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Synergy of sodium doping and nitrogen defects in carbon nitride for promoted photocatalytic synthesis of hydrogen peroxide

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Chinese Chemical Letters 2024年第8期35卷 324-329页

作者： fabrice Nelly Habarugira Ducheng Yao Wei Miao Chengcheng Chu Zhong Chen Shun Mao College of Environmental Science and Engineering State Key Laboratory of Pollution Control and Resource ReuseTongji UniversityShanghai 200092China Baowu Water Technology Co. Ltd.Research InstituteShanghai 201999China

Photocatalytic synthesis of hydrogen peroxide has gradually become a promising method for in-situ pro-duction of hydrogen peroxide,which relies on sustainable solar ***,the commonly used photocatalyst,i.e.,carbon nitride(CN),still suffers from the drawbacks of narrow light absorption range and fast charge ***,we report a facile method to introduce nitrogen defects into carbon nitride together with sodium *** adjusting the ratio of sodium dicyandiamide,the band gap of carbon nitride can be controlled,while the carrier separation and transfer ability of carbon nitride is *** modified CN with sodium doping and nitrogen defect(SD-CN)demonstrates outstanding H_(2)O_(2)pro-duction performance(H_(2)O_(2)yield rate of 297.2μmol L^(−1)h^(−1))under visible light irradiation,which is approximately 9.8 times higher than that of pristine *** work deepens the understanding of the coordinated effect of structural defect and element doping of carbon nitride on the photocatalytic H_(2)O_(2)production performance,and provides new insight into the design of photocatalytic system for efficient production of H_(2)O_(2).

关键词： Photocatalysis H_(2)O_(2)evolution Sodium doping Nitrogen defect Metal-free catalyst

Genome-Wide Discovery and Expression Profiling of the SWEET Sugar Transporter Gene Family in Woodland Strawberry (Fragaria vesca) under Developmental and Stress Conditions: Structural and Evolutionary Analysis

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Phyton-International Journal of Experimental Botany 2024年第7期93卷 1485-1502页

作者： Shoukai Lin Yifan Xiong Shichang Xu Manegdebwaoaga Arthur fabrice Kabore Fan Lin Fuxiang Qiu College of Environmental and Biological Engineering Putian UniversityPutian351100China College of Life Science Fujian Agriculture and Forestry UniversityFuzhou350002China Fujian Provincial Key Laboratory of Ecology-Toxicological Effects&Control for Emerging Contaminants Putian UniversityPutian351100China Key Laboratory of Ecological Environment and Information Atlas(Putian University) Fujian Provincial UniversityPutian351100China Affiliated Hospital of Putian University Putian351100China

The SWEET(sugar will eventually be exported transporter)family proteins are a recently identiﬁed class of sugar transporters that are essential for various physiological *** the functions of the SWEET proteins have been identiﬁed in a number of species,to date,there have been no reports of the functions of the SWEET genes in woodland strawberries(Fragaria vesca).In this study,we identiﬁed 15 genes that were highly homolo-gous to the *** AtSWEET genes and designated them as FvSWEET1–*** then conducted a structural and evolutionary analysis of these 15 FvSWEET *** phylogenetic analysis enabled us to categor-ize the predicted 15 SWEET proteins into four distinct *** observed slight variations in the exon‒intron structures of these genes,while the motifs and domain structures remained highly ***,the developmental and biological stress expression proﬁles of the 15 FvSWEET genes were extracted and ***,WGCNA coexpression network analysis was run to search for possible interacting genes of FvSWEET *** results showed that the FvSWEET10 genes interacted with 20 other genes,playing roles in response to bacterial and fungal *** outcomes of this study provide insights into the further study of FvSWEET genes and may also aid in the functional characterization of the FvSWEET genes in woodland strawberries.

关键词： Woodland strawberry SWEET gene sugar transporter genome-wide identiﬁcation characterization expression

Optical probing of ultrafast laser-induced solid-to-overdense-plasma transitions

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Light(Science & Applications) 2024年第5期13卷 973-984页

作者： Yasmina Azamoum Georg Alexander Becker Sebastian Keppler Guillaume Duchateau Stefan Skupin Mickael Grech fabrice Catoire Sebastian Hell Issa Tamer Marco Hornung Marco Hellwing Alexander Kessler Franck Schorcht Malte Christoph Kaluza GSI Helmholtzzentrum für Schwerionenforschung Planckstr.164291 DarmstadtGermany. Helmholtz Institute Jena Fröbelstieg 307743 JenaGermany. Institute of Optics and Quantum Electronics Friedrich-SchillerUniversität JenaMax-Wien-Platz 107743 JenaGermany. CEA-CESTA 15 Avenue des SablièresCS6000133116 Le BarpCedexFrance Institut Lumière Matière UMR 5306-CNRSUniversitéde Lyon 169622 VilleurbanneFrance. LULI CNRSCEASorbonne UniversitéInstitut Polytechnique de ParisPalaiseauFrance. Universitéde Bordeaux-CNRS-CEA CELIAUMR 5107 TalenceFrance

Understanding the solid target dynamics resulting from the interaction with an ultrashort laser pulse is a challenging fundamental multi-physics problem involving atomic and solid-state physics,plasma physics,and laser *** of the initial interplay of the underlying processes is essential to many applications ranging from lowpower laser regimes like laser-induced ablation to high-power laser regimes like laser-driven ion *** the properties of the so-called pre-plasma formed as the laser pulse’s rising edge ionizes the target is complicated from the theoretical and experimental point of view,and many aspects of this laser-induced transition from solid to overdense plasma over picosecond timescales are still open *** the one hand,laser-driven ion acceleration requires precise control of the pre-plasma because the efficiency of the acceleration process crucially depends on the target properties at the arrival of the relativistic intensity peak of the *** the other hand,efficient laser ablation requires,for example,preventing the so-called“plasma shielding”.By capturing the dynamics of the initial stage of the interaction,we report on a detailed visualization of the pre-plasma formation and ***-thin diamond-like carbon foils are shown to transition from solid to plasma during the laser rising edge with intensities<10^(16)W/cm^(2).Single-shot near-infrared probe transmission measurements evidence sub-picosecond dynamics of an expanding plasma with densities above 10^(23)cm^(−3)(about 100 times the critical plasma density).The complementarity of a solid-state interaction model and kinetic plasma description provides deep insight into the interplay of initial ionization,collisions,and expansion.

关键词： laser acceleration solid

Correlation between Total PSA Level and the Histoprognostic Gleason Score

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Open Journal of Pathology 2024年第2期14卷 69-80页

作者： fabrice Senghor Ibou Thiam Kor Ndiaye Kassoum Badji Department of Pathological Anatomy H&#244pital de La Paix Ziguinchor Senegal Department of Pathological Anatomy CHU Aristide le Dantec Dakar Senegal

Prostate cancer is a public health problem in Senegal. It is one of the most common cancers in men and can be detected early by PSA measurement and confirmed by the pathological study which specifies the histological type and evaluates the histoprognostic scores (Gleason and pTNM). We did not find any anatomopathological study highlighting a link between the PSA t rate and histoprognostic Gleason scores in Senegal. Objective: We carried out this work aimed at determining whether there is a correlation between the PSA t rate and the histoprognostic Gleason score, in our context. Methodology: This is a retrospective, descriptive and analytical study conducted from January 2013 to October 2021, based on histologically proven prostate cancer cases with a specified PSA level, diagnosed in the pathological anatomy and cytology laboratory of Aristide Le Dantec hospital. Results: We identified 654 cases of prostate cancer. The average age was 68.59 ± 5.8 years with extremes of 40 years to 92 years. More than half of our cohort presented a clinical stage T2c, i.e. 56.94%. The average prostate volume on ultrasound was 81.81 ± 66 cc. The median PSA t was 110.5 ng/ml, with extremes ranging from 2 ng/ml to 74,770 ng/ml. Prostatic adenocarcinoma was the only histological type found in our patients. There was a predominance of Gleason score 6 (PICU grade group 1) observed in 35.17% of patients. Well-differentiated cancers were predominant and represented 35.17%. There was a statistically significant positive correlation between PSA t level and Gleason score (Spearman’s Rho = 0.305, p = 0.000). Conclusion: This study shows that in the Senegalese population, in patients with prostate cancer, the higher the PSA t level rises above normal, the higher the Gleason score tends to be.

关键词： Prostate Cancer PSAt Gleason Dakar

New Fusion Approach of Spatial and Channel Attention for Semantic Segmentation of Very High Spatial Resolution Remote Sensing Images

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Open Journal of Applied Sciences 2024年第2期14卷 288-319页

作者： Armand Kodjo Atiampo Gokou Hervé fabrice Diédié Unité de Recherche et d’Expertise du Numerique (UREN) Université Virtuelle de Céte d’Ivoire Abidjan Ivory Coast Laboratoire de Mathématiques et Informatique Université Peleforo Gon Coulibaly Korhogo Ivory Coast

The semantic segmentation of very high spatial resolution remote sensing images is difficult due to the complexity of interpreting the interactions between the objects in the scene. Indeed, effective segmentation requires considering spatial local context and long-term dependencies. To address this problem, the proposed approach is inspired by the MAC-UNet network which is an extension of U-Net, densely connected combined with channel attention. The advantages of this solution are as follows: 4) The new model introduces a new attention called propagate attention to build an attention-based encoder. 2) The fusion of multi-scale information is achieved by a weighted linear combination of the attentions whose coefficients are learned during the training phase. 3) Introducing in the decoder, the Spatial-Channel-Global-Local block which is an attention layer that uniquely combines channel attention and spatial attention locally and globally. The performances of the model are evaluated on 2 datasets WHDLD and DLRSD and show results of mean intersection over union (mIoU) index in progress between 1.54% and 10.47% for DLRSD and between 1.04% and 4.37% for WHDLD compared with the most efficient algorithms with attention mechanisms like MAU-Net and transformers like TMNet.

关键词： Spatial-Channel Attention Super-Token Segmentation Self-Attention Vision Transformer

Contribution of Anti-p63 Antibodies in the Interpretation of Benign Label Prostatic Biopsies

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Open Journal of Pathology 2024年第2期14卷 31-44页

作者： Ibou Thiam fabrice Senghor Frenette Codja Kor Ndiaye Mohamed Moustapha Cherif Dial Pathological Anatomy Department Aristide Le Dantec University Hospital Dakar Senegal Pathological Anatomy Department H&#244pital de la Paix Ziguinchor Senegal Pathological Anatomy Department Idrissa Pouye University Hospital Dakar Senegal

Introduction: Prostate cancer is the second most common cancer in men. The diagnosis is most often based on the prostate biopsies’ analysis and on histological criteria recognizable on standard coloring. In some cases, the use of immunohistochemistry is important. Objectives: This paper aims to specify the p63 phenotypic profile of lesions diagnosed benign, with minimal suspect foci, difficult to interpret, HGPIN (high grade intraepithelial neoplasia) and LGPIN (low-grade prostatic intraepithelial neoplasia) and evaluate the manual technique of p63 immunohistochemistry. Patients and Method: This was a retrospective, descriptive study of prostate biopsies recorded in the PAC service of the HALD from January 1st, 2018 to December 31st, 2018. It was completed by a manual immunohistochemical study of the blocks enrolled from November 19th to December 4th, 2020 in the PAC department of the HPD. The studied parameters were: registry number, age, clinical stage, prostate volume, PSA level, microscopic appearance and p63 immunohistochemical profile. Results: Our study included 60 prostate biopsies. The ages of our patients varied from 45 to 77 years, with an average of 64.2 years and a standard deviation of 6.2. The majority of patients were at clinical stage cT2b (33%) with a prostate volume varying between 33.15 and 169.4 cc. The minimum value of PSA in our series is 5 ng/ml, the maximum being 100 ng/ml with an average level of 24.1 ng/ml and a standard deviation of 21.2. Our series included 50 adenomyomatous hyperplasias, 7 adenomyomatous hyperplasias associated with chronic prostatitis, 2 HGPIN and 1 LGPIN. After re-reading we found 5 discordant cases, which corresponded to minimal suspect foci (kappa = 0.5098). The p63 marking was informative in 53 cases, i.e. 88%, and non-informative in 7 cases, i.e. 12%. Among the uninformative markings, 2 were due to lack of tissue adhesion to the slides. Among the informative markings, 11 were negative. p63 immunohistochemistry was

关键词： Prostate Cancer Diagnosis Anti-p6 Antibody

Indirect Electroanalysis of 3-Methyl-4-Nitrophenol in Water Using Carbon Fiber Microelectrode Modified with Nickel Tetrasulfonated Phthalocyanine Complex

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Materials Sciences and Applications 2024年第2期15卷 25-35页

作者： Yibor fabrice Roland Bako Serge Foukmeniok Mbokou Boukaré Kaboré Issa Tapsoba Maxime Pontié Laboratoire de Chimie Analytique Environnementale et Bio-organique (LCAEBiO) Département de Chimie Université Joseph Ki-Zerbo Ouagadougou Burkina Faso Institut des Sciences et de Technologie Ecole Normale Supérieure Ouagadougou Burkina Faso Group of analysis and Processes Analysis (GA&P) Département de Chimie Université d’Angers Angers France Laboratoire de Sciences et Technologies (LaST) Université Thomas SANKARA Ouagadougou Burkina Faso

Electrochemical detection of 3-methyl-4-nitrophenol (MNP) in direct phenol oxidation occurs at high potentials and generally leads to progressive passivation of the electrochemical sensor. This study describes the use of a carbon fiber microelectrode modified with a tetrasulfonated nickel phthalocyanine complex for the detection of MNP at a lower potential than that of direct phenol oxidation. The MNP voltammogram showed the presence of an anodic peak at -0.11 V vs SCE, corresponding to the oxidation of the hydroxylamine group generated after the reduction of the nitro group. The effect of buffer pH on the peak current and SWV parameters such as frequency, scan increment, and pulse amplitude were studied and optimized to have better electrochemical response of the proposed sensor. With these optimal parameters, the calibration curve shows that the peak current varied linearly as a function of MNP concentration, leading to a limit of detection (LoD) of 1.1 μg/L. These results show an appreciable sensitivity of the sensor for detecting the MNP at relatively low potentials, making it possible to avoid passivation phenomena.

关键词： 3-Methyl-4-Nitrophenol Carbon Fiber Microelectrode Nickel Tetrasulfonated Phthalocyanine Indirect Electroanalysis Square Wave Voltammetry

Intraductal Prostatic Carcinoma: Epidemiological and Anatomopathological Aspects in Dakar

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Open Journal of Pathology 2024年第2期14卷 54-63页

作者： Ibou Thiam fabrice Senghor Omar Sow Kor Ndiaye Mohamed Moustapha Chérif Dial Anatomical Pathology Department Aristide Le Dantec University Hospital Dakar Senegal Anatomical Pathology Department Peace Hospital Ziguinchor Senegal General Surgery Department Peace Hospital Ziguinchor Senegal Anatomical Pathology Department Idrissa Pouye University Hospital Dakar Senegal

Introduction: Intraductal carcinoma is often associated with high-grade, high-stage adenocarcinoma. Its frequency is variable and it is considered a poor prognostic factor. In our context, when prostatic carcinoma is diagnosed, pathologists do not always report the presence of this anatomopathological entity. We therefore conducted a study to determine the epidemiological and anatomopathological profile of patients with this lesion in Dakar. Materials and Methods: This is a retrospective descriptive study covering a 1-year period from January to December 2022. It focused on cases of intraductal carcinoma diagnosed among prostatic carcinomas collected in the anatomopathology laboratories of Hôpital Général Idrissa Pouye (HOGIP) and Hôpital Militaire de Ouakam (HMO). It was based on archives of anatomopathological reports, blocks and slides. A total of 200 cases of prostatic carcinoma were collated and reviewed to identify those presenting with intraductal carcinoma according to the diagnostic criteria of Guo and Epstein. Results: 87 cases of intraductal carcinoma were found, representing 43.5% of prostatic carcinomas. The mean age was 71 years. Patients in their seventh decade were the most represented, i.e. 42.5%. The majority of samples examined were biopsies (72.4%). The mean PSA level was 965.91 ng/ml, with extremes ranging from 0.03 to 10,000 ng/ml. Histologically, 96.5% of cases (N = 84) were invasive prostatic carcinoma. Gleason score 8 (4 + 4) was the most common, accounting for 42.53% (N = 37). On average, the study found four (04) foci of intraductal carcinoma per specimen, with extremes ranging from 1 to 30. Dense cribriform architecture accounted for 78.16%, loose cribriform for 11.5%, solid for 8.04% and micropapillary for 2.3%. Six cases (6.9%) showed foci of comedonecrosis. The vast majority of radical prostatectomies (87.5%) were classified as pT3. Node invasion and perineural sheathing were observed in 12.5% and 52.32% of cases respectively. Conclusi

关键词： Intraductal Carcinoma Prostate Pathological Anatomy Senegal

Validation of the TOPAS Monte-Carlo Code of the Off-Field Dose of a 6 MV Synergy Linac

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Journal of Biosciences and Medicines 2024年第7期12卷 38-54页

作者： Kodjo Joel fabrice N’Guessan Ibrahima Sakho Bogbé D. L. H. Gogon Department of Physics and Chemistry Faculty of Sciences and Technology Iba Der Thiam University of This This Senegal International Cancer Center of Dakar Dakar Senegal Department of Physics Faculty of Sciences and Technology Flix Houphouet Boigny University of Abidjan Abidjan Cte dIvoire

The risk of radiation-induced second cancer and the late tissue loss due to Off-field doses in radiotherapy remain a serious concern. Monte Carlo (MC) simulation is currently one of the most accurate methods for calculating these doses. MC simulation model based on the Particle Simulation Tool (TOPAS) has been developed to simulate the off-field dose of an Elekta Synergy linear accelerator (Linac) emitting 6 MV photons. Measurements were taken in a water phantom using an ionization chamber to validate this model. The Percentage Depth Dose (PDD) at the depth of 0.0, 5.0, 10.0 and 15.0 cm from the beam axis for a 10 × 10 cm2 field size was measured and simulated. Off-field dose profiles at the depth of 1.5 (dmax), 5.0 and 10.0 cm for field sizes of 5 × 5, 10 × 10, 15 × 15, and 20 × 20 cm2 respectively were measured and simulated. Comparison of measured and simulated off-field dose values showed a good agreement. The average gamma passing rate of the PDDs and profiles curves for off-field doses were 87.5% and 98.11% respectively. The local dose difference based on the PDD curve between the measured and simulated was less than 6.0 % for all locations. For all field size considered in this study, the average difference between profile curves for off-field dose measured and simulated was 9.1%. PDDs and Profiles curves for off-field dose simulation uncertainties were less than 2.0% and 1.0% respectively. TOPAS-MC simulation model developed is a good representation of our 6 MV Linac Elekta Synergy for assessing off-field dose, which would be the primary cause of some secondary cancers.

关键词： Radiotherapy Off-Field Dose Secondary Cancer TOPAS-MC Simulation Dosimetry