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Defect Engineering in Earth-Abundant Cu2ZnSnSe4 Absorber Using Efficient Alkali Doping for Flexible and Tandem Solar Cell Applications

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Energy & Environmental Materials 2024年第2期7卷 253-260页

作者： Muhammad Rehan Ara Cho Inyoung Jeong Kihwan Kim Asmat Ullah Jun-Sik Cho Joo Hyung Park Yunae Jo Sung Jun Hong Seung Kyu Ahn SeJin Ahn Jae Ho Yun Jihye Gwak donghyeop shin Photovoltaics Research Department Korea Institute of Energy Research (KIER) Department of Renewable Energy Engineering University of Science and Technology (UST) Korea Institute of Energy Technology (KENTECH)

To demonstrate flexible and tandem device applications, a low-temperature Cu2ZnSnSe4（CZTSe） deposition process, combined with efficient alkali doping, was developed. First, high-quality CZTSe films were grown at480 °C by a single co-evaporation, which is applicable to polyimide（PI）substrate. Because of the alkali-free substrate, Na and K alkali doping were systematically studied and optimized to precisely control the alkali distribution in CZTSe. The bulk defect density was significantly reduced by suppression of deep acceptor states after the（Na F + KF） PDTs. Through the low-temperature deposition with（Na F + KF） PDTs, the CZTSe device on glass yields the best efficiency of 8.1% with an improved VOCdeficit of646 m V. The developed deposition technologies have been applied to *** the first time, we report the highest efficiency of 6.92% for flexible CZTSe solar cells on PI. Additionally, CZTSe devices were utilized as bottom cells to fabricate four-terminal CZTSe/perovskite tandem cells because of a low bandgap of CZTSe（～1.0 e V） so that the tandem cell yielded an efficiency of 20%. The obtained results show that CZTSe solar cells prepared by a low-temperature process with in-situ alkali doping can be utilized for flexible thin-film solar cells as well as tandem device applications.

关键词： alkali doping Earth-abundant Cu2ZnSnSe4 flexible solar cells four-terminal tandem cells low-temperature process

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