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Non-genetic photoacoustic stimulation of single neurons by a tapered fiber optoacoustic emitter

Light(Science & Applications) 2021年第8期10卷 1494-1506页

作者： Linli Shi Ying Jiang fernando r.fernandez Guo Chen Lu Lan Heng-Ye Man John A.White Ji-Xin Cheng Chen Yang Department of Chemistry Boston University580 Commonwealth AvenueBostonMA 02215USA. Department of Biomedical Engineering Boston University44 Cummington MallBostonMA 02215USA. Center for Systems Neuroscience Boston University610 Commonwealth AveBostonMA 02215USA. Neurophotonics Center Photonics CenterBoston University8 St.Mary's StreetBostonMA 02215USA. Department of Electrical and Computer Engineering 8 St.Mary's StreetBostonMA 02215USA. Department of Biology Boston University5 Cummington MallBostonMA 02215USA

Neuromodulation at high spatial resolution poses great significance in advancing fundamental knowledge in the field of neuroscience and offering novel clinical ***,we developed a tapered fiber optoacoustic emitter(TFOE)generating an ultrasound field with a high spatial precision of 39.6 pm,enabling optoacoustic activation of single neurons or subcellular structures,such as axons and ***,a single acoustic pulse of sub-microsecond converted by the TFOE from a single laser pulse of 3 ns is shown as the shortest acoustic stimuli so far for successful neuron *** precise ultrasound generated by the TFOE enabled the integration of the optoacoustic stimulation with highly stable patch-clamp recording on single *** measurements of the electrical response of single neurons to acoustic stimulation,which is difficult for conventional ultrasound stimulation,have been *** coupling TFOE with ex vivo brain slice electrophysiology,we unveil cell-type-specific responses of excitatory and inhibitory neurons to acoustic *** results demonstrate that TFOE is a non-genetic single-cell and sub-cellular modulation technology,which could shed new insights into the mechanism of ultrasound neurostimulation.

关键词： emitter fiber stimulation

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Integrating Levels of Hierarchical Organization in Porous Organic Molecular Materials

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Nano-Micro Letters 2024年第5期16卷 134-153页

作者： Jesus Ferrando‑Soria Antonio fernandez Instituto de Ciencia Molecular(ICMol) Universidad de Valencia46980 ValenciaSpain School of Science Loughborough UniversityLoughborough LE113TUUK

Porous organic molecular materials(POMMs)are an emergent class of molecular-based materials characterized by the formation of extended porous frameworks,mainly held by non-covalent *** represent a variety of chemical families,such as hydrogen-bonded organic frameworks,porous organic salts,porous organic cages,C-H···πmicroporous crystals,supramolecular organic frameworks,π-organic frameworks,halogen-bonded organic framework,and intrinsically porous molecular *** some porous materials such as zeolites and metal organic frameworks,the integration of multiscale has been adopted to build materials with multifunctionality and optimized ***,considering the significant role of hierarchy in porous materials and the growing importance of POMMs in the realm of synthetic porous materials,we consider it appropriate to dedicate for the first time a critical review covering both ***,we will provide a summary of literature examples showcasing hierarchical POMMs,with a focus on their main synthetic approaches,applications,and the advantages brought forth by introducing hierarchy.

关键词： Porous organic molecular materials Hierarchy Hydrogen-bonded organic frameworks Porous cages Fullerene

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E-Commerce Fraud Detection Based on Machine Learning Techniques:Systematic Literature review

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Big Data Mining and Analytics 2024年第2期7卷 419-444页

作者： Abed Mutemi fernando Bacao NOVA Information Management School(NOVA IMS) Universidade Nova de LisboaCampus de CampolideLisboa 1070-312Portugal

The e-commerce industry’s rapid growth,accelerated by the COVID-19 pandemic,has led to an alarming increase in digital fraud and associated *** establish a healthy e-commerce ecosystem,robust cyber security and anti-fraud measures are ***,research on fraud detection systems has struggled to keep pace due to limited real-world *** in artificial intelligence,Machine Learning(ML),and cloud computing have revitalized research and applications in this *** ML and data mining techniques are popular in fraud detection,specific reviews focusing on their application in e-commerce platforms like eBay and Facebook are lacking *** reviews provide broad overviews but fail to grasp the intricacies of ML algorithms in the e-commerce *** bridge this gap,our study conducts a systematic literature review using the Preferred reporting Items for Systematic reviews and Meta-Analysis(PrISMA)*** aim to explore the effectiveness of these techniques in fraud detection within digital marketplaces and the broader e-commerce *** the current state of the literature and emerging trends is crucial given the rising fraud incidents and associated *** our investigation,we identify research opportunities and provide insights to industry stakeholders on key ML and data mining techniques for combating e-commerce *** paper examines the research on these techniques as published in the past *** the PrISMA approach,we conducted a content analysis of 101 publications,identifying research gaps,recent techniques,and highlighting the increasing utilization of artificial neural networks in fraud detection within the industry.

关键词： E-commerce Machine Learning(ML) systematic review fraud detection organized retail fraud

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Conformational dynamics as an intrinsic determinant of prion protein misfolding and neurotoxicity

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Neural regeneration research 2024年第10期19卷 2095-2096页

作者： Alessandro Cembran Pedro fernandez-Funez Department of Chemistry and Biochemistry University of Minnesota DuluthDuluthMNUSA Department of Biomedical Sciences University of Minnesota Medical SchoolDuluth CampusDuluthMNUSA

The prion protein(PrP) is the key molecular and pathological mediator of prion diseases,a heterogeneous group of brain disorders with fatal *** diseases are rare but deserve special attention because of their unique f... 详细信息

关键词： folding intrinsic dynamics

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Exploring multifaceted factors in chronic kidney disease risk: A comprehensive analysis of biochemistry, lifestyle, and inflammation in elderly Chinese individuals

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World Journal of Clinical Cases 2024年第5期12卷 1033-1035页

作者： fernando Cardona Unitat de Genètica Molecular Instituto de Biomedicina de Valencia–CSICValencia 46010Spain Centro de investigación Biomédica en red Enfermedades Neurodegenerativas(CIBErNED) Instituto de Salud Carlos IIIMadrid 28029Spain Departamento de Biotecnología Escuela Técnica Superior de Ingeniería Agronómica y del Medio Natural(ETSIAMN)Univeristat Politècnica de ValenciaValencia 46022Spain

This letter praises a recent article in the World Journal of Clinical Cases(roles of biochemistry data,lifestyle,and inflammation in identifying abnormal renal function in old Chinese),examining factors affecting abnormal renal function in elderly Chinese using advanced machine *** highlights the importance of uric acid,age,hemoglobin,body mass index,sport hours,and systolic blood *** study's holistic approach,integrating lifestyle and inflammation,offers a nuanced understanding of chronic kidney disease risk *** letter suggests exploring mechanistic pathways of hyperuricemia,the link between anemia and renal function,and the connection between body mass index and estimated glomerular filtration *** advocates investigating physical activity's impact on renal health and the independent effects of blood *** study significantly contributes to chronic kidney disease understanding,proposing avenues for further exploration and *** are extended to the authors and the journal.

关键词： Biochemistry data Lifestyle Machine learning renal function

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Biotransformation of 6:2 fluorotelomer sulfonate(6:2 FTS)in sulfur-rich media by Trametopsis cervina

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Frontiers of Environmental Science & Engineering 2024年第9期18卷 17-26页

作者： Felix Grimberg Thomas M Holsen Sujan fernando Siwen Wang Department of Civil and Environmental Engineering Clarkson UniversityPotsdamNew York 13699USA

Biotransformation of 6:2 fluorotelomer sulfonate(6:2 FTS)by two species of white-rot fungi,Pleurotus ostreatus(***)and Trametopsis cervina(***),was investigated in a sulfurrich medium designed to stimulate production of lignin-degrading *** of 6:2 FTS was observed by *** over the study period of 30 d,but not by *** rates were comparable to those found in other studies investigating mixed culture degradation in nonsulfur limiting media,with approximately 50 mol%of applied 6:2 FTS removed after 30 *** transformation products were short-chain perfluorocarboxylic acids(PFCAs),including PFHxA(2.27 mol%),PFPeA(0.24 mol%),and PFBA(0.28 mol%).The main intermediate products include 5:2 sFTOH(16.3 mol%)and 5:3 FTCA(2.99 mol%),while 6:2 FTCA,6:2 FTuCA,and 5:2 ketone were also identified at low *** 60 mol%of detected products were assigned to the major pathway to 5:2 ketone,and 40 mol%were assigned to the minor pathway to 5:3 *** overall molar balance was found to decrease to 75 mol%by Day 30,however,was closed to near 95 mol%with a theoretical estimation for the volatile intermediates in the headspace,5:2 ketone and 5:2 *** different capabilities of the two white-rot fungal species for 6:2 FTS biotransformation in sulfur-rich media suggest that the enzyme processes of *** to de-sulfonate 6:2 FTS may be unrelated to sulfur metabolism.

关键词： White-rot fungus 6:2 fluorotelomer sulfonate(6:2 FTS) Biotransformation Sulfur-rich medium Intermediate products

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Pioneering the direct large-scale laser printing of flexible“graphenic silicon”self-standing thin films as ultrahigh-performance lithium-ion battery anodes

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Carbon Energy 2024年第7期6卷 26-40页

作者： Avinash Kothuru Adam Cohen Gil Daffan Yonatan Juhl fernando Patolsky School of Chemistry Faculty of Exact SciencesTel Aviv UniversityTel AvivIsrael Department of Materials Science and Engineering The Iby and Aladar Fleischman Faculty of EngineeringTel Aviv UniversityTel AvivIsrael

recent technological advancements,such as portable electronics and electric vehicles,have created a pressing need for more efficient energy storage ***-ion batteries(LIBs)have been the preferred choice for these applications,with graphite being the standard anode material due to its ***,graphite falls short of meeting the growing demand for higher energy density,possessing a theoretical capacity that lags *** address this,researchers are actively seeking alternative materials to replace graphite in commercial *** promising avenue involves lithiumalloying materials like silicon and phosphorus,which offer high theoretical ***-silicon composites have emerged as a viable option,showing improved capacity and performance over traditional graphite or pure silicon ***,the existing methods for synthesizing these composites remain complex,energy-intensive,and costly,preventing widespread adoption.A groundbreaking approach is presented here:the use of a laser writing strategy to rapidly transform common organic carbon precursors and silicon blends into efficient“graphenic silicon”composite thin *** films exhibit exceptional structural and energy storage *** resulting three-dimensional porous composite anodes showcase impressive attributes,including ultrahigh silicon content,remarkable cyclic stability(over 4500 cycles with∼40%retention),rapid charging rates(up to 10 A g^(-1)),substantial areal capacity(>5.1 mAh cm^(-2)),and excellent gravimetric capacity(>2400 mAh g^(-1) at 0.2 A g^(-1)).This strategy marks a significant step toward the scalable production of high-performance LIB *** widely available,cost-effective precursors,the laser-printed“graphenic silicon”composites demonstrate unparalleled performance,potentially streamlining anode production while maintaining exceptional *** innovation not only paves the way for advanced LIBs but also sets a precedent for

关键词： 4D printing energy storage fast-charging laser-induced graphene lithium-ion silicon carbon composite anodes

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Potential of Bamboo Species Guadua trinii and Guadua angustifolia for Nanocellulose Production

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Journal of renewable Materials 2024年第9期12卷 1541-1555页

作者： Agatha E.r.Prado Gárate fernando E.Felissia María Cristina Area Teresa Suirezs María Evangelina Vallejos Círculo de Investigación del Bambú Universidad Nacional Agraria La Molina(UNALM)Lima15026Perú Instituto de Materiales de Misiones(IMAM) Universidad Nacional de Misiones(UNaM)Consejo Nacional de Investigaciones Científicas y Técnicas(CONICET)Facultad de Ciencias ExactasQuímicas y Naturales(FCEQYN)Programa de Celulosa y Papel(PROCyP)Posadas3300Argentina Instituto de Materiales de Misiones(IMAM) Universidad Nacional de Misiones(UNaM)Consejo Nacional de Investigaciones Científicas y Técnicas(CONICET)Facultad de Ciencias Forestales(FCF)Eldorado3380Argentina

Non-traditional lignocellulosic materials are a significant resource for producing high-value products,including *** work studied the nanocellulose obtention from chemical pulps of the two fast-growing bamboo species,Guadua trinii,and Guadua *** pulps were produced by soda-anthraquinone(S)pulping from both autohydrolysis-pretreated(H)and unpretreated bamboo ***-pretreated(SHP)and unpretreated soda-anthraquinone(AQ)(SP)pulps were characterized by yield,Kappa number,alpha,beta,and gamma cellulose,degree of polymerization,water retention value,and *** nanocellulose was produced by a sequential chemical oxidation treatment(2,2,6,6-tetramethylpiperidine-1-oxyl,TEMPO reagent)and mechanical *** was characterized by carboxylic group content and *** results revealed that autohydrolysis pretreatment resulted in a higher hemicelluloses extraction in *** contrast,the pulping yield of unpretreated samples was higher for ***,and the soda-AQ pulps from this species exhibited better delignification than the autohydrolysis-pretreated *** crystallinity index values of the obtained pulps were high(>80%),and the alpha-cellulose contents were *** viscosities of the aqueous nanocellulose suspensions were higher for the nanocellulose solutions obtained from the unpretreated soda-AQ ***,nanocellulose from *** unpretreated soda-AQ pulps had a higher rate of carboxylic *** results of this work are significant in assessing the potential of both bamboo species as a source of high-value products within the biorefinery framework because the viscosities of the aqueous nanocellulose suspensions depend on the size and shape of *** has significant importance for industrial unit operations and potential applications.

关键词： Natural fiber Guadua angustifolia Guadua trinii soda-anthraquinone pulp nanocellulose

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Time-Series Embeddings from Language Models:A Tool for Wind Direction Nowcasting

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Journal of Meteorological research 2024年第3期38卷 558-569页

作者： Decio ALVES Fabio MENDONCA Sheikh Shanawaz MOSTAFA fernando MOrGADO-DIAS University of Madeira Campus Universitário da Penteada9020-105FunchalPortugal Interactive Technologies Institute/Laboratory for robotics and Engineering Systems and Agência regional para o Desenvolvimento da Investigação Tecnologia e InovaçãoEdif.Madeira TecnopoloCaminho da Penteada piso-29020-105FunchalPortugal

Wind direction nowcasting is crucial in various sectors,particularly for ensuring aviation operations and *** this context,the TELMo(Time-series Embeddings from Language Models)model,a sophisticated deep learning architecture,has been introduced in this work for enhanced wind-direction *** by using three years of data from multiple stations in the complex terrain of an international airport,TELMo incorporates the horizontal u(east-west)and v(north-south)wind components to significantly reduce forecasting *** a day with high wind direction variability,TELMo achieved mean absolute error values of 5.66 for 2-min,10.59 for 10-min,and 14.79 for 20-min forecasts,processed within a swift 9-ms/step *** degree-based analysis,in comparison,yielded lower performance,emphasizing the effectiveness of the u and v *** contrast,a Vanilla neural network,representing a shallow-learning approach,underperformed in all analyses,highlighting the superiority of deep learning methodologies in wind direction *** is an efficient model,capable of accurately forecasting wind direction for air traffic operations,with an error less than 20°in 97.49%of the predictions,aligning with recommended international *** model design enables its applicability across various geographical locations,making it a versatile tool in global aviation meteorology.

关键词： wind nowcasting wind components wind direction time series prediction deep learning

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‘Jelly to Joule’:Direct laser writing of sustainable jellyfish-based ‘graphenic silicon’ anodes for environmentally remediating high-performance lithium-ion batteries

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Journal of Energy Chemistry 2024年第10期97卷 553-565页

作者： Gil Daffan Adam Cohen Yuval Sharaby roman Nudelman Shachar richter fernando Patolsky Department of Materials Science and Engineering the Iby and Aladar Fleischman Faculty of Engineering Tel Aviv University School of Chemistry Faculty of Exact Sciences Tel Aviv University

The ramifications of global climate change and resource scarcities have made it imperative to re-examine the definition of sustainable energy-storage *** is crucial to recognize that not all renewable resources are inherently sustainable,and their full impact on the environment must be *** the proliferation of invasive jellyfish species wreaking havoc on marine ecosystems and economies worldwide,utilizing overabundant jellyfish as a carbon source presents an opportunity to create energy-storage systems that are both financially beneficial and environmentally ***,a comprehensive approach to sustainability also requires eco-friendly solutions throughout the entire lifecycle,from material sourcing to battery production,without compromising highperformance ***,most electrode syntheses for lithium-ion batteries(LIBs) employed are energy-intensive,multiple-steps,complex,and *** response,this work pioneers the straightforward use of low-energy laser irradiation of a jellyfish biomass/silicon nanoparticle blend to encapsulate the silicon nanoparticles in-situ within the as-forming conductive carbonized matrix,creating sustainable and additive-free composite *** self-standing anode is directly synthesized under ambient conditions and requires no ***,a laser-synthesized conductive threedimensional porous carbon/silicon composite anode from raw jellyfish biomass for LIBs is presented,displaying outstanding cyclic stability(>1000 cycles),excellent capacity retention(>50% retention after1000 cycles),exceptional coulombic efficiency(>99%),superb reversible gravimetric capacity(>2000 mAh/g),and high rate performance capability(>1.6 A/g),paving a new path to future sustainable energy production.

关键词： Biomass Carbon Jellyfish Laser Lithium Silicon Sustainable

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