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Evolution of copper species during heat treatment and its effect on CO oxidation reaction on CuCeZrO_(y) catalyst synthesized by a facile solvent-free route

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Journal of Rare Earths 2024年第4期42卷 660-667页

作者： Guangying fu Dongsen Mao Jun Yu Qiangsheng guo School of Chemical and Environmental Engineering Shanghai Institute of TechnologyShanghai21418 China The ZeoMat Group Qingdao Institute of Bioenergy and Bioprocess TechnologyCASQingdao26611China

Several ternary oxides CuCeZrO_(y)(CCZ)were synthesized by a facile grinding method followed by calcination at high temperatures,and used as catalysts for CO oxidation at low *** influences of calcination temperature(400-600℃)on the physicochemical properties of the assynthesized ternary oxides were investigated by thermogravimetric analysis/differential scanning calorimetry(TGA/DSC),X-ray diffraction(XRD),transmission electron microscopy(TEM),Raman,inductively coupled plasma-optical emission spectrometry(ICP-OES),N_(2) adsorption,H_(2)-temperature programmed reduction(H_(2)-TPR),and X-ray photoelectron spectroscopy(XPS)*** results show that the increase in calcination temperature from 400 to 500℃is conducive to the high dispersion of CuOx on catalyst surface and the incorporation of Cu species into the support to form the Cu-Ce-Zr-O solid *** raising of calcination temperature from 500 to 600℃,however,leads to the segregation of Cu species from the solid solution to aggregate on support surface and growth of highly dispersed CuOx *** highest catalytic activity is acquired over the CCZ calcined at 500℃,which can be ascribed to the largest contents of Cu+species and oxygen vacancies owing to the formation of the maximum amount of Cu-Ce-Zr-O solid solution.

关键词： CuCeZrO_(y)catalyst co oxidation Calcination temperature Grinding method Oxalate precursor Rare earths

Incorporating Lasso Regression to Physics-Informed Neural Network for Inverse PDE Problem

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Computer Modeling in Engineering & Sciences 2024年第10期141卷 385-399页

作者： MengMa Liu fu Xu guo Zhi Zhai National Key Lab of Aerospace Power System and Plasma Technology Xi’an Jiaotong UniversityXi’an710049China School of Mechanical Engineering Xi’an Jiaotong UniversityXi’an710049China Department of Electrical and Computer Engineering University of Massachusetts LowellLowellMA 01854USA

Partial Differential Equation(PDE)is among the most fundamental tools employed to model dynamic *** PDE modeling methods are typically derived from established knowledge and known phenomena,which are time-consuming and ***,discovering governing PDEs from collected actual data via Physics Informed Neural Networks(PINNs)provides a more efficient way to analyze fresh dynamic systems and establish *** study proposes Sequentially Threshold Least Squares-Lasso(STLasso),a module constructed by incorporating Lasso regression into the Sequentially Threshold Least Squares(STLS)algorithm,which can complete sparse regression of PDE coefficients with the constraints of l0 *** further introduces PINN-STLasso,a physics informed neural network combined with Lasso sparse regression,able to find underlying PDEs from data with reduced data requirements and better *** addition,this research conducts experiments on canonical inverse PDE problems and compares the results to several recent *** results demonstrated that the proposed PINN-STLasso outperforms other methods,achieving lower error rates even with less data.

关键词： Physics-informed neural network inverse partial differential equation Lasso regression scientific machine learning

An Intelligent Framework for Resilience Recovery of FANETs with Spatio-Temporal Aggregation and Multi-Head Attention Mechanism

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Computers, Materials & Continua 2024年第5期79卷 2375-2398页

作者： Zhijun guo Yun Sun YingWang Chaoqi fu Jilong Zhong Air Traffic Control and Navigation College Air Force Engineering UniversityXi’an710000China Institute of Systems Engineering Academy of Military ScienceBeijing100101China Equipment Management and UAV Engineering College Air Force Engineering UniversityXi’an710038China Defense Innovation Institute Academy of Military ScienceBeijing100071China

Due to the time-varying topology and possible disturbances in a conflict environment,it is still challenging to maintain the mission performance of flying Ad hoc networks(FANET),which limits the application of Unmanned Aerial Vehicle(UAV)swarms in harsh *** paper proposes an intelligent framework to quickly recover the cooperative coveragemission by aggregating the historical spatio-temporal network with the attention *** mission resilience metric is introduced in conjunction with connectivity and coverage status information to simplify the optimization model.A spatio-temporal node pooling method is proposed to ensure all node location features can be updated after destruction by capturing the temporal network *** with the corresponding Laplacian matrix as the hyperparameter,a recovery algorithm based on the multi-head attention graph network is designed to achieve rapid *** results showed that the proposed framework can facilitate rapid recovery of the connectivity and coverage more effectively compared to the existing *** results demonstrate that the average connectivity and coverage results is improved by 17.92%and 16.96%,respectively compared with the state-of-the-art ***,by the ablation study,the contributions of each different improvement are *** proposed model can be used to support resilient network design for real-time mission execution.

关键词： Resilience cooperative mission FANET spatio-temporal node pooling multi-head attention graph network

Sedimentary Environment and Mineralization of the Black Shale Polymetallic Layer in the Early Cambrian,SW China:Constraints from in situ LA-ICP-MS Analysis of Pyrite

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Acta Geologica Sinica(English Edition) 2024年第2期98卷 416-429页

作者： YANG Zhen fu Yong LI Chao CAI Xi guo Chuan College of Eco-Environmental Engineering Guizhou Minzu UniversityGuiyang 550025China College of Resources and Environmental Engineering Guizhou UniversityGuiyang 550025China Key Laboratory of Karst Georesources and the Environment Ministry of EducationGuizhou UniversityGuiyang 500025China National Research Center for Geoanalysis Chinese Academy of Geological SciencesBeijing 100037China

A polymetallic layer is usually developed at the bottom of the early Cambrian black shale in Guizhou *** mineral that makes up the polymetallic layer is related to the sedimentary *** analyze the differentiation mechanism between polymetallic deposits(Ni-Mo and V),the Zhijin Gezhongwu profile located in the outer shelf and the Sansui Haishan V deposit located in the lower slope are selected to study the in situ sulfur isotopes and trace elements of *** results show that δ^(34)S values of pyrite vary widely from−7.8‰to 28‰in the Gezhongwu profile,while the δ^(34)S values are relatively uniform(from 27.8‰to 38.4‰)in the Haishan *** isotopic S composition is consistent with the transition that occurs in the sedimentary phase from the shelf to the deep sea on the transgressive Yangtze platform;this indicates that the δ^(34)SO_(4)^(2−)values in seawater must be differently distributed in depositional *** sulfur in the Ni-Mo layer is produced after the mixing of seawater and hydrothermal fluid,while the V layer mainly originates from ***,the Ni-Mo and V deposits have been differentiated primarily on the basis of the combined effect of continental weathering and hydrothermal fluid.

关键词： sedimentary environment black shale polymetallic layer pyrite early Cambrian

Unbound^(28)O,the heaviest oxygen isotope observed:a cutting-edge probe for testing nuclear models

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Nuclear Science and Techniques 2024年第2期35卷 1-2页

作者： Jian-guo Li Bai-Shan Hu Shuang Zhang fu-Rong Xu School of Physics and State Key Laboratory of Nuclear Physics and TechnologyPeking UniversityBeijing 100871China Institute of Modern Physics Chinese Academy of SciencesLanzhou 730000China Southern Center for Nuclear-Science Theory(SCNT) Institute of Modern PhysicsChinese Academy of SciencesHuizhou 516000China

The beyond-dripline oxygen isotopes^(27,28)O were recently observed at RIKEN,and were found to be unbound decaying into^(24)O by emitting *** unbound feature of the heaviest oxygen isotope,^(28)O,provides an excellent test for stateof-the-art nuclear *** atomic nucleus is a self-organized quantum manybody system comprising specific numbers of protons Z and neutrons N.

关键词： testing quantum system

Investigation of Maxima Assumptions in Modelling Tropical Cyclone- Induced Hazards in the South China Sea

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China Ocean Engineering 2024年第3期38卷 491-504页

作者： WEN Ze-guo WANG fu-ming WAN Jing YANG Fan School of Civil Engineering Sun Yat-sen University&Southern Marine Science and Engineering Guangdong Laboratory(Zhuhai)Zhuhai 519082China Guangdong Academy of Safety Science and Technology Guangzhou 510060China Guangdong Key Laboratory of Oceanic Civil Engineering Guangzhou 510275China Advanced Energy Science and Technology Guangdong Laboratory(Yangjiang Offshore Wind Energy Laboratory) Yangjiang 529500China

The present study aims to examine the suitability of two commonly used assumptions that simplify modelling metoceanconditions for designing offshore wind turbines in the South China Sea (SCS). The first assumption assumes thatjoint N-year extreme wind and wave events can be independently estimated and subsequently combined. The secondone assumes peak wind and waves can be modelled as occurring simultaneously during a tropical cyclone (TC) *** better understand the potential TC activity, a set of 10000 years synthetic TC events are generated. The wind fieldmodel and the Mike 21 spectral wave model are employed to model the TC-induced hazards. Subsequently, theeffect of the assumptions is evaluated by analyzing the peak structural response of both monopile and semisubmersibleoffshore wind turbines during TC events. The results demonstrate that the examined assumptions are generally *** assessing the implications of these assumptions, valuable insights are obtained, which can inform andimprove the modelling of TC-induced hazards in the SCS region.

关键词： tropical cyclone numerical wave modelling hazards offshore wind turbines structural response

Engineered AAV13 variants with enhanced transduction and confined spread

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Zoological Research 2024年第4期45卷 781-790页

作者： Neng-Song Luo Yu-Xiang Cai Zeng-Peng Han Xiao-Kai Sui Wen-Jia Yuan Zi-lian Zhang Hao-Dong guo Jie Wang Kun-Zhang Lin fu-Qiang Xu Wuhan National Laboratory for Optoelectronics Huazhong University of Science and TechnologyWuhanHubei 430074China Shenzhen Key Laboratory of Viral Vectors for Biomedicine Shenzhen-Hong Kong Institute of Brain ScienceShenzhen Institute of Advanced TechnologyChinese Academy of SciencesShenzhenGuangdong 518055China Key Laboratory of Magnetic Resonance in Biological Systems State Key Laboratory of Magnetic Resonance and Atomic and Molecular PhysicsNational Center for Magnetic Resonance in WuhanInnovation Academy for Precision Measurement Science and TechnologyChinese Academy of SciencesWuhanHubei 430071China Key Laboratory of Quality Control Technology for Virus-Based Therapeutics Guangdong Provincial Medical Products AdministrationNMPA Key Laboratory for Research and Evaluation of Viral Vector Technology in Cell and Gene Therapy Medicinal ProductsBrain Cognition and Brain Disease InstituteShenzhen Institute of Advanced TechnologyChinese Academy of SciencesShenzhenGuangdong 518055China University of Chinese Academy of Sciences Beijing 100049China Zhongnan Hospital Wuhan UniversityWuhanHubei 430072China Brain Case Biotechnology Co. Ltd.ShenzhenGuangdong 518107China College of Life Sciences Wuhan UniversityWuhanHubei 430072China Center for Excellence in Brain Science and Intelligence Technology Chinese Academy of SciencesShanghai 200031China

Precise targeting of specific regions within the central nervous system(CNS)is crucial for both scientific research and gene therapy in the context of brain ***-associated virus 13(AAV13)is known for its restricted diffusion range within the CNS,making it an ideal choice for precise labeling and administration within small brain ***,AAV13 mediates relatively low expression of target ***,we introduced specifically engineered modifications to the AAV13 capsid protein to enhance its transduction *** first constructed AAV13-YF by mutating tyrosine to phenylalanine on the surface of the AAV13 *** then inserted the 7m8 peptide,known to enhance cell transduction,into positions 587/588 and 585/586 of the AAV13 capsid,resulting in two distinct variants named AAV13-587-7m8 and AAV13-585-7m8,*** found that AAV13-YF exhibited superior in vitro infectivity in HEK293T cells compared to AAV13,while AAV13-587-7m8 and AAV13-585-7m8 showed enhanced CNS infection capabilities in C57BL/6 mice,with AAV13-587-7m8 infection retaining a limited spread *** modified AAV13 variants hold promising potential for applications in gene therapy and neuroscience research.

关键词： Adeno-associated virus 13 AAV13-YF AAV13-587-7m8 AAV13-585-7m8 transduction efficiency

Freestanding MoSe_(2)nanoflowers for superior Li/Na storage properties

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Tungsten 2024年第1期6卷 238-247页

作者： Qiao Cu Chao-Qun Shang guo-fu Zhou Xin Wang Guangdong Provincial Key Laboratory of Optical Information Materials South China Normal UniversityGuangzhou 510006China School of Materials Science and Engineering and Hubei Key Laboratory of Plasma Chemistry and Advanced Materials Wuhan Institute of TechnologyWuhan 430205China International Academy of Optoelectronics at Zhaoqing South China Normal UniversityZhaoqing 526060China

MoSe_(2),with high theoretical specific capacity,has attracted a lot of *** remains an open challenge to effectively suppress the irreversible selenium dissolution and rapid capacity decrease induced by severe volume change during ***,we synthesize MoSe_(2)nanoflowers dispersed on one-dimensional(1D)N-doped carbon nanofibers(MoSe_(2)@NCNFs)for use as a freestanding *** this unique structure,the 1D N-doped carbon nanofibers are found to not only enhance the conductivity but also ensure the structural integrity during the Li^(+)/Na^(+)insertion/destraction *** expected,at 2 A·g^(-1),the specific capacity of the MoSe_(2)@NCNFs is maintained at 180 mAh·g^(-1)after 500 cycles when used in lithium storage ***,in the case of sodium storage,at 1 A·g^(-1),the MoSe_(2)@NCNFs shows a capacity of 122mAh·g^(-1)after 500 *** findings suggest that the MoSe_(2)@NCNF electrodes may be a promising candidate for use in reversible Li/Na storage applications.

关键词： Li/Na storage Freestanding electrode MoSe_(2) Electrochemical reaction kinetics Structural integrity

Integrative analysis of metabolome and transcriptome provides new insights into functional components of Lilii Bulbus

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Chinese Herbal Medicines 2024年第3期16卷 435-448页

作者： Wenjun Wei Tao guo Wenguang Fan Mengshan Ji Yu fu Conglong lian Suiqing Chen Wenjing Ma Wenfang Ma Shuying Feng School of Pharmacy Henan University of Chinese MedicineZhengzhou 450046China Henan Engineering Research Center of Medicinal and Edible Chinese Medicine Technology Zhengzhou 450046China School of Life Science and Engineering Lanzhou University of TechnologyLanzhou 730050China Lanzhou Shibai Agricultural Biotechnology Co. Ltd.Lanzhou 730050China Medical College Henan University of Chinese MedicineZhengzhou 450046China

Objective:Lilium brownii ***(LB)and ***(LL)are the main sources of medicinal lily(Lilii Bulbus,Baihe in Chinese)in ***,the functional components of these two species responsible for the treatment efficacy are yet not *** order to explore the therapeutic material basis of Lilii Bulbus,we selected *** ***(LD)only used for food as the control group to analyze the differences between LD and the other two(LB and LL).Methods:Metabolome and transcriptome were carried out to investigate the differences of active components in LD vs LB and LD vs *** of metabolome and transcriptome was analysed using various analysis methods,such as principal component analysis(PCA),hierarchical cluster analysis(HCA),and so *** expressed genes(DEGs)were enriched through KEGG and GO enrichment ***:The PCA and HCA of the metabolome indicated the metabolites were clearly separated and varied greatly in LL and LB contrasted with *** were 318 significantly differential metabolites(SDMs)in LD vs LB group and 298 SDMs in LD vs LL *** with LD group,the significant up-regulation of steroidal saponins and steroidal alkaloids were detected both in LB and LL groups,especially in LB *** HCA of transcriptome indicated that there was significant difference in LB vs LD group,while the difference between LL and LD varied ***,47540 DEGs in LD vs LB group and 18958 DEGs in LD vs LL group were ***,CYP450s involving in the biosynthesis of steroidal saponins and steroidal alkaloids were detected,and comparing with LD,CYP724,CYP710A,and CYP734A1 in LB and CYP90B in LL were all ***:This study suggested that steroidal saponins and steroidal alkaloids maybe the representative functional components of Lilii Bulbus,which can provide new insights for Lilii Bulbus used in the research and development of classic famous formula.

关键词： Lilium browniiF.E.Brown var.viridulum Baker Lilium davidii var.willmottiae(E.H.Wilson) Raffill Lilium lancifolium Thunb. metabolome transcriptome