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Design and synthesis of thermally stable single atom catalysts for thermochemical CO_(2) reduction

Journal of Energy Chemistry 2023年第11期86卷 246-262,I0006页

作者： eswaravara prasadarao komarala Ayesha A.Alkhoori Xiaolong Zhang Hui-Ming Cheng Kyriaki Polychronopoulou Department of Mechanical Engineering Khalifa University of Science and TechnologyMain CampusP.O.Box 127788Abu DhabiUnited Arab Emirates Center for Catalysis and Separations Khalifa University of Science and TechnologyP.O.Box 127788Abu DhabiUnited Arab Emirates Shenzhen Key Laboratory of Energy Materials for Carbon Neutrality Shenzhen Institutes of Advanced TechnologyChinese Academy of SciencesShenzhen 518055GuangdongChina Shenyang National Laboratory for Materials Science Institute of Metal ResearchChinese Academy of SciencesShenyang 110016LiaoningChina

The continuous and excessive emission of CO_(2)into the atmosphere presents a pressing challenge for global sustainable *** response,researchers have been devoting significant efforts to develop methods for converting CO_(2)into valuable chemicals and *** conversions have the potential to establish a closed artificial carbon cycle and provide an alternative resource to depleting fossil *** the various conversion routes,thermochemical CO_(2)reduction stands out as a promising candidate for *** the realm of heterogeneous catalysis,single atom catalysts(SACs)have garnered significant *** utilization of SACs offers tremendous potential for enhancing catalytic *** achieve optimal activity and selectivity of SACs in CO_(2)thermochemical reduction reactions,a comprehensive understanding of key factors such as single atom metal-support interactions,chemical coordination,and accessibility of active sites is *** extensive research in this field,the atomic-scale reaction mechanisms in different chemical environments remain largely *** SACs have been found successful applications in electrochemical and photochemical CO_(2)reduction reactions,their implementation in thermochemical CO_(2)reduction encounters challenges due to the sintering and/or agglomeration effects that occur at elevated *** this review,we present a unique approach that combines theoretical understanding with experimental strategies to guide researchers in the design of controlled and thermally stable *** elucidating the underlying principles,we aim to enable the creation of SACs that exhibit stable and efficient catalytic activity for thermochemical CO_(2)reduction ***,we provide a comprehensive overview of recent literature on noble metal-and transition metal-based SACs for thermochemical CO_(2)*** current review is focused on certain CO_(2)-derived products involving one

关键词： CO_(2) utilization CO_(2) conversion SACs Added-value products Thermochemical catalysis

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