material selection of a shared bicycle frame as an example,the proposed method was verified by the prediction and iterative optimization of the carbon emission index.

关键词： Product iterative design Digital twin(DT) Green material optimal selection Evolution mechanism Iterative optimization

High entropy rare earth hexaborides/tetraborides(HE REB_(6)/HE REB_(4)) composite powders with enhanced electromagnetic wave absorption performance

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Journal of Materials Science & Technology 2021年第28期87卷 155-166页

作者： Weiming Zhang Biao Zhao Na Ni Huimin xiang fu-Zhi Dai Shijiang Wu Yanchun zhou Science and Technology on Advanced functional Composite Laboratory Aerospace Research Institute of Materials&Processing TechnologyBeijing100076China Henan Key Laboratory of Aeronautical Materials and Application Technology School of Material Science and EngineeringZhengzhou University of AeronauticsZhengzhou450046China Key Lab of Education Ministry for Power Machinery and Engineering School of Mechanical EngineeringShanghai Jiao Tong UniversityShanghai200240China Zibo Firststar New Material Incorporated Co.Ltd. Zibo255000China

The increasing electromagnetic hazards including electromagnetic interference and electromagnetic pollution,which were stemmed from massive usage of electromagnetic technology,have triggered widespread *** cope with this challenge,electromagnetic wave absorbing materials with high performance are greatly *** construction has been widely applied in electromagnetic(EM)wave absorbing materials to achieve high permittivity,high permeability and impedance ***,high-temperature stability,oxidation and corrosion resistance are still unignorable ***,high entropy hexaborides/tetraborides(HE REB_(6)/HE REB_(4))composites with synergistic dielectric and magnetic losses were designed and successfully synthesized through a one-step boron carbide reduction *** five as-prepared(Y_(0.2) Nd_(0.2) Sm_(0.2) Eu_(0.2) Er_(0.2))B_(6)/(Y_(0.2) Nd_(0.2) Sm_(0.2) Eu_(0.2) Er_(0.2))B_(4),(Y_(0.2) Nd_(0.2) Sm_(0.2) Er_(0.2) Yb_(0.2))B_(6)/(Y_(0.2) Nd_(0.2) Sm_(0.2) Er_(0.2) Yb_(0.2))B_(4),(Y_(0.2) Nd_(0.2) Eu_(0.2) Er_(0.2) Yb_(0.2))B_(6)/(Y_(0.2) Nd_(0.2) Eu_(0.2) Er_(0.2) Yb_(0.2))B_(4),(Nd_(0.2) Sm_(0.2) Eu_(0.2) Er_(0.2) Yb_(0.2))B_(6)/(Nd_(0.2) Sm_(0.2) Eu_(0.2) Er_(0.2) Yb_(0.2))B_(4) and(Y_(0.2) Sm_(0.2) Eu_(0.2) Er_(0.2) Yb_(0.2))B_(6)/(Y_(0.2) Sm_(0.2) Eu_(0.2) Er_(0.2) Yb_(0.2))B_(4) contain two phases of HE REB_(6) and HE REB_(4).Among them(Y_(0.2) Nd_(0.2) Sm_(0.2) Eu_(0.2) Er_(0.2))B_(6)/(Y_(0.2) Nd_(0.2) Sm_(0.2) Eu_(0.2) Er_(0.2))B_(4)(HE REB_(6)/HE REB_(4)-1)and(Y_(0.2) Nd_(0.2) Sm_(0.2) Er_(0.2) Yb_(0.2))B_(6)/(Y_(0.2) Nd_(0.2) Sm_(0.2) Er_(0.2) Yb_(0.2))B_(4)(HE REB_(6)/HE REB_(4)-2)exhibit excellent EM wave absorption *** optimal minimum reflection loss(RL_(m in))and effective absorption bandwidth(E_(AB))of HE REB_(6)/HE REB_(4)-1 and HE REB_(6)/HE REB_(4)-2 are–53.3 dB(at 1.7 mm),4.2 GHz(at 1.5 mm)and–43.5 dB(1.3 mm),4.2 GHz(1.5 mm),*** combination of conducting HE REB_(4) with magnetism into HE REB_

关键词： High entropy ceramics Hexaborides/tetraborides composites One-step synthesis Electromagnetic wave absorption Synergistic dielectric and magnetic losses

High-entropy spinel ferrites MFe_(2)O_(4)(M=Mg,Mn,Fe,Co,Ni,Cu,Zn)with tunable electromagnetic properties and strong microwave absorption

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Journal of Advanced Ceramics 2022年第5期11卷 754-768页

作者： Jiabin MA Biao ZHAO Huimin xiang fu-Zhi DAI Yi LIU Rui ZHANG Yanchun zhou Henan Key Laboratory of Aeronautical Materials and Application Technology School of Materials Science and EngineeringZhengzhou University of AeronauticsZhengzhou 450046China Science and Technology on Advanced functional Composite Laboratory Aerospace Research Institute of Materials&Processing TechnologyBeijing 100076China School of Material Science and Engineering Shaanxi University of Science and TechnologyXi'an 710021China School of Materials Science and Engineering Luoyang Institute of Science and TechnologyLuoyang 471023China

Ferrites are the most widely used microwave absorbing materials to deal with the threat of electromagnetic(EM)***,the lack of sufficient dielectric loss capacity is the main challenge that limits their *** cope with this challenge,three high-entropy(HE)spineltype ferrite ceramics including(Mg_(0.2)Mn_(0.2)Fe_(0.2)Co_(0.2)Ni_(0.2))Fe_(2)O_(4),(Mg_(0.2)Fe_(0.2)Co_(0.2)Ni_(0.2)Cu_(0.2))Fe_(2)O_(4),and(Mg_(0.2)Fe_(0.2)Co_(0.2)Ni_(0.2)Zn_(0.2))Fe_(2)O_(4)were designed and successfully prepared through solid state *** results show that all three HE MFe_(2)O_(4) samples exhibit synergetic dielectric loss and magnetic *** good magnetic loss ability is due to the presence of magnetic components;while the enhanced dielectric properties are attributed to nano-domain,hopping mechanism of resonance effect and HE *** three HE spinels,(Mg_(0.2)Mn_(0.2)Fe_(0.2)Co_(0.2)Ni_(0.2))Fe_(2)O_(4)shows the best EM wave absorption performance,e.g.,its minimum reflection loss(RL_(min))reaches-35.10 dB at 6.78 GHz with a thickness of 3.5 mm,and the optimized effective absorption bandwidth(EAB)is 7.48 GHz from 8.48 to 15.96 GHz at the thickness of 2.4 *** to the easy preparation and strong EM dissipation ability,HE MFe_(2)O_(4) are promising as a new type of EM absorption materials.

关键词： high-entropy ceramics(HECs) spinel-type ferrite electromagnetic(EM)wave absorption dielectric loss magnetic loss

Electromagnetic wave absorbing properties of TMCs(TM=Ti,Zr,Hf,Nb and Ta)and high entropy(Ti0.2Zr0.2Hf0.2Nb0.2Ta0.2)C

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Journal of Materials Science & Technology 2021年第15期74卷 105-118页

作者： Yanchun zhou Biao Zhao Heng Chen Huimin xiang fu-Zi Dai Shijiang Wu Wei Xu Science and Technology on Advanced functional Composite Laboratory Aerospace Research Institute of Materials&Processing TechnologyBeijing100076China Henan Key Laboratory of Aeronautical Materials and Application Technology School of Material Science and EngineeringZhengzhou University of AeronauticsZhengzhou450046China Key Laboratory of Advanced Ceramics and Machining Technology of Ministry of Education School of Materials Science and EngineeringTianjin UniversityTianjin300072China Zibo Firstar New Material Incoqjorated Co.Ltd. Zibo255000China Shanghai Chenhua Science and Technology Coloration Ltd. Shanghai201804China

Electromagnetic wave(EMW)absorbing materials play a vital role in modern communication and information processing technologies to inhibit information leakage and prevent possible damages to environment and human ***,most of EMW absorbing materials are either composites of two or more phases or in the form of nanosheets,nanowires or nanofibers in order to enhance the EMW absorption performance through dielectric loss,magnetic loss and dielectric/magnetic loss ***,the combination of complex shapes/multi phases and nanosizes may compound the difficulties of materials processing,composition and interfaces control as well as performance maintenance during ***,searching for single phase materials with good stability and superior EMW absorbing properties is *** achieve this goal,the EMW absorbing properties of transition metal carbides TMCs(TM=Ti,Zr,Hf,Nb and Ta)and high entropy(Ti_(0.2)Zr_(0.2)Hf_(0.2)Nb_(0.2)Ta_(0.2))C which belong to ultrahigh temperature ceramics,were investigated in this *** to the good electrical conductivity and splitting of d orbitals into lower energy t2glevel and higher energy eglevel in TMC6octahedral arrangement,TMCs(TM=Ti,Zr,Hf,Nb and Ta)exhibit good EMW absorbing ***,Hf C and Ta C exhibit superior EMW absorbing *** minimum reflection loss(RLmin)value of Hf C is-55.8 d B at 6.0 GHz with the thickness of 3.8 mm and the effective absorption bandwidth(E_(AB))is 6.0 GHz from 12.0 to 18.0 GHz at thickness of 1.9 mm;the RL_(minvalue)of Ta C reaches-41.1 d B at 16.2 GHz with a thickness of 2.0 mm and the EABis 6.1 GHz with a thickness of 2.2 ***,the electromagnetic parameters,i.e.,complex permittivity and permeability are tunable by forming single phase solid solution or high entropy(Ti_(0.2)Zr_(0.2)Hf_(0.2)Nb_(0.2)Ta_(0.2))*** R_(Lminvalue)of high entropy(Ti_(0.2)Zr_(0.2)Hf_(0.2)Nb_(0.2)Ta_(0.2))C is-38.5 d B at 9.5 GHz with the thickness of 1.9 mm,and the EA

关键词： Transition metal carbides High entropy ceramics Microwave absorption Electromagnetic parameters Electronic structure Crystal field theory

Preparation and properties of CMAS resistant bixbyite structured high-entropy oxides RE_(2)O_(3)(RE=Sm,Eu,Er,Lu,Y,and Yb):Promising environmental barrier coating materials for Al_(2)O_(3)f/Al_(2)O_(3) composites

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Journal of Advanced Ceramics 2021年第3期10卷 596-613页

作者： Yanan SUN Huimin xiang fu-Zhi DAI Xiaohui WANG Yan XING Xiaojun ZHAO Yanchun zhou School of Materials Science and Engineering Central South UniversityChangsha 410083China Science and Technology on Advanced functional Composite Laboratory Aerospace Research Institute of Materials&Processing TechnologyBeijing 100076China Shenyang National Laboratory for Materials Science Institute of Metal ResearchChinese Academy of SciencesShenyang 110016China New Energy Technology Engineering Laboratory of Jiangsu Province Nanjing University of Posts and TelecommunicationsNanjing 210023China

Y_(2)O_(3) is regarded as one of the potential environmental barrier coating(EBC)materials for Al_(2)O_(3)f/Al_(2)O_(3)ceramic matrix composites owing to its high melting point and close thermal expansion coefficient to Al_(2)O_(3).However,the relatively high thermal conductivity and unsatisfactory calcium-magnesium-aluminosilicate(CMAS)resistance are the main obstacles for the practical application of Y_(2)O_(3).In order to reduce the thermal conductivity and increase the CMAS resistance,four cubic bixbyite structured high-entropy oxides RE_(2)O_(3),including(Eu_(0.2)Er_(0.2)Lu_(0.2)Y_(0.2)Yb_(0.2))2O_(3),(Sm_(0.2)Er_(0.2)Lu_(0.2)Y_(0.2)Yb_(0.2))2O_(3),(Sm_(0.2)Eu_(0.2)Er_(0.2)Y_(0.2)Yb_(0.2))2O_(3),and(Sm_(0.2)Eu_(0.2)Lu_(0.2)Y_(0.2)Yb_(0.2))2O_(3)were designed and synthesized,among which(Eu_(0.2)Er_(0.2)Lu_(0.2)Y_(0.2)Yb_(0.2))2O_(3)and(Sm_(0.2)Er_(0.2)Lu_(0.2)Y_(0.2)Yb_(0.2))2O_(3)bulks were prepared by spark plasma sintering(SPS)to investigate their mechanical and thermal properties as well as CMAS *** mechanical properties of(Eu_(0.2)Er_(0.2)Lu_(0.2)Y_(0.2)Yb_(0.2))2O_(3)and(Sm_(0.2)Er_(0.2)Lu_(0.2)Y_(0.2)Yb_(0.2))2O_(3) are close to those of Y_(2)O_(3) but become more brittle than Y_(2)O_(3).The thermal conductivities of(Eu_(0.2)Er_(0.2)Lu_(0.2)Y_(0.2)Yb_(0.2))2O_(3) and(Sm_(0.2)Er_(0.2)Lu_(0.2)Y_(0.2)Yb02)2O_(3)(5.1 and 4.6 W·m^(-1)·K^(-1))are only 23.8%and 21.5%respectively of that of Y_(2)O_(3)(21.4 W·m^(-1)·K^(-1)),while their thermal expansion coefficients are close to those of Y_(2)O_(3) and A12O_(3).Most importantly,HE RE_(2)O_(3) ceramics exhibit good CMAS *** being attacked by CMAS at 1350℃for 4 h,the HE RE_(2)O_(3) ceramics maintain their original morphologies without forming pores or cracks,making them promising as EBC materials for Al_(2)O_(3)f/Al_(2)O_(3) composites.

关键词： high-entropy ceramics rare earth oxides low thermal conductivity thermal expansion coefficient CMAS resistance

Superlubricitive engineering—future industry nearly getting rid of wear and frictional energy consumption

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Friction 2020年第4期8卷 643-665页

作者： Jianbin LUO xiang zhou State Key Laboratory of Tribology Tsinghua UniversityBeijing 100084China

Superlubricity has been developing very rapidly in recent years as a new and important area in tribology. Many new phenomena and materials, as well as some new mechanisms in both liquid and solid superlubricity have been obtained. In liquid superlubricity, tens of new kinds of liquids with superlubricity have been found (e.g., water-based liquids, oil-based lubricants, and liquids combined with additives of two-dimensional (2D) materials that exhibit very good superlubricity properties under high pressure). In the field of solid superlubricity, more materials with superlubricity have been observed, including graphene-to-graphene surfaces, highly oriented pyrolytic graphite to graphene surfaces, and heterostructure surfaces where a friction coefficient as low as 0.00004 has been obtained. However, superlubricity is still under laboratory research. What is the future of superlubricity? What is the barrier restricting superlubricity from industrial applications? How do we transfer superlubricity from scientific research to industrial application? These questions and application fields of superlubricity in near future have been analyzed, and the concept of"superlubricitive engineering"has been proposed in the present work.

关键词： superlubricitive engineering superlubricity liquid superlubricity solid superlubricity two-dimensional(2D)material lubrication