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Revealing the anti-sintering phenomenon on silica-supported nickel catalysts during CO_(2)hydrogenation

Journal of Environmental Sciences 2024年第6期140卷 270-278页

作者： Liuqingqing yang Tiancheng Pu feixiang Tian Yulian He Minghui Zhu State Key Laboratory of Chemical Engineering School of Chemical EngineeringEast China University of Science and TechnologyShanghai 200237China University of Michigan-Shanghai Jiao Tong University Joint Institute Shanghai Jiao Tong UniversityShanghai 200240China School of Chemistry and Chemical Engineering Shanghai Jiao Tong UniversityShanghai 200240China

The CO_(2)catalytic hydrogenation represents a promising approach for gas-phase CO_(2)utilization in a direct manner.Due to its excellent hydrogenation ability,nickel has been widely studied and has shown good activities in CO_(2)hydrogenation reactions,in addition to its high availability and low price.However,Ni-based catalysts are prone to sintering under elevated temperatures,leading to unstable catalytic performance.In the present study,various characterization techniques were employed to study the structural evolution of Ni/SiO_(2)during CO_(2)hydrogenation.An anti-sintering phenomenon is observed for both 9%Ni/SiO_(2)and 1%Ni/SiO_(2)during CO_(2)hydrogenation at 400℃.Results revealed that Ni species were re-dispersed into smaller-sized nanoparticles and formed Ni^(0)active species.While interestingly,this anti-sintering phenomenon leads to distinct outcomes for two catalysts,with a gradual increase in both reactivity and CH_(4)selectivity for 9%Ni/SiO_(2)presumably due to the formation of abundant surface Ni°from redispersion,while an apparent decreasing trend of CH_(4)selectivity for 1%Ni/SiO_(2)sample,presumably due to the formation of ultra-small nanoparticles that diffuse and partially filled the mesoporous pores of the silica support over time.Finally,the redispersion phenomenon was found relevant to the H_(2)gas in the reaction environment and enhanced as the H_(2)concentration increased.This finding is believed to provide in-depth insights into the structural evolution of Ni-based catalysts and product selectivity control in CO_(2)hydrogenation reactions.

关键词： Carbon dioxide utilization CO_(2)hydrogenation Nickel-based catalysts Anti-sintering Structural evolution

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Provably secure attribute-based authenticated encryption with keyword search from ideal lattices

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Science China(Information Sciences) 2024年第1期67卷 308-309页

作者： Lisha YAO Lin HOU Jian WENG feixiang ZHAO College of Cyber Security Jinan University

A public-key authenticated encryption with keyword search(PAEKS)[1, 2] system overcomes the problem of an inside adversary forging searchable ciphertexts and guessing the keyword information from the given token. This system allows the sender to encrypt and authenticate a keyword.However, traditional PAEKS schemes require the sender to specify the intended receiver in advance, losing much flexibility.

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Constructing a fluorinated interface layer enriched with Ge nanoparticles and Li-Ge alloy for stable lithium metal anodes

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Nano Research 2024年第6期17卷 5148-5158页

作者： Fulu Chu Jinwei Zhou Jiamin Liu Fengcheng Tang Liubin Song feixiang Wu School of Metallurgy and Environment Engineering Research Center of the Ministry of Education for Advanced Battery MaterialsHunan Provincial Key Laboratory of Nonferrous Value-added MetallurgyCentral South UniversityChangsha 410083China Hunan Provincial Key Laboratory of Materials Protection for Electric Power and Transportation School of Chemistry and Chemical EngineeringChangsha University of Science and TechnologyChangsha 410004China School of Materials Science&Engineering University of JinanJinan 250022China

Lithium metal batteries(LMBs)based on metallic Li exhibit high energy density to be competent for advanced energy storage applications.However,the unstable solid electrolyte interphase(SEI)layer due to continuous decomposition of electrolytes,and the attendant problem of Li dendrite growth frustrate their commercialization process.Herein,a hybrid SEI comprising abundant LiF,lithiophilic Li-Ge alloy,and Ge nanoparticles is constructed via a simple brush coating method.This fluorinated interface layer with embedded Ge-containing components isolates the Li anode from the corrosive electrolyte and facilitates homogenous Li nucleation as well as uniform growth.Consequently,the modified Li anode exhibits remarkable stability without notorious Li dendrites,delivering stable cycling lives of more than 1000 h for symmetric Li||Li cells and over 600 cycles for Li||Cu cells at 1 mA·cm^(−2).Moreover,the reinforced Li anodes endow multiple full-cell architectures with dramatically improved cyclability under different test conditions.This work provides rational guidance to design an artificial hybrid SEI layer and would stimulate more ideas to solve the dendrite issue and promote the further development of advanced LMBs.

关键词： lithium metal anode artificial solid electrolyte interphase(SEI) dendrite suppression lithium fluoride Li-Ge alloy

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There discovery of alpine oak (Heterobalanus group, Quercus section Ilex, Fagaceae) fossils from Mount Shisha Pangma and its significance

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ACTA PETROLOGICA SINICA 2024年第5期40卷 1382-1393页

作者： Su, Tao Liu, jia Chen, Linlin Huang, Jian Zhang, Xinwen Wu, feixiang Ni, Xijun Deng, Tao Zhou, Zhekun Chengdu Univ Technol Inst Sedimentary Geol MNR Key Lab Deeptime Geog & Environm Reconstruct Chengdu 610059 Peoples R China Chengdu Univ Technol State Key Lab Oil & Gas Reservoir Geol & Exploita Chengdu 610059 Peoples R China Chinese Acad Sci Xishuangbanna Trop Botan Garden CAS Key lab Trop Forest Ecol Mengla 666303 Peoples R China Univ Bristol Sch Geograph Sci Bristol BS8 1QU Avon England Chinese Acad Sci Inst Vertebrate Paleontol & Paleoanthropol CAS Key Lab Veribrate Evol & Human Origins Beijing 100044 Peoples R China

We reported alpine oak fossil leaves ( the Heterobalanus group, Quercus section Ilex, Fagaceae) rediscovered on Mount Shisha Pangma. According to twice field investigations, the fossil site is located at the front of the No. 5 glacier tongue on the south side of the Dasuopu Glacier at an altitude of about 5800m on the north slope of Shisha Pangma Peak. These fossils are from the siltstone interlayer dominated by sandy conglomerate in the lower part of the Yebokangjiale Group. These newly discovered fossil leaves have typical characteristics of alpine oaks, including oval or oblong leaf, thick and short petiole, entire or toothed leaf margin, and 5 similar to 6 pairs of secondary veins, which is completely consistent with the leaf morphology of alpine oaks from Mount Shisha Pangma reported previously. Through morphological comparison with living and fossil species in this group, as well as quantitative analysis combined with geometric morphometry, these fossil leaves from Mount Shisha Pangma were assigned to Quercus preguajavifolia Tao. Alpine oaks may originate in southeastern margin of the Qinghai -Tibetan Plateau, then thrive locally and spread into regions nearby accompanying by the uplift of the plateau. The implication of alpine oak fossil leaves from Mount Shisha Pangma on paleoelevation needs to be further investigated due to the present wide range and the uncertainty of these fossils. The rediscovery of alpine oak fossils from Mount Shisha Pangma not only helps to clarify the specific layers bearing these fossils, but also further enriches the morphological characteristics of this fossil record and its systematic position. This discovery would provide important basis for better revealing the evolution of biodiversity and environmental changes in the middle part of the Himalaya during the Cenozoic.

关键词： Heterobalanus Leaf fossil Himalaya Mountain uplift Biodiversity Neogene LATE MIOCENE TIBETAN PLATEAU ELEVATION EXHUMATION EVOLUTION HIMALAYA OROGEN UPLIFT

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Exploring the multicomponent synergy mechanism of Zuogui Wan(左归丸) on postmenopausal osteoporosis by a systems pharmacology strategy

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Journal of Traditional Chinese Medicine 2024年第3期44卷 489-495页

作者： FENG Yanchen LIU Yali DANG Xue LIN Zixuan ZHANG Yunke CHE Zhiying LI Xiang PAN Xiaolong LIU feixiang ZHENG Pan Traditional Chinese Medicine (Zhong Jing) School Henan University of Chinese Medicine Hospital of Encephalopathy the First Affiliated Hospital of Henan University of Chinese Medicine State Key Laboratory for Diagnosis and Treatment of Infectious Diseases National Clinical Research Center for Infectious DiseasesCollaborative Innovation Center for Diagnosis and Treatment of Infectious Diseasesthe First Affiliated HospitalZhejiang University School of MedicineResearch Units of Infectious Disease and MicroecologyChinese Academy of Medical Sciences

OBJECTIVE: To explore the multi-component synergistic mechanism of Zuogui Wan(左归丸, ZGW) in treating postmenopausal osteoporosis(PMOP). METHODS: The main components and target genes of ZGW were screened via the Traditional Chinese Medicine Systems Pharmacology(TCMSP). In addition, the target gene sets of PMOP were derived from the Gene Cards and Online Mendelian Inheritance in Man databases. The search tool for recurring instances of neighbouring genes(STRING) 11.0 software was used to analyze the interaction among intersecting genes. Cytoscape 3.6.1 software and the Matthews correlation coefficient(MCC) algorithm were used to screen the core genes. Fifty Sprague-Dawley female rats were randomly divided into the sham-operated(Sham) group and the four ovariectomized(OVX) subgroups. Rats subjected to Sham or OVX were administered with the vehicle(OVX, 1 m L water/100 g weight), 17β-estradiol(E2, 50 μg·kg-1·d-1), and lyophilized powder of ZGW at a low dose of 2.3(ZGW-L) and high dose of 4.6(ZGW-H) g·kg-1·d-1 for three months. The bone density and bone strength were assessed using dual-energy X-ray and three-point bending tests, respectively. Furthermore, enzyme-linked immunosorbent assay, Hematoxylin-eosin staining, and western blot analysis were used to determine the potential pharmacological mechanisms of action of ZGW in PMOP. RESULTS: A total of 117 active compounds of ZGW were screened from the TCMSP. Furthermore, 108 intersecting genes of drugs and diseases were identified. Using STRING software and the MCC algorithm, ten core genes, including C-X-C chemokine living 8(CXCL8), C-C chemokine receptor type 2(CCR2), alpha-2a active receptor(ADRA2A), melatonin receptor type 1B(MTNR1B), and amyloid-beta A4 protein(APP), were identified. The anti-osteoporosis regulation network of ZGW was constructed using the Cytoscape software. The animal experiments demonstrated that ZGW groups significantly reduced the serum levels of β-C-terminal telopeptide of type I collagen(β-CTX) and increased serum levels of bone-specific al

关键词： network pharmacology osteoporosis, postmenopausal Zuogui Wan

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Reliability and validity of the hidden hunger assessment scale in China-revised for high school students

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Global Health Journal 2023年第2期7卷 110-116页

作者： Ning Zhang Minao Wang Yuchen Zhang Huake Cao yang yang Yuhang Shi yang Pei feixiang yang Yinan Du School of Basic Medical Sciences Anhui Medical UniversityHefeiAnhui 230032China First School of Clinical Medicine Anhui Medical UniversityHefeiAnhui 230032China First Affiliated Hospital of Anhui Medical University HefeiAnhui 230022China Second School of Clinical Medicine Anhui Medical UniversityHefeiAnhui 230032China

Objective:Hidden hunger remains a severe public health problem that affects millions of people worldwide.In China,challenges related to dietary imbalance and hidden hunger persist.Micronutrient inadequacy deserves more attention among adolescents,given its vital role in their growth and development;however,this problem appears to have been largely ignored.High school students,in particular,are often at a high risk of hidden hunger but have limited assessment tools available.Therefore,this study aims to revise the hidden hunger assessment scale for high school students(HHAS-HSS)in China and assess its reliability and validity.Methods:Based on a literature review,expert consultation,pre-experiment,and formal survey,a hidden hunger assessment scale was revised for high school students.The formal survey involved 9336 high school students in 11 of the 16 cities in Anhui Province,China,and 9038 valid questionnaires were collected and included in the analysis.The item analysis,internal consistency reliability,test-retest reliability,content validity,exploratory factor analysis,and confirmatory factor analysis of the HHAS-HSS were examined.Results:The HHAS-HSS included a total of 4 dimensions and 12 items:"vegetables and food diversity"(three items),"fruits and dairy products"(three items),"micronutrient-dense foods"(four items),and"health condition and eating habits"(two items).The results showed a Cronbach's alpha of 0.758,a split-half reliability of 0.829,and a test-retest reliability of o.793,indicating good internal consistency.Using the Bartlett's test and Kaiser-Meyer-Olkin test(KMO)to test the exploratory factor analysis presented a four-factor model of the HHAS-HSS,the KMO0 value was 0.820(P<0.001),which indicated the possibility for factor confirmatory factor analysis.Using the maximum variance rotation method,four factors were obtained,and the cumulative variance explained rate was 57.974%.Confirmatory factor analysis also supported the division of the scale into four dimensions,and the fitting indices were x^

关键词： Hidden hunger Reliability and validity Assessment scale High school student Micronutrients

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Layered buserite Mg-Mn oxide cathode for aqueous rechargeable Mg-ion battery

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Journal of Magnesium and Alloys 2023年第3期11卷 840-850页

作者： Caiyun Sun Hailian Wang feixiang yang Aitao Tang Guangsheng Huang Lingjie Li Zhongting Wang Baihua Qu Chaohe Xu Shuangshuang Tan Xiaoyuan Zhou Jingfeng Wang Fusheng Pan College of Materials Science and Engineering Chongqing UniversityChongqing 400044China National Engineering Research Center for Magnesium Alloys College of Materials Science and EngineeringChongqing UniversityChongqing 400044China College of Chemistry and Chemical Engineering Chongqing UniversityChongqing 400044China College of Aerospace Engineering Chongqing UniversityChongqing 400044China College of Physics Chongqing UniversityChongqing401331China

Owing to the features(high safety,inexpensive and environmental friendliness)of aqueous rechargeable Mg-ion batteries(ARMIBs),they have drawn extensive attention in the future energy storage systems.However,the poor Mg^(2+)migration kinetics during the Mg^(2+)intercalation/extraction still hinders the progress of developing suitable cathode materials.Herein,a layered buserite Mg-Mn oxide(MMO)material with large interlayer space(~9.70A)and low-crystalline structure is studied as a high-performance cathode in ARMIBs.Compared with the counterpart,the Mg^(2+)migration kinetics of the MMO cathode can be enhanced by its unique structure(bigger interlayer spacing and low-crystalline structure).The layered buserite MMO as a high-performance ARMIBs cathode exhibits high Mg storage capacity(50 mAg^(-1):169.3 mAh g^(-1)),excellent rate capability(1000 mAg^(-1):98.3 mAh g^(-1)),and fast Mg^(2+)migration(an average diffusion coefficient:~4.21×10-^(10)cm^(2)s^(-1))in 0.5 M MgCl_(2)aqueous electrolyte.Moreover,the MMO-1//AC full battery achieved a high discharge capacity(100 mAg^(-1):111 mAh g^(-1)),and an ignored fading over 5000 cycles(1000 mAg^(-1)).Therefore,layered Mg-Mn oxide with large interlayer space may break a new path to develop the promising ARMIBs.

关键词： Layered buserite phase Low-crystalline Mg-Mn oxide Fast Mg ion migration kinetic Aqueous Mg-ion battery

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Neogene integrative stratigraphy,biotas,and paleogeographical evolution of the Qinghai-Tibetan Plateau and its surrounding areas

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Science China Earth Sciences 2024年第4期67卷 1326-1359页

作者： Tao DENG Xiaomin FANG Qiang LI Shiqi WANG feixiang WU Sukuan HOU Jiao MA Qigao JIANGZUO Danhui SUN Yan ZHENG Qinqin SHI Boyang SUN Lu LI Key Laboratory of Vertebrate Evolution and Human Origins Institute of Vertebrate Paleontology and PaleoanthropologyChinese Academy of SciencesBeijing 100044China CAS Center for Excellence in Life and Paleoenvironment Beijing 100044China University of Chinese Academy of Sciences Beijing 100049China CAS Center for Excellence in Tibetan Plateau Earth Sciences and Key Laboratory of Continental Collision and Plateau Uplift Institute of Tibetan Plateau ResearchChinese Academy of SciencesBeijing 100101China Key Laboratory of Orogenic Belts and Crustal Evolution School of Earth and Space SciencesPeking UniversityBeijing 100871China

The remarkable uplift of the Tibetan Plateau in the Neogene had great impacts on the climate and environment of East Asia and even the world.Therefore,establishment of the Neogene stratigraphic framework of the Tibetan Plateau is of great significance to research in various fields of geosciences.Based on marine sediments,the international chronostratigraphic system of the Neogene is divided into six stages in the Miocene and two stages in the Pliocene.Since the beginning of the Cenozoic,the share of terrestrial strata on continents has increased rapidly.By the Neogene,it had far exceeded that of marine strata,and almost all deposits on the Tibetan Plateau and its surrounding areas were terrestrial strata.In China,the Miocene includes five stages and the Pliocene includes two stages.Except for the Tunggurian of the Miocene,which has a lower boundary at 15 Ma,the other stages have the same paleomagnetic definitions and time intervals as the corresponding international marine stages.Mammalian fossils play a very important role in the division and correlation of Cenozoic terrestrial strata,and rodent,carnivore,proboscidean,perissodactyl and artiodactyl fossils are especially important in Neogene terrestrial biostratigraphy.There are many basins with well-exposed strata and abundant mammalian fossils in the Tibetan Plateau.The lower boundary stratotype sections of the Neogene Xiejian and Bahean stages are located respectively in the Xining and Linxia basins,and there are precise paleomagnetic dates in coordination with mammalian fossils.The lower boundary stratotypes of other stages can also be effectively determined in the Tibetan Plateau.Many first appearing mammalian genera in East Asia also appeared in the Tibetan Plateau and its surrounding areas,especially in the Linxia Basin on the northeast margin and in the Siwaliks on the southwest margin.Among them,Prodeinotherium first appeared at the bottom of the Miocene in the Siwaliks,and the earliest Hipparion of the Old World first appeared at the bottom of the Bahea

关键词： Tibetan Plateau Neogene Terrestrial stratum Mammalian fossil Paleomagnetism

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四轮独立转向车辆转向模式切换轨迹多目标优化方法研究

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机械工程学报 2024年第6期60卷 306-320页

作者：周晨徐飞翔中国矿业大学信息与控制工程学院徐州221100 福建省移动机械绿色智能驱动与传动重点实验室厦门361021

为了提高四轮独立转向车辆多种转向模式切换过程中的舒适性、安全性和切换效率,提出一种车辆转向模式切换轨迹多目标优化方法。首先,构建四轮独立转向车辆动力学和运动学模型,并建立基于B样条曲线的车辆瞬时转向中心切换轨迹;其次,选取... 详细信息

为了提高四轮独立转向车辆多种转向模式切换过程中的舒适性、安全性和切换效率,提出一种车辆转向模式切换轨迹多目标优化方法。首先,构建四轮独立转向车辆动力学和运动学模型,并建立基于B样条曲线的车辆瞬时转向中心切换轨迹;其次,选取车辆转向模式切换过程中安全性、舒适性、切换效率等性能评价指标,构建多性能目标协同优化目标函数和约束条件,运用粒子群算法对转向模式切换轨迹进行优化,实现多性能目标协同的四轮独立转向车辆转向模式切换轨迹最优规划;最后,基于仿真和自主研制的整车试验测试平台,对所提出的四轮独立转向车辆转向模式切换轨迹优化方法进行验证。在前轮转向模式切换到后轮转向模式的仿真工况下,相比于切换目标已知的多目标和双目标优化方法,所提出的优化方法使得切换效率分别提升了20.73%、27.78%,安全性分别提升了6.67%、15.15%。仿真和试验结果表明所提出的转向模式切换轨迹优化方法能够有效提高四轮独立转向车辆在转向模式切换过程中的切换效率、舒适性和安全性。

关键词：四轮独立转向车辆转向模式切换轨迹规划多目标优化实车试验测试

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新时期中国电影批评话语研究——以钟惦棐的“双翼论”为例

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当代电影 2024年第3期 97-104页

作者：王飞翔山西师范大学戏剧与影视学院

在当代中国电影批评话语的知识谱系中,钟惦棐无疑是一位旗帜性和标杆性的人物。目前,学界对钟惦棐的研究蔚然大观、成果颇丰——既有体大思精的著作,亦有构思精巧的短文。然而,此类研究多聚焦在钟惦棐的美学思想和历史地位,对其电影批... 详细信息

在当代中国电影批评话语的知识谱系中,钟惦棐无疑是一位旗帜性和标杆性的人物。目前,学界对钟惦棐的研究蔚然大观、成果颇丰——既有体大思精的著作,亦有构思精巧的短文。然而,此类研究多聚焦在钟惦棐的美学思想和历史地位,对其电影批评活动的考察却鲜有人关注。基于此,本文以钟惦棐在20世纪80年代与群众影评的交往为切入点,考察其在建构“电影观众学”的路径中,与全国群众影评协会之间的深刻关联,为我们提供一个重新审视20世纪80年代中国电影批评话语体系,甚至当代中国电影文化的窗口。

关键词：钟惦棐群众影评 20世纪80年代中国电影批评话语

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