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Research 2024年第2期6卷 171-179页

作者： Ran duan Weihong qi Panke Li Kewei Tang Guoliang Ru Weimin liu State Key Laboratory of Solidification Processing Center of Advanced Lubrication and Seal MaterialsNorthwestern Polytechnical UniversityXi'an 710072China Shandong Laboratory of Yantai Advanced Materials and Green Manufacturing Yantai 265503China State Key Laboratory of Solid Lubrication Lanzhou Institute of Chemical PhysicsChinese Academy of SciencesLanzhou 730000China

Recent advancements in two-dimensional materials have shown huge potential for optoelectronic *** is challenging to achieve highly effective and sensitive broadband photodetection based on MoS_(2)*** engineering,such as introducing vacancies,can narrow the bandgap and boost the separation of photogenerated carriers by defect states but leads to a slow response ***,we propose a nickel nanoparticle-induced gateless photogating effect with a unique energy band structure to enable the application of defect engineering and achieve high optoelectronic *** device based on Ni nanoparticle-decorated MoS_(2)with S vacancies exhibited high responsivities of 106.21 and 1.38 A W^(-1)and detectivities of 1.9×10^(12)and 8.9×10^(9)Jones under 532 and 980 nm illumination(visible to near infrared),respectively,with highly accelerated response *** strategy provides new insight into optimizing defect engineering to design high-performance optoelectronic devices capable of broadband photodetection.

关键词： defect Infrared illumination

Single-cell technologies: current and near future

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Science China Life Sciences 2025年第1期 1-4页

作者： Chenfei Wang qi liu Xiaohui Fan Tieliu Shi Key Laboratory of Spine and Spinal Cord Injury Repair and Regeneration Ministry of EducationOrthopedics DepartmentTongji HospitalBioinformatics DepartmentSchool of Life Sciences and TechnologyTongji University Frontier Science Center for Stem Cells School of Life Sciences and TechnologyTongji University Translational Medical Center for Stem Cell Therapy and Institute for Regenerative Medicine Shanghai East HospitalBioinformatics DepartmentSchool of Life Sciences and TechnologyTongji University Research Institute of Intelligent Computing Zhejiang Lab Pharmaceutical Informatics Institute College of Pharmaceutical SciencesZhejiang University National Key Laboratory of Chinese Medicine Modernization Innovation Center of Yangtze River DeltaZhejiang University Center for Bioinformatics and Computational Biology Shanghai Key Laboratory of Regulatory Biologythe Institute of Biomedical Sciences and School of Life SciencesEast China Normal University Key Laboratory of Advanced Theory and Application in Statistics and Data Science (MOE) School of StatisticsEast China Normal University

Single-cell technologies enable the indepth exploration of multiple biological hierarchies at the scale of individual cells,which have deepened our knowledge of cellular diversity, tissue organization, and overall organism function(Sun et al.,2024). In 2009, single-cell RNA sequencing(sc RNA-seq) was first developed as a powerful tool to dissect gene expression and uncover transcriptional *** the rapid advancement of technology, single-cell approaches have expanded to encompass other omics, such as genomics, epigenomics, proteomics,and metabolomics.

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High active amorphous Co(OH)_(2) nanocages as peroxymonosulfate activator for boosting acetaminophen degradation and DFT calculation

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Chinese Chemical Letters 2021年第5期32卷 1814-1818页

作者： Juanjuan qi Juzhe liu Fengbin Sun Taobo Huang Jun duan Wen liu The Key Laboratory of Resources and Environmental Systems Optimization Ministry of EducationCollege of Environmental Science and EngineeringNorth China Electric Power UniversityBeijing 102206China The Key Laboratory of Water and Sediment Sciences Ministry of EducationCollege of Environmental Sciences and EngineeringPeking UniversityBeijing 100871China School of Chemistry and Beijing Advanced Innovation Center for Biomedical Engineering Beihang UniversityBeijing 100191China State Environmental Protection Key Laboratory of All Material Fluxes in River Ecosystems Peking UniversityBeijing 100871China

Acetaminophen(ACE)is commonly used in analgesic and antipyretic drug,which is hardly removed by traditional wastewater treatment ***,amorphous Co(OH)_(2)nanocages were explored as peroxymonosulfate(PMS)activator for efficient degradation of *** the presence of amorphous Co(OH)_(2)nanocages,100%of ACE removal was reached within 2 min with a reaction rate constant k_(1)=3.68 min 1 at optimum pH 5,which was much better than that of crystallineβ-Co(OH)_(2)and Co_(3)O_(4).Amorphous materials(disorder atom arrangement)with hollow structures possess large specific surface area,more reactive sites,and abundant vacancies structures,which could efficiently facilitate the catalytic redox *** radicals quenching experiment demonstrated that SO_(4)^(·-)radicals dominated the ACE degradation rather than^(·)OH *** mechanism of ACE degradation was elucidated by the an alysis of degradation in termediates and theoretical calculation,indicating that the electrophilic SO_(4)^(·-)and^(·)OH tend to attack the atoms of ACE with high Fukui index(f).Our finding highlights the remarkable advantages of amorphous materials as heterogeneous catalysts in sulfate radicals-based AOPs and sheds new lights on water treatment for the degradation of emerging organic contaminants.

关键词： Amorphous Co(OH)_(2) Peroxymonosulfate(PMS) Acetaminophen(ACE) Intermediates DFT calculation

Formation Mechanism of the Accumulative Magnification Effect in a Financial Time Series

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Chinese Physics Letters 2012年第3期29卷 271-274页

作者： duan Wen-qi College of Economics and Management Zhejiang Normal UniversityJinhua 321004

Structural information contained in financial time series can be magnified effectively by constructing the accumulative *** order to make the magnification effects of different financial time series comparative,we first propose a standard method to characterize the strength of the accumulative magnification ***,we employ decomposed-randomized technology to uncover the formation mechanism of the accumulative magnification *** results show that(1)the standard deviation pattern is determined by volatility dependence,(2)the Hurst exponent pattern is induced by sign dependence,(3)an approximate entropy pattern is caused by the combined effect of sign dependence and volatility dependence.

关键词： effect strength pattern

Chondroitinase ABC combined with Schwann cell transplantation enhances restoration of neural connection and functional recovery following acute and chronic spinal cord injury

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Neural Regeneration Research 2025年第5期20卷 1467-1482页

作者： Wenrui Qu Xiangbing Wu Wei Wu Ying Wang Yan Sun Lingxiao Deng Melissa Walker Chen Chen Heqiao Dai qi Han Ying Ding Yongzhi Xia George Smith Rui Li Nai-Kui liu Xiao-Ming Xu Spinal Cord and Brain Injury Research Group Stark Neurosciences Research InstituteDepartment of Neurological SurgeryIndiana University School of MedicineIndianapolisINUSA Department of Hand Surgery the Second Hospital of Jilin UniversityChangchunJilin ProvinceChina Shriners Hospitals Pediatric Research Center Temple University School of MedicinePhiladelphiaPAUSA Department of Anatomy&Cell Biology Indiana University School of MedicineIndianapolisINUSA

Schwann cell transplantation is considered one of the most promising cell-based therapy to repair injured spinal cord due to its unique growth-promoting and myelin-forming properties.A the Food and Drug Administration-approved Phase I clinical trial has been conducted to evaluate the safety of transplanted human autologous Schwann cells to treat patients with spinal cord injury.A major challenge for Schwann cell transplantation is that grafted Schwann cells are confined within the lesion cavity,and they do not migrate into the host environment due to the inhibitory barrier formed by injury-induced glial scar,thus limiting axonal reentry into the host spinal *** we introduce a combinatorial strategy by suppressing the inhibitory extracellular environment with injection of lentivirus-mediated transfection of chondroitinase ABC gene at the rostral and caudal borders of the lesion site and simultaneously leveraging the repair capacity of transplanted Schwann cells in adult rats following a mid-thoracic contusive spinal cord *** report that when the glial scar was degraded by chondroitinase ABC at the rostral and caudal lesion borders,Schwann cells migrated for considerable distances in both rostral and caudal *** Schwann cell migration led to enhanced axonal regrowth,including the serotonergic and dopaminergic axons originating from supraspinal regions,and promoted recovery of locomotor and urinary bladder ***,the Schwann cell survival and axonal regrowth persisted up to 6 months after the injury,even when treatment was delayed for 3 months to mimic chronic spinal cord *** findings collectively show promising evidence for a combinatorial strategy with chondroitinase ABC and Schwann cells in promoting remodeling and recovery of function following spinal cord injury.

关键词： axonal regrowth bladder function chondroitinase ABC functional recovery glial scar lentivirus migration Schwann cell spinal cord injury transplantation

Study on buoyancy convection phenomenon in the crystal growth process

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Science China(Technological Sciences) 2009年第8期52卷 2367-2372页

作者： duan Li KANG qi National Microgravity Laboratory Institute of MechanicsChinese Academy of SciencesBeijing 100190China

Real-time phase shift Mach-Zehnder interference technique, imaging technique, and computer image processing technique were combined to perform a real-time diagnosis of NaClO3 crystal, which de- scribed both the dissolution process and the crystallization process of the NaClO3 crystal in real-time condition. The dissolution fringes and the growth fringes in the process were obtained. Moreover, a distribution of concentration field in this process was obtained by inversion calculation. Finally, the buoyancy convection phenomenon caused by gravity in the crystal growth process was analyzed. The results showed that this convection phenomenon directly influences the growth rate of each crystal face in the crystal.

关键词： crystal growth interferometry buoyancy convection

Oxygen vacancies with localized electrons direct a functionalized separator toward dendrite-free and high loading LiFePO_(4)for lithium metal batteries

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Journal of Energy Chemistry 2022年第12期75卷 38-45,I0002页

作者： qi An qing liu Shimin Wang Lixiang liu Han Wang Yongjiang Sun Lingyan duan Genfu Zhao Hong Guo School of Materials and Energy Yunnan UniversityNo.2Green Lake North RoadKunming 650091YunnanChina Institute for Integrative Nanosciences Leibniz IFW DresdenHelmholtzstraße 2001069 DresdenGermany

The pursuit of high energy density has promoted the development of high-performance lithium metal batteries(LMBs).However,the underestimated but non-negligible dendrites of Li anode have been observed to shorten battery ***,a composite separator(TiO_(2-x)@PP),in which TiO_(2)with electron-localized oxygen vacancies(TiO_(2-x))is coated on a commercial PP separator,is fabricated to homogenize lithium ion transport and stabilize the lithium anode *** the utilization of TiO_(2-x)@PP separators,the symmetric lithium metal battery displays enhanced cycle stability over 800 h under a high current density of 8 m A cm^(-2).Moreover,the LMBs assembled with high-loading LiFePO_(4)(9.24 mg cm^(-2))deliver a stable cycling performance over 900 cycles at a rate of 0.5 *** theoretical studies based on density functional theory(DFT)further unveil the *** favorable TiO_(2-x)is beneficial for facilitating fast Li+migration and impeding anions *** addressing the Li dendrite issues,the use of TiO_(2-x)@PP separator potentially provides a facile and attractive strategy for designing well-performing LMBs,which are expected to meet the application requirements of rechargeable batteries.

关键词： Oxygen vacancy Ionic transport regulation Dendrite-free Localized electrons High loading

Study of thermal decoherence of harmonic oscillators

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原子与分子物理学报 2025年第5期42卷 108-114页

作者： LI Jian ZHOU Gao-Liang YAN Zheng-Xin liu Wei WANG Zhao-qi College of Science Xi’an University of Science and TechnologyXi’an 710054China

The thermal decoherence of harmonic oscillators is investigated *** quantum system presented here is a one-dimensional oscillator with angular frequency,which is surrounded by a thermal bath of environmental *** are various environmental oscillators with different angular frequency(below an ultraviolet cutoff).At the beginning,the quantum system is a pure state and the environmental oscillators are in thermodynamic equilibrium with *** a period,the system-environment interactions inspire significant decoherence of the quantum *** decoherence is displayed by explicit calculations of the purity and von Neumann entropy of the quantum *** is worth noting that the decoherence could be significant even in the weak coupling and low temperature case due to the large amount of environmental degrees of *** the decoherence process is inspired between the quantum system and an ordinary thermal environment here,the thermal decoherence result is quite general.

关键词： Quantum decoherence Grand canonical ensemble Oscillators

Microwave-assisted continuous flow phytosynthesis of silver nanoparticle/reduced graphene oxide composites and related visible light catalytic performance

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Journal of Environmental Sciences 2022年第5期34卷 286-293页

作者： Houyu Wang Chun-Gang Yuan Chenchen liu Xuelei duan qi Guo Yiwen Shen Jingfu liu Yongsheng Chen Hebei Key Lab of Power Plant Flue Gas Multi-Pollutants Control Department of Environmental Science&EngineeringNorth China Electric Power UniversityBaoding 071000China Wetland Research Center for Baiyangdian Lake North China Electric Power UniversityBaoding 071000China State Key Laboratory of Environmental Chemistry and Ecotoxicology Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing 100085China School of Civil and Environmental Engineering Georgia Institute of TechnologyAtlantaGA 30332USA

The creation of an environmentally friendly synthesis method for silver nanomaterials(Ag-NPs)is an urgent concern for sustainable nanotechnology *** the present study,a novel straightforward and green method for the preparation of silver nanoparti-cle/reduced graphene oxide(AgNP/rGO)composites was successfully developed through the combination of phytosynthesis,continuous flow synthesis and *** persimmon(Diospyros kaki Thunb.)extracts were used as both plant reducing and capping agents for fast online synthesis of AgNP/rGO *** experimental param-eters were optimized and the morphologies of the prepared materials were *** characterization results reveal that spherical AgNPs were quickly synthesized and uni-formly dispersed on rGO sheets using the proposed online *** transform in-frared spectroscopy analysis confirmed that phenols,flavonoids,and other substances in the plant extracts played a decisive role in the synthesis of AgNP/rGO *** sodium borohydride(NaBH4)degradation of p-nitrophenol(4-NP)as a model,the catalytic activity of the prepared AgNP/rGO materials was *** complete degradation of 4-NP was achieved within 12 min through the use of AgNP/rGO materials,and the compos-ite had a much better catalytic activity than the bare AgNPs and rGO *** with the conventional chemical method,our online method is facile,fast,cost-efficient,and en-vironmentally friendly.

关键词： Microwave Continuous flow Phytosynthesis Silver nanocomposite Catalysis

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一种新型压配式腰椎椎间融合器的机械性能

中国组织工程研究 2025年第21期29卷 4492-4498页

作者：李世文于长水刘启王智博刘禹良祁全哈尔滨医科大学附属第一医院黑龙江省哈尔滨市150000

背景:行经皮微创椎间孔腰椎椎间融合置入椎间融合器时,由于入路操作范围狭窄,有牵拉神经根损伤或置入融合器位置不良等风险,为了解决以上问题作者课题组发明了一种新型机械结构可变形压配式cage(Press-fit cage,YP-cage)。目的:对新型... 详细信息

背景:行经皮微创椎间孔腰椎椎间融合置入椎间融合器时,由于入路操作范围狭窄,有牵拉神经根损伤或置入融合器位置不良等风险,为了解决以上问题作者课题组发明了一种新型机械结构可变形压配式cage(Press-fit cage,YP-cage)。目的:对新型腰椎融合器YP-cage的机械强度特性进行初步评估。方法:对不同尺寸9,11,13 mm高度的新型YP-cage(n=9)和聚醚醚酮-cage(n=9)进行了静态轴向压缩实验和静态轴向扭转实验,分别采集力-位移曲线计算屈服位移及载荷、极限载荷位移及刚度,屈服角位移及扭矩、极限载荷角位移扭矩及刚度,并进行对比分析。结果与结论:(1)在静态轴向压缩测试中,YP-cage在3组测试中(9,11,13 mm),其刚度、屈服载荷、极限位移和载荷极限方面均优于聚醚醚酮-cage(P <0.01),但YP-cage的屈服位移小于聚醚醚酮-cage(P <0.05);(2)在静态扭转测试中,除了9 mm组的YP-cage和聚醚醚酮-cage在极限扭转角度上差异无显著性意义,YP-cage在屈服扭矩、屈服扭转角度及极限扭矩均小于聚醚醚酮-cage(P <0.01),而YP-cage扭转刚度在9 mm组和11 mm组大于聚醚醚酮-ccage(P <0.01);(3)结果表明新型压配式机械结构椎间融合器相较于聚醚醚酮材质cage具有更高的抗压强度,但抗扭强度不如聚醚醚酮-cage。

关键词：椎间融合装置经孔椎体间融合术脊柱融合机械性能物理性质