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A justice and innovative way ahead of consumption-based emission accounting approach

Science China Earth Sciences 2024年第10期67卷 2999-3010页

作者： Qun SHEN Hongbo DUAN Yun tang Linbing tang Li SHANG Xinyu DOU Wei WEI Weiqiang CHEN Zhu LIU State Key Laboratory of Low Carbon Catalysis and Carbon Dioxide Utilization CAS Key Laboratory of Low-Carbon Conversion Science&EngineeringShanghai Advanced Research InstituteChinese Academy of SciencesShanghai 201210China School of Economics&Management University of Chinese Academy of SciencesBeijing 100190China Key Lab of Urban Environment and Health Institute of Urban EnvironmentChinese Academy of SciencesXiamen 361021China Department of Earth System Science Tsinghua UnivesityBeijing 100084China

Carbon emission accounting is an important basis for global climate *** on the consumption-based accounting(CBA)method,the characteristics of carbon flow between national,regional,and product processes could be more clearly ***,CBA is more conducive to clarifying the attribution of responsibilities between producers and consumers,with the principles of fairness and *** accounting for carbon emissions in typical countries from 1990 to 2019,we found that the CBA emissions are higher than the production-based accounting(PBA)emissions in major developed countries,while the results are reversed for developing *** the past 30 years,the CBA emissions in targeted developed countries generally have shown a downward trend,while in developing countries,they have shown an upward *** emissions in China have shown a continuous growth trend from 1990 to 2019,but the pace has slowed down significantly over the last ***,the embodied carbon intensity of China’s exports continues to decline,indicating that China is providing more green and low-carbon products to the *** the PV industry as an example,this study further reveals the contribution of specific product industries to the country’s carbon transfer through product carbon footprint *** order to provide a scientific basis for global mitigation and climate governance,it is urgent to innovate a scientific,practical,and standardized CBA technology system.

关键词： Consumption-based accounting Production-based accounting Carbon transfer Carbon footprint

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Catalytic Asymmetric Synthesis of Inherently Chiral Saddle- Shaped Dibenzo[b,fI[1,5]diazocines

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Chinese Journal of Chemistry 2024年第17期42卷 1953-1959页

作者： Jinmiao Zhou Mengyao tang Xiaoyu Yang Schoolof Physical Science and Technology ShanghaiTech UniversityShanghai 201210China

Dibenzo[b,fi[1,5]diazocines are a class of eight-membered heterocycles,which exhibit unique rigid saddle-shaped structure and possess inherent *** this study,we report a convenient and straightforward method for the catalytic enantioselective synthesis of these unique chiral molecules through chiral phosphoric acid-catalyzed dimerization of ***,the addition of corresponding 2-acylaniline as the co-catalyst significantly improved the efficiency of these reactions,and a simple phase separation operation resulted in products with excellent *** studies were performed to elucidate the mechanism behind these reactions,leading to the proposal of a plausible reaction mechanism based on the study findings.

关键词： Dibenzo[b,f]diazocines Saddle-shaped inherent chirality Organocatalysis Asymmetric catalysis Medium-ring compounds Cooperativecatalysis Chiral phosphoricacids

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Editorial for Machine learning and AI for underground metaverse

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Underground Space 2024年第6期19卷 1-3页

作者： Kok-Kwang Phoon Qiujing Pan Chong tang Information Systems Technology and Design/Architecture and Sustainable Design Singapore University of Technology and DesignSingapore 487372 School of Civil Engineering Central South UniversityChangsha 410075China State Key Laboratory of Coastal and Offshore Engineering Dalian University of TechnologyDalian 116024China

It is widely recognized that civil engineering practice,including underground construction,is lagging the fast pace digital transformation taking place in many *** key reason for this revolution is the emergence and convergence of digital technologies that include machine learning,artificial intelligence(AI),blockchain,cloud/edge computing,Internet of Things,5G communication,automation,digital twin,and *** parallel,Industry 4.0 is now complemented by Industry 5.0 that advocates a shift from economic value to societal value(sustainability,well-being,etc.).This means a shift from enterprises benefiting shareholders(profits)to stakeholders(people).

关键词： learning artificial underground

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一种基于用户行为分析的密钥管理异常检测方法

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通信技术 2023年第2期56卷 226-230页

作者：张文钦唐峯竹中国电子科技集团公司第三十研究所四川成都610041

云计算的发展带来了科技领域的深刻变革,因其便利性、经济性、可扩展性等优势获得了越来越多政企的青睐,与此同时云上应用的安全性也成为各方关注的焦点。密钥安全是密码安全的基础,在云计算环境中,不仅云上的各类应用需要更方便、安全... 详细信息

云计算的发展带来了科技领域的深刻变革,因其便利性、经济性、可扩展性等优势获得了越来越多政企的青睐,与此同时云上应用的安全性也成为各方关注的焦点。密钥安全是密码安全的基础,在云计算环境中,不仅云上的各类应用需要更方便、安全的密钥管理服务,云系统本身也面临着用户数量多、数据量大等问题,亟待划分粒度更细、使用更加灵活的密钥管理方式。在云环境密钥管理的背景下,提出了一种基于用户行为分析的异常检测方法,按各用户的历史行为分析其当前操作的合法性。所提方法具有动态灵活、智能性强的特点,对拒绝服务攻击也具有一定的防护作用。

关键词：用户行为分析云密钥管理异常检测云计算

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Nanoparticle targeting cGAS-STING signaling in disease therapy

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Nano Research 2024年第8期17卷 7315-7336页

作者： Lan Zhou Yu Huang Yuzhang Wu Shupei tang Frontier Medical Training Brigade Third Military Medical UniversityHutubi 831200China Department of Gastroenterology Xinqiao HospitalThird Military Medical UniversityChongqing 400037China Institute of Immunology Third Military Medical UniversityChongqing 400038China Shigatse Branch Xinqiao HospitalThird Military Medical UniversityShigatse 857000China

The cyclic guanosine monophosphate-adenosine monophosphate synthase-stimulator of interferon(IFN)genes(cGAS-STING)signaling pathway is crucial for sensing abnormal DNA accumulation in the *** binds to abnormal DNA,cGAS catalyzes the production of second messenger cyclic dinucleotides,followed by the activation of downstream *** activation induces the expression of type I interferon and other inflammatory cytokines,ultimately initiating an immune *** to the involvement of the cGAS-STING pathway in various diseases,including infection,tumor,autoimmune disease and kidney disease,ongoing research is focused on developing drugs and treatment methods to target and regulate this *** the development of nanotechnology,nanomedicines targeting cGAS-STING signaling are of great significance in clinical applications due to their targeted delivery,controlled drug release,improved solubility,multifunctionality,and enhanced *** comprehensive review focuses on the most recent progress of nanoplatforms targeting cGAS-STING in disease therapy,aiming to provide references and guidelines for further design and optimization of nanomedicines.

关键词： nanomedicine cGAS-STING pathway and related disease anti-tumor nanotherapy anti-viral nanotherapy

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Stability analysis and stabilization of semi-Markov jump linear systems with unavailable sojourn-time information

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Science China(Information Sciences) 2024年第7期67卷 211-223页

作者： Xiaotai WU Yang tang Shuai MAO Ying ZHAO School of Mathematics and Physics Anhui Polytechnic University Key Laboratory of Advanced Control and Optimization for Chemical Processes Ministry of EducationEast China University of Science and Technology

This study addresses the stability and stabilization problems of discrete-time semi-Markov jump linear systems(S-MJLSs) with unavailable sojourn-time information. The sojourn-time probability mass functions(S-TPMFs) of discrete-time semi-Markov chains are no longer confined to the geometric distribution, and it is difficult to obtain accurate and comprehensive information for S-TPMFs in practice. This is because S-TPMFs are usually deduced from the statistical characteristics according to the sampled-data, while adequate samples are often costly and time consuming. In this study, when the S-TPMFs for semi-Markov chains are assumed to be unavailable, the σ-error mean square stability is investigated for discrete-time S-MJLSs with some widely used assumptions; for semi-Markov chains, only the transition probability matrix of the embedded chain is used. In addition, the existence conditions of the effective controller are provided for closed-loop systems without using the information of S-TPMFs. Numerical examples are presented to illustrate the validity of the obtained theoretical results.

关键词： semi-Markov chain semi-Markov jump linear systems σ-error mean square stability unavailable sojourn-time information

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An interesting synergistic effect of heteronuclear dual-atom catalysts for hydrogen production:Offsetting or promoting

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Nano Research 2024年第6期17卷 5742-5752页

作者： Zhonghao Wang Wei tang Jialin Liu Gang Zhou School of Science Hubei University of TechnologyWuhan 430068China

To elucidate the synergistic effect of dual-atom catalysts(DACs)at the microscopic level,we propose and construct a prototype heteronuclear system,CuNi/TiO_(2),in which the two elements of a pair have significantly different d electron-donating abilities,as a piece in the *** density functional theory calculations,we investigate charge-dependent configurations of Cu-Ni dimers anchored on TiO_(2)by the mixing of individual constituent *** d electron-donating ability determines deposition sequence and position of transition metal atoms on oxides,establishing dimer pattern and metal-support *** interaction between Cu and Ni,beyond the coordination environment,predominately contributes to the synergistic effect.A complex adsorption-reduction behavior of H species on CuNi/TiO_(2)is *** reaction mechanism and catalytic activity of CuNi/TiO_(2)for hydrogen production are *** room temperature and high H coverages,CuNi/TiO_(2)shows better performance and efficiency than Ni1/TiO_(2).Our findings provide a new understanding of the synergistic effect on structure-activity relationships of supported dimers,which would be beneficial in the future design of various DACs or even atomically dispersed metal catalysts.

关键词： dual-atom catalysts heteronuclear/homonuclear dimers synergistic effect density functional theory hydrogen production

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Two-dimensional porous carbon derived from pollen with enlarged interlayer distance enhanced electrocatalytic oxidation of n-valeraldehyde to octane

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Nano Research 2024年第5期17卷 3455-3461页

作者： Meichun Qin Chaolong Liu Shouhen Xu Jianguo tang Institute of Hybrid Materials National Center of International Joint Research for Hybrid Materials TechnologyNational Base of International Sci.and Tech.Cooperation on Hybrid MaterialsCollege of Materials Science and EngineeringQingdao UniversityQingdao266071China Department of Pharmaceutics School of PharmacyQingdao UniversityQingdao266071China

Electrocatalytic n-valeraldehyde oxidation reaction was an inexpensive and eco-friendly method to control n-valeraldehyde contamination and produce high value-added ***,low-cost and readily available electrocatalysts with high current efficiency were urgently ***,two-dimensional porous carbon derived from pollen with enlarged interlayer distance was built by alkali activation method,applying in electrocatalytic n-valeraldehyde oxidation *** enlarged interlayer distance was verified by X-ray diffraction(XRD)and high-angle annular dark-field scanning transmission electron microscope(HAADF-STEM).Electrocatalytic experiments consequences showed activated biomass derived carbon possessed a higher electrocatalytic activity and octane selectivity than unactivated *** tests and in situ infrared experiments demonstrated that enlarged interlayer distance was positively correlated with specific surface area of catalysts,large specific surface area provided abundant absorption sites,facilitated the adsorption for n-valeraldehyde,and further promoted the transformation of n-valeraldehyde to *** work also provides a new avenue for creating high-performance electrocatalysts in terms of lattice engineering.

关键词： biomass derived carbon lattice expansion high specific surface area upgrade of n-valeraldehyde

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Causal reasoning in typical computer vision tasks

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Science China(Technological Sciences) 2024年第1期67卷 105-120页

作者： ZHANG KeXuan SUN QiYu ZHAO ChaoQiang tang Yang Key Laboratory of Advanced Control and Optimization for Chemical Process Ministry of EducationEast China University of Science and TechnologyShanghai 200237China National Key Laboratory of Air based Information Perception and Fusion Luoyang 471000China Luoyang Institute of Electro Optical Equipment of Avic Luoyang 471000China

Deep learning has revolutionized the field of artificial *** on the statistical correlations uncovered by deep learning-based methods,computer vision tasks,such as autonomous driving and robotics,are growing *** being the basis of deep learning,such correlation strongly depends on the distribution of the original data and is susceptible to uncontrolled *** the guidance of prior knowledge,statistical correlations alone cannot correctly reflect the essential causal relations and may even introduce spurious *** a result,researchers are now trying to enhance deep learningbased methods with causal *** theory can model the intrinsic causal structure unaffected by data bias and effectively avoids spurious *** paper aims to comprehensively review the existing causal methods in typical vision and visionlanguage tasks such as semantic segmentation,object detection,and image *** advantages of causality and the approaches for building causal paradigms will be *** roadmaps are also proposed,including facilitating the development of causal theory and its application in other complex scenarios and systems.

关键词： causal reasoning computer vision tasks vision-language tasks semantic segmentation object detection

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Underwater inertial error rectification with limited acoustic observations

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Satellite Navigation 2024年第1期5卷 207-223页

作者： Hongqiong tang Hongyang He Fangneng Li Jiangning Xu Department of Navigation Engineering Naval University of EngineeringWuhan430000China

Underwater inertial navigation is particularly difficult for the long-durance operations as many navigation systems such global satellite navigation systems are *** acoustic signal is a marvelous choice for underwater inertial error rectification due to its underwater penetration ***,the traditional Acoustic Positioning Systems(APS)are expensive and incapable of positioning with limited acoustic *** novel underwater inertial error rectification algorithms with limited acoustic observations are *** first one is the single acoustic-beacon Range-only Matching Aided Navigation(RMAN)method,which is inspired by matching navigation without reference maps and presented for the first *** second is the improved single acoustic-beacon Virtual Long Baseline(VLBL)method,which considers the impact of indicated relative position increments on virtual beacon *** RMAN and improved VLBL are further developed when multi acoustic-beacons are available,named mAB-RMAN and *** comprehensive simulations and field investigations were *** results demonstrated that the proposed methods achieved excellent accuracy and stability compared to the baseline,specifically,the mAB-RMAN and mAB-VLBL can reduce the inertial error by more than 90%and 98%when using single and double acoustic-beacons,*** proposed techniques will provide new perspectives for underwater positioning,navigation,and timing.

关键词： Underwater PNT Range-only matching aided navigation Virtual long baseline Inertial error rectification

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