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Chinese Chemical Letters 2024年第8期35卷 288-293页

作者： Lei wang Jun-Jie Wu Chang-Cun Yan Wan-Ying Yang Zong-Lu Che Xin-Yu Xia xue-dong wang Liang-Sheng Liao Jiangsu Key Laboratory for Carbon-Based Functional Materials&Devices Institute of Functional Nano&Soft Materials(FUNSOM)Soochow UniversitySuzhou 215123China Jiangsu Engineering Laboratory of Novel Functional Polymeric Materials College of ChemistryChemical Engineering and Materials ScienceSoochow UniversitySuzhou 215123China Macao Institute of Materials Science and Engineering Macao University of Science and TechnologyMacao SAR 999078China

Organic lasers with broad emission bands in near-infrared(NIR)region are crucial for their applications in laser communication,night-vision as well as bioimaging owing to the abundance of selectable lasing ***,for most organic gain materials,gain regions are limited in a small wavelength range because of the fixed energy level ***,we design a strategy to realize NIR organic lasers with broad emission bands based on tunable energy level systems induced by cascaded excited-state intramolecular proton transfer(ESIPT).A novel gain material named DHNN was developed,which can undergo a cascaded double-ESIPT process supporting four-level and six-level systems *** doping DHNN into polystyrene microspheres,NIR lasers with tunable emission bands can be achieved based on the careful modulation of ***,organic lasers with an ultra-broad emission band ranging from 700 nm to 900 nm was successfully achieved by harnessing four-level and six-level systems simultaneously.

关键词： Excited-state intramolecular proton transfer Organic solid-state laser Wide gain interval Near-infrared emission Molecular design

Organic near-infrared optoelectronic materials and devices:an overview

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Advanced Photonics 2024年第1期6卷 17-42页

作者： Zong-Lu Che Chang-Cun Yan xue-dong wang Liang-Sheng Liao Soochow University Institute of Functional Nano and Soft Materials(FUNSOM)Jiangsu Key Laboratory for Carbon-Based Functional Materials and DevicesSuzhouChina Soochow University College of ChemistryChemical Engineering and Materials ScienceJiangsu Engineering Laboratory of Novel Functional Polymeric MaterialsSuzhouChina Macao University of Science and Technology Macao Institute of Materials Science and EngineeringMacaoChina

Near-infrared(NIR)light has shown great potential for military and civilian applications owing to its advantages in the composition of sunlight,invisibility to human eyes,deeper penetration into biological tissues,and low optical loss in optical ***,organic optoelectronic materials that can absorb or emit NIR light have aroused great scientific interest in basic science and practical *** on these NIR organic optoelectronic materials,NIR optoelectronic devices have been greatly improved in performance and *** this review,the representative NIR organic optoelectronic materials used in organic solar cells,organic photodetectors,organic light-emitting diodes,organic lasers,and organic optical waveguide devices are briefly introduced,and the potential applications of each kind of device are briefly ***,we summarize and take up the development of NIR organic optoelectronic materials and devices.

关键词： near-infrared organic optoelectronic materials organic solar cells organic light-emitting devices organic optical waveguides

Unconventional Organic Low-Dimensional Crystals:Diversity and Potential Applications

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CCS Chemistry 2024年第7期6卷 1628-1653页

作者： Jin Feng Mao Sun Ying-Xin Ma Zhen-Yu Geng Chuan-Zeng wang Shu-Ping Zhuo Shu-Hai Chen Hong-Tao Lin xue-dong wang School of Chemistry and Chemical Engineering Shandong University of TechnologyZibo 255000 School of Resources and Environmental Engineering Shandong University of TechnologyZibo 255000 Institute of Functional Nano&Soft Materials(FUNSOM) Jiangsu Key Laboratory for Carbon-Based Functional Materials&DevicesSoochow UniversitySuzhou 215123

Organic low-dimensional crystals have garnered escalating interests in the realms of miniaturized optoelectronics and integrated *** continual expansion of molecular systems and improvement in experimental conditions have given rise to unconventional organic low-dimensional crystals,which showcase a variety of appealing structure-dependent properties in the realm of organic semiconductors,owing to their adaptable physicochemical characteristics and exceptional optoelectronics ***,the development of unconventional low-dimensional crystals is filled with abundant possibilities due to their diverse application ***,we present a comprehensive overview of advancements in research on representative cases of unconventional low-dimensional organic crystals,using a systematic and rational structural ***,we have also discussed the existing challenges and future directions,aspiring to deepen understanding and encourage further research exploration in this field.

关键词： organic semiconductor crystal growth precise synthesis noncovalent interaction integrat-ed photonics

Exercise promotes osteogenic differentiation by activating the long non-coding RNA H19/microRNA-149 axis

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World Journal of Orthopedics 2024年第4期15卷 363-378页

作者： Xu-Chang Zhou dong-xue wang Chun-Yu Zhang Ya-Jing Yang Ruo-Bing Zhao Sheng-Yao Liu Guo-Xin Ni School of Sport Medicine and Rehabilitation Beijing Sport UniversityBeijing 100084China Department of Acupuncture and Moxibustion Hubei University of Chinese MedicineWuhan 430065Hubei ProvinceChina Department of Spinal Surgery The Second Affiliated Hospital of Guangzhou Medical UniversityGuangzhou 510260Guangdong ProvinceChina Department of Rehabilitation Medicine The First Affiliated Hospital of Xiamen UniversityXiamen 361003Fujian ProvinceChina

BACKGROUND Regular physical activity during childhood and adolescence is beneficial to bone development,as evidenced by the ability to increase bone density and peak bone mass by promoting bone *** To investigate the effects of exercise on bone formation in growing mice and to investigate the underlying *** 20 growing mice were randomly divided into two groups:Con group(control group,n=10)and Ex group(treadmill exercise group,n=10).Hematoxylin-eosin staining,immunohistochemistry,and micro-CT scanning were used to assess the bone formation-related indexes of the mouse *** analysis was used to find potential miRNAs targets of long non-coding RNA H19(lncRNA H19).RT-qPCR and Western Blot were used to confirm potential miRNA target genes of lncRNA H19 and the role of lncRNA H19 in promoting osteogenic *** Compared with the Con group,the expression of bone morphogenetic protein 2 was also significantly *** micro-CT results showed that 8 wk moderate-intensity treadmill exercise significantly increased bone mineral density,bone volume fraction,and the number of trabeculae,and decreased trabecular segregation in the femur of *** of lncRNA H19 significantly upregulated the expression of miR-149 and suppressed the expression of markers of osteogenic *** addition,knockdown of lncRNA H19 significantly downregulated the expression of autophagy markers,which is consistent with the results of autophagy-related protein changes detected in mouse femurs by *** Appropriate treadmill exercise can effectively stimulate bone formation and promote the increase of bone density and bone volume in growing mice,thus enhancing the peak bone mass of *** lncRNA H19/miR-149 axis plays an important regulatory role in osteogenic differentiation.

关键词： Exercise Osteogenic differentiation Bone formation Bone mesenchymal stem cells Autophagy

调控动态生长过程以构筑嵌段可换和光谱可调的有机异质结构

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Science China Materials 2024年第7期67卷 2153-2160页

作者：赵帅许超飞余悦夏星宇王磊王雪东廖良生 Jiangsu Key Laboratory for Carbon-Based Functional Materials&Devices Institute of Functional Nano&Soft Materials(FUNSOM)Soochow UniversitySuzhou 215123China Macao Institute of Materials Science and Engineering Macao University of Science and TechnologyMacao 999078China

与单一结构相比,有机嵌段异质结构具有特殊的光电性能.然而,有机分子间的相互作用主导了异质结构构建单元的生长顺序,如有机单元A、B会自发形成BAB型结构而不是相反的ABA型结构,不能可控生长.在此,我们提出了次序结晶工程,结合晶种逐步... 详细信息

与单一结构相比,有机嵌段异质结构具有特殊的光电性能.然而,有机分子间的相互作用主导了异质结构构建单元的生长顺序,如有机单元A、B会自发形成BAB型结构而不是相反的ABA型结构,不能可控生长.在此,我们提出了次序结晶工程,结合晶种逐步自组装,控制共晶R与共晶N在彼此的两端纵向外延生长,从而精确合成具有可逆嵌段构型的有机嵌段异质结构:RNR和***有机嵌段异质结构,由于其逐渐掺杂的异质结而表现出渐变色的发射和波导特性,而NRN有机嵌段异质结构由于其明显的构筑异质结界限而表现出纯双色发射和波导特性.本工作实现了有机嵌段异质结构中嵌段块的有序可控生长,为未来光子学发展提供了制备合理复杂有机嵌段异质结构的途径.

关键词： organic heterostructure charge transfer cocrystal crystallization optical waveguide

Interception of Layered LP-N and HLP-N at Ambient Conditions by Confined Template

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Chinese Physics Letters 2024年第3期41卷 61-72页

作者：王冬雪付静李义姚震刘爽刘冰冰 State Key Laboratory of Superhard Materials College of PhysicsJilin UniversityChangchun 130012China Basic Science Department Jilin Institute of Architecture and TechnologyChangchun 130000China College of Science Liaoning University of TechnologyJinzhou 121000China

We propose a feasible strategy of intercepting the layered polymeric nitrogen(LP-N)and hexagonal layered polymeric nitrogen(HLP-N)at ambient conditions by using the confinement *** stable mechanism of confined LP-N an... 详细信息

关键词： ambient layered polymeric

可见光到近红外Ⅱ区内宽领域可调发射的芘基共晶

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Science China Materials 2024年第3期67卷 946-953页

作者：夏星宇吕强余悦车宗路王雪东廖良生李述汤 Jiangsu Key Laboratory for Carbon-Based Functional Materials&Devices Institute of Functional Nano&Soft Materials(FUNSOM)Soochow UniversitySuzhou 215123China Macao Institute of Materials Science and Engineering Macao University of Science and TechnologyMacao SAR 999078China

有机材料的可变发光在波导和显示应用方面具有广泛的潜力.然而,基于单一有机分子体系实现从可见光到近红外区域的大范围发光调节仍然是一项挑战.本文介绍了一系列基于芘的同构共晶体,可提供从可见光到近红外Ⅱ区的可调发射.它们的能级... 详细信息

有机材料的可变发光在波导和显示应用方面具有广泛的潜力.然而,基于单一有机分子体系实现从可见光到近红外区域的大范围发光调节仍然是一项挑战.本文介绍了一系列基于芘的同构共晶体,可提供从可见光到近红外Ⅱ区的可调发射.它们的能级是通过引入电荷转移和无氟芳烃-全氟芳烃相互作用而定制的.令人印象深刻的是,这项工作中的有机微晶可以成功地应用于微观层面的多色波导以及宏观层面的二维码显示,为先进的光子学开辟了新的道路.这项工作为获得400至1100 nm的有机晶体提供了一种简单而有效的方法,从而为制造多种光电子学的核心材料提供了可能性.

关键词： organic cocrystal tunable emission near-infraredⅡ(NIR-Ⅱ) optical waveguide quick response(QR)code

Shape-engineering of organic heterostructures via a sequential selfassembly strategy for multi-channel photon transportation

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Nano Research 2022年第4期15卷 3781-3787页

作者： Yue Yu Qiang Lv Yi Yuan xue-dong wang Liang-Sheng Liao Institute of Functional Nano&Soft Materials(FUNSOM) Jiangsu Key Laboratory for Carbon-Based Functional Materials&DevicesSoochow UniversitySuzhou 215123China Macao Institute of Materials Science and Engineering Macao University of Science and TechnologyTaipaMacao 999078MacaoChina

The controlled self-assembly of organic heterostructures(OHSs)with precisely defined compositions,architectures,and interfaces,have largely remained a ***,we introduce an effective approach to accurately construct three types of axial branching OHSs including unilateral axial OHSs,bilateral single-branching axial OHSs and bilateral multi-branching axial OHSs through modulating hierarchical charge-transfer intermolecular interactions and sequential crystal nucleation rate on account of the two different cocrystals with the low lattice mismatching rate of~2.2%.The present work opens an avenue for rationally designing and finely synthesizing more kinds of OHSs.

关键词： sequential self-assembly axial heterostructures non-covalent interaction lattice-match multi-channel outputs

Recent progress on the excited-state multiple proton transfer process in organic molecules

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Science China Chemistry 2022年第10期65卷 1843-1853页

作者： Wan-Ying Yang Chang-Cun Yan xue-dong wang Liang-Sheng Liao Institute of Functional Nano&Soft Materials(FUNSOM) Jiangsu Key Laboratory for Carbon-Based Functional Materials&DevicesSoochow UniversitySuzhou 215123China Macao Institute of Materials Science and Engineering Macao University of Science and TechnologyTaipa 999078China

In contrast to the widely reported excited-state single proton-transfer,excited-state multiple proton transfer(ESMPT)containing two or more intra-or inter-molecular proton transfers has greatly expanded the research scope of the excited-state proton *** recent decades,ESMPT-active organic molecules have attracted much attention owing to their unique photophysical properties,such as large magnitude Stokes shifts and dual *** photophysical properties facilitate the application of the organic molecules in organic solid-state lasers,fluorescent probes and sensors,and molecular ***,we introduce the fundamentals of the ESMPT and review the recent advances in different types of ESMPTs in organic ***,we present our conclusions and the future development prospects of the ESMPT in organic molecules.

关键词： excited-state multiple proton transfer hydrogen bond photoisomerization organic molecules photophysical properties

Longitudinal Quantitation of Tooth Displacement in Chinese Adolescents with Normal Occlusion

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Current Medical Science 2019年第2期39卷 317-324页

作者： Jie-ni ZHANG xue-dong wang Jiu-xiang LIN Department of Orthodontics Peking University School and Hospital of StomatologyBeijing 100081China

This longitudinal study aims to analyze the different modes of the maxillary and mandibular tooth displacement in subjects,who were aged 12.5-17.5 years(150-210 months),with untreated normal(Class I)*** lateral cephalograms for a set of 10 subjects(7 females and 3 males)at consecutive annual time points were selected and *** were analyzed on the basis of the superimpositions of serial tracings of lateral cephalograms on stable anterior cranial base,the anatomies of the maxillary and mandibular *** horizontal and vertical displacements of the first molar and incisor were assessed by *** local and the secondary tooth displacements with growth contributed to the total horizontal and vertical displacements of the molars and incisors of the *** the total tooth displacement,the horizontal growth of maxilla and mandible had the same contribution as the local tooth *** vertical maxillary growth played a smaller role than the local drift,and mandibular remodeling went in a reverse direction with the local tooth *** first molars moved more forward than the incisors in the upper and lower *** the upper and lower first molars showed forward *** analysis of tooth displacement may be utilized in making orthodontic treatment plan,including anchorage or torque control.

关键词： tooth movement growth evaluation cephalometries superimposition