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Tungsten 2024年第2期6卷 293-303页

作者： Hao-Zhe Xu Dong Li Ying Chen Pin fang Xiao-Xing ke Olga Demidenko Yu-Jing Li Beijing key Laboratory of Construction Tailorable Advanced Functional Materials and Green Applications Experimental Center of Advanced MaterialsSchool of Materials Science and EngineeringBeijing Institute of TechnologyBeijing 100081China Faculty of Materials and Manufacturing Beijing University of TechnologyBeijing 100124China Scientifi c-Practical Materials Research Centre National Academy of Sciences of Belarus220072 MinskBelarus

Platinum-group-metal-based alloy nanocrystals have been considered as the most effi cient catalysts for oxygen reduction reaction(ORR).However,the poor stability issues limit their further deployment in *** oxide(WO_(3))has received attention due to its intrinsic electrochemical stability and proton absorption/desorption *** this work,we prepared PtCuNi/WO_(3)/C hybrid catalyst with inter-diff usive alloy/WO_(3)interface on *** catalyst exhibits enhanced activity and stability associated with the WO_(3)*** characterization results suggest that the increased activity originates from the complementary proton supply of non-stoichiometric H_(x)WO_(3).Moreover,WO_(3)prevents the particle from dissolution and detachment under vigorous electrochemical *** enhanced stability originates from the electronic interaction established between Pt and *** work provides new strategies to design high-performance ORR catalysts by taking the merits of WO_(3)。

关键词： Tungsten oxide PtCuNi Interface Electronic interaction

FCF-LDH/BiVO4 with synergistic effect of physical enrichment and chemical adsorption for efficient reduction of nitrate

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Green Energy & Environment 2024年第7期9卷 1112-1121页

作者： Yajie Bai Zhenyuan fang Yong Lei Lijing Liu Huaiquan zhao Hongye Bai Weiqiang Fan Weidong Shi School of Chemistry and Chemical Engineering Jiangsu University School of Chemistry Beihang University Institute of Physics & IMN MacroNano Technische Universit?t Ilmenau

Photoelectrochemical NO3-reduction（PEC NITRR） not only provides a promising solution for promoting the global nitrogen cycle,but also converts NO3-to the important chemicals（NH3）.However,it is still a great challenge to prepare catalysts with excellent NO3-adsorption/activation capacity to achieve high ***,we designed a novel Fe2+～Cu2+Fe3+LDH/BiVO4（FCF-LDH/BVO） catalyst with synergistic effect of chemical adsorption and physical ***2+in FCF-LDH/BVO provides the rich Lewis acid sites for the adsorption of NO3-,and the appropriate layer spacing of FCF-LDH further promotes the physical enrichment of NO3-in its interior,thus realizing the effective contact between NO3-and active sites(Fe2+).FCF-LDH/BVO showed excellent NH3production performance(FENH3=66.1%,rNH3=13.8 μg h-1cm-2) and selectivity(FENO2-=2.5%,rNO2-=4.9 μg h-1cm-2) in 0.5 mol *** addition,FCF-LDH/BVO maintains the desirable PEC stability for six cycle experiments,showing great potential for practical ***14NO3-and15NO3-isotope test provides strong evidence for further verification of the origin of N in the generated *** LDH catalyst has a great potential in PEC removal of NO3-from groundwater.

关键词： LDH Lewis acid sites Physical enrichment Photoelectrochemical NO 3 − Reduction Ammonia

Dynamic recrystallization behavior and strengthening mechanism of a novel Mo-Ti_(3)AlC_(2) alloy at ultrahigh temperature

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Rare Metals 2024年第8期43卷 3946-3960页

作者： Lu Yang Xin-Yuan Zheng Yang zhao Xi-Ran Wang fang-Nao Xiao Shi-Zhong Wei School of Materials Science and Engineering Henan University of Science and TechnologyLuoyang 471023China National Joint Engineering Research Center for Abrasion Control and Molding of Metal Materials Henan University of Science and TechnologyLuoyang 471003China Department of Applied Mechanics Univ.Bourgogne FrancheComteFEMTO-ST InstituteCNRS/UF/ENSMM/UTBM25000BesangonFrance

Increasing the recrystallization temperature to achieve better high-temperature performance is critical in the development of molybdenum alloys for ultrahightemperature applications,such as the newest generation of multitype high-temperature nuclear *** this study,an innovative strategy was proposed to improve the performance of molybdenum alloys at high temperature by using the two-dimensional MAX(where M is an early transition metal,A is an A-group element and X is C or N)ceramic material Ti_(3)AlC_(2).The relationships between flow stress,strain rate and temperature were *** microstructure,distribution of misorientation and evolution of dislocations in the Mo-Ti_(3)AlC_(2) alloy were *** microscopic mechanism of the Ti_(3)AlC_(2) phase in the molybdenum alloy at high temperatures was *** experimental results showed that the peak flow stress of Mo-Ti_(3)AlC_(2) at 1600℃ reached 155 MPa,which was161.8% greater than that of pure *** activation energy of thermal deformation of Mo-Ti_(3)AlC_(2) was as large as537 kJ·mol~(-1),which was 17.6% more than that of pure *** recrystallization temperature reached 1600℃ or even *** topological reaction of the Ti_(3)AlC_(2) phase consumed a large amount of energy at high temperatures,resulting in increases in the deformation activation *** structures of AlTi_3 and Ti-O Magneli-phase oxides(Ti_nO_(2n-1)) were formed in-situ,which relied on kink bands and interlayer slip,resulting in many dislocations during ***,the special two-dimensional of the structure Ti_(3)AlC_(2) ceramic inhibited the recrystallization behavior of the Mo *** results of this study can provide theoretical guidance for the development of a new generation of molybdenum alloys for use in ultrahigh-temperature environments.

关键词： Mo alloy Two-dimensional reinforcement Dynamic recrystallization behavior Hot deformation Mechanical properties

Effect of electrical parameters and slag system on macrostructure of electroslag ingot

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China Foundry 2024年第1期21卷 44-50页

作者： Bing-jie Wang Yu Wang Meng-jun Wang Lei zhao Li-zhong Chang Xiao-fang Shi School of Metallurgy engineering Anhui University of TechnologyMa'anshan 243002AnhuiChina

To investigate the influence of electric parameters and slag system on the solidification quality of electroslag ingot during electroslag remelting,different power supply modes,current strengths and remelting slag systems were used to conduct electroslag remelting experiments on 304L austenitic stainless steel,and the macrostructure of electroslag ingots was *** results indicate that the depth of the metal pool decreases with the reduction of remelting frequency in the low frequency power supply *** effects of different power supply modes,such as low-frequency,direct current straight polarity(DCSP),and direct current reverse polarity(DCRP),on reducing the depth of the metal pool increase in that *** reducing the remelting current strength in the same power supply mode,the depth of metal pool is *** compared to the binary slag system of 70%CaF2+30%Al2O3,the ternary slag system of 60%CaF2+20%Al2O3+20%CaO is more effective in reducing the depth of the metal pool during *** the 60%CaF2+20%Al2O3+20%CaO ternary slag system results in a shallower and flatter metal pool,with columnar crystal growth occurring closer to the axial *** effect is observed for both low frequency and direct current(DC)power supply modes.

关键词： electroslag remelting frequency slag system solidification quality

Magnetic NiFe_(2)O_(4)@FeNi_(3)core-shell nanospheres derived from FeNi-LDH precursor anchoring on rGO nanosheets for enhanced electromagnetic wave absorption

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Journal of Materials Science & Technology 2024年第4期171卷 101-114页

作者： Kunyao Cao Yuan fang Shuai Wang Yue Zhang Jiayue Wen Jun Chen Rui zhao Weidong Xue School of Materials and Energy University of Electronic Science and Technology of ChinaChengdu 610054China

Graphene has been extensively utilized in the domain of electromagnetic wave(EMW)absorption ma-terials because of its excellent electrical ***,the inferior impedance matching per-formance and the single loss mechanism vastly restrict the ***,it’s an effective strat-egy to solve these issues by introducing magnetic ***,layer double hydroxide(LDH)is an appropriate template to obtain magnetic component *** that ferromagnetic met-als such as Fe,Co,Ni,and their corresponding metal oxides are usually treated as magnetic compo-nents which are promising candidates for EMW absorption ***,in this work,a FeNi-layered double hydroxide-reduced graphene oxide(FeNi-LDH-rGO)aerogel was synthesized through a series of processes such as electrostatic self-assembly,hydrothermal,freeze-drying,and *** magnetic NiFe_(2)O_(4)@FeNi_(3)core-shell nanospheres were obtained from FeNi-LDH precursor,anchoring on rGO nanosheets after the annealing ***,the effects of different mass ratios of LDH to GO as well as different annealing temperatures of LDH-rGO aerogel on the EMW absorption prop-erty and impedance matching performance were *** a consequence,the fabricated ultralight 600LDH-rGO 2:1 aerogel shows a broad effective absorption bandwidth(EAB)of 7.04 GHz at a thickness of 2.3 mm with a low filling content of only 6 wt%and a low density of 4.4 mg/cm^(3).In conclusion,the synthetic LDH-rGO aerogels offer an effective strategy for preparing EMW absorption materials that own three-dimensional porous network structure and unique magnetic NiFe_(2)O_(4)@FeNi_(3)core-shell struc-ture nanospheres.

关键词： Electrostatic self-assembly Electromagnetic wave absorption LDH-rGO aerogel Layered double hydroxide Reduced graphene oxide NiFe_(2)O_(4)@FeNi_(3)core-shell structure

Simultaneous detection of flare-associated kink oscillations and extreme-ultraviolet waves

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Science China(Technological Sciences) 2024年第5期67卷 1592-1601页

作者： LI Dong HOU ZhenYong BAI XianYong LI Chuan fang Matthew zhao HaiSheng WANG JinCheng NING ZongJun key Laboratory of Dark Matter and Space Astronomy Purple Mountain ObservatoryChinese Academy of SciencesNanjing210023China Yunnan key Laboratory of the Solar Physics and Space Science Kunming650216China School of Earth and Space Sciences Peking UniversityBeijing100871China National Astronomical Observatories Chinese Academy of SciencesBeijing100101China School of Astronomy and Space Science University of Chinese Academy of SciencesBeijing100049China School of Astronomy and Space Science Nanjing UniversityNanjing210023China key Laboratory of Modern Astronomy and Astrophysics Ministry of EducationNanjing UniversityNanjing210023China Columbus Academy GahannaOhio43230USA key Laboratory of Particle Astrophysics Institute of High Energy PhysicsChinese Academy of SciencesBeijing100049China Yunnan Observatories Chinese Academy of SciencesKunming650216China

Kink oscillations,which are frequently observed in coronal loops and prominences,are often accompanied by extreme-ultraviolet(EUV)***,much more needs to be explored regarding the causal relationships between kink oscillations and EUV *** this article,we report the simultaneous detection of kink oscillations and EUV waves that are both associated with an X2.1 flare on 2023 March 03(SOL2023-03-03T17:39).The kink oscillations,which are almost perpendicular to the axes of loop-like structures,are observed in three coronal loops and one *** short loop shows in-phase oscillation within the same period of 5.2 min at three *** oscillation could be triggered by the pushing of an expanding loop and interpreted as the standing kink *** lags are found between the kink oscillations of the short loop and two long loops,suggesting that the kink wave travels in different *** kink oscillations of one long loop and the prominence are possibly driven by the disturbance of the coronal mass ejection(CME),and that of another long loop might be attributed to the interaction of the EUV *** onset time of the kink oscillation of the short loop is nearly same as the beginning of an EUV *** fact demonstrates that they are almost *** EUV wave is most likely excited by the expanding loop structure and shows two *** leading component is a fast coronal wave,and the trailing one could be due to the stretching magnetic field lines.

关键词： coronal loops solar flares solar prominence solar oscillations extreme-ultraviolet wave magnetohydrodynamic

Countermeasure against blinding attack for single-photon detectors in quantum key distribution

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Journal of Semiconductors 2024年第4期45卷 76-81页

作者： Lianjun Jiang Dongdong Li Yuqiang fang Meisheng zhao Ming Liu Zhilin Xie Yukang zhao Yanlin Tang Wei Jiang Houlin fang Rui Ma Lei Cheng Weifeng Yang Songtao Han Shibiao Tang QuantumCTek Co. Ltd.Hefei 230088China Shandong Institute of Quantum Science and Technology Co. Ltd.Jinan 250101China QuantumCTek(Beijing)Co. Ltd.Beijing 100193China School of Cyber Science and Technology University of Science and Technology of ChinaHefei 230027China Anhui Armed Police Force Hefei 230026China School of Electrical Engineering and Automation Anhui UniversityHefei 230601China

Quantum key distribution(QKD),rooted in quantum mechanics,offers information-theoretic ***,practi-cal systems open security threats due to imperfections,notably bright-light blinding attacks targeting single-photon ***,we propose a concise,robust defense strategy for protecting single-photon detectors in QKD systems against blinding *** strategy uses a dual approach:detecting the bias current of the avalanche photodiode(APD)to defend against con-tinuous-wave blinding attacks,and monitoring the avalanche amplitude to protect against pulsed blinding *** integrat-ing these two branches,the proposed solution effectively identifies and mitigates a wide range of bright light injection attempts,significantly enhancing the resilience of QKD systems against various bright-light blinding *** method forti-fies the safeguards of quantum communications and offers a crucial contribution to the field of quantum information security.

关键词： quantum key distribution single photon detector blinding attack pulsed blinding attack countermeasure quan-tum communication

Oxygen-vacancy-rich MnO_(x)supported RuO_(x)for efficient base-free oxidation of 5-hydroxymethylfurfural and 5-methoxymethylfurfural to 2,5-furandicarboxylic acid

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Journal of Energy Chemistry 2024年第8期95卷 670-683,I0015页

作者： Jiali Wu Weizhen Xie Yining Zhang Xixian ke Tianyuan Li Huayu fang Yong Sun Xianhai Zeng Lu Lin Xing Tang Xiamen key Laboratory of Clean and High-valued Applications for Biomass Fujian Engineering and Research Center of Clean and High-valued Technologies for BiomassCollege of EnergyXiamen UniversityXiamen 361102FujianChina key Lab for Sport Shoes Upper Materials of Fujian Province Fujian Engineering and Research Center for New Functional Fiber Materials(Fujian Huafeng New Material Co.Ltd.Putian Dakai New Material Co.Ltd.)Putian 351144FujianChina

2,5-Furandicarboxylic acid(FDCA)is a promising biomass-derived polymeric monomer that serves as an attractive alternative to terephthalic acid derived from fossil ***,the green and efficient production of FDCA through the oxidation of 5-hydroxymethylfurfural(HMF)and its derivatives is still rudimentary under base-free *** this work,oxygen-vacancy-rich Mn Oxwas prepared and displayed a strong adsorption and anchoring ability to Ru species that mainly exposed the(210)plane of RuO_(2),bringing about highly dispersed and active interfacial Ru-O-Mn *** results and density functional theory calculations confirm that these above features greatly facilitate the adsorption/activation of oxygen and the dehydrogenation-oxidation of HMF/5-methoxymethylfurfural(MMF),which enables an efficient FDCA production under base-free and mild ***,a desirable FDCA yield of 86.56%was still obtained from concentrated HMF(10 wt%)under base-free conditions over oxygen-vacancy-rich Mn Oxsupported Ru Ox(1.0 MPaO_(2),120℃,6 h).This work delineates a facile catalyst preparation strategy for HMF/MMF oxidation,and might open a new avenue for the green synthesis of FDCA under base-free conditions.

关键词： Base-free oxidation Oxygen-vacancy-rich 5-Hydroxymethylfurfural 5-Methoxymethylfurfural 2 5-Furandicarboxylic acid

Minerals in edible insects:a review of content and potential for sustainable sourcing

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Food Science and Human Wellness 2024年第1期13卷 65-74页

作者： Mingxing Lu Chenxu Zhu Sergiy Smetana Ming zhao Haibo Zhang fang Zhang Yuzhou Du College of Plant Protection&Institute of Applied Entomology Yangzhou UniversityYangzhou 225009China German Institute of Food Technologies(DIL e.V.) Quakenbrück D-49610Germany Jiangsu Plant Protection and Plant Quarantine Station Nanjing 210036China Joint International Research Laboratory of Agriculture and Agri-Product Safety Yangzhou UniversityYangzhou 225009China

In response to the rapid increase in world population and subsequent demands for food,edible insects represent an alternative food source for humans that is rich in proteins,amino acids and *** is a tradition in many countries including China and Thailand,and edible insects have attracted a lot of attention in Western World due to their suitable nutrient composition,high mineral content(e.g.,Fe,Zn,Ca,Mg)and potential use as a supplement in human *** this study,we surveyed mineral content in seven insect orders and 67 species of mass produced and wild-harvested edible *** total content of essential elements in edible insects was very high in Tenebrio molitor,Bombyx mori,and Zonocerus *** heavy metal content(summarized for eight species)was below the maximum limit allowed for safe *** supply of minerals derived from insect biomass is complicated due to the high variations of mineral content in insects and the potential of its change due to processing.

关键词： Edible insects Minerals Nutrition Food safety Sustainability

Channel Correlation Based User Grouping Algorithm for Nonlinear Precoding Satellite Communication System

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China Communications 2024年第1期21卷 200-214页

作者： ke Wang Baorui Feng Jingui zhao Wenliang Lin Zhongliang Deng Dongdong Wang Yi Cen Genan Wu School of Information and Communication Engineering Beijing University of Posts and TelecommunicationsBeijing 100876China School of Information Engineering Minzu University of ChinaBeijing 100081China Institute of Spacecraft Application System Engineering China Academy of Space TechnologyBeijing 100094China Academy for Network and Communications of CETC Science and Technology on Communication Networks LaboratoryShijiazhuang 050081China

Low Earth Orbit(LEO)multibeam satellites will be widely used in the next generation of satellite communication systems,whose inter-beam interference will inevitably limit the performance of the whole *** precoding such as Tomlinson-Harashima precoding(THP)algorithm has been proved to be a promising technology to solve this problem,which has smaller noise amplification effect compared with linear ***,the similarity of different user channels(defined as channel correlation)will degrade the performance of THP *** this paper,we qualitatively analyze the inter-beam interference in the whole process of LEO satellite over a specific coverage area,and the impact of channel correlation on Signal-to-Noise Ratio(SNR)of receivers when THP is *** user grouping algorithm is proposed based on the analysis of channel correlation,which could decrease the number of users with high channel correlation in each precoding group,thus improve the performance of ***,our algorithm is designed under the premise of co-frequency deployment and orthogonal frequency division multiplexing(OFDM),which leads to more users under severe inter-beam interference compared to the existing research on geostationary orbit satellites broadcasting *** results show that the proposed user grouping algorithm possesses higher channel capacity and better bit error rate(BER)performance in high SNR conditions relative to existing works.

关键词： channel correlation inter-beam interference multibeam satellite Tomlinson-Harashima precoding user grouping