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Liquid-mediated Ostwald ripening of Ag-based clusters supported on oxides

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Nano Research 2024年第6期17卷 4971-4978页

作者： Conghui Liu Rongtan Li Yamei Fan Shiwen Li Xiaohui feng Lu feng Yanxiao Ning Qiang Fu School of Chemistry Dalian University of TechnologyDalian 116024China State Key Laboratory of Catalysis Chinese Academy of SciencesDalian Institute of Chemical PhysicsDalian 116023China

Reconstruction of supported nanocatalysts often occurs in gas-solid reactions and significantly affects the catalytic performance,yet it is much less explored in liquid-phase ***,we find that highly-dispersed Ag nanocatalysts,i.e.,AgOx clusters,supported on alumina,silica,and titania,can aggregate into larger Ag or Ag2. particles after immersing in liquid-phase media at room *** spontaneous aggregation of AgOx clusters in liquid water is attributed to liquid-phase Ostwald ripening through dissolution of AgOx clusters into water and subsequent redeposition to form Ag2. *** immersion into organic solvents such as ethanol leads to reduction of AgOx clusters and further growth into Ag *** work reveals that liquid-phase reaction media can induce substantial structural evolution of supported nanostructured catalysts,which should be carefully considered in liquid-solid interface catalytic reactions such as electrocatalysis,environmental catalysis,and organic synthesis in liquid phase.

关键词： Ag catalysts Ostwald ripening liquid phase media dissolution-deposition process

Upcycling electroplating sludge into bioengineering-enabled highly stable dual-site Fe-Ni_(2.P@C electrocatalysts for efficient oxygen evolution

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Nano Research 2024年第8期17卷 6984-6992页

作者： Jiawen Liu Zunpeng Zuo feng Gao Kai Yi Jiahui Lin Mengye Wang Zhang Lin feng Huang State Key Laboratory of Optoelectronic Materials and Technologies School of MaterialsSun Yat-Sen UniversityGuangzhou 510275China Department of Chemistry City University of Hong KongHong Kong 999077China School of Metallurgy and Environment Central South UniversityChangsha 410083China Ganjiang Innovation Academy Chinese Academy of SciencesGanzhou 341000China

The advancement of bimetallic catalysts holds significant promise for the innovation of oxygen evolution reaction(OER)*** from adsorbate evolution mechanism(AEM)and lattice oxygen oxidation mechanism(LOM),the incorporation of dual active sites has the potential to foster novel OER pathways,such as the coupled oxygen evolution mechanism(COM),which can surpass the limitations of OER and elevate catalytic *** this study,uniformly distributed Fe/Ni dual-site Fe-Ni_(2.P@C electrocatalysts are crafted by upcycling metals in electroplating sludge via an eco-friendly and sustainable microbial engineering *** findings indicate that a substantial number of defects emerge at the Ni2. crystal during the OER process,laying the groundwork for lattice oxygen ***,the displacement of Ni/Fe in the crystal lattice intensifies the asymmetry of the electronic structure at the metal active sites,facilitating the deprotonation *** research introduces an innovative paradigm for the synthesis of effective and robust transition metal-based OER catalysts,with implications for sustainable energy generation technologies.

关键词： oxygen evolution reaction dual active sites adsorbate evolution mechanism lattice oxygen mechanism bioengineering

Effects and mechanisms of acupuncture on women related health

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Frontiers of Medicine 2024年第1期18卷 46-67页

作者： Huichao Qin Jiaxing feng Xiaoke Wu Department of Reproductive Medicine Heilongjiang Provincial HospitalHarbin Institute of TechnologyHarbin150036China Department of Obstetrics and Gynecology First Affiliated HospitalHeilongjiang University of Chinese MedicineHarbin150040China

Globally,public health interventions have resulted in a 30-year increase in women’s life ***,women’s health has not increased when socioeconomic status is ***’s health has become a major public health concern,for those women from developing countries are still struggling with infectious and labor-related diseases,and their counterparts in developed countries are suffering from physical and psychological *** recent years,complementary and alternative medicine has attracted wide attentions with regards to maintaining women’s ***,a crucial component of traditional Chinese medicine,has been used to treat many obstetric and gynecological diseases for thousands of years due to its analgesic and anti-inflammatory effects and its effects on stimulating the sympathetic/parasympathetic nervous *** fully understand the mechanism through which acupuncture exerts its effects in these diseases would significantly extend the list of available interventions and would allow for more reasonable advice to be given to general ***,by searching PubMed and CNKI regarding the use of acupuncture in treating obstetric and gynecological diseases,we aimed to summarize the proven evidence of using acupuncture in maintaining women’s health by considering both its effectiveness and the underlying mechanisms behind its effects.

关键词： acupuncture women health clinical efficacy mechanism

Development of high-power microwave mechanical integrated continuous mining device

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Journal of Rock Mechanics and Geotechnical Engineering 2024年第9期16卷 3365-3377页

作者： Xia-Ting feng feng Lin Jiuyu Zhang Chengxiang Yang Yuntan Ao Tianyang Tong Key Laboratory of Ministry of Education on Safe Mining of Deep Metal Mines Northeastern UniversityShenyang110819China Key Laboratory of Liaoning Province on Deep Engineering and Intelligent Technology Northeastern UniversityShenyang110819China

This article introduces a high-power microwave mechanical integrated continuous mining device,which can achieve synchronous cutting of hard rocks by microwave and *** device includes a cutting system,a rotary translation system,a loading system,a high-power microwave system,and a control and monitoring *** technology of“master-slave follow-up”disc cutter alternating side cutting of rock was proposed,which could improve the effectiveness of rock *** integrated structure of a microwave-cut system was then proposed,and synchronous motion of the microwave-cut system and adjustment of the loading system could be *** automatic adjustment technology of the microwave working distance was developed to dynamically control the optimal microwave working *** basic functions of the equipment were verified by *** comparing the two types of disk cutters,it is found that the master-slave follow-up disk cutter can improve significantly the dust removal effect and rock breaking efficiency in rock breaking process versus the conventional large disc *** tests of slate with or without microwave were conducted using a master-slave follow-up disk *** results show that the cutting patterns of slates change from intermittent chunks(without microwave irradiation)to persistent debris(with microwave irradiation),and the cutting speed is significantly improved(170%).The development of the device provides a scientific basis for changing the conventional mining technology of metal mines and realizing the mechanical continuous mining in hard metal mines.

关键词： Hard metal mine Microwave machinery Continuous mining Master-slave follow-up disc cutter

Cloud Microphysical Characteristics of Typhoon Meranti(2.16)during Its Rapid Intensification:Model Validation and SST Sensitivity Experiments

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Journal of Meteorological Research 2024年第3期38卷 542-557页

作者： Rui WANG Yihong DUAN Jianing feng Department of Atmospheric and Oceanic Sciences&Institute of Atmospheric Sciences Fudan UniversityShanghai200438China State Key Laboratory of Severe Weather Chinese Academy of Meteorological SciencesChina Meteorological AdministrationBeijing100081China

Cloud microphysics plays an important role in determining the intensity and precipitation of tropical cyclones(TCs).In this study,a high-resolution numerical simulation by WRF(version 4.2.of Typhoon Meranti(2.16)during its rapid intensification(RI)period was conducted and validated by multi-source observations including Cloud-Sat and Global Precipitation Mission satellite *** snow and ice particles content were found to increase most rapidly compared with other hydrometeors during the RI *** all hydrometeors continued to *** graupel content only increased in the initial RI stage,and then decreased afterwards due to precipitation during the RI *** addition,sea surface temperature(SST)sensitivity experiments showed that,although the intensity of the TC increased with a higher SST,not all hydrometeors *** graupel content continued to increase with the increase in SST,mainly due to the accumulation of more lower-temperature supercooled water vapor at the corresponding *** content of snow decreased with the increase in SST because stronger vertical motion at the corresponding height affected the aggregation of ice crystals.

关键词： tropical cyclone rapid intensification cloud microphysical characteristics sea surface temperature(SST)

Beam Training and Tracking in mmWave Communication:A Survey

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China Communications 2024年第6期21卷 1-22页

作者： Wang Yi Wei Zhiqing feng Zhiyong Yangtze Delta Region Institute(Quzhou) University of Electronic Science and Technology of ChinaQuzhou 324003China School of Information and Communication Engineering University of Electronic Science and Technology of ChinaChengdu 611731China Key Laboratory of Universal Wireless Communications Ministry of EducationBeijing University of Posts and TelecommunicationsBeijing 100876China

Communicating on millimeter wave(mmWave)bands is ushering in a new epoch of mobile communication which provides the availability of 10 Gbps high data rate ***,mmWave links are easily prone to short transmission range communication because of the serious free space path loss and the blockage by *** overcome these challenges,highly directional beams are exploited to achieve robust links by hybrid *** aligning the transmitter and receiver beams,*** training,is vitally important to high data rate ***,it may cause huge overhead which has negative effects on initial access,handover,and ***,the mobility patterns of users are complicated and dynamic,which may cause tracking error and large tracking *** efficient beam tracking method has a positive effect on sustaining robust *** article provides an overview of the beam training and tracking technologies on mmWave bands and reveals the insights for future research in the 6th Generation(6G)mobile ***,some open research problems are proposed to realize fast,accurate,and robust beam training and *** hope that this survey provides guidelines for the researchers in the area of mmWave communications.

关键词： 6G beam tracking beam training beamforming mmWave

Higher-order expansions of powered extremes of logarithmic general error distribution

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Applied Mathematics(A Journal of Chinese Universities) 2024年第1期39卷 47-54页

作者： TAN Xiao-feng LI Li-hui School of Mathematics and Statistics Southwest UniversityChongqing 400715China

In this paper,Let M_(n)denote the maximum of logarithmic general error distribution with parameter v≥***-order expansions for distributions of powered extremes M_(n)^(p)are derived under an optimal choice of normalizing *** is shown that M_(n)^(p),when v=1,converges to the Frechet extreme value distribution at the rate of 1/n,and if v>1 then M_(n)^(p)converges to the Gumbel extreme value distribution at the rate of(loglogn)^(2.=(log n)^(1-1/v).

关键词： logarithmic general error distribution convergence rate higher-order expansion powered ex-treme

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军队保健医师能力素质建设

解放军医院管理杂志 2017年第6期24卷 555-558页

作者：刘畅孟晴晴冯大跃张杰冯雨来解放军第305医院医务部北京100017 中央军委机关事务管理总局保健处北京100034 中央军委政治工作部老干部服务管理局门诊部北京100036

干部保健工作不仅是医疗服务,也是政治任务,事关党、国家和军队的安定和稳定,其发展过程经历萌芽、发展、曲折中前进、壮大等几个过程,逐步形成一套科学的体系。保健医师是干部保健工作的主体,军队保健医师因保健对象的特殊性与临床医... 详细信息

干部保健工作不仅是医疗服务,也是政治任务,事关党、国家和军队的安定和稳定,其发展过程经历萌芽、发展、曲折中前进、壮大等几个过程,逐步形成一套科学的体系。保健医师是干部保健工作的主体,军队保健医师因保健对象的特殊性与临床医师相比有很大区别。但绝大多数由临床医师转来,与实际保健需求有一定差距。重视和开展军队保健医师的能力素质建设和模块化层级式培训,以符合新时期强军保健任务的需要,有利于保健医师能力的提高和技术的进步,为保健政策的制定提供科学的数据支撑。

关键词：干部保健工作保健医师能力素质

Covariate-Assisted Matrix Completion with Multiple Structural Breaks

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Journal of Systems Science & Complexity 2024年第2期37卷 692-728页

作者： MENG Jing feng Long ZOU Changliang WANG Zhaojun School of Statistics and Data Science KLMDASRLEBPSand LPMCNankai UniversityTianjin 300071China

In matrix completion,additional covariates often provide valuable information for completing the unobserved entries of a high-dimensional low-rank matrix *** this paper,the authors consider the matrix recovery problem when there are multiple structural breaks in the coefficient matrix β under the column-space-decomposition model A=Xβ+B.A cumulative sum(CUSUM)statistic is constructed based on the penalized estimation of β.Then the CUSUM is incorporated into the Wild Binary Segmentation(WBS)algorithm to consistently estimate the location of ***,a nearly-optimal recovery of A is *** findings are further corroborated via numerical experiments and a real-data application.

关键词： Additional covariates matrix completion multiple structural breaks wild Binary Segmentation