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Cationic ordering transition in oxygen-redox layered oxide cathodes

Carbon Energy 2024年第1期6卷 197-206页

作者： Xinyan Li Ang gao Qinghua Zhang Hao Yu Pengxiang Ji Dongdong Xiao Xuefeng Wang Dong Su Xiaohui Rong Xiqian Yu Hong Li Yong-sheng Hu Lin Gu Beijing National Laboratory for Condensed Matter Physics Institute of PhysicsChinese Academy of SciencesBeijingChina College of Materials Science and Opto-Electronic Technology University of Chinese Academy of SciencesBeijingChina Beijing National Center for Electron Microscopy and Laboratory of Advanced Materials School of Materials Science and EngineeringTsinghua UniversityBeijingChina Beijing Advanced Innovation Center for Materials Genome Engineering Huairou DivisionInstitute of PhysicsChinese Academy of SciencesBeijingChina

Understanding the structural origin of the competition between oxygen 2p and transition-metal 3d orbitals in oxygen-redox(OR)layered oxides is eminently desirable for exploring reversible and high-energy-density Li/Na-ion ***,we reveal the correlation between cationic ordering transition and OR degradation in ribbon-ordered P3-Na_(0.6)Li_(0.2)Mn_(0.8)O_(2) via in situ structural *** two different voltage windows,the OR capacity can be improved approximately twofold when suppressing the in-plane cationic ordering *** find that the intralayer cationic migration is promoted by electrochemical reduction from Mn^(4+)to Jahn–Teller Mn^(3+)and the concomitant NaO_(6) stacking transformation from triangular prisms to octahedra,resulting in the loss of ribbon ordering and electrochemical ***-principles calculations reveal that Mn^(4+)/Mn^(3+)charge ordering and alignment of the degenerate eg orbital induce lattice-level collective Jahn–Teller distortion,which favors intralayer Mn-ion migration and thereby accelerates OR *** findings unravel the relationship between in-plane cationic ordering and OR reversibility and highlight the importance of superstructure protection for the rational design of reversible OR-active layered oxide cathodes.

关键词： cationic ordering layered oxide cathodes oxygen redox sodium-ion batteries

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In vivo imaging reveals a synchronized correlation among neurotransmitter dynamics during propofol and sevoflurane anesthesia

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Zoological Research 2024年第3期45卷 679-690页

作者： gao-Lin Qiu Li-Jun Peng Peng Wang Zhi-Lai Yang Ji-Qian Zhang Hu Liu Xiao-Na Zhu Jin Rao Xue-sheng Liu Department of Anesthesiology First Affiliated Hospital of Anhui Medical UniversityHefeiAnhui 230022China School of Life Science and Technology ShanghaiTech UniversityShanghai 201210China

General anesthesia is widely applied in clinical ***,the precise mechanism of loss of consciousness induced by general anesthetics remains ***,we measured the dynamics of five neurotransmitters,includingγ-aminobutyric acid,glutamate,norepinephrine,acetylcholine,and dopamine,in the medial prefrontal cortex and primary visual cortex of C57BL/6 mice through in vivo fiber photometry and genetically encoded neurotransmitter sensors under anesthesia to reveal the mechanism of general anesthesia from a neurotransmitter *** revealed that the concentrations of γ-aminobutyric acid,glutamate,norepinephrine,and acetylcholine increased in the cortex during propofol-induced loss of *** levels did not change following the hypnotic dose of propofol but increased significantly following surgical doses of propofol ***,the concentrations of the five neurotransmitters generally decreased during sevoflurane-induced loss of ***,the neurotransmitter dynamic networks were not synchronized in the non-anesthesia groups but were highly synchronized in the anesthetic *** findings suggest that neurotransmitter dynamic network synchronization may cause anesthetic-induced loss of consciousness.

关键词： General anesthesia Loss of consciousness In vivo neurotransmitter imaging Medial prefrontal cortex Primary visual cortex

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The energy response of LaBr_(3)(Ce),LaBr_(3)(Ce,Sr),and NaI(Tl)crystals for GECAM

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Nuclear Science and Techniques 2024年第2期35卷 110-122页

作者： Pei-Yi Feng Xi-Lei Sun Zheng-Hua An Yong Deng Cheng-er Wang Huang Jiang Jun-Jie Li Da-Li Zhang Xin-Qiao Li Shao-Lin Xiong Chao Zheng Ke Gong sheng Yang Xiao-Jing Liu Min gao Xiang-Yang Wen Ya-Qing liu Yan-Bing Xu Xiao-Yun Zhao Jia-Cong Liu Fan Zhang Hong Lu Particle and Astrophysics Center Institute of High Energy PhysicsChinese Academy of SciencesBeijing 100049China Key Laboratory of Particle Astrophysics Institute of High Energy PhysicsChinese Academy of SciencesBeijing 100049China University of Chinese Academy of Sciences Chinese Academy of SciencesBeijing 100049China Experimental Physics Center Institute of High Energy PhysicsChinese Academy of SciencesBeijing 100049China State Key Laboratory of Particle Detection and Electronics Institute of High Energy PhysicsChinese Academy of SciencesBeijing 100049China School of Nuclear Science and Technology University of South ChinaHengyang 421001China National Engineering Research Center for Rare Earth Grirem Advanced Materials Co.Ltd.and General Research Institute for Nonferrous MetalsBeijing 100088China

The GECAM series of satellites utilizes LaBr_(3)(Ce),LaBr_(3)(Ce,Sr),and NaI(Tl)crystals as sensitive materials for gamma-ray detectors(GRDs).To investigate the nonlinearity in the detection of low-energy gamma rays and address the errors in the calibration of the E-C relationship,comprehensive tests and comparative studies of the three aforementioned crystals were conducted using Compton electrons,radioactive sources,and mono-energetic *** nonlinearity test results of the Compton electrons and X-rays demonstrated substantial differences,with all three crystals presenting a higher nonlinearity for X/-rays than for Compton *** the LaBr_(3)(Ce)and LaBr_(3)(Ce,Sr)crystals having higher absolute light yields,they exhibited a noticeable nonlinear decrease in the light yield,especially at energies below 400 *** NaI(Tl)crystal demonstrated an"excess"light output in the 6-200 keV range,reaching a maximum"excess"of 9.2%at 30 keV in the X-ray testing and up to 15.5%at 14 keV during Compton electron testing,indicating a significant advantage in the detection of low-energy gamma ***,we explored the underlying causes of the observed nonlinearity in these *** study not only elucidates the detector responses of GECAM,but also initiates a comprehensive investigation of the nonlinearity of domestically produced lanthanum bromide and sodium iodide crystals.

关键词： LaBr_(3)(Ce)detector LaBr_(3)(Ce,Sr)detector NaI(Tl)detector GECAM Energy response Light yield nonlinearity

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Survey on Pre-pregnancy Health Knowledge and Service Demands among Un-pregnant Married Women

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Journal of Reproduction and Contraception 2006年第3期17卷 195-200页

作者： Yu-hua LI Hong LIANG Li-feng ZHOU Ren-li WANB er-sheng gao Wen-ping SHEN Yue DONG Zhi-hui GU Rui-zhu CHEN Wei-jue CAO Guo-liang ZHOU Xiao-ping ZHOU Epidemiology and Social Science Department of Shanghai institnte of Planned parenthood Research Shanghai 20032 China Population and Family Planning Commission of Xuhui District Shanghai 200030 China

Objective To understand the pre-pregnancy health knowledge and service needs among un-pregnant married women in Shanghai. Methods A total of 968 newly-married un-pregnant women in Changqiao, Lingyun sub-districts and Huajing town of Xuhui district, Shanghai, were recruited and interviewed by structured questionnaire to collect the information on pre-pregnancy health knowledge and service demands. Results 1） Newly-married women thought the contraceptive methods suitable for them was male condom（84.4%）, followed by oral contraceptives（54%）, emergent contraceptive（52.5%） and contraceptive suppository （48.3%）. 2） The score of pre-pregnancy health knowledge was 54.7±14.5 among the subjects. The participants with junior college or a bachelor had more knowledge than those with junior or senior high school, and those who were engaged in medicine /education/science field had higher score. 3） They had higher knowing rate on the common knowledge, and the rate was above 80%. But the knowing rate on the knowledge of birth defect was low, and all below 50%. 4）A proportion of 52. 7% of the respondents knew that there was a station for reproductive health service in their communities, but only 45.5% received the service from the station, 87.0% thought they had insufficient or scarce knowledge, 73.6% planned to consult before pregnancy training courses on preparing pregnancy. and 63.6% were willing to attend the Conclusion The participants had certain pre-pregnancy health knowledge, but still need being improved,＂ in addition, they had higher needs on knowledge and service of birth defect prevention, at the same time they can＇t make full use of the existing reproductive health institution.

关键词： un-pregnant women pre-pregnancy health knowledge service use demand

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Removal and fluorescence detection of antibiotics from wastewater by layered double oxides/metal-organic frameworks with different topological configurations

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Chinese Chemical Letters 2024年第8期35卷 401-405页

作者： Zhiqiang Liu Qiang gao Wei Shen Meifeng Xu Yunxin Li Weilin Hou Hai-Wei Shi Yaozuo Yuan erwin Adams Hian Kee Lee sheng Tang School of Environmental and Chemical Engineering Jiangsu University of Science and TechnologyZhenjiang 212003China National Medical Products Administration Key Laboratory for Impurity Profile of Chemical Drugs Nanjing 210019China Chemical Drug Inspection Laboratory 2 Jiangsu Institute for Food and Drug ControlNanjing 210019China Department of Pharmaceutical and Pharmacological Sciences Pharmaceutical AnalysisKU LeuvenHerestraat 49O&N2PB 923Leuven B-3000Belgium Department of Chemistry National University of Singapore3 Science Drive 3Singapore 117543Singapore

Owing to the serious potential side-effects on the environment and human health,the rapid detection and removal of antibiotics have become an important research *** this work,four zinc-based metal-organic frameworks(MOFs)with different functional groups,i.e.,Zn-MOF,Zn-MOF-CH_(3),Zn-MOF-NO_(2),Zn-MOF-COOH,were utilized for the construction of LDO/MOF composite materials with a nickel-iron-cobalt-based layered double oxide,*** results showed that the LDO/MOF composites not only had high sensitivity in detecting sulfonamide and quinolone antibiotics,but also had an appreciable ability to adsorb them from *** maximum adsorption capacities of all the four types of LDO@Zn-MOFs to all antibiotics can at least reach 150 mg/g,and the limits of detection in relation to all four antibiotics were at least as low as 100μg/*** work suggested the dual-function extraction performance can be attributed to the synergistic effects between the LDO and the ***,the strong ferromagnetism derived from the LDO provided great convenience for the separation and regeneration of the LDO/MOF composites.

关键词： Light-emitting metal-organic frameworks Layered double oxides Antibiotics Topological configurations Fluorescence detection

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Multivariate relationships between microstructure evolution and strengthening mechanisms in laser powder bed fusion of Al-Mn-Sc alloy:towards improved fatigue performance

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Light(Advanced Manufacturing) 2024年第1期5卷 3-18页

作者： Huaping Tang Chaofeng gao Shiheng Zhang Xiaojing Xiong sheng Cao Xiaopeng Wu Yunjie Bi Jeremy Heng Rao Institute of Advanced Additive Manufacturing Ji Hua LaboratoryFoshanGuangdong528200China Department of Mechanical Engineering College of EngineeringShantou UniversityShantouGuangdong515063China School of Materials Science and Engineering Northeastern UniversityShenyang 110819China

The effects of direct aging treatment(at 300°C for 5 hours)on selective laser melted(SLMed)Al-4.5Mn-1.5Mg-0.9Sc-0.2Zr alloy were investigated in this work,with the microstructure,fatigue behaviors,and fracture characteristics examined to determine the primary cause of fatigue crack *** results revealed that the microstructure of the investigated alloy comprised fine equiaxed and columnar *** aging treatment,a significant number of nano-scaled Al3(Sc,Zr)precipitates were dispersed within the grains,leading to a substantial increase in *** yield strength improved from 431 MPa to 568 MPa,representing an increase of more than 32%,while the fatigue strength improved from 180 MPa to 220 MPa after aging ***,the fracture toughness decreased significantly from 25.1 MPa·√m to 12.3 MPa·√*** results of the fatigue fracture characteristics indicate that the Mn-rich phase and the formation of defects such as pores and poor powder fusion are the sources of fatigue *** direct aging treatment can significantly increase the yield strength,decrease the rate of fatigue crack propagation,and thus improve the fatigue performance,it deteriorates the fracture toughness,and thus shortens the fatigue life of the alloy as well.

关键词： Selective laser melting Al-Mn-Sc alloys High-cycle fatigue

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Alternaria TeA toxin activates a chloroplast retrograde signaling pathway to facilitate JAdependent pathogenicity

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Plant Communications 2024年第3期5卷 123-140页

作者： Jiale Shi He Wang Mengping Li Liru Mi Yazhi gao sheng Qiang Yu Zhang Dan Chen Xinbin Dai Hongyu Ma Huan Lu Chanhong Kim Shiguo Chen Weed Research Laboratory Nanjing Agricultural UniversityNanjing 210095China Shanghai Center for Plant Stress Biology Center for Excellence in Molecular Plant SciencesChinese Academy of SciencesShanghai 200032China Bioinformatics and Computational Biology Laboratory Noble Research Institute2510 Sam Noble ParkwayArdmoreOK 73401USA College of Plant Protection Nanjing Agricultural UniversityNanjing 210095China Department of Botany and Plant Biology University of GenevaGenevaSwitzerland

The chloroplast is a critical battleground in the arms race between plants and *** microbe-secreted mycotoxins,tenuazonic acid(TeA),produced by the genus Alternaria and other phytopathogenic fungi,inhibits photosynthesis,leading to a burst of photosynthetic singlet oxygen(1O2)that is implicated in damage and chloroplast-to-nucleus retrograde *** the signicant crop damage caused by Alternaria pathogens,our understanding of the molecular mechanism by which TeA promotes pathoge-nicity and cognate plant defense responses remains *** now reveal that *** induces necrotrophic foliar lesions by harnessing EXECUTer1(EX1)/EX2-mediated chloroplast-to-nucleus retro-grade signaling activated by TeA toxin–derived photosynthetic 1O2 in Arabidopsis *** of the 1O2-sensitive EX1-W643 residue or complete deletion of the EX1 singlet oxygen sensor domain compro-mises expression of 1O2-responsive nuclear genes and foliar *** also found that TeA toxin rapidly induces nuclear genes implicated in jasmonic acid(JA)synthesis and signaling,and EX1-mediated retro-grade signaling appears to be critical for establishing a signaling cascade from 1O2 to *** present study sheds new light on the foliar pathogenicity of ***,during which EX1-dependent 1O2 signaling in-duces JA-dependent foliar cell death.

关键词： TeA mycotoxin Alternaria pathogen chloroplast singlet oxygen retrograde signaling jasmonic acid

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生活技能培训对职校生生殖健康认知的影响

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生殖与避孕 2009年第1期29卷 31-37页

作者：楼超华王筱金涂晓雯高尔生上海市计划生育科研所上海200032

目的:评价生活技能培训对职校生生殖健康认知的影响。方法:上海市区3所职校为研究现场,其中2所为干预学校,1所为对照学校,研究对象为二年级的学生。干预组采取以生殖健康为核心的生活技能培训加同伴教育和单一生活技能培训2种不同的干... 详细信息

目的:评价生活技能培训对职校生生殖健康认知的影响。方法:上海市区3所职校为研究现场,其中2所为干预学校,1所为对照学校,研究对象为二年级的学生。干预组采取以生殖健康为核心的生活技能培训加同伴教育和单一生活技能培训2种不同的干预模式,干预活动持续1个学年。通过干预前后电脑问卷调查评价干预效果。结果:与基线调查时相比,干预后干预组对象的生殖健康风险(发生妊娠、感染性病和艾滋病)认知、避孕套使用的收益认知和避孕方法选择的自我效能上升,避孕套使用的障碍认知则下降,差异有统计学意义(P<0.05),而对照组的变化不明显。以基线和终线2次调查对象的生殖健康认知(即风险认知、收益认知、障碍认知和自我效能)评分为应变量,拟合重复测量资料的混合效应模型显示,在调整了其它可能的混杂因素后,组别与时间的交互作用项在4个模型中都有统计学意义(P<0.05),提示生活技能培训可提高职校生的生殖健康风险与避孕相关认知。2种干预模式(生活技能培训加同伴教育与单一生活技能培训)的作用仅在避孕套使用的收益认知上有差异。结论:生活技能培训可有效提高职校生的生殖健康认知,可以作为对年轻人进行性相关问题教育的一种重要方法。

关键词：生活技能培训生殖健康认知职校生

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Yinhuang granule alleviates carbon tetrachloride-induced liver fibrosis in mice and its mechanism

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World Journal of Hepatology 2024年第2期16卷 264-278页

作者： Hao Ouyang Hui Miao Zhen Li Duan Wu Si-Cheng gao Yao-Yao Dai Xiao-Di gao Hai-sheng Chai Wei-Ye Hu Jun-Feng Zhu Department of Liver Yueyang Hospital of Integrated Traditional Chinese and Western MedicineShanghai University of Traditional Chinese MedicineShanghai 201203China State Key Laboratory of Bioreactor Engineering East China University of Science and TechnologyShanghai 201203China

BACKGROUND Liver fibrosis is a formidable global medical challenge,with no effective clinical treatment currently *** granule(YHG)is a proprietary Chinese medicine comprising Scutellariae Radix and Lonicerae Japonicae *** is frequently used for upper respiratory tract infections,pharyngitis,as well as acute and chronic *** To investigate the potential of YHG in alleviating carbon tetrachloride(CCl4)-induced liver fibrosis in *** To induce a hepatic fibrosis model in mice,this study involved intraperitoneal injections of 2 mL/kg of CCl4 twice a week for 4 ***,liver fibrosis mice in the low dose of YHG(0.4 g/kg)and high dose of YHG(0.8 g/kg)groups were orally administered YHG once a day for 4 *** alanine/aspartate aminotransferase(ALT/AST)activity and liver hydroxyproline content were *** red and Masson's trichrome staining assay were *** polymerase chain reaction,western-blot and enzyme-linked immunosorbent assay were *** glutathione content,superoxide dismutase activity level,reactive oxygen species and protein carbonylation amount were *** The administration of YHG ameliorated hepatocellular injury in CCl4-treated mice,as reflected by decreased serum ALT/AST activity and improved liver histological *** also attenuated liver fibrosis,evident through reduced liver hydroxyproline content,improvements in Sirius red and Masson's trichrome staining,and lowered serum hyaluronic acid ***,YHG hindered the activation of hepatic stellate cells(HSCs)and ameliorated oxidative stress injury and inflammation in liver from CCl4-treated *** prompted the nuclear accumulation of nuclear factor erythroid 2-related factor 2(Nrf2)and upregulated the expression of Nrf2-dependent downstream antioxidant *** addition,YHG promoted mitochondrial biogenesis in liver from CCl4-treated mice,as demonstrated by increased liver adenosine triphosphate content,

关键词： Yinhuang granule Liver fibrosis Hepatic stellate cells Oxidative injury Nuclear factor erythroid 2-related factor 2 Inflammation

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职校生的性与生殖健康认知现况及需求

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生殖与避孕 2009年第2期29卷 88-91页

作者：陈晓涂晓雯楼超华应笑高尔生复旦大学公共卫生学院上海200032 上海市计划生育科学研究所上海200032

目的:了解上海市职校生性与生殖健康知识的认知程度和服务需求。方法:于2005年9月对上海市三所职校全体一年级1846名学生进行匿名自填式问卷横断面调查。结果:职校生的性与生殖健康知识水平普遍较低,总知识得分为33.5分;性态度开放,约... 详细信息

目的:了解上海市职校生性与生殖健康知识的认知程度和服务需求。方法:于2005年9月对上海市三所职校全体一年级1846名学生进行匿名自填式问卷横断面调查。结果:职校生的性与生殖健康知识水平普遍较低,总知识得分为33.5分;性态度开放,约有一半的学生认可婚前性行为;65%的职校生在青春期遇到过相关的困惑或问题;84%的学生觉得自己缺乏性与生殖健康知识;54%的职校生在初中时没接受过正规的性与生殖健康教育;65%的职校生认为有必要建立专门针对青少年的服务机构。结论:现有的性与生殖健康教育和服务不能满足职校生的需求,应进一步加强针对职校生的相关教育和服务,尤其是学校。

关键词：职校生性教育生殖健康服务需求

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