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Multiphase Interfacial Regulation Based on Hierarchical Porous Molybdenum Selenide to Build Anticorrosive and Multiband Tailorable Absorbers

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Nano-Micro Letters 2024年第1期16卷 85-105页

作者： Tianbao Zhao Zirui jia Jinkun Liu Yan Zhang Guanglei wu Pengfei Yin College of Science Sichuan Agricultural UniversityYa’an 625014People’s Republic of China Institute of Materials for Energy and Environment State Key Laboratory of Bio‑Fibers and Eco‑TextilesCollege of Materials Science and EngineeringQingdao UniversityQingdao 266071People’s Republic of China College of Chemistry and Chemical Engineering Qingdao UniversityQingdao 266071People’s Republic of China

Electromagnetic wave(EMW)absorbing materials have an irreplaceable position in the field of military stealth as well as in the field of electromagnetic pollution *** in order to cope with the complex electromagnetic environment,the design of multifunctional and multiband high efficiency EMW absorbers remains a tremendous *** this work,we designed a three-dimensional porous structure via the salt melt synthesis strategy to optimize the impedance matching of the ***,through interfacial engineering,a molybdenum carbide transition layer was introduced between the molybdenum selenide nanoparticles and the three-dimensional porous carbon matrix to improve the absorption behavior of the *** analysis indicates that the number and components of the heterogeneous interfaces have a significant impact on the EMW absorption performance of the absorber due to mechanisms such as interfacial polarization and conduction loss introduced by interfacial ***,the prepared MoSe_(2)/MoC/PNC composites showed excellent EMW absorption performance in C,X,and Ku bands,especially exhibiting a reflection loss of−59.09 dB and an effective absorption bandwidth of 6.96 GHz at 1.9 *** coordination between structure and components endows the absorber with strong absorption,broad bandwidth,thin thickness,and multi-frequency absorption ***,it can effectively reinforce the marine anticorrosion property of the epoxy resin coating on Q235 steel *** study contributes to a deeper understanding of the relationship between interfacial engineering and the performance of EMW absorbers,and provides a reference for the design of multifunctional,multiband EMW absorption materials.

关键词： Interfacial engineering Anticorrosion Multiband Electromagnetic wave absorber

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Unlocking the Potential of Poly(butylene succinate)through Incorporation of Vitrimeric Network Based on Dynamic Imine Bonds

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Chinese Journal of Polymer Science 2024年第10期42卷 1414-1424,I0006页

作者： Shan-Song wu Hui-Juan Lu Yi-dong Li Shui-dong Zhang jian-Bing Zeng Chongqing Key Laboratory of Soft-Matter Material Manufacturing School of Chemistry and Chemical EngineeringSouthwest UniversityChongqing400715China School of Mechanical and Automotive Engineering South China University of TechnologyGuangzhou510640China

Poly(butylene succinate)(PBS)exhibits many advantages,such as renewability,biodegradability,and impressive thermal and mechanical properties,but is limited by the low melt viscosity and strength resulted from the linear *** address this,vitrimeric network was introduced to synthesize PBS vitrimers(PBSVs)based on dynamic imine bonds through melt polymerization of hydroxyl-terminated PBS with vanillin derived imine containing compound and hexamethylene diisocyanate using trimethylolpropane as a crosslinking *** with different crosslinking degrees were synthesized through changing the content of the crosslinking *** effect of crosslinking degree on the thermal,theological,mechanical properties,and stress relaxation behavior of the PBSVs was studied in *** results demonstrated that the melt viscosity,melt strength,and heat resistance were enhanced substantially without obvious depression in crystallizability,thermal stability,and mechanical properties through increasing crosslinking *** addition,the PBSVs exhibit thermal reprocessability with mechanical properties recovered by more than 90%even after processing for three ***,PBSV with improved melt properties shows significantly improved foamability compared to commercial *** research contributes to the advancement of polymer technology by successfully developing PBS vitrimers with improved properties,showcasing their potential applications in sustainable and biodegradable materials.

关键词： Poly(butylene succinate) Vitrimer Imine bonds Foamability

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Association between the cumulative triglyceride-glucose index and the recurrence of atrial fibrillation after radiofrequency catheter ablation

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Journal of Geriatric Cardiology 2024年第2期21卷 200-210页

作者： Qing YAN jia-Qi LIANG Yi-De YUAN Yuan LI jia-Li FAN Wen-Huan wu Pan XU jia-Hong XUE Department of Cardiovascular Medicine the Second Affiliated Hospital of Xi’an Jiaotong UniversityShaanxiChina Department of Cardiovascular Medicine Zichang People’s HospitalShaanxiChina Department of Ultrasound Xijing HospitalAir Force Military Medical UniversityShaanxiChina

BACKGROUND Triglyceride-glucose(TyG)index values are a new surrogate marker for insulin *** study aimed to explore the relationship between cumulative TyG index values and atrial fibrillation(AF)recurrence after radiofrequency catheter ablation(RFCA).METHODS A total of 576 patients with AF who underwent RFCA at the Second Affiliated Hospital of Xi'an jiaotong University were included in this *** participants were grouped based on cumulative TyG index values tertiles within 3 months after *** regression and restricted cubic spline analyses were used to determine the relationship between cumulative TyG index values and AF *** predictive value of all risk factors was assessed by receiver operating curve *** There were 375 patients completed the study(age:63.23±10.73 years,64.27%male).The risk of AF recurrence increased with increasing cumulative TyG index values *** adjusting for potential confounders,patients in the medium cumulative TyG index group[hazard ratio(HR)=4.949,95%CI:1.778–13.778,P=0.002]and the high cumulative TyG index group(HR=8.716,95%CI:3.371–22.536,P<0.001)had a higher risk of AF recurrence than those in the low cumulative TyG index *** restricted cubic spline regression model also showed an increased risk of AF recurrence with increasing cumulative TyG index *** considering cumulative TyG index values,left atrial diameter,and lactate dehydrogenase levels as a comprehensive factor,the model could effectively predict AF recurrence after RFCA[area under the curve(AUC)=0.847,95%CI:0.797–0.897,P<0.001].CONCLUSIONS Cumulative TyG index values were a risk factor for AF recurrence after *** longitudinal TyG index values may assist with optimized for risk stratification and outcome prediction for AF recurrence.

关键词： atrial fibrillation index

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Innovative mesenchymal stem cell treatments for fatty liver disease

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World Journal of Stem Cells 2024年第9期16卷 846-853页

作者： Fei-Qiong Gao jia-Qi Zhu Xu-dong Feng Department of Endocrinology Affiliated Hangzhou First People’s HospitalSchool of MedicineWestlake UniversityHangzhou 310003Zhejiang ProvinceChina Laboratory Medicine Center Department of Clinical LaboratoryZhejiang Provincial People’s HospitalPeople’s Hospital of Hangzhou Medical CollegeHangzhou 310014Zhejiang ProvinceChina Department of Clinical Laboratory Ningbo Medical Center Lihuili HospitalAffiliated Lihuili Hospital of Ningbo UniversityNingbo 315000Zhejiang ProvinceChina

The incidence of non-alcoholic fatty liver disease(NAFLD)and alcohol-associated liver disease(ALD)is increasing year by year due to changes in the contemporary environment and dietary structure,and is an important public health problem *** is an urgent need to continuously improve the understanding of their disease mechanisms and develop novel therapeutic *** stem cells(MSCs)have shown promise as a potential therapeutic strategy in therapeutic studies of NAFLD and *** and ALD have different triggers and their specific mechanisms of disease progression are different,but both involve disease processes such as hepatocellular steatosis and potential fibrosis,cirrhosis,and even hepatocellular *** have metabolic regulatory,anti-apoptotic,antioxidant,and immunomodulatory effects that together promote liver injury repair and functional recovery,and have demonstrated positive results in preclinical *** editorial is a continuum of jiang et al’s review focusing on the advantages and limitations of MSCs and their derivatives as therapeutics for NAFLD and *** detail how MSCs attenuate the progression of NAFLD by modulating molecular pathways involved in glucolipid metabolism,inflammation,oxidative stress,endoplasmic reticulum stress,and *** on recent advances,we discuss MSCs and their derivatives as therapeutic strategies for NAFLD and ALD,providing useful information for their clinical application.

关键词： Alcohol-associated liver disease Non-alcoholic fatty liver disease Mesenchymal stem cells Cell therapy Inflammation

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Synthesis,Characterization of Polyethylene Ionomers and Their Antibacterial Properties

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Chinese Journal of Polymer Science 2024年第8期42卷 1077-1084页

作者： jia-jia wu Fei Wang Peng-Qi Wan Li Pan Chun-Sheng Xiao Zhe Ma Yue-Sheng Li Tianjin Key Lab Composite&Functional Materials School of Materials Science and EngineeringTianjin UniversityTianjin 300350China Key Lab Polymer Ecomaterials Changchun Institute of Applied ChemistryChinese Academy of SciencesChangchun 130022China

Owing to its high production volume and wide range of application s,polyethylene has gained a great deal of attention,but its low surface energy and non-polar nature have limited its application in some important *** this study,ethylene/11-iodo-1-undecene copolymers were prepared and used as the intermediates to afford a series of imidazolium-based ionomers bearing methanesulfonate(CH_(3)SO_(3)^(-)),trifluoromethanesulfonate(CF_(3)SO_(3)^(-)),or bis(trifluoromethane)sulfonimide(Tf_(2)N^(-))*** tensile test results showed that the stress-at-break(7.8-25.6 MPa)and the elongation-at-break(445%-847%)of the ionomers could be adjusted by changing the counterion species and the ionic group *** importantly,the ionomers exhibited marvelous antibacterial activities against Staphylococcus aureus(***)and Escherichia coli(***).The ionomers bearing Tf_(2)N^(-)exhibited antibacterial activities>99%against both *** and *** when ionic content reached 9.1%.The imidazolium-based ionomers prepared in this work demonstrated excellent comprehensive properties,especially highefficient and broad-spectrum antibacterial ability,exhibiting the potential fo r the application as the antibacterial materials in packaging,medical,and other fields.

关键词： Polyethylene Ionomer Polymerization catalysis Imidazolium Antibacterial material

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P_(c)(4457)Interpreted as a J^(P)=1/2+State byD^(0)∧_(c)^(+)(2595)-π^(0)P_(c)(4312)Interaction

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Chinese Physics Letters 2024年第9期41卷 23-27页

作者： Jin-Zi wu Jin-Yi Pang jia-Jun wu School of Physics Sciences University of Chinese Academy of SciencesBeijing 100049China Columbian College of Arts&Sciences George Washington University80122nd St.NW Washington DC 20052USA College of Science University of Shanghai for Science and TechnologyShanghai 200093China Southern Center for Nuclear-Science Theory Institute of Modern PhysicsChinese Academy of SciencesHuizhou 516000China

P_(c)(4457)has been discovered over five years,but the parity of this particle remains *** propose a new interpretation for P_(c)(4457),which is the state generated from the coupled-channel D^(0)Ac+(2595)andπ^(0)P_(c)(4312)since they can exchange an almost on-shell∑_(c)^(+).In this scenario,the parity of P_(c)(4457)will be positive,which is different from the candidate of the bound state of D*∑_(c).The main decay channel of P_(c)(4457)in this model is Pc(4312)π.We propose three processes∧_(b)^(0)→J/ψKapπ^(-),∧_(b)^(0)→J/ψK-pπ^(0),and∧_(b)^(0)→J/ψpπ^(-)π^(+)k^(-)to verify Pc(4457)→Pc(4312)π.

关键词： (0 parity verify

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Suppress oxygen evolution of lithium-rich manganese-based cathode materials via an integrated strategy

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Green Energy & Environment 2024年第1期9卷 138-151页

作者： Wenhua Yu Yanyan Wang Aimin wu Aikui Li Zhiwen Qiu Xufeng dong Chuang dong Hao Huang Key Laboratory of Energy Materials and Devices(Liaoning Province) School of Materials Science and EngineeringDalian University of TechnologyDalian116024Liaoning ProvinceChina Dalian Engineering Research Center for New Electric Power Systerms School of Electrical EngineeringDalian University of TechnologyDalian116024Liaoning ProvinceChina

Improving the reversibility of anionic redox and inhibiting irreversible oxygen evolution are the main challenges in the application of high reversible capacity Li-rich Mn-based cathode materials.A facile synchronous lithiation strategy combining the advantages of yttrium doping and LiYO_(2) surface coating is *** doping effectively suppresses the oxygen evolution during the delithiation process by increasing the energy barrier of oxygen evolution reaction through strong Y–O bond ***_(2) nanocoating has the function of structural constraint and protection,that protecting the lattice oxygen exposed to the surface,thus avoiding irreversible *** an Li^(+) conductor,LiYO_(2) nano-coating can provide a fast Li^(+) transfer channel,which enables the sample to have excellent rate *** synergistic effect of Y doping and nano-LiYO_(2) coating integration suppresses the oxygen release from the surface,accelerates the diffusion of Li^(+)from electrolyte to electrode and decreases the interfacial side reactions,enabling the lithium ion batteries to obtain good electrochemical *** lithium-ion full cell employing the Y-1 sample(cathode)and commercial graphite(anode)exhibit an excellent specific energy density of 442.9 Wh kg^(-1) at a current density of 0.1C,with very stable safety performance,which can be used in a wide temperature range(60 to-15℃)stable *** result illustrates a new integration strategy for advanced cathode materials to achieve high specific energy density.

关键词： Lithium-rich manganese-based cathodes Lithium ion batteries Oxygen redox Oxygen evolution Integrated strategy

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New insights into the DPR mechanism of elastic energy released by polymer gel for enhanced oil recovery

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PETROLEUM 2024年第3期10卷 539-547页

作者： jia, Hu wu, Junyi wu, Shaowei Liang, Yanbin Wang, Minghao Wan, Xiaojin Li, Pengwu Southwest Petr Univ State Key Lab Oil & Gas Reservoir Geol & Exploitat Chengdu Peoples R China CNOOC Zhanjiang Branch Zhanjiang Peoples R China PetroChina Dagang Oilfield Co Oil Prod Technol Inst Tianjin Peoples R China

Polymer gel was widely used as water shutoff agent in mature oil fields. And the results of single-phase plugging experiments show that the plugging rate of the polymer gel to the oil phase is lower than that of the water phase. However, the disproportionate permeability reduction (DPR) mechanism of polymer gels still remains controversial. In this paper, we used four gel formulations including polyethyleneimine (PEI) and phenol-formaldehyde crosslinked gel with and without adding laponite to investigate the effect of gel elastic property on the water shutoff mechanism. The result of sand pack flooding experiments shown that the gel with higher elastic modulus has better effects on decreasing water cut and increasing oil recovery. After adding laponite, the elastic modulus of phenol-formaldehyde crosslinked gel increased from 64.2 Pa to 192 Pa, and the elastic modulus of PEI crosslinked gel increased from 27.4 Pa to 36.5 Pa. Compared to the phenol-formaldehyde-HAPM gel, the oil recovery of laponite-phenol-formaldehyde-HPAM gel increased by 5.2% and the maximum water cut decreased by 8.3%. Besides, comparing with PEI-HPAM gel, the oil recovery of laponite-PEI-HPAM gel increased by 2.7% and the water cut dropped by 27.8%. In the meanwhile, the laponite-phenol-formaldehyde-HPAM gel with higher elastic modulus obviously swells in the formation water but almost remains constant in oil at 105 degrees C. The mass of gel soaked in the formation water increased from 42 g to 96 g and the gel volume increased by 300% within 48 hours. This study improves the understanding of the DPR mechanism of polymer gel for water shutoff. (c) 2022 Southwest Petroleum University. Publishing services by Elsevier B.V. on behalf of KeAi Communications Co. Ltd. This is an open access article under the CC BY-NC-ND license (http://***/licenses/by-nc-nd/4.0/).

关键词： Gel elasticity Water shutoff DPR Laponite Oil recovery DISPROPORTIONATE PERMEABILITY REDUCTION NONIONIC POLYACRYLAMIDE WATER PERMEABILITY PHENOLIC RESIN

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Ambarzumyan's Theorem for the Dirac Operator on Equilateral Tree Graphs

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Acta Mathematicae Applicatae Sinica 2024年第2期40卷 568-576页

作者： dong-Jie wu Xin-jian XU Chuan-Fu YANG Department of Mathematics School of Mathematics and StatisticsNanjing University of Science and TechnologyNanjing 210094China

The classical Ambarzumyan’s theorem states that if the Neumann eigenvalues of the Sturm-Liouville operator-d^(2)/dx^(2)+q with an integrable real-valued potential q on[0,π] are {n^(2):n≥0},then q=0 for almost all x∈[0,π].In this work,the classical Ambarzumyan’s theorem is extended to the Dirac operator on equilateral tree *** prove that if the spectrum of the Dirac operator on graphs coincides with the unperturbed case,then the potential is identically zero.

关键词： dirac operator quantum graph Ambarzumyan’s theorem inverse spectral problem

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Frontiers of Computer Science 2024年第3期18卷 227-229页

作者： Qianwen GOU Yunwei dong Yujiao wu Qiao KE School of Computer Science Northwestern Polytechnical UniversityXi’an 710129China School of Mathematics and Statistics Northwestern Polytechnical UniversityXi’an 710129China

1 Introduction Program retrieval aims to enable the flexible retrieval of program snippets based on a natural language query,significantly accelerating software development *** shows that over 60%of developers perform program retrieval daily[1].Recent years have witnessed an increasing interest in deep learning-based program retrieval,which aims to construct embedding representations for program snippets and ***,the distribution of natural languages and programs is inconsistent,resulting in a semantic *** critical challenge is to bridge the semantic gap between the programming language and natural language,and accurately measure their similarity.

关键词： semantic similarity retrieval

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