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A new perspective to develop regiorandom polymer acceptors with high active layer ductility,excellent device stability,and high efficiency approaching 17%

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Carbon Energy 2023年第2期5卷 216-224页

作者： Qunping Fan Ruijie Ma Wenyan Su Qinglian Zhu Zhenghui Luo Kai Chen Yabing Tang francis RLin Yuxiang Li He Yan Chuluo Yang Alex K.-Y.jen Wei Ma State Key Laboratory for Mechanical Behavior of Materials Xi'an Jiaotong UniversityXi'anShaanxiChina Department of Chemistry Hong Kong University of Science and TechnologyKowloonHong KongChina School of Materials Science and Engineering Xi'an University of Science and TechnologyXi'anShaanxiChina Shenzhen Key Laboratory of Polymer Science and Technology Shenzhen UniversityShenzhenGuangdongChina Department of Chemistry City University of Hong KongKowloonHong KongChina

The recently reported efficient polymerized small-molecule acceptors(PSMAs)usually adopt a regioregular backbone by polymerizing small-molecule acceptors precursors with a low-reactivity 5-brominated 3-(dicyanomethylidene)indan-1-one(IC)end group or its derivatives,leading to low molecular weight,and thus reduce active layer mechanical ***,a series of newly designed chlorinated PSMAs originating from isomeric IC end groups are developed by adjusting chlorinated positions and copolymerized sites on end groups to achieve high molecular weight,favorable intermolecular interaction,and improved physicochemical *** with regioregular PY2Se-Cl-o and PY2Se-Cl-m,regiorandom PY2Se-Cl-ran has a similar absorption profile,moderate lowest unoccupied molecular orbital level,and favorable intermolecular packing and crystallization ***,the binary PM6:PY2Se-Cl-ran blend achieves better ductility with a crack-onset strain of 17.5% and improved power conversion efficiency(PCE)of 16.23% in all-polymer solar cells(all-PSCs)due to the higher molecular weight of PY2Se-Cl-ran and optimized blend morphology,while the ternary PM6:j71:PY2Se-Cl-ran blend offers an impressive PCE approaching 17% and excellent device stability,which are all crucial for potential practical applications of all-PSCs in wearable *** date,the efficiency of 16.86% is the highest value reported for the regiorandom PSMAs-based all-PSCs and is also one of the best values reported for the *** work provides a new perspective to develop efficient all-PSCs,with all high active layer ductility,impressive PCE,and excellent device stability,towards practical applications.

关键词： all-polymer solar cells chlorination ductility power conversion efficiency regiorandom polymer acceptors

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Blockade of Endogenous Angiotensin-(1–7) in Hypothalamic Paraventricular Nucleus Attenuates High Salt-Induced Sympathoexcitation and Hypertension

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Neuroscience Bulletin 2019年第1期35卷 47-56页

作者： Xiao-jing Yu Yu-Wang Miao Hong-Bao Li Qing Su Kai-Li Liu Li-Yan Fu Yi-Kang Hou Xiao-Lian Shi Ying Li jian-jun Mu Wen-Sheng Chen Wei Cui Guo-Qing Zhu Philip j.Ebenezer joseph francis Yu-Ming Kang Department of Physiology and Pathophysiology Xi’an Jiaotong University School of Basic Medical SciencesKey Laboratory of Environment and Genes Related to DiseasesMinistry of EducationXi’an 710061China Comparative Biomedical Sciences School of Veterinary MedicineLouisiana State UniversityBaton RougeLA 70803USA Genetic Engineering Laboratory College of BiotechnologyXi’an UniversityXi’an 710065China Department of Plastic and Cosmetic Surgery Gansu Provincial HospitalLanzhou 730000China Department of Pharmacology School of Basic Medical SciencesXi’an Jiaotong University Health Science CenterXi’an 710061China Department of Cardiovascular Medicine First Affiliated Hospital of the Medical College of Xi’an Jiaotong UniversityXi’an 710061China Department of Cardiovascular Surgery Xijing HospitalFourth Military Medical UniversityXi’an 710032China Department of Endocrinology and Metabolism The First Affiliated Hospital of Xi’an Jiaotong UniversityXi’an Jiaotong University Health Science CenterXi’an 710061China Key Laboratory of Cardiovascular Disease and Molecular Intervention Department of PhysiologyNanjing Medical UniversityNanjing 210029China

Angiotensin(Ang)-(1–7) is an important biologically-active peptide of the renin-angiotensin system. This study was designed to determine whether inhibition of Ang-(1–7) in the hypothalamic paraventricular nucleus(PVN) attenuates sympathetic activity and elevates blood pressure by modulating pro-inflammatory cytokines(PICs)and oxidative stress in the PVN in salt-induced hypertension. Rats were fed either a high-salt(8% NaCl) or a normal salt diet(0.3% NaCl) for 10 weeks, followed by bilateral microinjections of the Ang-(1–7) antagonist A-779 or vehicle into the PVN. We found that the mean arterial pressure(MAP), renal sympathetic nerve activity(RSNA), and plasma norepinephrine(NE) were significantly increased in salt-induced hypertensive rats. The high-salt diet also resulted in higher levels of the PICs interleukin-6, interleukin-1 beta, tumor necrosis factor alpha, and monocyte chemotactic protein-1, as well as higher gp91 phoxexpression and superoxide production in the PVN. Microinjection of A-779(3 nmol/50 nL) into the bilateral PVN of hypertensive rats not only attenuated MAP, RSNA, and NE, but also decreased the PICs and oxidative stress in the PVN. These results suggest that the increased MAP and sympathetic activity in salt-induced hypertension can be suppressed by blockade of endogenous Ang-(1–7) in the PVN, through modulation of PICs and oxidative stress.

关键词： High-salt diet Hypertension Angiotensin(1–7) Paraventricular nucleus Pro-inflammatory cytokines

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供料不足对橡胶挤出性能的影响

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橡胶参考资料 1998年第3期28卷 39-43页

作者： P.j.j.francis 高桂芝

通常采用供料不足的方法来改善单螺杆挤出机的操作灵活性。例如,相同的螺杆挤出机采用供料不足法可加工大量的材料,工作特性也常常优于采用高功率利用率的挤出机。

关键词：橡胶挤出成型性能供料不足

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竹纤维增强聚双环戊二烯复合材料的研究

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塑料科技 2019年第5期47卷 21-26页

作者：梅雯陈琦陈宬 Verpoort francis 武汉理工大学材料科学与工程学院湖北武汉430070 武汉理工大学材料复合新技术国家重点实验室湖北武汉430070

将竹纤维(BF)和聚双环戊二烯(PDCPD)通过反应注塑成型制备竹纤维增强PDCPD复合材料。采用干燥法、碱处理法、硅烷偶联剂处理法分别对竹纤维进行表面改性,结合力学性能、红外光谱、扫描电镜(SEM)等分析检测手段,确定最佳竹纤维处理方法... 详细信息

将竹纤维(BF)和聚双环戊二烯(PDCPD)通过反应注塑成型制备竹纤维增强PDCPD复合材料。采用干燥法、碱处理法、硅烷偶联剂处理法分别对竹纤维进行表面改性,结合力学性能、红外光谱、扫描电镜(SEM)等分析检测手段,确定最佳竹纤维处理方法和最佳竹纤维用量。结果表明:采用硅烷偶联剂处理后的竹纤维用量为2%时,PDCPD/BF复合材料的拉伸强度、弯曲强度、冲击强度分别为49.824 MPa、99.903 MPa和94.34 j/m^2,比改性前分别提高了104.7%、61.82%和624.6%;改性后PDCPD/BF复合材料的热变形温度(HDT)达到108.2℃,比改性前提高了53.2%。

关键词：竹纤维聚双环戊二烯硅烷偶联剂复合材料力学性能热变形温度

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Isoreactive Manipulation of Bioadhesive Polymers Impacts Tissue-Specific Interactions

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journal of Biomedical Science and Engineering 2017年第5期10卷 287-303页

作者： jahid Ferdous Eva Romito Heather Doviak Alexandra Moreira Mark j. Uline francis G. Spinale Tarek Shazly College of Engineering and Computing University of South Carolina Columbia SC USA Cardiovascular Translational Research Center School of Medicine University of South Carolina Columbia SC USA Department of Cell Biology and Anatomy School of Medicine University of South Carolina Columbia SC USA WjB Dorn Veteran Affairs Medical Center Columbia SC USA

Bioadhesive polymers can serve as surgical sealants with a wide range of potential clinical applications, including augmentation of wound closure and acute induction of hemostasis. Key determinants of sealant efficacy include the strength and duration of tissue-material adhesion, as well as material biocompatibility. Canonical bioadhesive materials, however, are limited by a tradeoff among performance criteria that is largely governed by the efficiency of tissue-material interactions. In general, increasingly bioreactive materials are endowed with greater bioadhesive potential and protracted residence time, but incite more tissue damage and localized inflammation. one emergent strategy to improve sealant clinical performance is application-specific material design, with the goal of leveraging both local soft tissue surface chemistry and environmental factors to promote adhesive tissue-material interactions. We hypothesize that copolymer systems with equivalent bioreactive group densities (isoreactive) but different amounts/oxidation states of constituent polymers will exhibit differential interactions across soft tissue types. We synthesized an isoreactive family of aldehyde-mediated co-polymers, and subjected these materials to physical (gelation time), mechanical (bulk modulus and adhesion strength), and biological (in-vitro cytotoxicity and in-vivo biocompatibility) assays indicative of sealant performance. Results show that while bioadhesion to a range of soft tissue surfaces (porcine aortic adventitia, renal artery adventitia, renal cortex, and pericardium) varies with isoreactive manipulation, general indicators of material biocompatibility remain constant. Together these findings suggest that isore-active tuning of polymeric systems is a promising strategy to circumvent current challenges in surgical sealant applications.

关键词： Bioadhesion Dextran Aldehyde Soft Tissue Polymer Surgical Sealant

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保护性耕作小麦—玉米农田生态系统能流特点的研究

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生态农业研究 1995年第2期3卷 71-74页

作者：孙海国李卫任图生 francis j.Larney C.Wayne Lindwall 河北省农林科学院土壤肥料研究所石家庄050051 加拿大农业部烈桥研究站

通过在黑龙港地区主要土壤类型壤质潮土上连续3年的耕作试验,研究在不同耕作条件下农田生态系统的能流特点与能量分配的合理性。结果表明,与传统耕作制度相比,保护性耕作(免耕)能够明显提高小麦—玉米一年两作农田生态系统的能量转化率... 详细信息

通过在黑龙港地区主要土壤类型壤质潮土上连续3年的耕作试验,研究在不同耕作条件下农田生态系统的能流特点与能量分配的合理性。结果表明,与传统耕作制度相比,保护性耕作(免耕)能够明显提高小麦—玉米一年两作农田生态系统的能量转化率,能量投产比间的差异显著(P<0.01);不同耕作农田生态系统的熵变和自由能绝对值的差异均无统计学意义,但在一定程度上表明免耕增强了农田生态系统的有序性,从而提高了系统的相对生产力。

关键词：保护性耕作农田生态系统能量小麦玉米

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Intrahepatic flow diversion prior to segmental Yttrium-90 radioembolization for challenging tumor vasculature

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journal of Interventional Medicine 2022年第2期5卷 79-83页

作者： Lindsay B.Young Marcin Kolber Michael j.King Mona Ranade Vivian L.Bishay Rahul S.Patel francis S.Nowakowski Aaron M.Fischman Robert A.Lookstein Edward Kim Icahn School of Medicine at Mount Sinai Deparmnent of Dignostc Molecular and lterventionl RadiologyOne Gustave L.Levry Place Box 1234NY100296574New YorkUSA University of Teras Southwestem Medical Center Division of Vascular and Inerentional Radiology5323 Hary Hines BhvdTx753909316DallasUSA David Geffen School of Medicine at the Univerity of Calfornia-LoS Angeles Deparment of Itrentionol Radiology27235 Toumey RoadSuite 1500Califormia91355ValenciaUSA

Background: Hepatic tumors with complex vascular supply or poor relative perfusion are prone to decreased rates of objective response. This is compounded in the setting of Yttrium-90(Y90) transarterial radioembolization(TARE), which is minimally embolic and flow-dependent, relying on high threshold dose for complete ***: We describe our experience with intrahepatic flow diversion(FD) prior to TARE of hepatocellular carcinoma(HCC) with challenging vascular *** and methods: Between April 2014 and january 2020, 886 cases of coinciding MAA or TARE and bland embolization or temporary occlusion were *** embolizations performed for more routine purposes were excluded. FD was performed by bland embolization or temporary occlusion of vessels supplying non-malignant parenchyma in cases where flow was not preferential to target tumor. Lesion characteristics, vascular supply, treatment approach, angiography, and adverse events(AEs) were reviewed. Radiographic response was assessed using mRECIST ***: 22 cases of FD of focal HCC were identified. Embolics included calibrated microspheres(n = 11), microcoils(n = 4), gelfoam(n = 3), temporary balloon occlusion(n = 2) and temporary deployment of a microvascular plug(n = 1). Post-treatment SPECT-CT dosimetry coverage was concordant with target lesions in all cases. Mean follow-up was 16.7 months(1.4–45 mos). Tumor-specific response per m RECIST was 41% complete response, 50% objective response, and 59% disease control rate. No major adverse events or grade 3/4 hepatotoxicity were ***: our findings suggest that FD prior to TARE is safe and potentially effective in treating HCC with complex vascular supply or poor tumor perfusion.

关键词： embolization routine balloon

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复测水平点样本的林木株数和断面积的一致性估计

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林草资源研究 1992年第3期 78-84页

作者： francis A.Roesch ,jr.Edwin j.Green ,Charles T. Scott ,林昌庚

本文检视了Roesch等（1989）讨论的保留木生长量（S）、进界生长量（j）和时期1总量（V1）用于估计断面积和株数变化时的一致性估计值。Martin（1982）用符号明确表示出复测水平点样本中6种可能类型。“o”和“n”两类是在第1期测定时... 详细信息

本文检视了Roesch等（1989）讨论的保留木生长量（S）、进界生长量（j）和时期1总量（V1）用于估计断面积和株数变化时的一致性估计值。Martin（1982）用符号明确表示出复测水平点样本中6种可能类型。“o”和“n”两类是在第1期测定时为“在外”的（未被抽中）活立木,但在第2期测定时“在内”（被抽中）。

关键词：估计值点样本林木进界生长量协方差株数断面积复测

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黄金、美元与权力

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作者： (美)弗朗西斯·加文(francis j. Gavin)

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Co_(3)Mo_(3)N—An efficient multifunctional electrocatalyst

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The Innovation 2021年第2期2卷 40-46页

作者： Yao Yuan Samira Adimi Tiju Thomas jiacheng Wang Haichuan Guo jian Chen j.Paul Attfield francis j.DiSalvo Minghui Yang Ningbo Institute of Materials Technology and Engineering Chinese Academy of SciencesNingbo315201China Dalian Institute of Chemical Physics Chinese Academy of SciencesDalian116023China Department of Metallurgical and Materials Engineering Indian Institute of Technology Madras AdyarChennai 600036Tamil NaduIndia State Key Laboratory of High Performance Ceramics and Superfine Microstructure Shanghai Institute of CeramicsChinese Academy of SciencesShanghai200050China Centre for Science at Extreme Conditions and School of Chemistry University of EdinburghEdinburghEH93JZUK Department of Chemistry and Chemical Biology Cornell UniversityNew York14853USA

Efficient catalysts are required for both oxidative and reductive reactions of hydrogen and oxygen in sustainable energy conversion ***,current precious metal-based electrocatalysts do not perform well across the full range of reactions and reported multifunctional catalysts are all complex ***,we show that singlephase porous Co3Mo3N prepared via a facile method is an efficient and reliable electrocatalyst for three essential energy conversion reactions;oxygen evolution reaction(oER),oxygen reduction reaction(oRR),and hydrogen evolution reaction(HER)in alkaline ***3-Mo3N presents outstanding oER,oRR,and HER activity with high durability,comparable with the commercial catalysts Ruo2 for oER and Pt/C for oRR and *** practical demonstrations,Co3Mo3N gives high specific capacity(850 mA h gZn^(-1) at 10 mA cm^(-2))as the cathode in a zinc-air battery,and a low potential(1.63 V at 10 mA cm^(-2))used in a water-splitting *** of Co and Mo d-states appear to result in high oRR and HER performance,while the oER properties result from a cobalt oxide-rich activation surface *** findings will inspire further development of bimetallic nitrides as cost-effective and versatile multifunctional catalysts that will enable scalable usage of electrochemical energy devices.

关键词： ternary nitrides multifunctional electrocatalysts rechargeable Zn-air batteries water splitting

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