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Optimization of the gain in Yb^(3+)-doped cubic laser crystals of 99.99% purity

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Journal of Rare Earths 2009年第4期27卷 616-618页

作者： Georges Boulon Yannick guyot Akira Yoshikawa Physical Chemistry of Luminescent Materials University Claude Berna rd/Lyon1 UMR 5620 CNRS Bt.A.Kastler Domaine Scientifique de La Doua 69622 Villeurbanne France IMRAM Tohoku University 2-1-1 Katahira Aoba-ku Sendai 980-8577 Japan

This was an outlook on the prediction of the infrared laser potentiality from concentration dependences of the 2F5/2 experimental decay time in Yb3＋-doped solid-state crystals mainly on cubic crystals with 99.99% pur... 详细信息

关键词： ytterbium fluoride garnet sesquioxide laser crystals concentration quenching self trapping lifetime

Dissipation of S-metolachlor and butachlor in agricultural soils and responses of bacterial communities:Insights from compound-specific isotope and biomolecular analyses

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Journal of Environmental Sciences 2020年第6期32卷 163-175页

作者： Ehssan Torabi Charline Wiegert Benoit guyot Stéphane Vuilleumier Gwenael Imfeld Department of Plant Protection Faculty of Agricultural Science and EngineeringCollege of Agriculture and Natural ResourcesUniversity of TehranDaneshkadeh St.P.O.Box#***-4111KarajIran Laboratory of Hydrology and Geochemistry of Strasbourg(LHyGeS) Universitéde StrasbourgUMR 7517 CNRS/EOST1 Rue Blessig67084Strasbourg CedexFrance Génétique Moléculaire GénomiqueMicrobiologie(GMGM)Universitéde StrasbourgUMR 7156 CNRS4 Allee Konrad Roentgen67000StrasbourgFrance

The soil dissipation of the widely used herbicides S-metolachlor(SM)and butachlor(BUT)was evaluated in laboratory microcosms at two environmentally relevant doses(15 and 150μg/g)and for two agricultural soils(crop and paddy).Over 80%of SM and BUT were dissipated within 60 and 30 days,respectively,except in experiments with crop soil at 150μg/*** on compound-specific isotope analysis(CSIA)and observed dissipation,biodegradation was the main process responsible for the observed decrease of SM and BUT in the paddy *** SM,biodegradation dominated over other dissipation processes,with changes of carbon isotope ratios(Δδ13C)of up to 6.5‰after 60 days,and concomitant production of ethane sulfonic acid(ESA)and oxanilic acid(OXA)transformation *** crop soil experiments,biodegradation of SM occurred to a lesser extent than in paddy soil,and sorption was the main driver of apparent BUT *** of the 16 S rRNA gene showed that soil type and duration of herbicide exposure were the main determinants of bacterial community *** contrast,herbicide identity and spiking dose had no significant *** paddy soil experiments,a high(4:1,V/V)ESA to OXA ratio for SM was observed,and phylotypes assigned to anaerobic Clostridiales and sulfur reducers such as Desulfuromonadales and Syntrophobacterales were dominant for both *** soil microcosms,in contrast,were associated with a reverse,low(1:3,V/V)ratio of ESA to OXA for SM,and Alphaproteobacteria,Actinobacteria,and Bacillales dominated regardless of the *** results emphasize the variability in the extent and modes of SM and BUT dissipation in agricultural soils,and in associated changes in bacterial communities.

关键词： Chloroacetanilide herbicides Carbon isotope fractionation Pesticide degradation Bacterial diversity

Structural and optical studies of Yb^(3+),Er^(3+) and Er^(3+)/Yb^(3+) co-doped phosphate glasses

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Journal of Rare Earths 2013年第7期31卷 685-693页

作者： S.Hraiech M.Ferid Y.guyot G.Boulon Physical Chemistry Laboratory of Mineral Materials and Their Applications National Center of Research in Materials ScienceTechnologic Park of Borj Cedria B.P.738020 SolimanTunisia Physical Chemistry of Luminescent Materials(LPCML) University of LyonClaude Bernard/Lyon 1 UniversityUMR 5620 CNRSLa Doua69622 VilleurbanneFrance

Phosphate glass samples with various Yb2O3 and Er2O3 contents were synthesized by the conventional melt quenching technique and characterized by X-ray diffraction, IR absorption spectroscopy and Raman scattering spectroscopy. The absorption, emission spectra and fluorescence decay studies were carried out both at low and room temperatures. Results showed the existence of several sites occupied by the rare earth ions in the phosphate glass. Up-conversion and cooperative fluorescence were also discussed.

关键词： Yb3+/Er3+ co-doped phosphate glass energy transfer upconversion co-operative fluorescence rare earths

Raman and optical absorption spectroscopic investigation of Yb-Er codoped phosphate glasses containing SiO_2

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Chinese Optics Letters 2009年第1期7卷 56-59页

作者：陈尤阔温磊胡丽丽陈伟 Y.guyot G.Boulon Shanghai Institute of Optics and Fine Mechanics Chinese Academy of Sciences Physical Chemistry of Luminescent Materials University of LyonUMR CNRS 5620Villeurbanne 69622France

Yb-Er codoped Na2O-Al2O3-P2O5-xSiO2 glasses containing 0 - 20 mol% SiO2 were prepared successfully. The addition of SiO2 to the phosphate glass not only lengthens the bond between pS＋ and non-bridging oxygen but also reduces the number of P=O bond. In contrast with silicate glass in which there is only four-fold coordinated Si4＋, most probably there coexist [SiO4] tetrahedron and [SiO6] oetahedron in our glasses. Within the range of 0 - 20 mol% SiO2 addition, the stimulated emission cross-section of Era＋ ion only decreases no more than 10%. The Judd-Ofelt intensity parameters of Er3＋, Ω2 does not change greatly, but Ω4 and Ω6 decrease obviously with increasing SiO2 addition, because the bond between Er3＋ and O2- is more strongly eovalently bonded.

关键词： Absorption spectroscopy Erbium Fiber lasers Glass Oxygen Silicates Ytterbium

Determination of energy transfer and upconversion constants for Yb^(3+)/Er^(3+) codoped phosphate glass

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Chinese Optics Letters 2010年第2期8卷 190-193页

作者：冯素雅栾飞李顺光陈力王标陈伟胡丽丽 Y.guyot G.Boulon Key Laboratory of Material for High Power Lasers Shanghai Institute of Optics and Fine MechanicsChinese Academy of Sciences Physical Chemistry of Luminescent Materials University of Lyon

The energy transfer and cooperation upconversion processes are investigated in Yb3＋/Er3＋ codoped phos- phate glass. Based on the measured curves of output power versus incident power, the laser and spectroscopic parameters of the glass are fitted and analyzed. We focus on the resonant energy transfer constant k from Yb3＋ to Er3＋ as well as the cooperation upconversion coefficient Cup from 4113/2 of Era＋. The fitted k and Cup can give almost the same results for different thicknesses of glass disk with the same dop- ing concentrations. The determination of these parameters is helpful for the development of Yb3＋/Er3＋ codoped laser glass.

关键词： Determination of energy transfer and upconversion constants for Yb codoped phosphate glass Er

Smoothelin,a new marker to determine the origin of liver fibrogenic cells

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World Journal of Gastroenterology 2013年第48期19卷 9343-9350页

作者： Sébastien Lepreux Christelle guyot Fabrice Billet Chantal Combe Charles Balabaud Paulette Bioulac-Sage Alexis Desmoulière CHU Bordeaux Hopital Pellegrin Service d’Anatomie Pathologique F-33076 Bordeaux France U889 and Université Victor Segalen Bordeaux 2 F-33076 Bordeaux France Division of Clinical Pharmacology and Toxicology Department of Medicine University Hospital Zurich 8006 Zurich Switzerland Facultés de Médecine et de Pharmacie Université de Limoges EA 6309 F-87025 LimogesFrance

AIM: To explore this hypothesis that smooth muscle cells may be capable of acquiring a myofibroblastic phenotype, we have studied the expression of smoothelin in fibrotic conditions.

关键词： Smooth muscle cells, Myofibroblasts, α -smooth muscle actin, Smoothelin, Fibrosis/cirrhosis, Hepatocellular carcinoma

Measurement of iron characteristics under ramp compression

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Chinese Physics B 2017年第11期26卷 360-364页

作者：魏会冈 E Brambrink N Amadou A Benuzzi-Mounaix A Ravasio G Morard F guyot T de Rességuier N Ozaki K Miyanishi 赵刚 M Koenig Key Laboratory of Optical Astronomy National Astronomical Observatories Chinese Academy of Sciences LULI-CNRS Ecole Polytechnique CEA Université Paris-Saclay Sorbonne Universités UPMC Univ Paris 06 CNRS laboratoire d'utilisation des lasers intenses (LULI) Département de Physique Université Abdou Moumouni de Niamey Institut de Minéralogie de Physique des Matériaux et de Cosmochimie (IMPMC) Sorbonne Universités-UPMC UMR CNRS 7590Muséum National d'Histoire Naturelle Institut Pprime CNRS ENSMA Univ.Poitiers Graduate School of Engineering Osaka University

Laser-driven ramp compression was used to investigate iron characteristics along the isentropic path. The iterative Lagrangian analysis method was employed to analyze the free surface velocity profiles in iron stepped target measured with two VISARs. The onset stress for the α to ε phase transformation was determined from the sudden change in the sound velocity and was found over-pressurized compared to the static and shock results. The derived stress（26 GPa） and strain rate（up to 10-8 s^-1） are consistent with our previous experimental results. The stress-density relations were compared with those from previous ramp experiments and good agreements were found, which experimentally confirms the simulations,showing that iterative Lagrangian analysis can be applied to the ramp-compression data with weak shock.

关键词： isentropic compression iron phase transformation

Study of intracellular anabolism of 5-fluorouracil and incorporation in nucleic acids based on an LC-HRMS method

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Journal of Pharmaceutical Analysis 2021年第1期11卷 77-87页

作者： Christelle Machon Frederic Catez Nicole Dalla Venezia Floriane Vanhalle Laetitia guyot Anne Vincent Maxime Garcia Beatrice Roy Jean-Jacques Diaz Jerome Guitton Laboratoire de Chimie Analytique Faculte de Pharmacie de LyonUniversite Lyon 18 Avenue RockefellerLyon69373France Laboratoire de Biochimie et de Pharmaco-toxicologie Centre Hospitalier Lyon-SudeHCLPierre Benite69495France Inserm U1052 CNRS UMR5286 Centre de Recherche en Cancerologie de LyonF-69000 LyonFrance.Centre Leon BerardF-69008 LyonFranceUniversite de Lyon 1F-69000 LyonFrance Institut des Biomolecules Max Mousseron(IBMM) UMR 5247 CNRSUniversite de MontpellierENSCMCampus TrioletMontpellierFrance Laboratoire de toxicologie Faculte de pharmacie de Lyon8 avenue RockefellerF-69373 LyonFrance

5-Fluorouracil(5-FU)is an anticancer drug extensively used for different *** metabolic activation leads to several nucleoside and nucleotide metabolites essential to exert its cytotoxic activity on multiple cellular targets such as enzymes,DNA and *** this paper,we describe the development of a method based on liquid chromatography coupled with high resolution mass spectrometry suitable for the simultaneous determination of the ten anabolic metabolites(nucleoside,nucleotide and sugar nucleotide)of *** chromatographic separationwas optimized on a porous graphitic carbon column allowing the analysis of the metabolites of 5-FU as well as endogenous *** detection was performed on an Orbitrap■tandem mass *** of the method was verified in intracellular content and in RNA *** limit of detection was equal to 12 pg injected on column for nucleoside metabolites of 5-FU and 150 pg injected on column for mono-and tri-phosphate nucleotide *** effect was evaluated in cellular contents,DNA and RNA extracts for nucleoside and nucleotides *** method was successfully applied to i)measure the proportion of each anabolic metabolite of 5-FU in cellular contents,ii)follow the consequence of inhibition of enzymes on the endogenous nucleotide pools,iii)study the incorporation of metabolites of 5-FU into RNA and DNA,and iv)to determine the incorporation rate of 5-FUrd into 18 S and 28 S sub-units of rRNA.

关键词： 5-Fluorouracil LC-MS-HRMS Nucleotide RNA DNA Incorporation rate

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不同端基聚氨酯-丙烯酸酯复合细乳液的表征

高分子材料科学与工程 2006年第5期22卷 90-94页

作者：王春鹏储富祥金立维林明涛 guyot Alain 中国林业科学研究院林产化学工业研究所江苏南京210042 法国国家研究中心聚合物反应工程实验室法国69616

采用异佛尔酮二异氰酸酯、聚丙二醇经1,4-丁二醇扩链的聚氨酯(PU),再经过甲醇或甲基丙烯酸羟乙酯封端后溶解在丙烯酸酯单体中,超声乳化后进行自由基细乳液聚合。NCO和OCH3为端基的PU构成的复合乳液GPC谱图都呈现两个峰,DSC和FT-IR分析发... 详细信息

采用异佛尔酮二异氰酸酯、聚丙二醇经1,4-丁二醇扩链的聚氨酯(PU),再经过甲醇或甲基丙烯酸羟乙酯封端后溶解在丙烯酸酯单体中,超声乳化后进行自由基细乳液聚合。NCO和OCH3为端基的PU构成的复合乳液GPC谱图都呈现两个峰,DSC和FT-IR分析发现,复合后增加了PU软段和硬段相分离的程度。甲基丙烯酸封端的复合乳液生成交联型聚合物,PU的硬段和硬段间的氢键也受到破坏。复合聚合物膜表面元素含量和本体接近,表明复合细乳液粒子未形成核-壳型结构。

关键词：聚氯酯丙烯酸酯复合细乳液端基