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Efficient concentration of trace analyte with ordered hotspot construction for a robust and sensitive SERS platform

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International Journal of Extreme Manufacturing 2024年第3期6卷 532-542页

作者： Youdi hu Yanlei hu Zhenyu Wang Jiale Yong Wei Xiong dong Wu Shixiang Xu Shenzhen Key Laboratory of Micro-Nano Photonic Information Technology College of Physics and Optoelectronic EngineeringShenzhen UniversityShenzhenGuangdong 518060People’s Republic of China CAS Key Laboratory of Mechanical Behavior and Design of Materials Key Laboratory of Precision Scientific Instrumentation of Anhui Higher Education InstitutesDepartment of Precision Machinery and Precision InstrumentationUniversity of Science and Technology of ChinaHefeiAnhui 230027People’s Republic of China Wuhan National Laboratory for Optoelectronics Huazhong University of Science and TechnologyWuhanHubeiPeople’s Republic of China

Surface-enhanced Raman scattering(SERS)platform,which enables trace analyte detection,has important application *** structuring/modifying the surface of the SERSsubstrate,analyte in highly diluted solutions can be concentrated into localized active areas for highly sensitive ***,subject to the difficulty of the fabrication process,itremains challenging to balance hot-spot construction and the concentration capacity of analyte ***,preparing SERS substrates with densely ordered hot spots andefficient concentration capacity is of great significance for highly sensitive ***,we propose an Ag and fluoroalkyl-modified hierarchical armour substrate(Ag/F-HA),which has a double-layer stacking design to combine analyte concentration with hotspot *** microarmour structure is fabricated by femtosecond-laser processing to serve as asuperhydrophobic and low-adhesive surface to concentrate analyte,while the anodic aluminium oxide(AAO)template creates a nanopillar array serving as dense and ordered hot *** the synergistic action of hot spots and analyte concentration,Ag/F-HA achieves a detectionlimit down to 10^(-7)M doxorubicin(DOX)molecules with a RSD of 7.69%.Additionally,Ag/F-HA exhibits excellent robustness to resist external disturbances such as liquid splash or *** on our strategy,SERS substrates with directional analyte concentrations are further explored by patterning microcone arrays with *** work opens a way to the realistic implementation of SERS in diverse scenarios.

关键词： surface-enhanced Raman scattering anodic aluminium oxide femtosecond laser processing concentration of trace analytes mechanical robustness

Strong invariance principle for a counterbalanced random walk

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Applied Mathematics(A Journal of Chinese Universities) 2024年第2期39卷 370-380页

作者： TAN hui-qun hu Zhi-shui dong Liang International Institute of Finance School of ManagementUniversity of Science and Technology of ChinaHefei 230026China Center for Basic Teaching and Experiment Nanjing University of Science and TechnologyJiangyin 214443China

We study a counterbalanced random walkS_(n)=X_(1)+…+X_(n),which is a discrete time non-Markovian process andX_(n) are given recursively as *** n≥2,X_(n) is a new independent sample from some fixed law̸=0 with a fixed probability p,andX_(n)=−X_(v(n))with probability 1−p,where v(n)is a uniform random variable on{1;…;n−1}.We apply martingale method to obtain a strong invariance principle forS_(n).

关键词： random walk martingale invariance principle

Enhancement in the Hg^(0) oxidation efficiency and sulfur resistance of CuCl_(2)-modified MnO_(x)-CeO_(x) nanorod catalysts

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Journal of Zhejiang University-Science A(Applied Physics & Engineering) 2024年第8期25卷 680-686页

作者： Shujie GAO Yongjin hu Zhichang JIANG Xiaoxiang WANG dong YE Changxing hu College of Quality&Safety Engineering China Jiliang UniversityHangzhou 310018China Key Laboratory of Biomass Chemical Engineering of Ministry of Education Institute of Industrial Ecology and EnvironmentCollege of Chemical and Biological EngineeringZhejiang UniversityHangzhou 310027China School of Mechatronics and Energy Engineering Ningbo Tech UniversityNingbo 315100China

In this study,a series of CuCl_(2)-modified MnO_(x)-CeO_(x)nanorods were synthesized for the oxidation of Hg^(0).The addition of CuCl_(2)resulted in an enhancement in the catalyst’s Hg^(0)oxidation ability,and Hg^(0)oxidation efficiency reached>97%from 150 to 250°*** the MnO_(x)-CeO_(x)catalysts,Mn^(4+)played the role of the active species for Hg^(0)oxidization,but in the CuCl_(2)-doped catalysts Cl−also contributed to Hg^(0)oxidation,conferring the superior performance of these *** introduction of SO_(2) led to a decrease in the availability of Mn^(4+),and the Hg^(0)oxidation efficiency of MnO_(x)-CeO_(x)decreased from about 100%to about 78%.By contrast,CuCl_(2)-promoted samples maintained a Hg^(0)oxidation efficiency of about 100%during the SO_(2) deactivation cycle due to the high reactivity of Cl−.

关键词： Hg^(0)oxidation CuCl_(2)modification MnO_(x)-CeO_(x)nanorods Sulfur resistance O_(x)idation activity

A Retrodirective Array Enabled by CMOS Chips for Two-Way Wireless Communication with Automatic Beam Tracking

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Engineering 2024年第6期37卷 196-207页

作者： Jiacheng Guo Yizhu Shen Guoqing dong Zhuang Han Sanming hu State Key Laboratory of Millimeter Waves School of Information Science and EngineeringSoutheast UniversityNanjing 210096China Purple Mountain Laboratories Nanjing 211111China

This article proposes and demonstrates a retrodirective array(RDA)for two-way wireless communication with automatic beam *** proposed RDA is enabled by specifically designed chips made using a domestic complementary metal-oxide semiconductor(CMOS)*** highly integrated CMOS chip includes a receiving(Rx)chain,a transmitting(Tx)chain,and a unique tracking phaselocked loop(PLL)for the crucial conjugated phase recovery in the *** article also proposes a method to reduce the beam pointing error(BPE)in a conventional *** validate the above ideas simply yet without loss of generality,a 2.4 GHz RDA is demonstrated through two-way communication links between the Rx and Tx chains,and an on-chip quadrature coupler is designed to achieve a nonretrodirective signal suppression of 23 *** experimental results demonstrate that the proposed RDA,which incorporates domestically manufactured low-cost 0.18 lm CMOS chips,is capable of automatically tracking beams covering±40with a reduced *** CMOS chip in the RDA has a compact size of 4.62 mm^(2) and a low power consumption of 0.15 *** the best of the authors’knowledge,this is the first research to demonstrate an RDA with a fully customized CMOS chip for wireless communication with automatic beam tracking。

关键词： Automatic beam tracking CMOS Retrodirective array Two-way communication

PCA-Net: a heart segmentation model based on the meta-learning method

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Optoelectronics Letters 2024年第11期20卷 697-704页

作者： YANG Mengzhu Zhu dong dong Hao hu Shunbo WANG Yongfang School of Information Science and Engineering Linyi University

In order to effectively prevent and treat heart-based diseases, the study of precise segmentation of heart parts is particularly important. The heart is divided into four parts: the left and right ventricles and the left and right atria, and the left main trunk is more important, thus the left ventricular muscle(LV-MYO), which is located in the middle part of the heart, has become the object of many researches.

关键词： A

Prediction of dissolved gas content in transformer oil based on multi-information fusion

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High Voltage 2024年第3期9卷 685-699页

作者： Tongliang Yang Yun Fang Chengming Zhang Chao Tang dong hu College of Engineering and Technology Southwest UniversityChongqingChina International R&D Center for New Technologies of Smart Grid and Equipment Southwest UniversityChongqingChina

In order to accurately predict the content and variation trend of dissolved gas in trans-former oil and guide the condition maintenance of power transformers,a combined prediction model based on multi-information fusion is proposed and its effectiveness is *** of all,based on the possibility of pathological and missing historical sample data,a detection and filling method based on variable weight combination samples is ***,the authors propose two *** at the non-linear and non-stationary characteristics of gas content,a univariate decomposition prediction mode HBA-VMD-TCN which based on the Honey Badger algorithm,variational mode decomposition and time convolutional network(TCN)is *** the multi-variate Informer prediction model is established for gas content affected by multiple ***,the cross-entropy theory is used to determine the weight coefficients of the two models,and the multi-information fusion combined prediction model is ***,on the basis of the above,a method to determine the time step and the position information of the transition point adaptively in the process of prediction is proposed to further improve the prediction *** results show that,through a series of simulation experiments of model comparison and transformer anomaly prediction,the accuracy and effectiveness of the combined prediction model are verified.

关键词： content prediction dissolved

Transcriptome analysis reveals immune-related genes in tissues of Vibrio anguillarum-infected turbot Scophthalmus maximus

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Journal of Oceanology and Limnology 2024年第1期42卷 332-344页

作者： Yuting SONG Maqsood Ahmed SOOMRO Xianzhi dong Guobin hu College of Marine Life Sciences Ocean University of ChinaQingdao 266003China Institute of Evolution&Marine Biodiversity Ocean University of ChinaQingdao 266003China Institute of Biophysis Chinese Academy of SciencesBeijing 100101China

Turbot Scophthalmus maximus is an important mariculture fish species with high economic ***,the bacterial diseases caused by Vibrio anguillarum infection bring huge economic losses to the turbot aquaculture *** understand the immune response of the turbot against *** infection and to explore novel immune-related genes,the transcriptome analysis of turbot spleen and gills were conducted after *** *** expressed genes(DEGs)were identified in spleen and gill of the turbot amounted to 17261 and 16436,respectively.A large number of immunerelated DEGs were enriched in cytokine-cytokine receptor interaction signaling pathway,and the others by the kyoto encyclopedia of genes and genomes(KEGG)*** gene ontology(GO)classification analysis revealed that *** infection had the greatest effect on biological processes and cellular *** immune-related DEGs were identified in the spleen(cstl.1,egfl6,lamb21,v2rx4,calcr,and gpr78a)and gills(ghra,sh3gl2a,cst12,inhbaa,cxcl8,and il-1b)by heat *** proteinprotein interaction(PPI)networks were constructed to analyze the immune *** results demonstrate that the maturation and antigen processing of major histocompatibility complex(MHC)class II molecule,and calcitonin-or adrenomedullin-regulated physiological activity were important events in the immunity of turbot against *** *** the gills,the protein interactions in TGF-βsignaling pathway,production of inflammatory factors,and endocytosis regulation were most *** research laid a foundation for discovering novel immune-related genes and enriching the knowledge of immune mechanisms of turbot against *** infection.

关键词： Scophthalmus maximus Vibrio anguillarum transcriptome differentially expressed genes immune mechanism

Ferrite features in simulated transition zone of EH36 shipbuilding steel submerged arc welded by CaF_(2)-SiO_(2)-MnO fluxes

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Journal of Iron and Steel Research International 2024年第4期31卷 790-796页

作者： Ming Zhong dong hu Da-ming Guo Somnath Basu Cong Wang Key Laboratory for Ecological Metallurgy of Multimetallic Mineral(Ministry of Education) Northeastern UniversityShenyang 110819LiaoningChina School of Metallurgy Northeastern UniversityShenyang 110819LiaoningChina The State Key Laboratory of Refractories and Metallurgy Wuhan University of Science and TechnologyWuhan 430081HubeiChina Department of Metallurgical Engineering and Materials Science Indian Institute of Technology BombayMumbai 400076MaharashtraIndia

Ferrite features in the simulated transition zone welded with CaF_(2)-SiO_(2)-MnO fluxes containing various MnO contents have been *** laser scanning microscopy has been applied to simulate the thermal cycling of the transition zone and the phase transformations during cooling have been in-situ *** has been found that the appearance temperature for ferrite side plate decreases with increasing Mn content in the weld metals caused by MnO content ***,growth rates for both ferrite side plate and acicular ferrite are significantly enhanced with a higher Mn content of weld ***,from the statistical fractions of salient microstructures,for all samples,the acicular ferrite,grain boundary ferrite,and polygonal ferrite take over more than 90%.It has also been demonstrated that with the increase in Mn content,the ferrite side plate fraction increases slightly from 5%to 10%and the acicular ferrite fraction shows a tendency of first increasing and then decreasing,which experiences the maximum with the flux containing 30 wt.%*** phenomenon is believed to be controlled by the O and Mn contents in weld metals synergistically.

关键词： Submerged arc welding Transition zone Phase transformation Microstructure

On the Responsible Use of Chatbots in Bioinformatics

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Genomics, Proteomics & Bioinformatics 2024年第1期22卷 1-3页

作者： Gangqing hu Li Liu dong Xu Department of Microbiology Immunology&Cell BiologyWest Virginia UniversityMorgantownWV 26506USA College of Health Solutions Arizona State UniversityPhoenixAZ 85004USA Biodesign Institute Arizona State UniversityTempeAZ 85281USA Department of Electrical Engineer and Computer Science Christopher S.Bond Life Sciences CenterUniversity of MissouriColumbiaMO 65211USA

Large language model(LLM)-based chatbots like Chat Generative Pre-trained Transformer(ChatGPT),equipped with broad biological knowledge[1],have demonstrated an impressive capability for bioinformatics coding[2].When given well-crafted instructions,these chatbots hold the potential to significantly augment bioinformatics education and research[3,4].However,opportunities entail both rewards and *** commentary explores the challenges of using chatbots in bioinformatics and proposes strategies to manage the associated risks while maximizing the benefits.

关键词： equipped while education