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Wearable sensors and supercapacitors using electroplated-Ni/ZnO antibacterial fabric

Journal of Materials Science & Technology 2022年第5期100卷 254-264页

作者： Taegun Kim Chanwoo park edmund p.samuel Yong-Il Kim Seongpil An Sam S.Yoon School of Mechanical Engineering Korea UniversitySeoul 02841Republic of Korea KU-KIST Green School Korea UniversitySeoul 136-713Republic of Korea SKKU Advanced Institute of Nanotechnology(SAINT)and Department of Nano Engineering Sungkyunkwan University(SKKU)Suwon 16419Republic of Korea

Herein,nickel nanocones and zinc oxide nanosheets were electroplated onto a fabric to produce multifunctional(wearable,stretchable,washable,hydrophobic,and antibacterial)materials with sensing,heating,and supercapacitive *** these functionalities are integrated into a one-layered fabric that can be used as a portable intelligent electronic textile for potential application in healthcare monitoring,smart sportswear,and energy *** nickel enhances the electrical conductivity and thus increases the electron charge transfer for supercapacitor *** integration of ZnO with the Ni-plated fabric provides pseudocapacitance via redox reactions with the *** resistance of the Ni/ZnO fabric changes in response to external stimuli such as temperature and *** voltage is applied,the fabric generates heat through Joule heating,demonstrating its potential application as winter *** superior mechanical durability of the fabric was confirmed through bending and stretching *** hydrophobic surface prevents viruses contained in liquid droplets from infiltrating the *** addition,bacterial growth is inhibited because of the antibacterial properties of the Ni/ZnO fabric and because of Joule *** one-layered fabric integrated with such multiple functionalities is expected to be applicable in the development of next-generation portable and wearable electronic textiles in various industries.

关键词： Multifunctional conductive fabric Fabric supercapacitor Fabric heater Thermal and strain sensors Electroplating

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Supersonically sprayed self-aligne d rGO nanosheets and ZnO/ZnMn_(2)O_(4)nanowires for high-energy and high-power-density supercapacitors

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Journal of Materials Science & Technology 2023年第6期137卷 193-204页

作者： Chanwoo park edmund samuel Byeong-Yeop Kim Seongpil An Hae-Seok Lee Sam S.Yoon School of Mechanical Engineering Korea UniversitySeoul 02841Republic of Korea Energy Environment policy and Technology Graduate School of Energy and Environment(KU-KIST Green School)Korea UniversityRepublic of Korea SKKU Advanced Institute of Nanotechnology(SAINT)and Department of Nano Engineering Sungkyunkwan University(SKKU)Suwon 16419Republic of Korea

Core-shell-type bimetallic oxide and carbon composites comprising zinc oxide(ZnO)nanospheres and zinc manganese oxide(ZnMn_(2)O_(4))nanowires were produced by a hydrothermal method,and supersoni-cally sprayed together with reduced graphene oxide(rGO)nanosheets onto Ni foil to fabricate flexible *** supersonic impact facilitated the exfoliation of the rGO nanosheets,thereby increasing the surface area and adhesion of the composite particles to the *** rGO nanosheets were vertically aligned during the supersonic impact and formed localized zones,enabling optimal accommodation of the ZnO/ZnMn_(2)O_(4)*** localization,with the addition of rGO,reduced the agglomeration of ZnO/ZnMn_(2)O_(4)*** molar concentration of MnSO_(4)used in the synthesis of ZnO/ZnMn_(2)O_(4)was varied from 0.05 to 0.15 mol/L to determine the optimal MnSO_(4)concentration that would result in the highest energy storage *** unique nanostructure of ZnO/ZnMn_(2)O_(4)and the self-alignment of rGO sheets facilitated a favorable environment for high energy storage capability with a specific capaci-tance of 276.3 mF·cm^(−2)at a current density of 0.5 mA·cm^(−2)and an energy density of 98.2μWh·cm^(−2)at a power density of 1600μW·cm^(−2).The width of the potential window was increased to 1.2 V,imply-ing a significant increase in the energy storage capability of the *** retention of 88%was achieved after 10,000 charge/discharge cycles for the supercapacitor fabricated using an optimal MnSO_(4)concentration(0.10 mol/L)during the composite synthesis.

关键词： ZnO/ZnMn_(2)O_(4)nanowires rGO nanosheets Hydrothermal method Supersonic spraying Supercapacitor

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Bimetallic zeolitic imidazolate framework-derived substrate-free anode with superior cyclability for high-capacity lithium-ion batteries

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Journal of Materials Science & Technology 2021年第8期67卷 116-126页

作者： Bhavana Joshi edmund samuel Yong-il Kim Govindasami periyasami Mostafizur Rahaman Sam S.Yoon School of Mechanical Engineering Korea UniversitySeoul136-713Republic of Korea Department of physics NES Science CollegeSwami Ramanand Teerth Marathwada UniversityLatur RoadNandedMaharashtra431606India Department of Chemistry College of ScienceKing Saud UniversityRiyadh11451Saudi Arabia

Freestanding carbon nanofibers loaded with bimetallic hollow nanocage structures were *** nanocages inherited the rhombic dodecahedral morphology of the zeolitic imidazolate framework(ZIF)precursors,ZIF-8 and *** anode materials for lithium-ion batteries(LIBs),the bimetallic nanocage-loaded freestanding carbon nanofibers effectively buffered volume expansions and alleviated pulverization through their different reduction and oxidation *** higher capacities of the composite anodes arose via the formation of the Li_(x)Zn alloy and Li_(2)O by Zn and Co ions,respectively,and the enhanced conductivity conferred by the carbon nanofibers.A synergistic effect of the composite components toward the strong electrochemical performance(688 m A h·g^(-1)at 1200 m A·g^(-1))of the bimetallic nanocage-loaded fibers was demonstrated through the superior long-term stability of the anode(1048 m A h·g^(-1)after 300 cycles at 100 m A·g^(-1)),suggesting that the fabricated anode can be a promising material for use in portable LIBs.

关键词： Carbon nanofiber Nanostructure Composite anode Zeolitic imidazolate framework

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Reduced graphene oxide supersonically sprayed on wearable fabric and decorated with iron oxide for supercapacitor applications

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Journal of Materials Science & Technology 2021年第23期82卷 47-56页

作者： Ali Aldalbahi edmund samuel Bander S.Alotaibi Hany El-Hamshary Sam S.Yoon Department of Chemistry College of ScienceKing Saud UniversityRiyadh11451Saudi Arabia School of Mechanical Engineering Korea UniversitySeoul136-713Republic of Korea

We demonstrate the fabrication of wearable supercapacitor *** electrodes were applied to wearable fabric by supersonically spraying the fabric with reduced graphene oxide(r GO)followed by decoration with iron oxide(Fe_(2)O_(3))nanoparticles via a hydrothermal *** integration of iron oxide with r GO flakes on wearable fabric demonstrates immense potential for applications in high-energystorage *** synergetic impact of the intermingled r GO flakes and Fe_(2)O_(3) nanoparticles enhances the charge transport within the composite electrode,ultimately improving the overall electrochemical *** advantage of the porous nature of the fabric,electrolyte diffusion into the active r GO and Fe_(2)O_(3) materials was significantly enhanced and subsequently increased the electrochemical interfacial *** effect of the Fe_(2)O_(3) concentration on the overall electrochemical performance was *** optimal composition yields a specific capacitance of 360 F g^(-1) at a current density of 1 Ag^(-1) with a capacitance retention rate of 89%after 8500 galvanostatic cycles,confirming the long-term stability of the Fe_(2)O_(3)/r GO fabric electrode.

关键词： Supersonic spraying Conductive textile Wearable energy devices Reduced graphene oxide Iron oxide Supercapacitor

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