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Pathways of birnessite formation in alkali medium

Science china Earth Sciences 2005年第9期48卷 1438-1451页

作者： feng xionghan1, tan wenfeng1,{2., huang qiaoyun1 & liu Xiangwen2.1. college of resources and environment, huazhong agricultural university, Wuhan 43.070, china 2. Testing Center, china university of Geosciences, Wuhan 430074, china 1. college of resources and {2. Huazhong Agricultural University 430070 Wuhan China 2. Testing Center China University of Geosciences 430074 Wuhan China

Birnessite is a common weathering and oxidation product of manganese-bearing rocks. An O2.oxidation procedure of Mn(OH)2.in the alkali medium has been used to synthesize birnessite. Fast and powder X-ray diffraction (XRD), transmission electron microscopy (TEM), electron diffraction (ED), energy dispersed X-ray analysis (EDAX), infrared spectroscopy (IR) techniques and chemical composition analysis, Eh-pH equilibrium diagram approaches were employed to investigate the reaction process and pathways of birnessite formation. Results showed that the process of the birnessite formation could be divided into four stages: (1) forma- tion stage for hausmannite and feitknechtite, (2. stage of transformation of hausmannite and feitknechtite to buserite, (3) buserite crystal growing stage, and (4) stage of conversion of buser- ite into birnessite. Mn(OH)2.was mainly present as amorphous state only for a short initial time of oxidation reaction. In the oxidation process, buserite formed following two pathways by recrys- tallization after dissolution of the intermediates, and the transformations of the minerals de- pended on the Eh determined by the dissolved O2.concentration on their surfaces. The results are fundamental in further exploration on the mechanism of birnessite formation in the alkali medium. A great practical significance would also be expected with respect to the areas of mate- rial sciences.

关键词： birnessite, pathway of formation, reaction process, Eh-pH diagram, hausmannite, feitknechtite.

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Stochastic community assembly of abundant taxa maintains the relationship of soil biodiversity-multifunctionality under mercury stress

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Soil Ecology Letters 2024年第2期6卷 163-177页

作者： Shuai Du Xin-Qi Li Li Bi Dong Zhu Hang-Wei Hu Xiuli Hao Jiao feng qiaoyun {2. Yu-Rong liu Key Laboratory of Urban environment and Health Ningbo Urban Environment Observation and Research StationInstitute of Urban EnvironmentChinese Academy of SciencesXiamen361021China college of resources and {2. Huazhong Agricultural UniversityWuhan430070China School of Agriculture and Food Faculty of Veterinary and Agricultural SciencesThe University of MelbourneParkvilleVIC3010Australia Hubei Key Laboratory of Soil environment and Pollution Remediation Huazhong Agricultural UniversityWuhan430070China

Soil abundant taxa diversity positively related to multifunctionality under Hg stress.•Microbial network complexity of soil abundant taxa supported the strength of SBF.•Stochastic assembly of soil abundant subcommunity supported the strength of SBF.•Stochastic ratio was the most important predictor for the strength of *** is known that soil microbial communities are intricately linked to multiple ecosystem functions and can maintain the relationship between soil biodiversity and multifunctionality(SBF)under environmental ***,the relative contributions and driving forces of abundant and rare taxa within the communities in maintaining soil biodiversity-multifunctionality relationship under pollution stresses are still ***,we conducted microcosm experiments to estimate the importance of soil abundant and rare taxa in predicting these relationships under heavy metal mercury(Hg)stress in paired paddy and upland *** results revealed that the diversity of abundant taxa,rather than rare taxa,was positively related to multifunctionality,with the abundant subcommunity tending to maintain a larger proportion of soil functions including chitin degradation,protein degradation,and phosphorus *** multitrophic network complexity consisting of abundant species showed positive correlations with biodiversity and multifunctionality,and supported the strength of SBF within a network complexity *** assembly processes of the abundant subcommunity were positively correlated with the strength of SBF,although stochastic processes decreased the biodiversity and the multifunctionality,*** simultaneously accounting for multiple factors on the strength of SBF,we found that the stochastic community assembly ratio of abundant taxa was the most important predictor for SBF strength under Hg *** results highlight the importance of abundant taxa in supporting soil multifunctionality,and elucidate the linkages between co

关键词： abundant taxa biodiversity-multifunctionality relationship community assembly network complexity environmental stresses

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Elemental Composition and Geochemical Characteristics of Iron-Manganese Nodules in Main Soils of china

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Pedosphere 2006年第1期16卷 72-81页

作者： tan Wen-feng {2. fan LI Yong-Hua HU Hong-Qing huang Qiao-Yun college of resources and {2. Huazhong Agricultural University Wuhan 430070 （China）. Institute of Geographical Sciences and Natural resources Research Chinese Academy of Sciences Beijing 100101（China）

Elemental composition and geochemical characteristics of iron-manganese nodules from nine main soils in china were studied by chemical and multivariate statistical analyses to better understand the reactions and functions of iron-manganese nodules in soils and sediment. Compared to the corresponding soils, Mn, Ba, Cd, Co and Pb had strong accumulation, Ni had moderate accumulation, while Ca, Cu, Fe, Na, P, Sr and Zn accumulated to a minor degree in the iron-manganese nodules. In contrast, Si, Al, K, Mg and Ti were reduced in the iron-manganese nodules. The contents of Ba, Cd, Co, Cu, Ni, Pb and Zn were positively and significantly correlated with that of MnO2.in the iron-manganese nodules, while the contents of Cr, Cu, Ni, Pb and Zn were positively and significantly correlated with that of Fe2.3 in soils. Based on a principle component analysis, the elements of iron-manganese nodules were divided into four groups: 1) Mn, Ba, Cd, Co, Cu, Li, Ni, Pb and Zn that were associated with Mn oxides, 2. Fe, Cr and P that were associated with Fe oxides, 3) Si, K, and Mg that were included in the elemental composition of phyllosilicate, and 4) Ca, Na, Al and Ti that existed in todorokite, birnessite, lithiophorite and phyllosilicate. It was suggested that accumulation, mineralization and specific adsorption were involved in the formation processes of soil iron-manganese nodules.

关键词： elemental composition geochemical characteristics iron-manganese nodule soil

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Status of aquatic organisms resources and their environments in Yangtze River system(2.17-2.2.)⋆

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Aquaculture and Fisheries 2024年第5期9卷 833-850页

作者： Haile Yang Li Shen Yongfeng He Huiwu Tian Lei Gao Jinming Wu Zhigang Mei Nian Wei Lin Wang Tingbing Zhu Feifei Hu Jinling Gong Hongchun Du Xinbin Duan Huatang Deng Daoqun Wang fengyue Zhu Yunfeng Li fan Wu Huijun Ru Yan Zhang Junyi Li Junlin Yang Yuntao Zhou Dongdong fang Yinping Wang Danqing Lin Yanping Yang Peijie Li Silei liu Jian Yang Ping Zhuang Sikai Wang Tao Zhang Gang Yang Wenbo Yang Lilai Yuan Kun Cao Shuo Xu Huiyuan liu Zhiqiang Liang Chongrui Wang Hong Li Xiping Yuan Xin Yang Yilong Fu Yanping Zhang Haixin Zhang Zhiying Tao Sheng Wang Xiaoping Gao Binsong Jin Kemao Li Guojie Wang Shenglong Jian Yingqin Li Chenjiang Xue Chunyun Lei Shaowei Xue Yi Sun Bin Zhu Ke Shao Xingkun Hu Meihua Xiong Jun Du Bin He Tao Yan Yingying huang Yuanchao Zou Biwen Xie Yongming Wang Bin Li Fei liu Yaoyao Zhang Fei fan Zhijian Wang Jing huang Haoran Gu Hailong Ge Yan Dan Yan Li Shuqiao Wang Chuang Zhang Lu Zhou Xue Wang Sheng Zeng Yan Xiang Xugang He Jianhui Qin Chengxing Xia Jie Hou Yifu Shi Lifang Gao Zhiqiang Zhu Hongbao Shen Yun Du Xuejun Duan Jiawu Xiong Deguo Yang Shaoping liu Zhaohui Ni Hui Zhang Kai liu feng Zhao Yingren Li Jianwei Wang Qiwei Wei Yangtze River Fisheries Research Institute Chinese Academy of Fishery SciencesWuhan430223China Institute of Hydrobiology Chinese Academy of SciencesWuhan430072China Fishery Resource and environment Research Center Chinese Academy of Fishery SciencesBeijing100141China Key Laboratory of Freshwater Fisheries and Germplasm resources Utilization Ministry of Agriculture and Rural AffairsFreshwater Fisheries Research CenterChinese Academy of Fishery SciencesWuxi214081China East china Sea Fisheries Research Institute Chinese Academy of Fishery SciencesShanghai200090China Institute of Fisheries Engineering Chinese Academy of Fishery SciencesBeijing100141China Hunan Fisheries Science Institute Changsha410153China Jiangxi Fisheries Research Institute Nanchang330039China Jiujiang Academy of Fishery Sciences Jiujiang332000China School of Life Sciences Nanchang UniversityNanchang330031China Qinghai Provincial Fishery Technology Extension Center Xining810012China Yunnan Academy of Fishery Sciences Kunming650111China Institute of Hydroecology Ministry of Water Resources and Chinese Academy of SciencesWuhan430079China Fisheries Institute Sichuan Academy of Agricultural SciencesChengdu611731China School of Life Sciences Neijiang Normal UniversityNeijiang641100China School of Life Sciences Southwest UniversityChongqing400715China Chongqing Fishery Sciences Research Institute Chongqing401120China Guizhou Fisheries Research Institute Guiyang550025China college of Fisheries Huazhong Agricultural UniversityWuhan430072China Hubei Fisheries Science Research Institute Wuhan430070China Shaanxi Fisheries Research Institute Xi’an710086China Innovation Academy for Precision Measurement Science and Technology Chinese Academy of SciencesWuhan430077China Nanjing Institute of Geography and Limnology Chinese Academy of SciencesNanjing210008China Central South Inventory and Planning Institute of State Forestry and Grassland Administration Changsha410014China

The Yangtze River is the mother river of *** promote the aquatic ecosystem protection of the great river,the Project of Yangtze Fisheries resources and environment Investigation(2.17-2.2.)supported by the Ministry of Agriculture and Rural Affairs,*** carried out by 2. institutes and universities that located in the Yangtze River basin surveys the status of(1)fish species composition and spatial distribution,(2.current fish abundance,(3)endangered fishes,(4)Yangtze finless porpoise,(5)aquatic eco-environments,(6)water-level fluctuation areas,(7)capture fisheries and recreational fisheries of the Yangtze River mainstream and 10 of its main tributaries,including Yalong River,Heng River,Min River(including Dadu River),Chishui River,Tuo River,Jialing River,Wu River,Han River,Dongting Lake and Poyang *** results showed that there were 443 fish species(belonging to 163 genus,37 families,and 18 orders)before 2.17,but only 32. fish species(including 15 new recorded exotic species)were recorded in the project of *** them,Cyprinus carpio,Carassius auratus,Hypophthalmichthys molitrix,Pelteobagrus fulvidraco,Coilia brachygnathus,Silurus asotus,Saurogobio dabryi,Ctenopharyngodon idellus,Pelteobagrus nitidus,Hemiculter leucisculus,Siniperca chuatsi,Coreius heterodon,Culter alburnus,Parabramis pekinensis,and Aristichthys nobilis were the dominant species across the whole Yangtze River *** is estimated that there were 886 million individuals weighing 12..8 million kg,merely equivalent to 2..3%of the resources in 1950s,30.9%of the resources in 1960s,or 58.7%of the resources in *** the new list of protected fishes that recorded in the Yangtze River system,only 15 of 2. were collected in this project of *** gladius has been affirmed to be Extinct by International Union for Conservation of Nature(IUCN).The wild individuals of Tenualosa reevesii and Luciobrama macrocephalus have disappeared for many years and maybe have been extinct

关键词： Fishes Yangtze finless porpoise resources Aquatic ecosystem Fisheries Background investigation Yangtze river system

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As(V)浓度和环境因子对硫酸盐绿锈转化的影响及其机制

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化学学报 2017年第6期75卷 608-616页

作者：王小明彭晶徐欢欢谭文峰刘凡黄巧云冯雄汉华中农业大学资源与环境学院农业部长江中下游耕地保育重点实验室武汉430070 华中农业大学农业微生物国家重点实验室武汉430070

绿锈与As(V)可共存于土壤、沉积物和地下水等缺氧环境,但As(V)如何影响绿锈转化过程和机制了解甚少.本工作通过溶液化学和光谱学方法,系统研究了As(V)浓度、pH、温度和空气流速对硫酸盐绿锈(GR)转化的影响.GR转化过程中通过吸附和共沉... 详细信息

绿锈与As(V)可共存于土壤、沉积物和地下水等缺氧环境,但As(V)如何影响绿锈转化过程和机制了解甚少.本工作通过溶液化学和光谱学方法,系统研究了As(V)浓度、pH、温度和空气流速对硫酸盐绿锈(GR)转化的影响.GR转化过程中通过吸附和共沉淀作用对As(V)有极强的去除能力,同时As(V)增强了GR的稳定性,显著影响转化产物的结晶度、矿物类型和生成机制.随As(V)浓度增加,GR氧化转化由溶解-氧化-沉淀机制向固态氧化机制过渡,产物由针铁矿和纤铁矿混合相向纯纤铁矿向纤铁矿、水铁矿和高铁绿锈混合相转变;高As(V)浓度时形成无定形FAsO_4表面沉淀.Fe/As=2.时,pH 6.5~9、温度(5~45℃)和空气流速(0~0.05 m3/h)条件下纤铁矿均为主要产物,随pH和空气流速增加或温度减小纤铁矿结晶度逐渐减弱;高pH或高空气流速或低温有利于高铁绿锈和水铁矿形成,高温有利于针铁矿形成.上述结果对深入理解环境中各种铁氧化物的形成转化机制和As(V)的环境行为有重要意义.

关键词：绿锈 As(V) pH 温度空气流速转化

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稻虾综合种养模式对土壤生物多样性和多重功能的影响

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Science Bulletin 2023年第20期68卷 2311-2315,M0004页

作者：冯娇潘荣胡行伟黄巧云郑娇莉谭文峰刘玉荣 Manuel Delgado-Baquerizo National Key Laboratory of agricultural Microbiology Huazhong Agricultural UniversityWuhan 430070China college of resources and {2. Huazhong Agricultural UniversityWuhan 430070China Faculty of Veterinary and agricultural Sciences The University of MelbourneMelbourne VIC 3010Australia Biopesticide Engineering Research Center Hubei Academy of Agricultural SciencesWuhan 430070China Hubei Key Laboratory of Soil environment and Pollution Remediation Huazhong Agricultural UniversityWuhan 430070China Instituto de Recursos Naturales y Agrobiología de Sevilla(IRNAS) Consejo Superior de Investigaciones CientíficasSevilla E-41012Spain

将水产养殖与农业种植相结合(稻渔综合种养)是提高农产品产量、推动农业绿色发展的重要途径.然而,稻渔综合种养对多营养级土壤生物多样性和多重功能的影响仍然未知.通过对中国19个地区(~1300 km跨度)的131个农田(包含水稻单作和稻虾综... 详细信息

将水产养殖与农业种植相结合(稻渔综合种养)是提高农产品产量、推动农业绿色发展的重要途径.然而,稻渔综合种养对多营养级土壤生物多样性和多重功能的影响仍然未知.通过对中国19个地区(~1300 km跨度)的131个农田(包含水稻单作和稻虾综合种养)进行野外调查发现,与水稻单作相比,稻虾综合种养导致土壤多营养级生物多样性(如真菌vs.无脊椎动物)和生态系统多重服务功能(如支持vs.调节服务)的权衡.本研究为综合评估稻虾综合种养的经济和环境效益提供了新的见解,呼吁在区域范围内合理布局水稻单作和稻虾综合种养面积以优化农田多重生态系统服务功能.

关键词：农产品产量水产养殖营养级农业种植综合种养生态系统多重功能生物多样性

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高校“教研一体化”创新型人才培养模式的探索——以华中农业大学农业资源与环境专业为例

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华中农业大学学报(社会科学版) 2012年第5期 122-126页

作者：黄巧云刘凡刘震冯永平谭文峰戴珂华中农业大学资源与环境学院

培养创新型人才,是当代中国高等教育最重要的历史使命,而"教研一体化"是高校培养创新型人才的重要途径。为了深入推进人才培养改革、加快创新型人才培养,华中农业大学农业资源与环境专业围绕"教研一体化"本科创新型人才培养模式展开了... 详细信息

培养创新型人才,是当代中国高等教育最重要的历史使命,而"教研一体化"是高校培养创新型人才的重要途径。为了深入推进人才培养改革、加快创新型人才培养,华中农业大学农业资源与环境专业围绕"教研一体化"本科创新型人才培养模式展开了一系列探索与实践:开展研究型、探究式、分层次教学和考试评价体系改革;实施本科生科研训练与实践;以高水平的科研支撑高质量的教学;建设教学科研一体化师资和平台等。构建出"教学为基础、科研为支撑,寓教于研、教研融合,教学科研互促共进、协同发展"的教研一体化创新型人才培养模式。

关键词：教研一体化互促共进协同发展创新型人才人才培养模式

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2.05年中国城市CO2.放数据集

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中国人口·资源与环境 2018年第4期28卷 1-7页

作者：蔡博峰刘晓曼陆军王金南刘红光陈洋陈占明丛建辉崔志鹏代春艳董会娟方恺冯彤郭杰李芬孟凡鑫唐伟王庚哲谢运生张建军阿依吐尔逊·沙木西布买日也木·买买提蔡伟光曾胜常盼陈前利陈振国单钰理丁冠乔独威范敏冯相昭干晓宇高壮飞谷雨何凌昊何姚胡鸣明黄丽珍黄桥贾小平菊春燕蓝菁李爽李松李耀光李照令刘合林刘婧文刘庆燕刘竹逯飞马贤磊欧金沛潘栋沈杨税月孙露谭效时唐敏唐袆祺王柯王思亓王香爱王晓培吴家杰吴雪萍肖连香邢文婷徐丽笑叶瑞克袁子坤张飞云张袆张明张琦峰张曦文张宇赵晶赵胜男郑思伟周来友朱天琦曹丽斌冯乐李栋李一静龙瀛孙瑞红环境保护部环境规划院北京100012 中国科学院大气物理研究所北京100029 南京农业大学公共管理学院江苏南京210095 上海财经大学城市与区域科学学院上海200433 中国人民大学经济学院北京100872 山西大学经济与管理学院山西太原030006 E2.环境平台咨询部北京100195 重庆工商大学长江上游经济研究中心重庆400067 上海交通大学环境科学与工程学院上海200240 浙江大学公共管理学院浙江杭州310058 天津大学管理与经济学部天津300072 南京农业大学土地管理学院江苏南京210095 深圳市建筑科学研究院股份有限公司北京研创中心广东深圳518049 华南理工大学环境与能源学院广东广州510006 杭州市环境保护科学研究院环境政策研究中心浙江杭州310014 埃因霍芬理工大学建筑学院荷兰埃因霍芬5616SC 江西省科学院能源研究所江西南昌330000 中国地质大学(北京)土地科学技术学院北京100083 新疆农业大学管理学院新疆乌鲁木齐830052 重庆大学建设管理与房地产学院重庆400044 重庆工商大学财政金融学院重庆400067 东安格利亚大学国际发展学院英国诺维奇NR47TJ 环境保护部环境发展中心北京100029 环境保护部环境与经济政策研究中心北京100029 四川大学建筑与环境学院四川成都610065 浙江工业大学政治与公共管理学院浙江杭州310023 美国绿色建筑委员会城市与社区部北京100085 挪威科技大学工程学院挪威约尔维克2815 北京师范大学统计学院北京100875 青岛科技大学环境学院山东青岛266000 北京大学遥感与地理信息系统研究所北京100871 北京师范大学环境学院北京100875 筑波大学日本筑波305-0005 华中科技大学建筑与城市规划学院湖北武汉430074 美国东北大学工学院美国波士顿02115 河北省环境科学研究院规划所河北石家庄050037 中山大学地理科学与规划学院广东广州北京林业大学环境科学与工程学院北京宁波职业技术学院商贸外语学院浙江宁波重庆工商大学土地管理学院重庆日本国立环境研究所社会环境系统研究中心日本筑波中国船舶重工集团公司第七一四研究所北京重庆工商大学管理学院重庆渭南师范学院化学与材料学院陕西渭南福州大学经济与管理学院福建福州扬州大学环境科学与工程学院江苏扬州中国矿业大学管理学院江苏徐州北京大学城市与环境学院北京内蒙古大学公共管理学院内蒙古呼和浩特江苏大学财经学院江苏镇江赤峰学院资源与环境科学学院内蒙古赤峰新余学院经济管理学院江西新余北京市环境保护科学研究院生态与城市环境研究所北京北京清华同衡规划设计研究院有限公司技术创新中心北京100085 北京大学汇丰商学院英国校区华威大学交叉学科研究方法中心英国牛津100871 清华大学建筑学院北京100062 上海工程技术大学管理学院上海021620

2.05年是中国承诺碳减排目标的基准年份,因而也是中国城市碳减排战略制定和近中期低碳转型的基准年份和对照年份。中国城市2.05年CO_2.放数据的一致性、全面性和精准性对于中国所有城市和每个具体城市的目标考核和评估都有重要意义。... 详细信息

2.05年是中国承诺碳减排目标的基准年份,因而也是中国城市碳减排战略制定和近中期低碳转型的基准年份和对照年份。中国城市2.05年CO_2.放数据的一致性、全面性和精准性对于中国所有城市和每个具体城市的目标考核和评估都有重要意义。基于中国高空间分辨率网格数据(CHRED 2.0)、城市层面统计数据以及大量现场调研和走访,建立2.05年中国城市CO_2.放数据集,包括工业能源排放、工业过程排放、农业排放、服务业排放、城镇生活排放、农村生活排放、交通排放7个部门的直接排放数据和间接排放数据。该数据集的建立汇总了86名研究人员的工作成果,在企业、城市不同行业与部门、城市工业和城市总化石能源等不同层面进行了大量的交叉验证和数据分析,有效保障了数据的精确性和准确性。结果显示,2.05年中国城市碳排放呈现出较大的体量差异和空间格局差异。排放前10的城市几乎比排放后10的城市的排放量高出两个数量级。高排放城市基本都是城市群的核心城市。东部城市直接排放占全国直接排放比例最高,达到44.59%,其次是西部城市2..76%,中部城市2..70%,东北城市10.95%。

关键词：城市 CO 2.放数据集中国高空间分辨率网格

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