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Multiphase flow physics of room temperature liquid metals and its applications

Science China(Technological Sciences) 2023年第6期66卷 1483-1510页

作者： QIAO MengWen XING ZeRong fu jun-heng LIU Jing CAS Key Laboratory of Cryogenics Technical Institute of Physics and ChemistryBeijing 100190China School of future Technology University of Chinese Academy of SciencesBeijing 100049China Beijing Key Laboratory of Cryo-Biomedical Engineering Beijing 100190China College of Water Conservancy and Hydropower Engineering Sichuan Agricultural UniversityYa’an 625014China Department of Biomedical Engineering School of MedicineTsinghua UniversityBeijing 100084China

Multiphase flow existing everywhere in the motion evolution of nature,industrial processes,and daily life,has been an interdisciplinary cutting-edge frontier covering rather diverse *** multiphase flow of high melting metals typically involves gas/vapor-liquid two-phase fluidics which usually requests intense energy processes and therefore limits their applications to a large *** from this,the newly emerging room-temperature liquid metals(RTLMs)with fascinating metallic fluidic properties and multifunctional behaviors,not only well resolve the existing challenges facing conventional technologies,but also open up a series of new scientific and engineering *** the conceptual introduction of multiphase composites endows liquid metal with many unconventional fluidic *** further push forward the advancement of this new area,the present article is dedicated to systematically outlining the scientific category of RTLMs multiphase flow physics and interpreting its fundamental and practical *** vision is to provide insights into promising developmental directions of RTLMs multiphase flow and thus facilitate synergetic research and progress among different ***,the traditional metal multiphase flow was briefly ***,we summarized the physics of RTLMs multiphase flow,the common types of liquid metals,the basic physical and chemical properties of their multiphase flow and governing equations,*** that,various typical driving modalities and manipulation methods of RTLMs were ***,important implementations of RTLMs multiphase flow into thermal management,energy harvesting,catalysis,soft machines,biomedicine,and printed electronics were ***,the multiphase flow physics of RTLMs is currently still in its incubation stage and there exist tremendous opportunities and challenges which are worth further pursuing in the coming time.

关键词： room-temperature liquid metals multiphase flow physics composite solution nanofluids fluid mechanics micro-/nanodroplets

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Oxidating liquid metal interface integrated capacitive pressure detection

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Science China(Technological Sciences) 2023年第6期66卷 1629-1639页

作者： fu jun-heng ZHAN Fei XING ZeRong ZHANG Teng SUN XinLong ZENG Yun YAN MingLei TANG Wei LIU Jing WANG Lei ZHAO Yang College of Water Conservancy and Hydropower Engineering Sichuan Agricultural UniversityYa’an 625014China School of Electrical and Electronic Engineering Shijiazhuang Tiedao UniversityShijiazhuang 050043China Beijing Key Laboratory of Cryo-Biomedical Engineering Technical Institute of Physics and ChemistryChinese Academy of SciencesBeijing 100190China Department of Materials Science and Engineering The University of SheffieldSheffield S13JDUK School of future Technology University of Chinese Academy of SciencesBeijing 100049China Department of Biomedical Engineering School of MedicineTsinghua UniversityBeijing 100084China

The characteristics of real-time monitoring and flexible integration based on passive capacitive detection are becoming the preferred sensing strategy for wearable ***,the currently designed capacitive sensors mostly focused on the bionic microstructures to improve sensitivity and measurement accuracy,while ignoring the inherent mechanical wear and resistance of multilayer *** this paper,an integrated monolithic capacitive pressure detection based on room temperature liquid metal is designed and fabricated,avoiding the tightness problem of the multi-layer *** oxidized paste-like liquid metal owning superior interfacial wetting properties can stably adhere to the surface of the porous *** gas-filled porous framework endows the capacitive sensor with a mechanical response of 0.0557 g with a response and recovery time of 1.26 and 0.63 s under a load condition of 150 Pa,and steadily maintained in 1600 cycle ***,the capacitive sensor is employed to detect human physiological signals and force shock responses,which could clearly distinguish different action signals,providing a new platform for the subsequent development and design of integrated capacitive sensors.

关键词： liquid metal interfacial wetting capacitive detection motion monitoring

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Effects of 1-MCP on Ethylene Synthesis and Metabolismof Apple During Storage

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Agricultural Sciences in China 2003年第11期2卷 1259-1265页

作者： LI fu-jun, ZHAI heng, YANG Hong-qiang, ZHANG Xin-hua, SHU Huai-rui and ZHOU Jie(Horticultural College , Shandong Agricultural University, Tai’an 271018 , P.R. China) Horticultural College Shandong Agricultural University Tai'an 271018 P. R. China

Red fuji apple(Malus domestica Borkh var. Red fuji)fruits were used to study the effect of 1-MCP on ethylene biosynthesis metabolism during storage. The results showed that 1-MCP maintained the firmness and inhibited the respiration rate, LOX activity and ethylene production rate of fruits. further study indicated that 1-MCP inhibited ACS(ACC synthase)activity from the 15th day, increased ACC accumulation, and delayed the appearance of ACO(ACC oxidase)activity peak. The increase of protein kinase activity was also inhibited by 1-MCP during fruit ethylene climacteric time.

关键词： Apple fruit Ethylene 1-MCP Protein kinase activity Storage

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De novo synthesis of atropisomeric benzofurans via Cu/SPDO complex catalyzed asymmetric formal [3 + 2] annulation

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Science China Chemistry 2025年第1期68卷 174-180页

作者： Fan-Xiao Meng Xing-Yu Wang Ka Lu Ju-Song Yang fu-Min Zhang Ai-jun Ma Bao Du Yong-Qiang Tu State Key Laboratory of Applied Organic Chemistry College of Chemistry and Chemical Engineering Lanzhou University School of Chemistry and Chemical Engineering Shanghai Jiao Tong University School of Biotechnology and Health Sciences Wuyi University

Herein, the de novo synthesis of atropisomeric benzofurans through the Cu/spirocyclic-pyrrolidine-oxazoline(SPDO) complex catalyze asymmetric formal [3 + 2] cycloaddition between quinones and ynamides is explored, producing a range of structurally diverse axially chiral benzofurans in satisfactory yields with good to excellent enantioselectivities. furthermore, density functional theory calculations were applied to explain the possible reaction mechanism.

关键词： benzofuran atropisomers novel de novo synthetic strategy asymmetric formal [3 + 2] cycladdition Cu/SPDO complex DFT calculations

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Discovery of a new family member of arsenic–vanadium polyoxometalates with high catalytic performance for one-pot coupling of CO2, epoxides and amines

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Tungsten 2025年第1期7卷 80-87页

作者： Fang-Qian Wang Yin Zhang Wei-Wei Wang Mei-Qian fu Hong-Bing Mo Wei-Dong Yu Chao Liu jun Yan College of Chemistry and Chemical Engineering Central South University junior Education Department Changsha Normal University School of Science Hunan University of Technology and Business

Arsenic-vanadium polyoxometalates（POMs） represent a family of tremendous potential catalysts owing to their peculiar physical and chemical *** in CO2conversion,using POMs to catalyze the conversion of CO2and epoxide into chemical intermediates is the research ***,A new family number of arsenic-vanadium POMs,[N（CH3）4]4[As8V12O38（H2O）]·2H2O({As8V12O38}),was reported and characterized by single-crystal X-ray diffraction,fourier transform infrared spectroscopy,X-ray photoelectron spectroscopy,*** from other allotropicity,{As8V12O38}shows a different structure pattern with an I-43d *** obtained {As8V12O38} was employed as a catalyst for the *** initial catalytic reaction confirmed that {As8V12O38} can catalyze the formation of epoxy carbonate by using 1.01 kPa CO2and epoxide at 70℃.furtherly,when added amine in the catalytic system,oxazolidinone could be obtained by high yields,which provides an efficient way to convert CO2into profitable ***,a possible catalytic reaction mechanism was proposed by using different characterization analyses.{As8V12O38} first catalyzes the epoxide and CO2to form an epoxy carbonate and then catalyzes epoxy carbonate and benzylamine into oxazolidinone.

关键词： Arsenic CO2 conversion Oxazolidinone Polyoxometalates Vanadium

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Staged dendrite suppression for high safe and stable lithium-sulfur batteries

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Journal of Energy Chemistry 2025年第1期100卷 674-683页

作者： jun Jiang Zhenjie Lu Yanwen Ding Shujun Liu Zhijie Qi Tian Tang Yunfan Zhang Zhiyuan Ma Jingwen Sun Liang Xue Wenyao Zhang Pan Xiong Xin Wang junwu Zhu Yongsheng fu Key Laboratory for Soft Chemistry and functional Materials of Ministry of Education Nanjing University of Science and Technology Jiangsu Pylon Battery Co.Ltd

The unavoidable dendrite growth and shuttle effect have long been stranglehold challenges limiting the safety and practicality of lithium-sulfur ***,we propose a dual-action strategy to address the lithium dendrite issue in stages by constructing a multifunctional surface-negatively-charged nanodiamond layer with high ductility and robust puncture resistance on polypropylene （PP） *** uniformly loaded compact negative layer can not only significantly enhance electron transmission efficiency and promote uniform lithium deposition,but also reduce the formation of dendrite during early deposition *** importantly,under the strong puncture stress encountered during the deterioration of lithium dendrite growth under limiting current,the high ductility and robust puncture resistance（145.88 MPa） of as-obtained nanodiamond layer can effectively prevent short circuits caused by unavoidable lithium *** Li||Li symmetrical cells assembled with nanodiamond layer modified PP demonstrated a stable cycle of over 1000 h at 2 mA cm-2with a polarization voltage of only 29.3 ***,the negative charged layer serves as a physical barrier blocking lithium polysulfide ions,effectively mitigating capacity *** improved cells achieved a capacity decay of only 0.042%per cycle after 700 cycles at 3 C,demonstrating effective suppression of dendrite growth and capacity attenuation,showing promising prospect.

关键词： Ductility

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Engineering N3C vacancies in hierarchical porous carbon nitride nanosheets for room temperature ultradeep photocatalytic aerobic oxidative desulfurization

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Science China Chemistry 2025年

作者： Yina Nie Weijie Yang Xin Wang Xiang Li Lele Wei Xiaolin Bai Lin Liu Feng fu jun Wan College of Chemistry & Chemical Engineering Research Institute of Comprehensive Energy Industrial Technology Shaanxi Key Laboratory of Chemical Reaction Engineering Yan'an University Anhui Engineering Research Center of Carbon Neutrality College of Chemistry and Materials Science Anhui Normal University

The production of ultra-low sulfur clean fuels holds global significance for improving energy efficiency and reducing environmental pollution. Photocatalytic aerobic oxidative desulfurization（PODS） offers an attractive approach to efficiently remove refractory heterocyclic aromatic sulfur compounds under mild conditions. However, the sluggish charge dynamics,insufficient molecule activation, and slow mass transfer within photocatalysts restrict the overall desulfurization efficiency,hindering the widespread application of this technology. Herein, we developed a defective g-C3N4（M1U3CN） photocatalyst with bridged N3Cvacancies and hierarchical porous structures to address these limitations. This catalyst not only demonstrates outstanding dibenzothiophene（DBT） removal efficiency of 99.6% for model oil with high conversion and selectivity but also achieves complete sulfur removal from gasoline as well as 96.7% sulfur removal for distilled diesel at room temperature,successfully achieving ultradeep aerobic oxidative desulfurization. The introduction of rich N3Cvacancies and abundant micromeso-macroporous distribution in M1U3CN enhances kinetic efficiencies by promoting charge carrier separation, mass transfer,and molecular activation simultaneously; resulting in exceptional PODS performance. This work provides a collaborative strategy to overcome kinetic challenges in aerobic oxidative desulfurization via defect and structural engineering of the catalyst.

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Single-cell omics: experimental workflow, data analyses and applications

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Science China Life Sciences 2025年第1期68卷 5-102页

作者： Fengying Sun Haoyan Li Dongqing Sun Shaliu fu Lei Gu Xin Shao Qinqin Wang Xin Dong Bin Duan Feiyang Xing jun Wu Minmin Xiao Fangqing Zhao Jing-Dong J.Han Qi Liu Xiaohui Fan Chen Li Chenfei Wang Tieliu Shi Department of Clinical Laboratory the Affiliated Wuhu Hospital of East China Normal University (The Second People's Hospital of Wuhu City) Pharmaceutical Informatics Institute College of Pharmaceutical SciencesZhejiang University Key Laboratory of Spine and Spinal Cord Injury Repair and Regeneration (Tongji University) Ministry of EducationOrthopaedic DepartmentTongji HospitalBioinformatics DepartmentSchool of Life Sciences and TechnologyTongji University Frontier Science Center for Stem Cells School of Life Sciences and TechnologyTongji University Translational Medical Center for Stem Cell Therapy and Institute for Regenerative Medicine Shanghai East HospitalBioinformatics DepartmentSchool of Life Sciences and TechnologyTongji University Research Institute of Intelligent Computing Zhejiang Lab Shanghai Research Institute for Intelligent Autonomous Systems Center for Single-cell Omics School of Public HealthShanghai Jiao Tong University School of Medicine National Key Laboratory of Chinese Medicine Modernization Innovation Center of Yangtze River DeltaZhejiang University Center for Bioinformatics and Computational Biology Shanghai Key Laboratory of Regulatory Biologythe Institute of Biomedical Sciences and School of Life SciencesEast China Normal University Beijing Institutes of Life Science Chinese Academy of Sciences Peking-Tsinghua Center for Life Sciences Academy for Advanced Interdisciplinary StudiesCenter for Quantitative Biology (CQB)Peking University Zhejiang Key Laboratory of Precision Diagnosis and Therapy for Major Gynecological Diseases Women's HospitalZhejiang University School of Medicine Key Laboratory of Advanced Theory and Application in Statistics and Data Science-MOE School of StatisticsEast China Normal University

Cells are the fundamental units of biological systems and exhibit unique development trajectories and molecular features. Our exploration of how the genomes orchestrate the formation and maintenance of each cell, and control the cellular phenotypes of various organismsis, is both captivating and intricate. Since the inception of the first single-cell RNA technology, technologies related to single-cell sequencing have experienced rapid advancements in recent years. These technologies have expanded horizontally to include single-cell genome, epigenome,proteome, and metabolome, while vertically, they have progressed to integrate multiple omics data and incorporate additional information such as spatial sc RNA-seq and CRISPR screening. Single-cell omics represent a groundbreaking advancement in the biomedical field,offering profound insights into the understanding of complex diseases, including cancers. Here, we comprehensively summarize recent advances in single-cell omics technologies, with a specific focus on the methodology section. This overview aims to guide researchers in selecting appropriate methods for single-cell sequencing and related data analysis.

关键词： single-cell sequencing genome epigenome proteomics metabolomics multimodal spatial transcriptomics CRISPR screening

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Growth characteristics of directionally solidified Al_2O_3/YAG/ZrO_2 ternary hypereutectic in situ composites under ultra-high temperature gradient

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International Journal of Minerals,Metallurgy and Materials 2011年第1期18卷 121-125页

作者： Hai-jun Su jun Zhang Lin Liu heng-zhi fu State Key Laboratory of Solidification Processing Northwestern Polytechnical University Xi＇an 710072 China

Oxide eutectic ceramic in situ composites have attracted significant interest in the application of high-temperature structural materials because of their excellent high-temperature strength,oxidation and creep resistance,as well as outstanding microstructural *** directionally solidified ternary Al2O3/YAG/ZrO2 hypereutectic in situ composite was successfully prepared by a laser zone remelting method,aiming to investigate the growth characteristic under ultra-high temperature *** microstructures and phase composition of the as-solidified hypereutectic were characterized by using scanning electron microscopy（SEM）,energy dispersive spectroscopy（EDS）,and X-ray diffraction（XRD）.The results show that the composite presents a typical hypereutectic lamellar microstructure consisting of fine Al2O3 and YAG phases,and the enriched ZrO2 phases with smaller sizes are randomly distributed at the Al2O3/YAG interface and in Al2O3 *** power and scanning rate strongly affect the sample quality and microstructure ***,coarse colony microstructures were also observed,and their formation and the effect of temperature gradient on the microstructure were discussed.

关键词： eutectics ceramic materials microstructure thermal gradients remelting solidification

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双因子显式二阶积分法

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工程力学 2025年第1期42卷 20-31页

作者：刘慧鹏刘付钧周福霖傅向荣广州大学工程抗震中心广州510006 广州容联建筑科技有限公司广州510180 中国农业大学土木工程系北京100083

研究了一类超收敛的显式二阶积分方法。该方法从哈密顿体系动力相场出发，利用二阶泰勒展开式，构造了动力时程分析迭代算法的基本格式。采用高斯积分处理在迭代步内荷载项的积分，并引入超收敛因子\begin{document}$ \alpha $\end{docu... 详细信息

研究了一类超收敛的显式二阶积分方法。该方法从哈密顿体系动力相场出发，利用二阶泰勒展开式，构造了动力时程分析迭代算法的基本格式。采用高斯积分处理在迭代步内荷载项的积分，并引入超收敛因子\begin{document}$ \alpha $\end{document}和\begin{document}$ \beta $\end{document}来提高算法的收敛步长和计算稳定性。该方法避免了整体刚度矩阵的求逆和相乘，因此不需要进行整体刚度矩阵的组集，是一种快速的新型动力显式积分法。引入超收敛因子后，该算法可大幅提高收敛步长，可在理论时间步长下稳定收敛。数值算例表明：双因子超收敛显式二阶积分法比传统精细积分法具有更高算法稳定性和精度;在合适分析步长下可与常用积分算法保持一致的精度和稳定性，且随着分析步长的增大具有更好的精度稳定性。

关键词：精细积分显式积分超收敛动力时程分析哈密顿体系

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