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Reconfigurable Mechanochromic Patterns into Chameleon-Inspired Photonic Papers

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Research 2022年第4期2022卷 421-433页

作者： dongpeng yang yang Hu Dekun Ma Jianping Ge Shaoming Huang School of Materials and Energy Guangzhou Key Laboratory of Low-Dimensional Materials and Energy Storage DevicesGuangdongUniversityof TechnologyGuangzhou510006China Zhejiang Key Laboratory of Alternative Technologies for Fine Chemicals Process Shaoxing UniversityShaoxing 312000China School of Chemistry and Molecular Engineering Shanghai Key Laboratory of Green Chemistry and Chemical Processes East China Normal UniversityShanghai200062China

Photonic crystal(PC)patterns have shown wide applications in optical devices,information encryption,anticounterfeiting,etc.Unfortunately,it is stll a great challenge to reconfigure the PC patterns once fabricated.Herein,a new strategy is presented to reconfigure self-recordable PC patterns by printing local patterns into the chameleon-inspired PC papers using the phase change material(PCM)as ink and then erasing the patterns in ethanol.Multicolor and high-resolution(25 and 75μm for dot and lines,respectively)patterns can be eficiently and repeatedly reconfigured.In addition,the photonic patterns based on the PC paper and PCM combinations are gifted with mechanochromic characteristics and can show programmable and reversible color change under pressure.The high melting point of the ink,nonclosely packed structures of the PC paper,and the similar solubility parameter of PC paper,PCM,and ethanol are the keys for all these characteristics.This work offers a simple,flexible,efficient way to reconfigure PC patterns with mechanochromic properties and could open up exciting applications for novel hand-operation-based anticounterfeiting and opticaldevices.

关键词： packed repeatedly printing

On-demand molecular design for efficient blue phosphorescence

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Science China Chemistry 2024年第7期67卷 2124-2126页

作者： Meiqi Dai dongpeng Yan Beijing Key Laboratory of Energy Conversion and Storage Materials Key Laboratory of RadiopharmaceuticalsMinistry of EducationCollege of ChemistryBeijing Normal UniversityBeijing 100875China

Blue luminescence(including both fluorescence and phosphorescence)is one of the core elements in solid-state lighting and full-color displays.Up to now,ultralong room temperature phosphorescence(RTP)with a long lifetime over 0.1 s has been continuously reported.Most ultralong phosphorescence emission bands are in the region of 500 to600 nm.However,high-energy blue phosphorescence remains an immense challenge[1].

关键词： blue lifetime bands

MIR1868 negatively regulates rice cold tolerance at both the seedling and booting stages

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The Crop Journal 2024年第2期12卷 375-383页

作者： yang Shen Xiaoxi Cai Yan Wang Wanhong Li dongpeng Li Hao Wu Weifeng Dong Bowei Jia Mingzhe Sun Xiaoli Sun Crop Stress Molecular Biology Laboratory Heilongjiang Bayi Agricultural UniversityDaqing 163319HeilongjiangChina

Low temperature causes rice yield losses of up to 30%–40%,therefore increasing its cold tolerance is a breeding target.Few genes in rice are reported to confer cold tolerance at both the vegetative and reproductive stages.This study revealed a rice-specific 24-nt miRNA,miR1868,whose accumulation was suppressed by cold stress.Knockdown of MIR1868 increased seedling survival,pollen fertility,seed setting,and grain yield under cold stress,whereas its overexpression conferred the opposite phenotype.Knockdown of MIR1868 increased reactive oxygen species(ROS)scavenging and soluble sugar content under cold stress by increasing the expression of peroxidase genes and sugar metabolism genes,and its overexpression produced the opposite effect.Thus,MIR1868 negatively regulated rice cold tolerance via ROS scavenging and sugar accumulation.

关键词： Rice Cold tolerance miRNA ROS scavenging Soluble sugar accumulation

Wear-resistant CoCrNi multi-principal element alloy at cryogenic temperature

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Science Bulletin 2024年第2期69卷 227-236页

作者： Yue Ren Qing Zhou dongpeng Hua Zhuobin Huang Yulong Li Qian Jia Peter Gumbsch Christian Greiner Haifeng Wang Weimin Liu State Key Laboratory of Solidification Processing Center of Advanced Lubrication and Seal MaterialsNorthwestern Polytechnical UniversityXi’an 710072China Institute for Applied Materials Karlsruhe Institute of TechnologyKarlsruhe 76131Germany IAM-ZM MicroTribology CenterμTC Karlsruhe Institute of TechnologyKarlsruhe 76131Germany Fraunhofer IWM Freiburg 79108Germany State Key Laboratory of Solid Lubrication Lanzhou Institute of Chemical PhysicsChinese Academy of SciencesLanzhou 730000China

Traditional high strength engineering alloys suffer from serious surface brittleness and inferior wear performance when servicing under sliding contact at cryogenic temperature.Here,we report that the recently emerging CoCrNi multi-principal element alloy defies this trend and presents dramatically enhanced wear resistance when temperature decreases from 273 to 153 K,surpassing those of cryogenic austenitic steels.The temperature-dependent structure characteristics and deformation mechanisms influencing the cryogenic wear resistance of CoCrNi are clarified through microscopic observation and atomistic simulation.It is found that sliding-induced subsurface structures show distinct scenarios at different deformation temperatures.At cryogenic condition,significant grain refinement and a deep plastic zone give rise to an extended microstructural gradient below the surface,which can accommodate massive sliding deformation,in direct contrast to the strain localization and delamination at 273 K.Meanwhile,the temperature-dependent cryogenic deformation mechanisms(stacking fault networks and phase transformation)also provide additional strengthening and toughening of the subsurface material.These features make the CoCrNi alloy particularly wear resistant at cryogenic conditions and an excellent candidate for safety–critical applications.

关键词： Multi-principal element alloy Cryogenic temperature Wear CoCrNi

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深海海底山引起的混响杂波联合预报方法

哈尔滨工程大学学报 2024年第3期45卷 466-473页

作者：杨华秦继兴莫东鹏高博中国科学院声学研究所声场声信息国家重点实验室北京100190 中国科学院大学物理学院北京100190 中国人民解放军92578部队北京100161 中国海洋大学信息海洋技术学院山东青岛266100

针对深海复杂海域的主动探测混响杂波干扰的联合工程预报问题,本文基于三维射线-简正波理论建立了深海海底山引起的混响杂波联合预报方法,将海底山当作一类具有强散射特征的体积散射源,提出了对海底山的体积散射函数在水平和垂直维度上... 详细信息

针对深海复杂海域的主动探测混响杂波干扰的联合工程预报问题,本文基于三维射线-简正波理论建立了深海海底山引起的混响杂波联合预报方法,将海底山当作一类具有强散射特征的体积散射源,提出了对海底山的体积散射函数在水平和垂直维度上进行网格划分的数值积分方法。研究了不同水平方位,不同地形条件下的海底混响和海底山杂波强度特征。实现了小起伏水平海底和海底山地形的深海海底混响和海底山杂波的统一预报。研究结果表明:海底山的体积散射源经过水平和垂直维度的划分后,可以和水平海底的小尺度散射过程形成有效耦合,而海底山杂波的时间尺度和包络强度分别受海底山的水平宽度和垂直高度影响。通过海上实验数据比对,验证了本文所提预报方法的准确性。

关键词：深海混响海底山杂波混响杂波模型射线理论主动声呐体积散射混响预报

One-dimensional molecular co-crystal alloys capable of full-color emission for low-loss optical waveguide and optical logic gate

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Aggregate 2024年第1期5卷 299-308页

作者： Zhenhong Qi Yu-Juan Ma dongpeng Yan Beijing Key Laboratory of Energy Conversion and Storage Materials College of ChemistryKey Laboratory of Radio-pharmaceuticals Ministry of EducationBeijing Normal UniversityBeijingChina

The luminescence color of molecule-based photoactive materials is the key to the applications in lighting and optical communication.Realizing continuous regulation of emission color in molecular systems is highly desirable but still remains a challenge due to the individual emission band of purely organic molecules.Herein,a novel alloy strategy based on molecular co-crystals is reported.By adjusting the molar ratio of pyrene(Py)and fluorathene(Flu),three types of molecular co-crystal alloys(MCAs)assemblies are prepared involving Py-Flu-OFN-x%,Py-Flu-TFP-x%,Py-Flu-TCNB-x%.Multiple energy level structure and Förster resonance energy transfer(FRET)process endow materials with tunable full-spectra emission color in visible region.Impressively,these MCAs and co-crystals can be successfully applied to low optical loss waveguide and optical logic gate by virtue of all-color luminescence from blue across green to red,together with smooth surface of onedimensional microrods,which show promising applications as continuous light emitters for advance photonics applications.

关键词： full-color emission microrods molecular co-crystal optical waveguide organic alloys

Selective nano-buckling improves the performance of graphene logic transistors

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National Science Review 2024年第2期11卷 95-96页

作者： Tong yang Ming yang Department of Applied Physics The Hong Kong Polytechnic University Research Centre for Nanoscience and Nanotechnology The Hong Kong Polytechnic University

The massive integration of silicon-based transistors into modern electronic devices greatly increases power consumption and heat generation/dissipation[1]. In this concern, transistors based on atomically-thin graphene that exhibit high electric and thermoelectric conductivities with negligible contact resistance,

关键词：

Deep Insight of Design,Mechanism,and Cancer Theranostic Strategy of Nanozymes

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Nano-Micro Letters 2024年第2期16卷 165-217页

作者： Lu yang Shuming Dong Shili Gai Dan yang He Ding Lili Feng Guixin yang Ziaur Rehman Piaoping yang Key Laboratory of Superlight Materials and Surface Technology Ministry of EducationCollege of Materials Science and Chemical EngineeringHarbin Engineering UniversityHarbin 150001People’s Republic of China Yantai Research Institute Harbin Engineering UniversityYantai 264000People’s Republic of China Key Laboratory of Green Chemical Engineering and Technology of Heilongjiang Province College of Material Science and Chemical EngineeringHarbin University of Science and TechnologyHarbin 150040People’s Republic of China Department of Chemistry Quaid-i-Azam UniversityIslamabad 45320Pakistan

Since the discovery of enzyme-like activity of Fe3O4 nanoparticles in 2007,nanozymes are becoming the promising substitutes for natural enzymes due to their advantages of high catalytic activity,low cost,mild reaction conditions,good stability,and suitable for large-scale production.Recently,with the cross fusion of nanomedicine and nanocatalysis,nanozyme-based theranostic strategies attract great attention,since the enzymatic reactions can be triggered in the tumor microenvironment to achieve good curative effect with substrate specificity and low side effects.Thus,various nanozymes have been developed and used for tumor therapy.In this review,more than 270 research articles are discussed systematically to present progress in the past five years.First,the discovery and development of nanozymes are summarized.Second,classification and catalytic mechanism of nanozymes are discussed.Third,activity prediction and rational design of nanozymes are focused by highlighting the methods of density functional theory,machine learning,biomimetic and chemical design.Then,synergistic theranostic strategy of nanozymes are introduced.Finally,current challenges and future prospects of nanozymes used for tumor theranostic are outlined,including selectivity,biosafety,repeatability and stability,in-depth catalytic mechanism,predicting and evaluating activities.

关键词： Nanozymes Classification Prediction and design Catalytic mechanism Tumor theranostics

Fresh-Keeping Decision and Coordination of Fresh Agricultural Product Supply Chain Considering Carbon Cap-and-Trade under Different Dominance

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Journal of Systems Science and Systems Engineering 2024年第1期33卷 30-51页

作者： yang yang Guanxin Yao China Institute for Agricultural Equipment Industrial Development Jiangsu UniversityZhenjiang212013China Jiangsu Modern Logistics Research Base Yangzhou UniversityYangzhou225009China

In the context of low carbon,this paper discussed the impact of the carbon cap-and-trade policy on the fresh-keeping decision-making of two-echelon fresh agricultural product supply chains under different dominance,and designed cost-sharing contracts to coordinate the supply chain of fresh agricultural products dominated by suppliers and retailers respectively.The results showed that:dominance has no effect on the fresh-keeping decision and total revenue of fresh agricultural product supply chain,but it affects the internal income distribution,and dominance does not always bring more benefits;the implementation of carbon cap-and-trade reduces the fresh-keeping decision-making of fresh agricultural products supply chain and reduces the free-rider income of followers;the role of higher carbon trading price is twofold,which not only brings about the speculation of leading enterprises,but also promotes the application of low-carbon technologies;consumers’high preference for freshness,low-cost and high-efficiency low-carbon technology are all conducive to improving the fresh-keeping efforts and benefits of the supply chain;cost-sharing contracts can coordinate the supply chain of fresh agricultural products.

关键词： Dominant power carbon cap-and-trade policy fresh agricultural product supply chain fresh-keeping decision-making