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Recent progress in flexible sensors based on 2D materials

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Journal of Semiconductors 2025年第1期46卷 130-142页

作者： Xiang Li Guancheng Wu Caofeng Pan Rongrong bao School of Physics Beihang UniversityBeijing 100191China Institute of Atomic Manufacturing Beihang UniversityBeijing 100191China Beijing Institute of Nanoenergy and Nanosystems Chinese Academy of SciencesBeijing 101400China School of Nanoscience and Engineering University of Chinese Academy of SciencesBeijing 100049China

With the rapid development of the internet of things(IoT)and wearable electronics,the role of flexible sensors is becoming increasingly irreplaceable,due to their ability to process and convert information ***-dimensional(2D)materials have been widely welcomed by researchers as sensitive layers,which broadens the range and application of flexible sensors due to the advantages of their large specific surface area,tunable energy bands,controllable thickness at the atomic level,stable mechanical properties,and excellent optoelectronic *** review focuses on five different types of 2D materials for monitoring pressure,humidity,sound,gas,and so on,to realize the recognition and conversion of human body and environmental ***,the main problems and possible solutions of flexible sensors based on 2D materials as sensitive layers are summarized.

关键词： 2D materials flexible sensors layered structure solution method

Spatial Pattern and Influencing Factors of China’s Digital Trade Resilience under the Impact of Trade Frictions

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Chinese Geographical Science 2025年第1期35卷 203-216页

作者： LI Chunli ZHU Huayou bao Weiping QIN Manman School of E-Commerce Yiwu Industrial and Commercial CollegeJinhua 322000China College of Economics and Management Zhejiang Normal UniversityJinhua 321004China

In the era of the digital economy,digital trade has demonstrated strong vitality,becoming a crucial driving force for the highquality development of national and regional ***,understanding the resilience of digital trade in the face of external crises is an important *** the backdrop of Sino-US trade friction,this paper constructs a resilience index system for digital *** utilizes entropy method,kernel density estimation,and ArcGIS mapping to calculate and visually analyze the resilience of China’s digital trade from 2017 to ***,a Tobit model is constructed to explore the main influencing factors of digital trade resilience *** research findings indicate:1)temporally,during the period of Sino-US trade friction,China’s digital trade resilience shows an overall upward trend,but there are regional differences in resilience levels across the country,with a severe polarization phenomenon.2)Spatially,high resilience is observed in the eastern and central regions of China,while the western and northeastern regions exhibit low resilience.3)From a dimensional perspective,the resistance of digital trade resilience displays a spatial distribution of high values in the east and low values in the *** recovery force is aggregated along coastal areas,and the renewal force tends to aggregate along the eastern coastline.4)Factors such as economic scale,industrial structure,urbanization rate,government fiscal expenditure,and technological talents significantly promote the enhancement of digital trade *** study reveals the dynamic characteristics and influencing factors of digital trade resilience in responding to external shocks,providing theoretical basis and policy suggestions for enhancing digital trade resilience,and promoting high-quality economic development in China.

关键词： digital trade resilience trade friction resilience pattern resilience factors China

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The human limb cell atlas:charting uncharted territories and setting sail on the new voyage of limb development research

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Science Bulletin 2025年第1期70卷 10-13页

作者： bao Zhang Hongbo Zhang The Key Laboratory for Stem Cells and Tissue Engineering Ministry of EducationZhongshan School of MedicineSun Yat-sen UniversityGuangzhou 510080China Advanced Medical Technology Center The First Affiliated HospitalZhongshan School of MedicineSun Yat-sen UniversityGuangzhou 510080China Medical College of Jiaying University Meizhou 514015China The SYSU-Perfect Diary Joint Skin Science Research Laboratory Sun Yat-sen UniversityGuangzhou 510080China

The vertebrate limb development serves as an excellent model in morphology,developmental biology,and evolutionary studies owing to its remarkable morphological and functional *** and hindlimbs originate from the lateral plate mesoderm(LPM),located along the embryo’s flank,with the initiation of differential expression of the transcription factors TBX5 for the forelimb and TBX4 and PITX1 for the ***,limbs emerge as small buds comprising an undifferentiated mesodermal core covered by a layer of ectoderm[1].

关键词： limbs limb remarkable

Visible-light-responsive homologous heterostructure of oxynitrides constructed to boost charge separation and water splitting

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Science China Chemistry 2025年第1期68卷 186-191页

作者： Hai Zou Yunfeng bao Xueshang Xin Yu Qi Tengfeng Xie Fuxiang Zhang State Key Laboratory of Catalysis Dalian National Laboratory for Clean EnergyDalian Institute of Chemical PhysicsChinese Academy of SciencesDalian 116023China School of Chemistry and Chemical Engineering Liaoning Normal UniversityDalian 116029China College of Chemistry Jilin UniversityChangchun 130012China

Constructing typeⅡheterostructures represents a widely recognized strategy for enhancing charge separation and photocatalytic efficiency,but it remains challenging to fabricate homologous heterostructures based on visible-light-responsive semiconductors,especially for popularly investigated(oxy)nitrides with low thermal ***,we synthesized a homologous heterostructure(denoted as YTON_H)based on the oxynitrides of YTaO_(4-x)N_(y)and YTa ON_(2).This heterostructure exhibits type Ⅱ band structure alignment and intimate interface achieved through a magnesium(Mg)powder-assisted nitridation *** with widely reported heterologous heterostructures,the as-obtained YTON_H homologous heterostructure could similarly exhibit enhanced charge separation as well as photocatalytic water splitting performance with respect to its counterparts(YTaO_(4-x)N_(y)and YTaON_(2)).Meanwhile,detailed structural characterizations and spectroscopy analysis have been made to confirm the formation of heterostructure and promotion of spatial charge separation.

关键词： charge separation heterostructure oxynitride photocatalysis visible light

Advances in enhancing hydrodeoxygenation selectivity of lignin-derived oxygenates:From synthetic strategies to fundamental techniques

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Green Energy & Environment 2025年第2期10卷 292-321页

作者： Xinru Wu Hongwei Zhang Cejun Hu Xiaojun bao Pei Yuan National Engineering Research Center of Chemical Fertilizer Catalyst College of Chemical EngineeringFuzhou UniversityFuzhou350002China College of Materials Science and Engineering Fuzhou UniversityFuzhou350108China Qingyuan Innovation Laboratory Quanzhou362801China

In recent years,studies focusing on the conversion of renewable lignin-derived oxygenates(LDOs)have emphasized their potential as alternatives to fossil-based ***,LDOs,existing as complex aromatic mixtures with diverse oxygen-containing functional groups,pose a challenge as they cannot be easily separated via distillation for direct utilization.A promising solution to this challenge lies in the efficient removal of oxygen-containing functional groups from LDOs through hydrodeoxygenation(HDO),aiming to yield biomass products with singular ***,the high dissociation energy of the carbon-oxygen bond,coupled with its similarity to the hydrogenation energy of the benzene ring,creates a competition between deoxygenation and benzene ring *** hydrogen consumption and lignin properties,the preference is directed towards generating aromatic hydrocarbons rather than saturated ***,the goal is to selectively remove oxygen-containing functional groups while preserving the benzene ring *** on LDOs conversion have indicated that the design of active components and optimization of reaction conditions play pivotal roles in achieving selective deoxygenation,but a summary of the correlation between these factors and the reaction mechanism is *** review addresses this gap in knowledge by firstly summarizing the various reaction pathways for HDO of *** explores the impact of catalyst design strategies,including morphology modulation,elemental doping,and surface modification,on the adsorption-desorption dynamics between reactants and ***,we delve into the application of advanced techniques such as spectroscopic techniques and computational modeling,aiding in uncovering the true active sites in HDO reactions and understanding the interaction of reactive reactants with catalyst ***,fundamental insights into selective deoxygenation obtained through these techniqu

关键词： Hydrodeoxygenation Lignin-derived oxygenates Targeted deoxidation Catalyst design Techniques and theoretical calculation

Role of iron ore in enhancing gasification of iron coke:Structural evolution,influence mechanism and kinetic analysis

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International Journal of Minerals,Metallurgy and Materials 2025年第1期32卷 58-69页

作者： Jie Wang Wei Wang Xuheng Chen Junfang bao Qiuyue Hao Heng Zheng Runsheng Xu School of Chemistry and Materials Science Hubei Engineering UniversityXiaogan 432000China Key Laboratory for Ferrous Metallurgy and Resources Utilization of Ministry of Education Wuhan University of Science and TechnologyWuhan 430081China Institue of Ironmaking Technology Baosteel Central Research InstituteShanghai 201999China State Key Laboratory of Advanced Metallurgy University of Science and Technology BeijingBeijing 100083China

The utilization of iron coke provides a green pathway for low-carbon *** uncover the influence mechanism of iron ore on the behavior and kinetics of iron coke gasification,the effect of iron ore on the microstructure of iron coke was ***,a comparative study of the gasification reactions between iron coke and coke was conducted through non-isothermal thermogravimetric *** findings indicate that compared to coke,iron coke exhibits an augmentation in micropores and specific surface area,and the micropores further extend and *** provides more adsorption sites for CO_(2) molecules during the gasification process,resulting in a reduction in the initial gasification temperature of iron *** the heating rate in non-isothermal gasification can enhance the reactivity of iron *** metallic iron reduced from iron ore is embedded in the carbon matrix,reducing the orderliness of the carbon structure,which is primarily responsible for the heightened reactivity of the carbon *** kinetic study indicates that the random pore model can effectively represent the gasification process of iron coke due to its rich pore ***,as the proportion of iron ore increases,the activation energy for the carbon gasification gradually decreases,from 246.2 kJ/mol for coke to 192.5 kJ/mol for iron coke 15wt%.

关键词： low-carbon ironmaking iron coke gasification structural evolution kinetic model

Interpretable Machine Learning-Based Spring Algal Bloom Forecast Model for the Coastal Waters of Zhejiang

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Journal of Ocean University of China 2025年第1期24卷 1-12页

作者： HUANG Guoqiang bao Min ZHANG Zhao GU Dongming LIANG Liansong TAO Bangyi State Key Laboratory of Satellite Ocean Environment Dynamics Second Institute of OceanographyMinistry of Natural ResourceHangzhou 310012China Wenzhou Marine Center Ministry of Natural ResourcesWenzhou 325000China Observation and Research Station of Yangtze River Delta Marine Ecosystems Ministry of Natural ResourcesZhoushan 316000China Key Laboratory of Marine Ecological Monitoring and Restoration Technologies Ministry of Natural ResourceShanghai 201206China

The 2016–2022 monitoring data from three ecological buoys in the Wenzhou coastal region of Zhejiang Province and the dataset European Centre for Medium-Range Weather Forecasts were examined to clarify the elaborate relationship between variations in ecological parameters during spring algal bloom incidents and the associated changes in temperature and wind fields in this study.A long short-term memory recurrent neural network was employed,and a predictive model for spring algal bloom in this region was *** model integrated various inputs,including temperature,wind speed,and other pertinent variables,and chlorophyll concentration served as the primary output *** model training used chlorophyll concentration data,which were supplemented by reanalysis and forecast temperature and wind field *** model demonstrated proficiency in forecasting next-day chlorophyll concentrations and assessing the likelihood of spring algal bloom occurrences using a defined chlorophyll concentration *** historical validation from 2016 to 2019 corroborated the model's accuracy with an 81.71%probability of correct prediction,which was further proven by its precise prediction of two spring algal bloom incidents in late April 2023 and early May *** interpretable machine learning-based model for spring algal bloom prediction,displaying effective forecasting with limited data,was established through the detailed analysis of the spring algal bloom mechanism and the careful selection of input *** insights gained from this study offer valuable contributions to the development of early warning systems for spring algal bloom in the Wenzhou coastal area of Zhejiang Province.

关键词： spring algal bloom forecast LSTM interpretable

Quantum public-key crypto via EPR pairs

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Science China(Physics,Mechanics & Astronomy) 2025年第1期68卷 54-59页

作者： Xiang-Qun Fu Hong-Wei Li Jian-Hong Shi Tan Li Wan-Su bao Henan Key Laboratory of Quantum Information and Cryptography Information Engineering UniversityZhengzhou 450004China Synergetic Innovation Center of Quantum Information and Quantum Physics University of Science and Technology of ChinaHefei 230026China

With the development of quantum computing technology,quantum public-key cryptography is gradually becoming an alternative to the existing classical public-key *** paper designs a quantum trapdoor one-way function via EPR pairs and quantum *** on this,a new quantum public-key cryptosystem is presented,which offers forward security,and can resist the chosen-plaintext attack and chosen-ciphertext *** with the existing quantum public-key cryptos,eavesdropping can be automatically detected in this new quantum public-key cryptosystem under a necessary condition,which is also detailed in the paper.

关键词： quantum public-key crypto trapdoor one-way function EPR pairs

Biisoindolylidene solvatochromic fluorophores: Synthesis and photophysical properties

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Chinese Chemical Letters 2025年第2期36卷 394-399页

作者： Xiaoyu Chen Jiahao Hu Jingyi Lin Haiyang Huang Changqing Ye Hongli bao College of Chemistry Fuzhou University State Key Laboratory of Structural Chemistry Key Laboratory of Coal to Ethylene Glycol and Its Related TechnologyCenter for Excellence in Molecular SynthesisFujian Science&Technology Innovation Laboratory for Optoelectronic Information of China Fujian College University of Chinese Academy of SciencesFuzhou 350002China dUniversity of Chinese Academy of Sciences

Environment-sensitive fluorescent probes are commonly utilized in various fields, including fluorescence sensing and imaging. This paper describes the synthesis and photophysical properties of a novel class of solvatochromic fluorophores that incorporate biisoindolylidene as the core backbone. This study investigates the structure-property relationships of these newly developed fluorophores. The central biisoindolylidene acts as an efficient electron acceptor, and by modifying the aryl ring substituent at the 3,3 position, the photophysical properties of the fluorophores can be significantly enhanced, particularly in terms of photoluminescence quantum efficiency. Furthermore, when an electron-donor group replaces the aryl ring at the 3,3 position, intriguing solvatochromic behavior is observed. This leads to a red-shift in the maximum emission wavelength and an increase in the Stokes shift with increasing solvent polarity. In solvent dimethyl sulfoxide(DMSO), the maximum emission wavelength can reach up to 750 nm,with a Stokes shift of approximately 150 nm. Finally, the potential application of the fluorophore in the detection of volatile acids is explored in a preliminary manner.

关键词： Acid sensitive Biisoindolylidene Electron receptor New fluorophores Solvatochromic