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Eliminating H_(2)O/HF and regulating interphase with bifunctional tolylene-2,4-diisocyanate(TDI)additive for long life Li-ion battery

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Journal of Energy Chemistry 2024年第8期95卷 519-528,I0011页

作者： Xueyi zeng Xiang Gao Peiqi Zhou Haijia Li Xin He Weizhen fan Chaojun fan Tianxiang Yang Zhen Ma Xiaoyang Zhao Junmin Nan School of Chemistry South China Normal UniversityGuangzhou 510006GuangdongChina Guangzhou Tinci Materials Technology Co.Ltd. Guangzhou 510760GuangdongChina School of Environmental Engineering and Chemistry Luoyang Institute of Science and TechnologyLuoyang 471023HenanChina School of Geomatic and Environmental Engineering Henan Polytechnic InstituteNanyang 473000HenanChina

Lithium-ion batteries(LIBs)featuring a Ni-rich cathode exhibit increased specific capacity,but the establishment of a stable interphase through the implementation of a functional electrolyte strategy remains *** when the battery is operated under high temperature,the trace water present in the electrolyte will accelerate the hydrolysis of the electrolyte and the resulting HF will further erode the *** order to enhance the long-term cycling performance of graphite/LiNi_(0.8)Co_(0.1)Mn_(0.1)O_(2)(NCM811)LIBs,herein,Tolylene-2,4-diisocyanate(TDI)additive containing lone-pair electrons is employed to formulate a novel bifunctional electrolyte aimed at eliminating H_(2)O/HF generated at elevated *** 1000 cycles at 25℃,the battery incorporating the TDI-containing electrolyte exhibits an impressive capacity retention of 94%at 1 *** contrast,the battery utilizing the blank electrolyte has a lower capacity retention of only 78%.Furthermore,after undergoing 550 cycles at 1 C under45℃,the inclusion of TDI results in a notable enhancement of capacity,increasing it from 68%to 80%.This indicates TDI has a favorable influence on the cycling performance of LIBs,especially at elevated *** analysis of the film formation mechanism suggests that the lone pair of electrons of the isocyanate group in TDI play a crucial role in inhibiting the generation of H_(2)O and HF,which leads to the formation of a thin and dense *** existence of this interphase is thought to substantially enhance the cycling performance of the *** work not only improves the performance of graphite/NCM811 batteries at room temperature and high temperature by eliminating H_(2)O/HF but also presents a novel strategy for advancing functional electrolyte development.

关键词： Graphite/LiNi_(0.8)Co_(0.1)Mn_(0.1)O_(2)battery Tolylene-2 4-diisocyanate Long-cycling performance H_(2)O/HF eliminated additive

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Lath-like phases formed at an extremely high temperature in a Mg-RE(RE=rare earth)-Al alloy

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Rare Metals 2024年第8期43卷 3937-3945页

作者： bo Deng Shu-Hui Lv Qiang Yang Dong-Yue Zhao Jun-Yuan fan Xin Qiu School of Materials Science and Engineering Changchun University of Science and TechnologyChangchun 130022China State Key Laboratory of Rare Earth Resource Utilization Changchun Institute of Applied ChemistryChinese Academy of SciencesChangchun 130022China Chongqing Research Institute Changchun University of Science and TechnologyChongqing 401135China

Thermal stable intermetallic particles are important for the heat resistance of magnesium(Mg)*** this work,many lath-like particles formed in α-Mg grains of a Mg-8Gd-3Sm-0.7Al casting alloy when heat-treated at 873 ***-resolution high-angle annular dark field scanning transmission electron microscopy(HAADF-STEM) characterizations indicate that most of them are Mg-containing Al_(2)(Gd,Sm),with the atomic ratio of Mg:Al:(Gd,Sm) being ~1:1:1;a small part of them with relatively wider thickness are long-period stacking ordered(LPSO) phases simultaneously containing both 14H and 18R *** followed common orientation relationships with Mg matrix as those reported in previous *** addition,many Mg laths were observed in the primary blocky Al_(2)(Gd,Sm) phase at grain boundaries,where the atomic ratio of Al:(Gd,Sm) in the Al_(2)(Gd,Sm) matrix was 2:***,density functional theory(DFT) calculations illustrated the detail structure of the re-constructed Mg/Al_(2)RE interface and simultaneously deduced the underlying reason for the re-dissolution of the newly formed Mg-containing Al_(2)(Gd,Sm) plates in α-Mg matrix.

关键词： Magnesium alloy HAADF-STEM Microstructures Intermetallic particles Orientation relationships Interfaces

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Multi-functional and multi-scenario applications for MXene aerogels with synergistically enhanced asymmetric modules

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Nano Research 2024年第4期17卷 3359-3368页

作者： Junru Yao Jintang Zhou Feng Yang Guiyu Peng Yijie Liu Zhengjun Yao fan Wu Haibo zeng College of Materials Science and Technology Nanjing University of Aeronautics and AstronauticsNanjing 211100China Key Laboratory of Material Preparation and Protection for Harsh Environment(Nanjing University of Aeronautics and Astronautics) Ministry of Industry and Information TechnologyNanjing 211100China School of Mechanical Engineering Nanjing University of Science and TechnologyNanjing 210094China

The development of multifunctional materials and synergistic applications of various functions are important conditions for integrated and miniaturized ***,we developed asymmetric MXene/aramid nanofibers/polyimides(AMAP)aerogels with different modules using an integrated molding *** asymmetric modules(layered MXene/aramid nanofibers section and porous MXene/aramid nanofibers/polyimides section)interactions are beneficial for enhanced performances,resulting in low reflection electromagnetic interference(EMI)shielding(specific shielding effectiveness of 2483(dB·cm^(3))/g and a low R-value of 0.0138),high-efficiency infrared radiation(IR)stealth(ultra-low thermal conductivity of 0.045 W/(m·K)and IR emissivity of 0.32 at 3–5μm and 0.28 at 8–14μm),and excellent thermal management performances of insulated Joule ***,these multifunctional AMAP aerogels are suitable for various application scenarios such as personal and building protection against electromagnetic pollution and cold,as well as military equipment protection against infrared detection and EMI.

关键词： multifunctional material electromagnetic interference shielding low reflection infrared radiation stealth thermal insulation Joule heating

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Subclinical impairment of left ventricular myocardium function in type 2 diabetes mellitus patients with or without hypertension

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World Journal of Diabetes 2024年第6期15卷 1272-1279页

作者： zeng-Guang Chen Guang-An Li Jun Huang Li fan Department of Cardiology The Affiliated Changzhou Second People’s Hospital with Nanjing Medical UniversityChangzhou 213000Jiangsu ProvinceChina Department of Echocardiography The Affiliated Changzhou Second People’s Hospital with Nanjing Medical UniversityChangzhou 213000Jiangsu ProvinceChina

BACKGROUND Cardiovascular disease has been the leading cause of morbidity and mortality for type 2 diabetes mellitus(T2DM)patients over the last *** To determine whether layer-specific global longitudinal strain(GLS)combined with peak strain dispersion(PSD)can be used to assess left ventricle(LV)myocardium systolic dysfunction in T2DM patients or without hypertension(HP).METHODS We enrolled 97 T2DM patients,70 T2DM+HP patients and 101 healthy ***-specific GLS and PSD were calculated by EchoPAC software in apical three-,four-and two-chamber *** of the epimyocardial,middle-layer and endomyocardial(GLSepi,GLSmid,and GLSendo)were measured and *** operating characteristic analysis was performed to detect LV myocardium systolic dysfunction in T2DM *** There were significant differences in GLSepi,GLSmid,GLSendo,and PSD between healthy subjects,T2DM patients and T2DM patients with HP(PT2DM patients>T2DM with HP patients in the absolute values of GLSepi,GLSmid and GLSendo(P<0.001),while PSD was ranked healthy subjects

关键词： Type 2 diabetes mellitus Hypertension Speckle tracking echocardiography Global longitudinal strain Peak strain dispersion

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Two Stages Segmentation Algorithm of Breast Tumor in DCE-MRI Based on Multi-Scale Feature and boundary Attention Mechanism

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Computers, Materials & Continua 2024年第7期80卷 1543-1561页

作者： Bing Li Liangyu Wang Xia Liu Hongbin fan bo Wang Shoudi Tong School of Automation Harbin University of Science and TechnologyHarbin150080China Heilongjiang Provincial Key Laboratory of Complex Intelligent System and Integration Harbin150080China School of Computer Engineering Technology Guangdong Institute of Science and TechnologyZhuhai519090China

Nuclearmagnetic resonance imaging of breasts often presents complex *** tumors exhibit varying sizes,uneven intensity,and indistinct *** characteristics can lead to challenges such as low accuracy and incorrect segmentation during tumor ***,we propose a two-stage breast tumor segmentation method leveraging multi-scale features and boundary attention ***,the breast region of interest is extracted to isolate the breast area from surrounding tissues and ***,we devise a fusion network incorporatingmulti-scale features and boundary attentionmechanisms for breast tumor *** incorporate multi-scale parallel dilated convolution modules into the network,enhancing its capability to segment tumors of various sizes through multi-scale convolution and novel fusion ***,attention and boundary detection modules are included to augment the network’s capacity to locate tumors by capturing nonlocal dependencies in both spatial and channel ***,a hybrid loss function with boundary weight is employed to address sample class imbalance issues and enhance the network’s boundary maintenance capability through additional *** was evaluated using breast data from 207 patients at RuijinHospital,resulting in a 6.64%increase in Dice similarity coefficient compared to the *** results demonstrate the superiority of the method over other segmentation techniques,with fewer model parameters.

关键词： Dynamic contrast-enhanced magnetic resonance imaging(DCE-MRI) breast tumor segmentation multi-scale dilated convolution boundary attention the hybrid loss function with boundary weight

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OpBench: an operator-level GPU benchmark for deep learning

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Science China(Information Sciences) 2024年第9期67卷 76-87页

作者： Qingwen GU bo fan Zhengning LIU Kaicheng CAO Songhai ZHANG Shimin HU Department of Computer Science and Technology Tsinghua University National Innovation Institute of Defense Technology Academy of Military Science Beijing Fitten Technology Co. Ltd.

Operators(such as Conv and ReLU) play an important role in deep neural networks. Every neural network is composed of a series of differentiable operators. However, existing AI benchmarks mainly focus on accessing model training and inference performance of deep learning systems on specific models. To help GPU hardware find computing bottlenecks and intuitively evaluate GPU performance on specific deep learning tasks, this paper focuses on evaluating GPU performance at the operator level. We statistically analyze the information of operators on 12 representative deep learning models from six prominent AI tasks and provide an operator dataset to show the different importance of various types of operators in different networks. An operator-level benchmark, OpBench, is proposed on the basis of this dataset, allowing users to choose from a given range of models and set the input sizes according to their demands. This benchmark offers a detailed operator-level performance report for AI and hardware developers. We also evaluate four GPU models on OpBench and find that their performances differ on various types of operators and are not fully consistent with the performance metric FLOPS(floating point operations per second).

关键词： deep learning operator benchmark model benchmark GPU performance analysis deep neural networks

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Slope-climbing of cropland and its effects in China

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Journal of Mountain Science 2024年第8期21卷 2754-2769页

作者： CHEN Wanxu XIE Youping YUAN Jintao zeng Jie YANG Liyan GU Tianci LEI fan Hubei Key Laboratory of Regional Ecology and Environmental Change School of Geography and Information EngineeringChina University of GeosciencesWuhan 430074China Key Laboratory of Natural Resources Monitoring and Supervision in Southern Hilly Region Ministry of Natural ResourcesChangsha 410118China Yunnan Key Laboratory of Plateau Geographic Processes and Environmental Changes Faculty of GeographyYunnan Normal UniversityKunming 650500China

In recent decades,the spatio-temporal patterns of China’s croplands have been reshaped by disturbances from anthropogenic activities,with complex changes in the topographic characteristics of ***-climbing of croplands(SCCL)is an important issue that threatens sustainable agricultural *** providing land with prominent location advantages,SCCL weakens the water and fertilizer retention capacity for cropland,intensifies various geological disasters,and adversely affects the ecological environment and food yield of these *** is crucial to determine the spatio-temporal variation features and effects of SCCL in China to formulate more accurate cropland protection policies and to maintain food security;however,the current lack of relevant studies is detrimental for capturing trends in cropland resources and sustainable cropland *** this study,we constructed a multi-scale slope spectrum for cropland and total terrain to explore the spatial differences and trends of SCCL from a three-dimensional *** evaluated the natural and socioeconomic effects of SCCL in China from multiple *** indicate that the proportion of cropland with slopes below 2°,5°,and 6°in China decreased by 0.43%,0.47%,and 0.50%from 1980 to 2020,*** became apparent during 1980-1990 and 2010-2020,especially over the recent *** cropland climbing index(CCI)and upper limited slope change(ULSC)to measure the spatio-temporal pattern of SCCL were 0.99%and 1.17°,respectively,during *** the agricultural regional scale,the SCCL was also concentrated in 1980-1990 and 2010-2020,and it is more pronounced in the southern *** proportion of provinces and prefecture-level cities with high-intensity SCCL during 1980-2020 were 87.10%and 49.73%,*** was comparatively more pronounced and broader from 2010 to *** this period,17.84%of prefecture-level cities had no SCCL,and the average CCI for all prefecture-level citi

关键词： Croplands Slope spectrum Slope-climbing Three-dimensional perspective Multi-scale China

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Degree of shade tolerance shapes seasonality of chlorophyll, nitrogen and phosphorus levels of trees and herbs in a temperate deciduous forest

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Journal of Forestry Research 2024年第4期35卷 60-72页

作者： Jiajia zeng fan Liu Yuan Zhu Jiayi Li Ying Ruan Xiankui Quan Chuankuan Wang Xingchang Wang Aulin College Northeast Forestry UniversityHarbin 150040People’s Republic of China Center for Ecological Research Northeast Forestry UniversityHarbin 150040People’s Republic of China Key Laboratory of Agricultural Water Resources Center for Agricultural Resources ResearchInstitute of Genetics and Developmental BiologyChinese Academy of SciencesShijiazhuang 050021People’s Republic of China Institute of Applied Ecology Chinese Academy of SciencesShenyang 110016People’s Republic of China Key Laboratory of Sustainable Forest Ecosystem Management Ministry of EducationNortheast Forestry UniversityHarbin 150040People’s Republic of China

Forest productivity is closely linked to seasonal variations and vertical differentiation in leaf ***,leaf structural and chemical traits variation among co-existing species,and plant functional types within the canopy are poorly *** this study,the seasonality of leaf chlorophyll,nitrogen(N),and phosphorus(P)were quantified vertically along the canopy of four major tree species and two types of herbs in a temperate deciduous *** role of shade tolerance in shaping the seasonal variation and vertical differentiation was *** the entire season,chlorophyll content showed a distinct asymmetric unimodal pattern for all species,with greater chlorophyll levels in autumn than in spring,and the timing of peak chlorophyll per leaf area gradually decreased as shade tolerance *** a:b ratios gradually decreased with increasing shade *** N and P contents sharply declined during leaf expansion,remained steady in the mature stage and decreased again during leaf *** the seasons,the lower canopy layer had significantly higher chlorophyll per leaf mass but not chlorophyll per leaf area than the upper canopy layer regardless of degree of shade ***,N and P per leaf area of intermediate shade-tolerant and fully shade-tolerant tree species were significantly higher in the upper canopy than in the *** variations in N:P ratios suggest changes in N or P *** findings indicate that shade tolerance is a key feature shaping inter-specific differences in leaf chlorophyll,N,and P contents as well as their seasonality in temperate deciduous forests,which have significant implications for modeling leaf photosynthesis and ecosystem production.

关键词： Leaf traits Leaf nutrients Seasonal variations Chlorophyll Nitrogen Phosphorus Shade tolerance Canopy layers

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Plasmon coupling-driven enhanced high-order multiphoton excited fluorescent performance of metal-organic frameworks

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Nano Research 2024年第7期17卷 6502-6508页

作者： Tong Meng bo Li Linlin zeng Xianshun Sun Yupeng Tian Hongping Zhou Meng Zhou Dandan Li Institutes of Physical Science and Information Technology Key Laboratory of Structure and Functional Regulation of Hybrid MaterialsMinistry of EducationAnhui UniversityHefei 230601China School of Chemistry and Chemical Engineering Anhui UniversityHefei 230601China Hefei National Research Center for Physical Sciences at the Microscale University of Science and Technology of ChinaHefei 230026China

Accessing high-order multiphoton excited fluorescence(H-MPEF)materials is challenging yet and needs complicated synthesis *** this study,we successfully assembled plasmonic Au nanorods(Au NRs)with multiphoton responsive metalorganic frameworks(MOFs),resulting in a significant several-fold enhancement of *** extent of multiphoton enhancement was found to be strongly dependent on the degree of overlap between the multiphoton excitation wavelength of MOFs and the localized surface plasmon resonance absorbance of Au NRs,indicating the importance of plasmon-induced resonance energy ***,plasmon-induced hot electron transfer played a vital role in enhanced multiphoton activity as ***,the optimum H-MPEF enhancement occurs at the second near-infrared(NIR-II)region,which provides a promising platform for fluorescent *** findings provide a feasible and practical method to fabricate optimized H-MPEF materials for biological imaging using tissue-penetrating NIR-II light.

关键词： metal-organic framework(MOF) plasmon resonance multiphoton activity fluorescence imaging

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A Review of Magnesium Alloys as Structure–Function Integrated Materials

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Acta Metallurgica Sinica(English Letters) 2024年第8期37卷 1301-1338页

作者： Zhenfei Jiang bo Hu Zixin Li fanjin Yao Jiaxuan Han Dejiang Li Xiaoqin zeng Wenjiang Ding National Engineering Research Center of Light Alloy Net Forming and State Key Laboratory of Metal Matrix Composites Shanghai Jiao Tong UniversityShanghai 200240China

Magnesium alloys have a significant advantage,lower density over the other structure materials;hence,they have been widely used in various fields such as transportation and *** the development of research and the enlargement of the research scope,more advantages have been revealed:excellent shielding efficiency,extraordinarily high damping capacity,as well as impressive thermal ***,Mg alloys have the potential to be various functional materials,such as electromagnetic shielding material,damping material,and thermal conductive *** review comprehensively summarizes the research progress and the up-to-date summary of Mg alloys as structure–function integrated materials in recent *** atoms,heat treatment,deformation,secondary phase,and temperature,which have a significant influence on the properties of magnesium alloys,are *** expect this review to be helpful for those who are working on developing structure–function integrated materials with superior comprehensive performance.

关键词： Magnesium alloys Structure-function integrated Electromagnetic shielding Damping capacity Thermal conductivity

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