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Methane Direct Conversion on Mo/ZSM-5 Catalysts Modified by Pd and Ru

Journal of Natural Gas Chemistry 2006年第2期15卷 82-86页

作者： Priscila Dias Sily fabio Bellot Noronha fabio barboza passos Departamento de Engenharia Química Universidade Federal FluminenseRua Passo da Pátria156 Niterói -RJ CEP 24210-240Brazil Instituto Nacional de Tecnologia Av. Venezuela 82Rio de Janeiro -RJ CEP 20081-312Brazil Departamento de Engenharia Química Universidade Federal FluminenseRua Passo da Pátria156 Niterói-RJ CEP 24210-240Brazil

The effect of addition of Ru and Pd to Mo/HZSM-5 catalysts used in the dehydroaromatization of methane was investigated. Catalytic tests and temperature-programmed oxidation results showed that Pd-based catalysts were more selective to naphthalene and suffered strong deactivation. The presence of Ru improved the activity and stability, with a decrease in the carbonaceous deposit probably because of a mechanism of protection of the Mo2C surface.

关键词： methane Pd Ru Mo ZSM-5 dehydroaromatization

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Production of Filler Aggregate from Waste of Bivalves Molluscs Shells

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Journal of Civil Engineering and Architecture 2011年第4期5卷 363-367页

作者： Ulisses Targino Bezerra fabio Luiz P. Almeida Lucineide Balbino Silva Normando Perazzo Barbosa TiberioA. passos Danielle G. L. Cavalcante Federal Institute of Paraiba Av. 1°de Maio 720 Jaguaribe Joao Pessoa-PB Brazil Federal University of Paralba Castelo Branco S/N Joao Pessoa-PB Brazil

The work presents an experimental study held with shells of molluscs of the species Anomalocardia brasiliana and Tivela mactroides, commonly found in the Northeast coast of Brazil. A local community living from the collection of these animals was the motivation of the work. This community wishes to install an industry for processing these molluscs; however, as government agencies require making an appropriate allocation of discarded shells, the community needs an environmental project of final destination of waste. Thus, the expectation of the work was to obtain a material to be added to Portland cement to act as filler, and also obtain a limestone that can be used as ink, because the material is composed of 80% calcium carbonate. The shells were ground and passed the sieve 325 mesh （0.044 mm）. The material was characterized by X-ray diffraction and X-ray fluorescence. Mortars specimens were prepared with percentages： 0%, 5%, 10%, 15%, 20% and 30% replacement of Portland cement. Two conditions were analyzed： with shells in a raw and burned state. The obtained results confirm the filler material effect, which suggests its use as a partial replacement of cement. However, due to the short silicas＇s concentration, the pozzolanic effect was not observed.

关键词： Bivalves molluscs shells filler Portland cement mortar

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