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A novel Ce_(0.485)Zr_(0.485)Y_(0.03)O_(2) composite oxide with surface doping of Y and its application in Pd-only three-way catalyst

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Rare Metals 2024年第2期43卷 749-757页

作者： Zheng Zhao wei-Xin Zhao Yong-Qi Zhang Mei-sheng Cui Yong-Ke Hou Dong-Ming Chen Juan-Yu Yang Zong-Yu Feng Xiao-wei Huang National Engineering Research Center for Rare Earth Grirem Advanced Materials Co.Ltd.GRINM Group Corporation LimitedBeijing100088China Griem Hi-Tech Co.Ltd. Langfang065000China Rare Earth functional Materials(Xiong’an)Innovation Venter Co.Ltd. Baoding071700China

The ceria-zirconia compound oxide-supported noble metal Pd(Pd@CZ)is widely used in three-way ***,the surface structure of CZ plays an important role in catalytic activity of ***,how to regulate the surface structure of CZ and clarify the structure–activity relationship is still a *** this paper,a strategy is proposed to develop high activity Pd@CZ nanocatalysts by tuning Y doping sites in *** precipitate-deposition method is developed to prepare the novel Ce_(0.485)Zr_(0.485)Y_(0.03)O_(2) composite with surface doping of Y(CZ-Y-S).In addition,the Pd@CZ-Y-S(Pd supported on CZ-Y-S)exhibits superior catalytic activity for HC,CO,and NO oxide,wherein,for CO and C_(3)H_(6) oxidation,the low-temperature activity of Pd@CZ-Y-S is still 20%higher than that of Pd@CZ-Y-B(Y bulk doping)and commercial Pd@CZ after 1000℃/4 h *** effect mechanism is further studied by density functional theory(DFT)*** with Pd@CZ-Y-B,Pd@CZ-Y-S shows the lower CO oxide reaction energy barriers due to the weaker adsorption strength of *** Y surface doping strategy could provide valuable insights for the development of highly efficient Pd@CZ catalyst with extensive applications.

关键词： Rare earth Ceria-zirconia-supported Pd Surface doping Experiment and theory Catalytic application

Theoretical Exploration of Alloying Effects on Stabilities and Mechanical Properties ofγʹPhase in Novel Co–Al–Nb-Base Superalloys

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Acta Metallurgica Sinica(English Letters) 2024年第7期37卷 1238-1248页

作者： Guan-Cheng Gu Zhao-Jing Han Ze-Yu Chen Zhao-Xuan Li sheng-Bao Xia Zheng-Ning Li Hua Jin wei-wei Xu Xing-Jun Liu Shenzhen Research Institute of Xiamen University School of Aerospace EngineeringXiamen UniversityXiamen361005China Institute of Materials Genome and Big Data Harbin Institute of TechnologyShenzhen518055China

The new developedγ/γʹCo–Al–Nb-base alloys show great potentials as high-temperature ***,finding appropriate compositions to improve performance of alloys still poses a great challenge to the development of Co–Al–Nb-base *** by the lack of alloying effects on fundamental properties of criticalγʹphase,we systematically performed a theoretical investigation on the effect of alloying elements TM(TM:Ti,V,Cr,Zr,Mo,Ta,W,Re,and Ru)on phase stabilities and mechanical properties of L1_(2)-typeγʹ(Co,Ni)_(3)(Al,Nb).By analyzing the stability ofγʹphase with respect to its competitive B2 and D0_(19) phases,the results shown that Ti,V,and Cr enhance the L1_(2) stability and widen the L1_(2)–D0_(19) energy barrier,in which V yields the maximum *** analysis of electronic structure indicated that the alternation of valence electrons at fermi level would be the atomic origin for doping TM inγʹ*** calculated results of mechanical properties shown that V and Cr are expected to be optimal dopant for enhancing the strength and the ductility ofγʹ*** addition of Ta is also beneficial for enhancing the strength at the slight expense of ductility ofγʹ*** drawing the mechanical maps,the preferred composition range for the phases with desired properties is roughly demarcated in theory for the multi-addition of V/Cr and V/Ta inγʹ*** findings would be useful for optimizing the performance of novelγ/γʹCo–Al–Nb-base superalloys.

关键词： Co-Al-Nb-base superalloys γ/γʹdual-phase Phase stability Mechanical properties First-principle methods

超临界水堆滑压启堆工况下堆芯热工水力动态模拟

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核动力工程 2011年第5期32卷 69-74页

作者：傅晟威周翀许志红杨燕华海军工程大学武汉430000 上海交通大学上海200240

对ATHLET-SC系统程序进行改进,实现了两流体模型下的跨临界瞬态计算。以该程序为基础,采用超临界轻水堆型(SCLWR-H)的滑压启堆方案,针对混合谱堆型的堆芯部分进行启堆工况下的热工水力动态模拟。模拟结果表明,整个启堆过程中燃料棒包壳... 详细信息

对ATHLET-SC系统程序进行改进,实现了两流体模型下的跨临界瞬态计算。以该程序为基础,采用超临界轻水堆型(SCLWR-H)的滑压启堆方案,针对混合谱堆型的堆芯部分进行启堆工况下的热工水力动态模拟。模拟结果表明,整个启堆过程中燃料棒包壳表面温度均未超过限值(650℃),跨临界瞬态下水的物性突变不会对堆芯燃料棒包壳传热造成不良影响。

关键词：滑压启堆动态模拟 ATHLET-SC 超临界水堆

Spatio-temporal variation of water salinity in mangroves revealed by continuous monitoring and its relationship to floristic diversity

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Plant Diversity 2024年第1期46卷 134-143页

作者： wei Wang Kun Xin Yujun Chen Yuechao Chen Zhongmao Jiang Nong sheng Baowen Liao Yanmei Xiong Research Institute of Tropical Forestry Chinese Academy of ForestryGuangzhou 510520PR China Guangdong Zhanjiang Mangrove National Nature Reserve Administration Zhanjiang 524088PR China

Salinity is among the most critical factors limiting the growth and species distribution of coastal *** salinity in estuarine ecosystems varies temporally and spatially,but the variation patterns across different time scales and salinity fluctuation have rarely been *** effects of salinity on floristic diversity in mangroves are not fully understood due to the temporal and spatial heterogeneity of *** this study,we monitored water salinity at an interval of 10-min over one year in three mangrove catchment areas representing the outer part,middle part,and inner part respectively of Dongzhai Bay,Hainan,*** number of mangrove community types and dominant mangrove species of the three catchment areas were also *** found that the diurnal variation and dry-season intra-month variation in water salinity were driven by tidal *** seasonal variation in water salinity was mainly driven by rainfall with higher salinity occurring in the dry season and lower salinity occurring in the wet ***,water salinity was highest at the outer part,intermediate at the middle part,and lowest at the inner part of the *** intra-month and annual fluctuations of water salinity were highest at the middle part and lowest at the outer part of the *** number of mangrove community types and dominant species were lowest at the outer part,intermediate at the middle part,and highest at the inner part of the *** results suggest that the temporal variation of water salinity in mangroves is driven by different factors at different time scales and therefore it is necessary to measure water salinity at different time scales to get a complete picture of the saline environment that mangroves ***,lower salinity levels benefit mangrove species richness within a bay landscape,however,further research is needed to distinguish the effects of salinity fluctuation and salinity level in affecting mangrove species richness.

关键词： Coastal wetlands Mangroves Salinity fluctuation Species diversity Species richness

Detection of SARS-CoV-2 based on artificial intelligence-assisted smartphone:A review

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Chinese Chemical Letters 2024年第7期35卷 25-34页

作者： Yunxin Li Jinghui Zhang Jisen Chen Feng Zhu Zhiqiang Liu Peng Bao wei Shen sheng Tang School of Environmental and Chemical Engineering Jiangsu University of Science and TechnologyZhenjiang 212003China Programme in Emerging Infectious Diseases Duke-NUS Medical SchoolSingapore 169857Singapore

In recent years,the application of smartphone in various fields has received great attention,and it has become a promising tool in virus detection,data processing and data *** the rapid spread of COVID-19 around the world,many traditional detection methods have been combined with smartphone to assist in the analysis and detection of the novel coronavirus(SARS-CoV-2),including electrochemistry,fluorescence and *** the gradual development of artificial intelligence(AI),the combination of AI and smartphone to analyze SARS-CoV-2 was also the focus of *** on the summary of the traditional methods combined with smartphone to detect SARS-CoV-2 virus,in addition to AI-based data processing,AI algorithms are also employed for SARS-CoV-2 detection *** review discussed both strategies and focused on the application of the *** combination of AI algorithm and smartphone to detect SARS-CoV-2 has high accuracy,which is more conducive to meeting the needs of portable *** addition,the classification of SARS-CoV-2 virus samples in biological fluids such as blood and saliva was also ***,this paper briefly discussed the limitations of using smartphone analysis to detect SARS-CoV-2,as well as the prospect and future development of virus *** conclusion,the detection methods based on smartphone and AI algorithms show great potential in the detection of SARS-CoV-2 and can be a valuable complement to traditional analysis methods.

关键词： COVID-19 SARS-CoV-2 virus Detection method Smartphone analysis Artificial intelligence

Safety and efficacy of transcatheter arterial embolization in autosomal dominant polycystic kidney patients with gross hematuria: Six case reports

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World Journal of Clinical Cases 2024年第11期12卷 1954-1959页

作者： wei-Fan Sui Yun-Xin Duan Jian-Yun Li wei-Bin Shao Jian-Hua fu Department of Interventional Radiology Zhenjiang First People's HospitalZhenjiang 212000Jiangsu ProvinceChina Department of Nephrology Zhenjiang First People’s HospitalZhenjiang 212000Jiangsu ProvinceChina

BACKGROUND To retrospectively report the safety and efficacy of renal transcatheter arterial embolization for treating autosomal dominant polycystic kidney disease(ADPKD)patients with gross *** SUMMARY The purpose of this study is to retrospectively report the safety and efficacy of renal transcatheter arterial embolization for treating ADPKD patients with gross *** and methods:During the period from January 2018 to December 2019,renal transcatheter arterial embolization was carried out on 6 patients with polycystic kidneys and gross *** arteriography was performed first,and then we determined the location of the hemorrhage and performed embolization under digital subtraction angiography *** in routine blood test results,routine urine test results,urine color and postoperative reactions were observed and ***:Renal transcatheter arterial embolization was successfully conducted in 6 *** indices of 5 patients and the color of gross hematuria improved after surgery compared with before *** severe complication reactions *** For autosomal dominant polycystic kidney syndrome patients with gross hematuria,transcatheter arterial embolization was safe and effective.

关键词： Renal artery Autosomal dominant polycystic kidney disease Gross hematuria Interventional radiology Embolization Case report

Divergent driving mechanisms of community temporal stability in China's drylands

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Environmental Science and Ecotechnology 2024年第4期20卷 237-246页

作者： Kai Wang Cong Wang Bojie fu Jianbei Huang Fangli wei Xuejing Leng Xiaoming Feng Zongshan Li wei Jiang State Key Laboratory of Urban and Regional Ecology Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing100085China College of Resources and Environment University of Chinese Academy of SciencesBeijing100049China Max Planck Institute for Biogeochemistry Hans-Kn€oll-Str.1007745JenaGermany Key Laboratory of Ecosystem Network Observation and Modeling Institute of Geographic Sciences and Natural Resources ResearchChinese Academy of SciencesBeijing100101China Shaanxi Yan'an Forest Ecosystem National Observation and Research Station Beijing100085China National Observation and Research Station of Earth Critical Zone on the Loess Plateau in Shaanxi Xi'an710061China

Climate change and anthropogenic activities are reshaping dryland ecosystems globally at an unprecedented pace,jeopardizing their *** stability of these ecosystems is crucial for maintaining ecological balance and supporting local ***,the mechanisms governing their stability are poorly understood,largely due to the scarcity of comprehensive field *** we show the patterns of community temporal stability and its determinants across an aridity spectrum by integrating a transect survey across China's drylands with remote *** results revealed a U-shaped relationship between community temporal stability and aridity,with a pivotal shift occurring around an aridity level of *** less arid areas(aridity level below 0.88),enhanced precipitation and biodiversity were associated with increased community productivity and ***,in more arid zones(aridity level above 0.88),elevated soil organic carbon and biodiversity were linked to greater fluctuations in community productivity and reduced *** study identifies a critical aridity threshold that precipitates significant changes in community stability in China's drylands,underscoring the importance of distinct mechanisms driving ecosystem stability in varying aridity *** insights are pivotal for developing informed ecosystem management and policy strategies tailored to the unique challenges of dryland conservation.

关键词： Dryland ecosystems Community stability Ecosystem management Species richness Aridity threshold

Highly Integrated Perovskite Solar Cells-Based Photorechargeable System with Excellent Photoelectric Conversion and Energy Storage Ability

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Energy & Environmental Materials 2024年第5期7卷 336-344页

作者： Jinxin Bi Shaoyin Li Dongtao Liu Bowei Li Kai Yang Ming Xu Chaopeng fu Yunlong Zhao wei Zhang Advanced Technology Institute University of Surrey School of Materials Science and Engineering Shanghai Jiao Tong University Dyson School of Design Engineering Imperial College London National Physical Laboratory

Perovskite solar cells have emerged as a promising technology for renewable energy generation. However, the successful integration of perovskite solar cells with energy storage devices to establish high-efficiency and long-term stable photorechargeable systems remains a persistent challenge. Issues such as electrical mismatch and restricted integration levels contribute to elevated internal resistance, leading to suboptimal overall efficiency (ηoverall) within photorechargeable systems. Additionally, the compatibility of perovskite solar cells with electrolytes from energy storage devices poses another significant concern regarding their stability. To address these limitations, we demonstrate a highly integrated photorechargeable system that combines perovskite solar cells with a solid-state zinc-ion hybrid capacitor using a streamlined process. Our study employs a novel ultraviolet-cured ionogel electrolyte to prevent moisture-induced degradation of the perovskite layer in integrated photorechargeable system, enabling perovskite solar cells to achieve maximum power conversion efficiencies and facilitating the monolithic design of the system with minimal energy loss. By precisely matching voltages between the two modules and leveraging the superior energy storage efficiency, our integrated photorechargeable system achieves a remarkable ηoverallof 10.01%while maintaining excellent cycling stability.

关键词： ionogel electrolyte perovskite solar cells photorechargeable system self-powered electronics zinc-ion hybrid capacitor

Highly Stretchable and Tunable Thermo-fluorochromic Polymer Elastomer through Eu^(3+)Dynamic Coordination Cross-linking

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Chinese Journal of Polymer Science 2024年第10期42卷 1449-1458,I0008页

作者： Qiu-Li Tan Kai Gou Jing-Zhi Tang Ming-Hui wei Chong Wang Yi-Jing Nie Geng-sheng Weng School of Materials Science and Chemical Engineering State Key Laboratory Base of Novel Functional Materials and Preparation ScienceNingbo UniversityNingbo315211China Institute of Polymer Materials School of Materials Science and EngineeringJiangsu UniversityZhenjiang212013China

Thermochromic polymers with tunable thermochromism,high stretchability and mechanical strength are of interests for optical information storage and *** this work,we demonstrate a new design of thermo-fluorochromic carboxylated nitrile butadiene rubber(XNBR)elastomer cross-linked by Eu^(3+)-COOH dynamic coordination with deprotonated imidazole(DPIm)as the ancillary *** presence of DPIm not only improves the mechanical strength and stretchability,but also dramatically intensifies the fluorescence emission and lifetime of the Eu-containing *** elastomer behaves reversible thermo-fluorochromism with easily tunable transition temperature and emission intensity by the simple change of the deprotonation degree of *** facile tunable thermo-fluorochromism,exceptional mechanical strength,and high stretchability(up to about 5000%)enable the Eu-containing XNBR elastomer with potential applications in soft electronics where optical information storage and encryption are required.

关键词： Dynamic coordination Thermochromism Highly stretchable Elastomer Europium